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Efficient and selective recovery of Gd(Ⅲ)via polyethyleneimine modification of lanthanum-based metal-organic frameworks

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Journal of Rare Earths 2024年第1期42卷 210-219,I0007页

作者： Wenhao li lijinhong Huang Bin xiao xiaoguang Duan Haike li Lang li Wanfu Huang Ganzhou Key Laboratory of Basin Pollution Simulation and Control Jiangxi University of Science and TechnologyGanzhou341000China Innovation Center for Water Quality Security Technology at Ganjiang River Basin Jiangxi University of Science and TechnologyGanzhou341000China Faculty of Science and Engineering WA School of Mines:MineralsEnergy and Chemical EngineeringCurtin UniversityWAAustralia School of Architecture and Design Jiangxi University of Science and TechnologyGanzhou341000China School of Resources and Architectural Engineering Gannan University of Science and TechnologyGanzhou341000China School of Chemical Engineering and Advanced Materials The University of AdelaideAdelaideSA5005Australia School of Resource and Environmental Engineering Jiangxi University of Science and TechnologyGanzhou341000China

With the development of the economy and the increasing demand for environmental protection,the efficient and selective recovery of Gd(Ⅲ)from actual wastewater is of critical *** this work,lanthanum-based metal-organic framework(LaBDC)materials were prepared by a hydrothermal method,and then polyethyleneimine(PEI)and LaBDC were combined by an impregnation method to form a novel LaBDC@xPEI *** prepared materials were characterized using Fourier transfo rm infrared spectroscopy(FTIR),X-ray diffraction(XRD),scanning electron microscopy(SEM),energy dispersive X-ray spectroscopy(EDX),B runauer-Emmett-Teller(BET),thermogravimetric analysis(TGA)and X-ray photoelectron spectroscopy(XPS).Experiments show that LaBDC@50%PEI has the highest adsorption capacity(181.77 mg/g)among lanthanum-based MOFs with different PEI loadings at pH=5.5,which is about 5.1 times that of bare *** adsorption isotherm analysis shows that LaBDC@50%PEI follows the Langmuir *** addition,the adsorption kinetics of LaBDC@50%PEI follows a pseudo-second-order kinetic model,indicating that the adsorption process is chemical *** is worth noting that LaBDC@50%PEI maintains good adsorption performance and stability after three recycling tests,and exhibits excellent selectivity in cation interference ***,the LaBDC@50%PEI composites possess good stability and hold great promises in rapid recovery of Gd(Ⅲ)from practical aqueous environments.

关键词： Wet-impregnation method Polyethylene imine Metaleorganic frameworks Lanthanum Recovery of Gd(Ⅲ) Rare earths

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Sliced Average Variance Estimation for Tensor Data

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Acta Mathematicae Applicatae Sinica 2024年第3期40卷 630-655页

作者： Chuan-quan li Pei-wen xiao Chao Ying xiao-hui liU School of Statistics Jiangxi University of Finance and EconomicsNanchang 330013China Key Laboratory of Data Science in Finance and Economics Jiangxi University of Finance and EconomicsNanchang 330013China Biostatistics and Medical Informatics University of Wisconsin MadisonMadison 53726USA

Tensor data have been widely used in many fields,e.g.,modern biomedical imaging,chemometrics,and economics,but often suffer from some common issues as in high dimensional *** to find their low-dimensional latent structure has been of great interest for *** this end,we develop two efficient tensor sufficient dimension reduction methods based on the sliced average variance estimation(SAVE)to estimate the corresponding dimension reduction *** first one,entitled tensor sliced average variance estimation(TSAVE),works well when the response is discrete or takes finite values,but is not■consistent for continuous response;the second one,named bias-correction tensor sliced average variance estimation(CTSAVE),is a de-biased version of the TSAVE *** asymptotic properties of both methods are derived under mild *** and real data examples are also provided to show the superiority of the efficiency of the developed methods.

关键词： tensor data sliced average variance estimation sufficient dimension reduction central subspace

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Study on impedance spectroscopy based on dynamic equivalent circuit of solar cell

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Optoelectronics Letters 2024年第8期20卷 449-453页

作者： xiao Wenbo li Ao WU Huaming li Yongbo xiao Bangzhi Key Laboratory of Nondestructive Testing Ministry of EducationNanchang Hangkong UniversityNanchang 330063China Jiangxi Engineering Laboratory for Optoelectronics Testing Technology Nanchang 330063China College of Science and Technology Nanchang Hangkong UniversityGongqingcheng 332020China School of Engineering and Construction Nanchang UniversityNanchang 330031China

This paper investigates the impedance spectroscopy of monocrystalline silicon solar cells(MSSC)and dye-sensitized solar cells(DSSC)using solar cell dynamic equivalent resistor-capacitance(RC)and capacitor sum capacitor(CSC)***,these circuits effectively represent the dynamic behavior of MSSC and ***,the measurement method significantly impacts the accuracy of impedance measurements in the high-frequency ***,the series resistance affects the distance between the left end of the impedance spectroscopy and the origin,while the parallel resistance influences the size of the impedance *** the CSC circuit,the relative magnitudes of dielectric relaxation capacitance and chemical capacitance affect the number and position of arc in the impedance *** value of the dielectric relaxation capacitor determines the number of impedance spectroscopy *** conclusions provide guidelines for improving the accuracy of solar cell impedance measurements.

关键词： spectroscopy impedance capacitance

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Uniqueness on Difference Operators of Meromorphic Functions of Infinite Order

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Acta Mathematica Sinica,English Series 2024年第2期40卷 511-527页

作者： Hui li Ming liang FANG xiao YAO School of Science China University of Mining and TechnologyBeijing 100083P.R.China Institute of Mathematics Academy of Mathematics and System SciencesChinese Academy of SciencesBeijing 100190P.R.China School of Sciences Hangzhou Dianzi UniversityHangzhou 310012P.R.China School of Mathematical sciences and LPMC Nankai UniversityTianjin 300071P.R.China

We investigate the uniqueness problems of meromorphic functions and their difference operators by using a new *** is proved that if a non-constant meromorphic function f shares a non-zero constant and ∞ counting multiplicities with its difference operators Δcf(z) and Δ_(c)^(2)f(z), thenΔcf(z)≡Δ_(c)^(2)f(z).In particular,we give a difference analogue of a result of *** method has two distinct features:(ⅰ) It converts the relations between functions into the corresponding *** makes it possible to deal with the uniqueness problem by linear algebra and combinatorics.(ⅱ) It circumvents the obstacle of the difference logarithmic derivative lemma for meromorphic functions of infinite order,since this method does not depend on the growth of the ***,the idea in this paper can also be applied to the case for several variables.

关键词： Uniqueness meromorphic functions difference operators infinite order

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DepthGAN: GAN-based depth generation from semantic layouts

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Computational Visual Media 2024年第3期10卷 505-522页

作者： Yidi li Jun xiao Yiqun Wang Zhengda Lu School of Artificial Intelligence University of Chinese Academy of SciencesBeijingChina College of Computer Science Chongqing UniversityChongqingChina

Existing GAN-based generative methodsare typically used for semantic image synthesis. Wepose the question of whether GAN-based architecturescan generate plausible depth maps and find thatexisting methods have difficulty in generating depthmaps which reasonably represent 3D scene structuredue to the lack of global geometric ***, we propose DepthGAN, a novel method ofgenerating a depth map using a semantic layout asinput to aid construction, and manipulation of wellstructured 3D scene point clouds. Specifically, wefirst build a feature generation model with a cascadeof semantically-aware transformer blocks to obtaindepth features with global structural *** our semantically aware transformer block, wepropose a mixed attention module and a semanticallyaware layer normalization module to better exploitsemantic consistency for depth features ***, we present a novel semantically weighteddepth synthesis module, which generates adaptivedepth intervals for the current scene. We generate thefinal depth map by using a weighted combination ofsemantically aware depth weights for different depthranges. In this manner, we obtain a more accuratedepth map. Extensive experiments on indoor andoutdoor datasets demonstrate that DepthGAN achievessuperior results both quantitatively and visually for thedepth generation task.

关键词： depth map generation generative model transformer scene generation

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Signifying quantum uncertainty relations by optimal observable sets and the tightest uncertainty constants

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Science China(Physics,Mechanics & Astronomy) 2024年第9期67卷 43-50页

作者： xiao-Bin liang Bo li Shao-Ming Fei School of Mathematics and Computer Science Shangrao Normal UniversityShangrao 334001China Quantum Information Research Center Shangrao Normal UniversityShangrao 334001China School of Mathematical Sciences Capital Normal UniversityBeijing 100048China

Quantum uncertainty relations constrain the precision of measurements across multiple non-commuting quantum mechanical ***,we introduce the concept of optimal observable sets and define the tightest uncertainty constants to accurately describe these measurement *** any quantum state,we establish optimal sets of three observables for both product and summation forms of uncertainty relations,and analytically derive the corresponding tightest uncertainty *** demonstrate that the optimality of these sets remains consistent regardless of the uncertainty relation ***,the existence of the tightest constants excludes the validity of standard real quantum mechanics,underscoring the essential role of complex numbers in this ***,our findings resolve the conjecture posed in[***.118,180402(2017)],offering novel insights and potential applications in understanding preparation uncertainties.

关键词： uncertainty relation the tightest uncertainty constants optimal observable sets

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mRNA vaccine technology for infectious diseases and beyond

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Science China(life Sciences) 2024年第10期67卷 2267-2270页

作者： Pei Hao xiao li Xuan li Wu Zhong Key Laboratory of Molecular Virology and Immunology Shanghai Institute of Immunity and InfectionChinese Academy of SciencesShanghai 200031China Changchun Veterinary Research Institute Chinese Academy of Agricultural SciencesChangchun 130122China Key Laboratory of Synthetic Biology CAS Center for Excellence in Molecular Plant SciencesInstitute of Plant Physiology and EcologyChinese Academy of SciencesShanghai 200032China National Engineering Research Center for the Emergency Drug Beijing Institute of Pharmacology and ToxicologyBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China

The rise of mRNA vaccine technology Vaccines stand as one of the most significant medical advancements,playing a crucial role in the prevention of infectious diseases and the improvement of global *** triumph of smallpox vaccination stands as a towering achievement in the annals of healthcare,leading to the complete elimination of a oncedevastating disease and showcasing the efficacy of vaccination methods.

关键词： methods vaccination prevention

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Sustainable Intensification and Large-scale Operation of Cultivated Land Use at the Farmers’ Scale:A Case Study of Shandong Province,China

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Chinese Geographical Science 2024年第1期34卷 149-167页

作者： li li LYU xiao ZHANG Anlu NIU Shandong PENG Wenlong School of Public Administration Huazhong Agricultural UniversityWuhan430070China Department of Geography University of ZurichZurich8057Switzerland School of Humanities and Law Northeastern UniversityShenyang110169China School of Geography and Tourism Qufu Normal UniversityRizhao276800China

Sustainable intensification of cultivated land use(SICLU) and large-scale operations(LSO) are widely acknowledged strategies for enhancing agricultural ***,the existing literature has faced challenges in precisely defining SICLU and constructing comprehensive indicators,which has hindered the exploration of factors influencing LSO within the SICLU *** address this gap,we integrated self-efficacy theory into the design of an index framework for evaluating *** subsequently employed econometric models to analyze the significant factors that impact *** findings reveal that SICLU can be divided into four key dimensions:intensive management,efficient output,resource conservation,and ecological environment ***,it is crucial to incorporate belief-based cognitive factors into the index system,as farmers’ understanding of fertilizer and pesticide application significantly influences their willingness to engage in ***,we identify grain market turnover as the most influential factor in promoting LSO,with single-factor contribution rates reaching 70.9% for cultivated land transfer willingness and 62.5% for the total planting ***,unlike irrigation and agricultural machinery inputs,increased labor inputs correspond to larger planting areas for *** trend may be attributed to reduced labor availability because of rural labor migration,whereas the reduction in irrigation and agricultural input is contingent on innovations in production practices and the transfer of cultivated land management ***,SICLU dynamically influences LSO,with each index related to SICLU having an optimal range that fosters *** insights offer valuable guidance for policymakers,emphasizing farmers as their central focus,with the adjustment of input and output factors as a means to achieve LSO as the ultimate *** conclusion,we propose research avenues for further enriching the SICLU framework to ensur

关键词： sustainable intensification of cultivated land use(SICLU) self-efficacy status quo bias input and output Boosted Regression Tree willingness to transfer cultivated land cultivated land planting areas Shandong,China

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Local environment regulation of transition metal dichalcogenide-based single-atom catalysts

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Rare Metals 2024年第9期43卷 4019-4037页

作者： Ming-Hui li Jing li xiao-Yu Zheng Yao Zhou Advanced Research Institute of Multidisciplinary Science and School of Chemistry and Chemical Engineering Beijing Institute of TechnologyBeijing 100081China Laser Micro/Nano Fabrication Laboratory School of Mechanical EngineeringBeijing Institute of TechnologyBeijing 100081China

Single-atom catalysts have risen significant attention in the realm of green electrocatalytic energy conversion to address energy and environmental sustainability *** metal dichalcogenide(TMD)-based single-atom catalysts are considered highly effective in electrocatalysis due to the TMDs'notable specific surface area,tunable elemental species and efficient utilization of single *** order to enhance electrocatalytic performance,it is imperative to elaborately engineer the local environment surrounding the active sites of single atoms within *** this review,we initially explore the effects of synthesis methods on single-atom active sites and the influence of loading of single atoms on catalytic performance for *** modulation strategies of the local environment surrounding single-atom sites in TMDs are elaborated,including substitution engineering,surface adsorption,vacancies,spatial confinement and dual-atom site *** each modulation strategy,the effects of diverse local environments on various electrocatalytic applications are presented,such as the oxygen evolution reaction,oxygen reduction reaction,nitrogen reduction reaction,CO_(2)reduction reaction and CO ***,this study presents a comprehensive overview of the challenges encountered and the potential directions for the advancement of single-atom catalysts based on TMDs in the realm of electrocatalysis.

关键词： Single-atom catalysts Transition metal dichalcogenide Local environment Electrocatalysis

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The Response of Carbonate System to Watershed Urbanization Process in a Semi-Arid River

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Journal of Ocean University of China 2024年第4期23卷 991-1002页

作者： li Yunxiao DANG Jiajia HUANG xiao YANG Hong WANG xiao li lina BAI Jie CHEN Xi Department of Environmental Science College of Resource and EnvironmentShanxi Agricultural UniversityTaigu 030801China Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control Collaborative Innovation Center of Atmospheric Environment and Equipment TechnologySchool of Environmental Science and EngineeringNanjing University of Information Science and TechnologyNanjing 210044China Department of Geography and Environmental Science University of ReadingWhiteknightsReading RG66ABUK Marine Agriculture Research Center Tobacco Research InstituteChinese Academy of Agricultural SciencesQingdao 266101China 5 Key Laboratory of Marine Environmental Science and Ecology Ministry of EducationCollege of Environmental Science and EngineeringOcean University of ChinaQingdao 266100China

Different from rivers in humid areas,the variability of riverine CO_(2) system in arid areas is heavily impacted by anthropogenic disturbance with the increasing urbanization and water *** this study,the water chemistry and the controls of carbonate system in an urbanized river(the Fenhe River)on the semi-arid Loess Plateau were *** water chemistry of the river water showed that the high dissolved inorganic carbon(DIC)concentration(about 37 mg L^(-1))in the upstream with a karst land type was mainly sourced from carbonate weathering involved by H_(2)CO_(3) and H_(2)SO_(4),resulting in an oversaturated partial pressure of CO_(2)(pCO_(2))(about 800μatm).In comparison,damming resulted in the widespread appearance of non-free flowing river segments,and aquatic photosynthesis dominated the DIC and pCO_(2) spatiality demonstrated by the enriched stable isotope of DIC(δ^(13)CDIC).Especially in the mid-downstream flowing through major cities in warm and low-runoff August,some river segments even acted as an atmospheric CO_(2) *** noteworthy is wastewater input leading to a sudden increase in DIC(>55 mg L^(-1))and pCO_(2)(>4500μatm)in the downstream of Taiyuan City,and in cold November the increased DIC even extended to the outlet of the *** results highlight the effects of aquatic production induced by damming and urban sewage input on riverine CO_(2) system in semi-arid areas,and reducing sewage discharge may mitigate CO_(2) emission from the rivers.

关键词： dissolved inorganic carbon stable carbon isotope carbonate weathering aquatic photosynthesis sewage input the Fenhe River

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