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Characterizing the behavior of surge-type glaciers in the Puruogangri Ice Field, Tibetan Plateau

Journal of Geographical Sciences 2024年第6期34卷 1174-1194页

作者： ZHOU Sugang WANG Ninglian LI Zhijie YAO xiaojun ZHANG Yuje QIN Gexia Shaanxi Key Laboratory of Earth Surface System and Environmental Carrying Capacity College of Urban and Environmental SciencesNorthwest UniversityXi'an 710127China Institute of Earth Surface System and Hazards College of Urban and Environmental SciencesNorthwest UniversityXi'an 710127China College of Geography and Environmental Science Northwest Normal UniversityLanzhou 730070China

The Puruogangri Ice Field(PIF), classified as an ultra-continental glacier, is considered extremely stable. However, several glaciers in this area have recently experienced surge events with significant instability and information on surge-type glaciers(STGs) in this region remains scarce. In this study, we identified six STGs and reported the observed characteristics of their surging behavior in the region by mapping glacier boundaries, surface flow velocity information, and glacier surface elevation changes using recent Landsat satellite imagery and shuttle radar topography mission(SRTM), TanDEM, and ASTER digital elevation model(AST14DEM) data. These data provide valuable insights into recent glacial processes, flow instability, and rapid glacial movement. During the active phase of the glaciers,all exhibited frontal advances and changes in surface elevation. Owing to limitations in the satellite imagery, flow velocity profiles were only available for glaciers N1(G089071E33998N),NE1(G089128E33943N), and SE3(G089278E33913N) during the active phase. However,these results effectively reflect the velocity variations in both glaciers before, during, and after the surge. Based on the characteristics of the STG, scientific expeditions, and meteorological data, we believe that the surge in PIF was largely influenced by glacier meltwater and changes in subglacial drainage systems.

关键词： glacier surge glacier surface elevation changes glacier surface velocity Puruogangri Ice Field

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Nanostructured AlFeO_(3) thin films as a novel photoanode for photoelectrochemical water splitting

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Nano Research 2024年第3期17卷 1075-1085页

作者： Xin Sun Min Wang Qi Geng Shuailin Chen xiaojun Lv Xunlei Ding Meicheng Li State Key Laboratory of Alternate Electrical Power System with Renewable Energy Sources School of New EnergyNorth China Electric Power UniversityBeijing 102206China School of Mathematics and Physics North China Electric Power UniversityBeijing 102206China

The earth-abundant and robust aluminum ferrite,AlFeO_(3)(AFO),is mainly studied in the context of ferroelectrics.herein,we demonstrate that AFO can be used as a stable solar absorber in photoelectrochemical cells for solar water splitting,exhibiting attractive performance.This is the first report on the photoelectrochemical activity of AFO.AFO thin-film photoelectrodes prepared by solution-processing methods are composed of vertically oriented thin nanosheets,featuring the rhombohedral symmetry(R3c)and n-type conductivity.The as-prepared AFO photoanodes generate a photocurrent density of+0.78 mA·cm^(-2) at 1.23 V vs.reversible hydrogen electrode(Rhe)with the photocurrent _(onset) potential(U_(onset))close to the flat band potential of 0.5 V vs.Rhe in the presence of hole scavengers.Remarkably,the U_(onset) of AFO for solar water splitting coincides with the flat band potential as well,which is rare in n-type inorganic absorbers.We also report other properties of AFO associated with photoelectrochemical performance.AFO films exhibit a band gap energy of 2.31 eV and positive band edges with low dispersion.Moreover,the carrier lifetimes in AFO films are up to millisecond timescales under the mediation of defect traps.Based on the photoelectrochemical behavior and optoelectronic properties,we believe that AFO has great potential for application in photoelectrochemical cells.

关键词： AlFeO_(3) photoanode nanosheets photoelectrochemistry onset potential

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Dual-aligned porous electrodes for enhanced hydrogen evolution in alkaline water electrolysis

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Nano Research 2024年第5期17卷 3835-3843页

作者： Yuqi Zhang Wenzhi Cui Longjian Li Chongbo Wang Chen Zhan xiaojun Quan School of Energy and Power Engineering Chongqing UniversityChongqing 400030China Key Laboratory of Low-grade Energy Utilization Technologies and Systems Chongqing UniversityChongqing 400030China School of Mechanical Engineering Shanghai Jiao-Tong UniversityShanghai 200240China

The efficiency of water electrolysis is significantly affected by the bubbles on the surface and inside the electrode.To enhance the gas-liquid transfer within the porous electrodes,we developed an innovative design termed dual-aligned porous electrode(D-APE),achieved by integrating magnetic alignment with freeze casting techniques.This paper investigates the hydrogen evolution performance of porous electrodes prepared using four different methods:evaporation,magnetic-aligned evaporation,freeze casting,and dual-aligned methods.The findings demonstrate that the magnetic-aligned process effectively alters the electrode structure,resulting in improved hydrogen evolution performance.Notably,among all the examined electrodes,the D-APE exhibits the highest hydrogen evolution performance,with further enhancements observed with prolonged the time of magnetic alignment.Furthermore,a comparison is made between electrodes prepared using the freeze casting method and the dual-aligned method at various thickness.The results show that the thinner D-APE exhibits excellent hydrogen evolution performance at high current density.Moreover,the D-APE demonstrates significantly improved material utilization rates compared to the conventional freeze casting method,offering promising prospects for enhancing the efficiency of water electrolysis.

关键词： hydrogen evolution reaction dual-aligned magnetic-aligned freeze casting

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MAX-DOAS and in-situ measurements of aerosols and trace gases over Dongying,China:Insight into ozone formation sensitivity based on secondary HCHO

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Journal of Environmental Sciences 2024年第1期135卷 656-668页

作者： xiaojun Zheng Zeeshan Javed Cheng Liu Aimon Tanvir Osama Sandhu Haoran Liu Xiangguang Ji Chengzhi Xing Hua Lin Daolin Du Institute of Environment and Ecology School of the Environment and Safety EngineeringJiangsu UniversityZhenjiang 212013China Department of Precision Machinery and Precision Instrumentation University of Science and Technology of ChinaHefei 230026China Key Laboratory of Environmental Optics&Technology Anhui Institute of Optics and Fine MechanicsHefei Institutes of Physical ScienceChinese Academy of SciencesHefei 230031China Center for Excellence in Regional Atmospheric Environment Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China Key Laboratory of Precision Scientific Instrumentation of Anhui Higher Education Institutes University of Science and Technology of ChinaHefei 230026China Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention(LAP3) Department of Environmental Science and EngineeringFudan UniversityShanghai 200433China National Agromet Center Pakistan Meteorological DepartmentIslamabad 44000Pakistan Institute of Physical Science and Information Technology Anhui UniversityHefei 230601China Information Materials and Intelligent Sensing Laboratory of Anhui Province Anhui UniversityHefei 230601China School of Environmental Science and Optoelectronic Technology University of Science and Technology of ChinaHefei 230026China

This study presents a comprehensive overview of the atmospheric pollutants including Sulfur dioxide(SO_(2)),Nitrogen dioxide(NO_(2)),Formaldehyde(HCHO),Particulate Matter PM;PM_(10):diameter≤10μm,and PM_(2.5):diameter≤2.5μm,and Ozone(O_(3)),over Dongying(Shandong Province)from March-April 2018 and September-October 2019 by employing ground-based Multiple Axis Differential Optical Absorption Spectroscopy(MAX-DOAS)observations along with the in-situ measurements attained by the national air quality monitoring platform.The concentrations of SO_(2)and NO_(2)were under the acceptable level,while both PM_(2.5),and PM_(10)were higher than the safe levels as prescribed by national and international air quality standards.The results depict that 21%of the total observation days were found to be complex polluted days(PM_(2.5)>35μg/m^(3) and O_(3)>160μg/m^(3)).The secondary HCHO was used for accurate analysis of O_(3)sensitivity.A difference of 11.40%and 10%during March-April 2018 and September-October 2019 respectively in O_(3)sensitivity was found between HCHO_(total)/NO_(2)and HCHO_(sec)/NO_(2).The results indicate that primary HCHO have significant contribution in HCHO.O_(3)formation predominantly remained to be in VOC-limited and transitional regime during March-April 2018 and September-October 2019 in Dongying.These results imply that concurrent control of both NO_(x) and VOCs would benefit in ozone reductions.Additionally,the criteria pollutants(PM,SO_(2),and NO_(2))depicted strong correlations with each other except for O_(3)for which weak correlation coefficient was obtained with all the species.This study will prove to be baseline for designing of air pollution control strategies.

关键词： MAX-DOAS Trace gases Ozone sensitivity Secondary HCHO Complex Pollution

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Metal–Organic Gel Leading to Customized Magnetic‑Coupling Engineering in Carbon Aerogels for Excellent Radar Stealth and Thermal Insulation Performances

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Nano-Micro Letters 2024年第3期16卷 36-52页

作者： Xin Li Ruizhe Hu Zhiqiang Xiong Dan Wang Zhixia Zhang Chongbo Liu xiaojun Zeng Dezhi Chen Renchao Che Xuliang Nie Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle Nanchang Hangkong UniversityNanchang 330063People’s Republic of China School of Environmental and Chemical Engineering Nanchang Hangkong UniversityNanchang 330063People’s Republic of China Laboratory of Advanced Materials Department of Materials Science and Collaborative Innovation Center of Chemistry for Energy Materials and Collaborative Innovation Center of Chemistry for Energy MaterialsFudan UniversityShanghai 200438People’s Republic of China School of Materials Science and Engineering Jingdezhen Ceramic UniversityJingdezhen 333403People’s Republic of China College of Chemistry and Materials Jiangxi Agricultural UniversityNanchang 330045People’s Republic of China

Metal–organic gel(MOG)derived composites are promising multi-functional materials due to their alterable composition,identifiable chemical homogeneity,tunable shape,and porous structure.herein,stable metal–organic hydrogels are prepared by regulating the complexation effect,solution polarity and curing speed.Meanwhile,collagen peptide is used to facilitate the fabrication of a porous aerogel with excellent physical properties as well as the homogeneous dispersion of magnetic particles during calcination.Subsequently,two kinds of heterometallic magnetic coupling systems are obtained through the application of Kirkendall effect.FeCo/nitrogen-doped carbon(NC)aerogel demonstrates an ultra-strong microwave absorption of−85 dB at an ultra-low loading of 5%.After reducing the time taken by atom shifting,a FeCo/Fe3O4/NC aerogel containing virus-shaped particles is obtained,which achieves an ultra-broad absorption of 7.44 GHz at an ultra-thin thickness of 1.59 mm due to the coupling effect offered by dual-soft-magnetic particles.Furthermore,both aerogels show excellent thermal insulation property,and their outstanding radar stealth performances in J-20 aircraft are confirmed by computer simulation technology.The formation mechanism of MOG is also discussed along with the thermal insulation and electromagnetic wave absorption mechanism of the aerogels,which will enable the development and application of novel and lightweight stealth coatings.

关键词： Metal-organic gels heterometallic magnetic coupling Radar stealth Thermal insulation Computer simulation technology

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Enhancing Strength-Ductility Synergy of CoCrNi-Based Medium-Entropy Alloy Through Coherent L1_(2)Nanoprecipitates and Grain Boundary Precipitates

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Acta Metallurgica Sinica(English Letters) 2024年第1期37卷 78-88页

作者： Leilei Li Kaikai Song Qingwei Gao Changshan Zhou Xiaoming Liu Yaocen Wang xiaojun Bai Chongde Cao School of Physical Science and Technology Northwestern Polytechnical UniversityXi’an710016China Weihai Research Institute of Industrial Technology Shandong UniversityWeihai264209China Research and Development Institute of Northwestern Polytechnical University in ShenzhenShenzhen518057China

The L1_(2)-strengthened Co_(34)Cr_(32)Ni_(27)Al_(4)Ti_(3)medium-entropy alloy(MEA)with precipitations of grain boundaries has been developed through selective laser melting(SLM)followed by cold rolling and annealing,exhibiting excellent strength-ductility synergy.The as-printed alloy exhibits low yield strength(YS)of~384 MPa,ultimate tensile strength(UTS)of~453 MPa,and uniform elongation(UE)of 1.5%due to the existence of the SLM-induced defects.After cold rolling and annealing,the YS,UTS,and UE are significantly increased to~739 MPa,~1230 MPa,and~47%,respectively.This enhancement primarily originates from the refined grain structure induced by cold rolling and annealing.The presence of coherent sphericalγ'precipitates(L1_(2)phases)and Al/Ti-rich precipitates at the grain boundaries,coupled with increased lattice defects such as dislocations,stacking faults,and ultrafine deformation twins,further contribute to the property’s improvement.Our study highlights the potential of SLM in producing high-strength and ductile MEA with coherent L1_(2)nanoprecipitates,which can be further optimized through subsequent rolling and annealing processes.These findings offer valuable insights for the development of high-performance alloys for future engineering applications.

关键词： Medium-entropy alloy Selective laser melting Precipitation Strength Ductility

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mtDNA-triggered pH response signal-amplified fluorescent probe for multiple cell discrimination

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Chinese Chemical Letters 2024年第3期35卷 363-368页

作者： Tianping Xia Yanxian Hou Zhuoran Xia Gengwen Chen Peichen Tang Jiangli Fan xiaojun Peng State Key Laboratory of Fine Chemicals Frontiers Science Center for Smart Materials Oriented Chemical EngineeringDalian University of TechnologyDalian 116024China hematology Reagent R&D Department Mindray Bio-medical Electronics Co.Ltd.Shenzhen 518132China Research Institute of Dalian University of Technology in Shenzhen Shenzhen 518057China

Developing fluorescence probes with multiple responses has vital significance but remains challenging.herein,for the first time,we present a mitochondrial DNA(mtDNA)-triggered pH response signalamplified fluorescent probe(QCY-DBT)for multiple cell detection.The probe exhibited a large stokes shift(229 nm),excellent DNA selectivity over RNA,and ultrasensitivity of detection limit(DL;74.0 ng/mL).Thus,QCY-DBT was successfully applied to analyze multiple human peripheral blood cells and visualize mtDNA in healthy and apoptotic cells.In the tumor acidic environment(pH 6.0–7.0),the absorbance of QCY-DBT at 436 nm increased,and the fluorescence signal(665 nm)was amplified by mtDNA,which enabled the direct observation of tumor cells.Our study provides help in designing smart probes with multiple responses for efficient abnormal cell detection.

关键词： Fluorescence probe Mitochondrial DNA pH response Peripheral blood cells Multiple cell detection

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Relationships between blood chromium exposure and liver injury:Exploring the mediating role of systemic inflammation in a chromate-exposed population

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Journal of Environmental Sciences 2024年第9期143卷 224-234页

作者： Zekang Su Yali Zhang Shiyi Hong Qiaojian Zhang Jiayu Xu Guiping Hu xiaojun Zhu Fang Yuan Shanfa Yu Tianchen Wang Guang Jia Department of Occupational and Environmental health Sciences School of Public HealthPeking UniversityBeijing 100191China School of Engineering Medicine and Beijing Advanced Innovation Center for Big Data-Based Precision Medicine Beihang UniversityBeijing 100191China National Center for Occupational Safety and health Beijing 102308China Department of Occupational health and Radiological health Chongqing Centers for Disease Control and PreventionChongqing 400042China henan Institute for Occupational Medicine Zhengzhou 450052China Department of Clinical Laboratory Third Hospital of Peking UniversityBeijing 100191China

hexavalent chromium and its compounds are prevalent pollutants,especially in the work environment,pose a significant risk for multisystem toxicity and cancers.While it is known that chromium accumulation in the liver can cause damage,the dose-response relationship between blood chromium(Cr)and liver injury,as well as the possible potential toxic mechanisms involved,remains poorly understood.To address this,we conducted a follow-up study of 590 visits from 305 participants to investigate the associations of blood Cr with biomarkers for liver injury,including serum alanine aminotransferase(ALT),aspartate aminotransferase(AST),total bilirubin(TBIL),and direct bilirubin(DBIL),and to evaluate the mediating effects of systemic inflammation.Platelet(PLT)and the platelet-to-lymphocyte ratio(PLR)were utilized as biomarkers of systemic inflammation.In the linear mixed-effects analyses,each 1-unit increase in blood Cr level was associated with estimated effect percentage increases of 0.82%(0.11%,1.53%)in TBIL,1.67%(0.06%,3.28%)in DBIL,0.73%(0.04%,1.43%)in ALT and 2.08%(0.29%,3.87%)in AST,respectively.Furthermore,PLT mediated 10.04%,11.35%,and 10.77%increases in TBIL,DBIL,and ALT levels induced by chromate,respectively.In addition,PLR mediated 8.26%and 15.58%of the association between blood Cr and TBIL or ALT.These findings shed light on the mechanisms underlying blood Cr-induced liver injury,which is partly due to worsening systemic inflammation.

关键词： Blood chromate Liver injury Systemic inflammation Mediation analysis

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Geochronology,Geochemistry,and Sr-Nd-Hf Isotopes of the Diorite Porphyrites from the Weining Beishan Area,Ningxia Hui Autonomous Region:Constraints on Their Source and Tectonic Implications

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Journal of Earth Science 2024年第2期35卷 462-475页

作者： Anlu Liu Lianfu Hai Jinke Liu xiaojun Zhang Haifeng Li Fengshun Zhao Guoliang Zhao Jinhe Bai Yifu Museum China University of GeosciencesWuhan430074China School of Earth Resources China University of GeosciencesWuhan430074China Mineral Geological Survey Institute of Ningxia Hui Autonomous Region Yinchuan750021China National Demonstration Center for Experimental Mineral Exploration Education China University of GeosciencesWuhan430074China Coal Geological Survey Institute of Ningxia Hui Autonomous Region Yinchuan750021China Zhuhai Engineering Investigation Institute of Guangdong Province Zhuhai519000China

The Weining Beishan area of Ningxia Hui Autonomous Region is located at on the western edge of the helanshan tectonic belt,which is a tectonic joint among Alxa Block,Ordos Block,and North Qilian orogenic belt.However,the tectonic evolution of this area remains unclear due to the lack of magmatic information.This paper conducted researches on geochronology,geochemistry,and Sr-Nd-Hf isotopes of the diorite porphyrites exposed in the Weining Beishan area.The zircon U-Pb dating yields two ages of 145.0±1.1 and 146.2±1.5 Ma,and the whole-rock geochemical data indicate that the diorite porphyrites are metaluminous to weakly peraluminous and high-K calc-alkaline series.The characteristics of highly initial^(87)Sr/^(86)Sr ratios(0.70816 to 0.71047),negativeε_(Nd)(t)(−8.9 to−8.4),and negativeε_(Hf)(t)(−13.8 to−21.2)indicate that the diorite porphyrites originated from partial melting of the middle-lower ancient crust related to the North China Craton.Combined with the regional geology,we suggested that partial melting was triggered by a tectonic activity of deep faults cutting through the crust under the regional stress transformation from compressing to extension during the Late Jurassic–Early Cretaceous,which is probably related to the westward subduction of the Paleo-Pacific Plate.

关键词： zircon U-Pb dating Sr-Nd-Hf isotopes magma source diorite porphyrite Weining Beishan area Ningxia Hui Autonomous Region geochronology geochemistry

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Hierarchical assembly of NiFe-PB-derived bimetallic phosphides on 3D Ti_(3)C_(2) MXene ribbon networks for efficient oxygen evolution

ChemPhysMater

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ChemPhysMater 2024年第1期3卷 118-124页

作者： Chulong Jin Hanlei Peng xiaojun Zeng Zhenyuan Liu Deng Ding School of Materials Science and Engineering Jingdezhen Ceramic UniversityJingdezhen 333403China School of Materials Science and Engineering Jiangsu University of Science and TechnologyZhenjiang 212100China College of Chemistry and Environmental Engineering Wuhan Polytechnic UniversityWuhan 430023China

The development of MXene-based heterostructures for electrocatalysis has garnered significant attention owing to their potential as high-performance catalysts that play a pivotal role in hydrogen energy.herein,we present a multistep strategy for the synthesis of a Ti_(3)C_(2) MXene ribbon/NiFePx@graphitic N-doped carbon(NC)heterostructure that enables the formation of three-dimensional(3D)Ti_(3)C_(2) MXene ribbon networks and bimetallic phosphide nanoarrays.With the assistance of HF etching and KOH shearing,the MXene sheets were successfully transformed into 3D MXene networks with interlaced MXene ribbons.Notably,a hydrothermal method,ion exchange route,and phosphorization process were used to anchor NiFeP_(x)@NC nanocubes derived from Ni(OH)_(2)/NiFe-based Prussian blue(NiFe-PB)onto the MXene ribbon network.The resulting MXene ribbon/NiFeP_(x)@NC heterostructure demonstrated enhanced oxygen evolution reaction(OER)activity,characterized by a low overpotential(164 mV at a current density of 10 mA cm^(-2))and a low Tafel slope(45 mV dec^(-1)).At the same time,the MXene ribbons/NiFeP_(x)@NC heterostructure exhibited outstanding long-term stability,with a 12 mV potential decay after 5000 cyclic voltammetry(CV)cycles.This study provides a robust pathway for the design of efficient MXene-based heterostructured electrocatalysts for water splitting.

关键词： Metal phosphides Prussian blue nanocubes Ti_(3)C_(2)MXene ribbons Interfacial matching OER

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