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Selective photocatalytic oxidation of methane to C1 oxygenates by regulating sizes and facets over Au/ZnO

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Nano Research 2024年第5期17卷 3810-3818页

作者： Qiang zhou Xinyu Wang xiaojie Tan Qinhua Zhang Hao Yang Tao Xing Mingqing Wang Mingbo Wu Wenting Wu State Key Laboratory of Heavy Oil Processing College of Chemistry and Chemical Engineering&Institute of New EnergyChina University of Petroleum(East China)Qingdao 266580China National Engineering Research Center of Coal Gasification and Coal-Based Advanced Materials ShanDong Energy Group CO.LTDJinan 250101China

Photocatalytic oxidation of methane to value-added chemicals is a promising process under mild conditions,nevertheless confronting great challenges in efficiently activating C-H bonds and inhibiting over-oxidation.Herein,we propose a comprehensive strategy for the selective generation of reactive oxygen species(ROS)by regulating the sizes and facets of Au nanoparticles loaded on ZnO.For photocatalytic methane oxidation at ambient temperature,a high oxygenates yield of 36.4 mmol·g^(-1)·h^(-1) with a nearly 100%selectivity has been achieved over the optimized 1.0%Au/ZnO-9.6(1%Au with(111)facet and 9.6 nm size on ZnO)photocatalyst,exceeding most reported literatures.Mechanism investigations reveal that 1.0%Au/ZnO-9.6 with the medium size and Au(111)facet guarantees the favourable formation of superoxide radicals(·OOH)through mild oxygen reduction,ultimately leading to excellent photocatalytic methane oxidation performance.This work provides some guidance for the delicate design of photocatalysts for efficient photocatalytic methane oxidation and oxygen utilization.

关键词： photocatalysis methane oxidation radical regulation oxygen activation nanomaterial

基于COMSOL的多中继线圈无线电能传输特性分析

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牡丹江师范学院学报（自然科学版） 2024年第2期 31-35页

作者：李新恒尹文凯周小杰汪婵孙雯国海王鑫鑫赵传奇安徽科技学院电气与电子工程学院安徽蚌埠233000

采用COMSOL Multiphysics软件,对含有多中继线圈结构的无线电能传输系统建模并分析.多中继线圈无线电能传输系统中,随着中继线圈个数的增加,系统传输功率和效率的最佳传输距离随之增加,但其功率和效率值逐渐减小,系统谐振频率发生频率偏... 详细信息

采用COMSOL Multiphysics软件,对含有多中继线圈结构的无线电能传输系统建模并分析.多中继线圈无线电能传输系统中,随着中继线圈个数的增加,系统传输功率和效率的最佳传输距离随之增加,但其功率和效率值逐渐减小,系统谐振频率发生频率偏移,在近距离会发生明显的频率分裂现象.研究结果表明,在临界耦合距离下,保持各线圈均匀放置在传输系统中,具有较高的功率和效率值.在实际的应用中,要根据需要增加线圈个数,合理设置传输距离这一关键参数.

关键词：无线电能传输中继线圈有限元法

WEAK APPROXIMATIONS OF STOCHASTIC PARTIAL DIFFERENTIAL EQUATIONS WITH FRACTIONAL NOISE

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Journal of Computational Mathematics 2024年第3期42卷 735-754页

作者： Meng Cai Siqing Gan xiaojie Wang School of Mathematics and Statistics HNP-LAMACentral South UniversityChangshaChina

This paper aims to analyze the weak approximation error of a fully discrete scheme for a class of semi-linear parabolic stochastic partial differential equations(SPDEs)driven by additive fractional Brownian motions with the Hurst parameter H∈(1/2,1).The spatial approximation is performed by a spectral Galerkin method and the temporal discretization by an exponential Euler method.As far as we know,the weak error analysis for approximations of fractional noise driven SPDEs is absent in the literature.A key difficulty in the analysis is caused by the lack of the associated Kolmogorov equations.In the present work,a novel and efficient approach is presented to carry out the weak error analysis for the approximations,which does not rely on the associated Kolmogorov equations but relies on the Malliavin calculus.To the best of our knowledge,the rates of weak convergence,shown to be higher than the strong convergence rates,are revealed in the fractional noise driven SPDE setting for the first time.Numerical examples corroborate the claimed weak orders of convergence.

关键词： Parabolic SPDEs Fractional Brownian motion Weak convergence rates Spec-tral Galerkin method Exponential Euler method Malliavin calculus

IQABC-Based Hybrid Deployment Algorithm for Mobile Robotic Agents Providing Network Coverage

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Tsinghua Science and Technology 2024年第2期29卷 589-604页

作者： Shuang Xu xiaojie Liu Dengao Li Jumin Zhao College of Computer Science and Technology(College of Data Science) Taiyuan University of TechnologyTaiyuan 030024China Pengcheng Laboratory Shenzhen 518055China College of Information and Computer Taiyuan University of TechnologyTaiyuan 030024China

Working as aerial base stations,mobile robotic agents can be formed as a wireless robotic network to provide network services for on-ground mobile devices in a target area.Herein,a challenging issue is how to deploy these mobile robotic agents to provide network services with good quality for more users,while considering the mobility of on-ground devices.In this paper,to solve this issue,we decouple the coverage problem into the vertical dimension and the horizontal dimension without any loss of optimization and introduce the network coverage model with maximum coverage range.Then,we propose a hybrid deployment algorithm based on the improved quick artificial bee colony.The algorithm is composed of a centralized deployment algorithm and a distributed one.The proposed deployment algorithm deploy a given number of mobile robotic agents to provide network services for the on-ground devices that are independent and identically distributed.Simulation results have demonstrated that the proposed algorithm deploys agents appropriately to cover more ground area and provide better coverage uniformity.

关键词： wireless robotic networks network coverage deployment algorithm improved quick artificial bee colony

Glutathione-depleted cyclodextrin pseudo-polyrotaxane nanoparticles for anti-inflammatory oxaliplatin(Ⅳ) prodrug delivery and enhanced colorectal cancer therapy

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Chinese Chemical Letters 2024年第4期35卷 280-286页

作者： Wenjia Wang Xingyue He xiaojie Wang Tiantian Zhao Osamu Muraoka Genzoh Tanabe Weijia Xie Tianjiao zhou Lei Xing Qingri Jin Hulin Jiang State Key Laboratory of Natural Medicines China Pharmaceutical UniversityNanjing 210009China Faculty of Pharmacy Kinki University HigashiosakaOsaka 577-8502Japan State Key Laboratory of Natural Medicines(SKLNM)and Department of Medicinal Chemistry School of PharmacyChina Pharmaceutical UniversityNanjing 210009China School of Pharmacy Hangzhou Medical CollegeHangzhou 311399China College of Pharmacy Yanbian UniversityYanji 133002China

Oxaliplatin(Oxa) is the first-line chemotherapeutic drug for the treatment of colorectal cancer(CRC). However, long-term Oxa chemotherapy can induce inflammation and increase the levels of cyclooxygenase-2(COX-2) and prostaglandin E2(PGE2), which can promote tumor metastasis. Moreover,high glutathione(GSH) levels in CRC cells significantly reduce Oxa sensitivity and seriously restrict the clinical application of Oxa. Herein, an Oxa(Ⅳ) prodrug with anti-inflammatory properties(desmethyl naproxe, DN) and GSH-depleting cyclodextrin pseudo-polyrotaxane carriers were prepared and further self-assembled into micellar nanoparticles(designated DNPt@PPRI). The relesae of DN from DNPt@PPRI can reduce the level of PGE2 to inhibit inflammation and tumor metastasis by decreasing COX-2 protein,and also synergize with Oxa to inhibit tumor. More importantly, GSH depletion can reduce the detoxification of Oxa and further enhance chemotherapy-induced apoptosis. DNPt@PPRI have a good GSH depletion ability to enhance the sensitivity of Oxa, indicating a potential in the synergistic chemotherapy and chemo-sensitization of colorectal cancer.

关键词： Oxaliplatin Glutathione depletion Tetravalent platinum prodrug Synergistic therapy Colorectal cancer

PAPS: Progressive Attention-Based Pan-sharpening

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IEEE/CAA Journal of Automatica Sinica 2024年第2期11卷 391-404页

作者： Yanan Jia Qiming Hu Renwei Dian Jiayi Ma xiaojie Guo College of Intelligence and Computing Tianjin UniversityTianjin 300350 China IEEE School of Robotics Hunan UniversityChangsha 410082China Electronic Information School Wuhan UniversityWuhan 430072China

Pan-sharpening aims to seek high-resolution multispectral(HRMS) images from paired multispectral images of low resolution(LRMS) and panchromatic(PAN) images, the key to which is how to maximally integrate spatial and spectral information from PAN and LRMS images. Following the principle of gradual advance, this paper designs a novel network that contains two main logical functions, i.e., detail enhancement and progressive fusion, to solve the problem. More specifically, the detail enhancement module attempts to produce enhanced MS results with the same spatial sizes as corresponding PAN images, which are of higher quality than directly up-sampling LRMS images.Having a better MS base(enhanced MS) and its PAN, we progressively extract information from the PAN and enhanced MS images, expecting to capture pivotal and complementary information of the two modalities for the purpose of constructing the desired HRMS. Extensive experiments together with ablation studies on widely-used datasets are provided to verify the efficacy of our design, and demonstrate its superiority over other state-of-the-art methods both quantitatively and qualitatively. Our code has been released at https://***/JiaYN1/PAPS.

关键词： High-resolution multispectral image image fusion pan-sharpening progressive enhancement

Infrared Photodissociation Spectroscopy of Mass Selected Homoleptic Copper Carbonyl Cluster Cations in the Gas Phase

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Infrared Photodissociation Spectroscopy of Mass Selected Hom...

Fault Analysis on AES:A Property-Based Verification Perspective

第十三届全国化学动力学会议

作者： Jieming Cui xiaojie zhou Guanjun Wang Chaoxian Chi Zhipan Liu Mingfei zhou Department of Chemistry Shanghai Key Laboratory of Molecular Catalysts and Innovative Materials Fudan University

＜正＞Homoleptic transition metal carbonyls have been studied extensively because of their role in organometallic chemistry and catalysis. [1-3] Here, infrared spectra of mass-selected homoleptic copper

关键词： transition metal carbonyl cluster cation infrared photodissociation spectroscopy density functional calculation copper carbonyl

来源： cnki会议评论

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Tsinghua Science and Technology 2024年第2期29卷 576-588页

作者： xiaojie Dai Xingxin Wang Xue Qu Baolei Mao Wei Hu School of Cybersecurity Northwestern Polytechnical UniversityXi’an 710072China School of Cyber Science and Engineering Zhengzhou UniversityZhengzhou 450001China

Fault analysis is a frequently used side-channel attack for cryptanalysis.However,existing fault attack methods usually involve complex fault fusion analysis or computation-intensive statistical analysis of massive fault traces.In this work,we take a property-based formal verification approach to fault analysis.We derive fine-grained formal models for automatic fault propagation and fusion,which establish a mathematical foundation for precise measurement and formal reasoning of fault effects.We extract the correlations in fault effects in order to create properties for fault verification.We further propose a method for key recovery,by formally checking when the extracted properties can be satisfied with partial keys as the search variables.Experimental results using both unprotected and masked advanced encryption standard(AES)implementations show that our method has a key search complexity of 216,which only requires two correct and faulty ciphertext pairs to determine the secret key,and does not assume knowledge about fault location or pattern.

关键词： side-channel attack fault analysis fault propagation model property extraction fault verification

Identification, pathogenicity, and fungicide sensitivity of Eutiarosporella dactylidis associated with leaf blight on maize in China

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Journal of Integrative Agriculture 2024年第3期23卷 888-900页

作者： Cheng Guo xiaojie Zhang Baobao Wang Zhihuan Yang Jiping Li Shengjun Xu Chunming Wang Zhijie Guo Tianwang zhou Liu Hong Xiaoming Wang Canxing Duan Institute of Plant Protection Gansu Academy of Agricultural SciencesLanzhou 730070China Pratacultural College Gansu Agricultural UniversityLanzhou 730070China Shijiazhuang Academy of Agriculture and Forestry Sciences Shijiazhuang 050050China Institute of Crop Sciences Chinese Academy of Agricultural SciencesBejing 100081China

Maize(Zea mays L.) is an economically vital grain crop that is cultivated worldwide. In 2011, a maize foliar disease was detected in Lingtai and Lintao counties in Gansu Province, China. The characteristic signs and symptoms of this disease include irregular chlorotic lesions on the tips and edges of infected leaves and black punctate fruiting bodies in dead leaf tissues. Given favourable environmental conditions, this disease spread to areas surrounding Gansu. In this study, infected leaves were collected from Gansu and Ningxia Hui Autonomous Region between 2018and 2020 to identify the disease-causing pathogen. Based on morphological features, pathogenicity tests, and multilocus phylogenetic analysis involving internal transcribed spacer(ITS), 18S small subunit rDNA(SSU), 28S large subunit rDNA(LSU), translation elongation factor 1-alpha(TEF), and β-tubulin(TUB) sequences, Eutiarosporella dactylidis was identified as the causative pathogen of this newly discovered leaf blight. Furthermore, an in vitro bioassay was conducted on representative strains using six fungicides, and both fludioxonil and carbendazim were found to significantly inhibit the mycelial growth of E. dactylidis. The results of this study provide a reference for the detection and management of Eutiarosporella leaf blight.

关键词： maize leaf blight morphology molecular phylogeny Eutiarosporella dactylidis fungicide sensitivity