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Unconventional Fluorescent and Multi-responsive Polysiloxane:Synthesis,Characterization and Biological Applications

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Chinese Journal of Polymer Science 2024年第5期42卷 579-590,I0006页

作者： xiao-Di li Shu-Sheng li Xu-Bao Jiang xiao-li Zhu Xiang Zheng Kong College of Chemistry and Chemical Engineering University of JinanJinan250022China College of Chemical Engineering Tianjin UniversityTianjin300072China Foshan(Southern China)institute for New Materials Foshan528200China

Owing to their high significance in fundamental study and diverse applications,stimuli-responsive and fluorescent polymers,particularly those with cluster-triggered emission(CTE)featured by non-conjugated chromophores,have drawn tremendous attention in recent *** this work,fluorescent and multi-responsive polysiloxane(FRPS)was synthesized by hydrolytic condensation polymerization of 3-aminopropyl methyl diethoxysilane(APMS)with 3-(N-isopropyl propionamide)iminopropyl methyl diethoxysilane(APMS-NiP),which was formed in situ through aza-Michael addition between APMS and N-isopropyl *** was not only highly sensitive to temperature,pH and CO_(2) in water,but also showed an enhanced and stimuli-adjustable fluorescence *** effects of monomer feeding,pH and CO_(2) on its lower critical solution temperature and fluorescent property were *** fluorescence emission was ascribed to CTE *** addition,FRPS was shown to be highly potential as physiological indicator for cell imaging,and for controlled release and trace detection of *** study provides therefore a type of stimuli-responsive and fluorescent material for potential applications in biomedical fields,and it is also of great significance for understanding of the fluorescence mechanism of polysiloxane-based stimuli-responsive polymers.

关键词： Polysiloxane Multi-responsiveness Cluster-triggered emission Cell imaging Controlled drug release

Effects of microplastic polystyrene,simulated acid rain and arbuscular mycorrhizal fungi on Trifolium repens growth and soil microbial community composition

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Pedosphere 2024年第2期34卷 424-437页

作者： Wanlin li Yan xiao College of Agro-grassland Science Nanjing Agricultural UniversityNanjing 210095China

Microplastic pollution is a global and ubiquitous environmental problem in the oceans as well as in the terrestrial *** examined the fate of microplastic polystyrene(MPS)beads in experimental soil in the presence and absence of symbiotic arbuscular mycorrhizal fungi(AMF)and simulated acid rain(SAR)to determine whether the combinations of these three factors altered the growth of white clover Trifolium *** found that MPS,SAR,or AMF added singly to soil did not alter *** growth or *** contrast,MPS and AMF together significantly reduced shoot biomass,while SAR and MPS together significantly reduced soil available phosphorus independent of AMF *** polystyrene,AMF,and SAR together significantly reduced soil NO_(3)^(-)-*** mycorrhizal fungi added singly also enriched the beneficial soil bacteria(genus Solirubrobacter),while MPS combined with AMF significantly enriched the potential plant pathogenic fungus *** mycorrhizal fungi inoculation with MPS increased the abundance of soil hydrocarbon degraders independent of the presence of *** addition,the abundance of soil nitrate reducers was increased by MPS,especially in the presence of AMF and ***,SAR alone increased the abundance of soil pathogens within the fungal community including antibiotic *** findings indicate that the coexistence of MPS,SAR,and AMF may exacerbate the adverse effects of MPS on soil and plant health.

关键词： acid deposition arbuscular mycorrhizal fungi symbiosis hydrocarbon degradation microbial alpha diversity microplastic pollution pathogen

Higher-order expansions of powered extremes of logarithmic general error distribution

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Applied Mathematics(A Journal of Chinese Universities) 2024年第1期39卷 47-54页

作者： TAN xiao-feng li li-hui School of Mathematics and Statistics Southwest UniversityChongqing 400715China

in this paper,Let M_(n)denote the maximum of logarithmic general error distribution with parameter v≥***-order expansions for distributions of powered extremes M_(n)^(p)are derived under an optimal choice of normalizing *** is shown that M_(n)^(p),when v=1,converges to the Frechet extreme value distribution at the rate of 1/n,and if v>1 then M_(n)^(p)converges to the Gumbel extreme value distribution at the rate of(loglogn)^(2)=(log n)^(1-1/v).

关键词： logarithmic general error distribution convergence rate higher-order expansion powered ex-treme

Analysis of Piezoelectric Semiconductor Structures Considering Both Physical and Geometric Nonlinearities

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Acta Mechanica Solida Sinica 2024年第1期37卷 72-81页

作者： Zhengguang xiao Shuangpeng li Chunli Zhang Key Laboratory of Soft Machines and Smart Devices of Zhejiang Province Department of Engineering MechanicsZhejiang UniversityHangzhou 310027China Huanjiang Laboratory Zhuji 311816China

Piezoelectric semiconductors(PSs),such as ZnO and GaN,known as the third-generation semiconductors,have promising applications in electronic and optoelectronic devices due to the coexistence and interaction of piezoelectricity and semiconductor *** modeling of PS structures under external loads,such as thermal and mechanical loads,plays a crucial role in the design of PS *** this work,we propose a nonlinear fully coupling theoretical model and investigate the multi-field coupling behaviors of PS structures and PN junctions under thermal and mechanical loads,considering physical and geometric *** electromechanical and semiconducting behaviors of a PS rod-like structure with flexural deformations under different combinations of temperature changes and mechanical loads are *** tuning effect of temperature changes and mechanical loads on multi-field coupling behaviors of PSs is *** current–voltage characteristics of PS PN junctions are studied under different combinations of temperature changes and mechanical *** obtained results are helpful for the development of novel PS devices.

关键词： Piezoelectric semiconductor Nonlinearity Multi-field Coupling Tuning

Proposing a development framework for sustainable architecture, engineering, and construction industry in China: Challenges, best practice, and future directions

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Frontiers of Structural and Civil Engineering 2024年第5期18卷 805-814页

作者： Peixian li Yujie LU Xuwen xiao College of Architecture and Urban Planning Tongji UniversityShanghai 200092China Key Laboratory of Ecology and Energy Saving Study of Dense Habitat(Tongji University) Ministry of EducationShanghai 200092China College of Civil Engineering Tongji UniversityShanghai 200092China Key Laboratory of Performance Evolution and Control for Engineering Structures of Ministry of Education Tongji UniversityShanghai 200092China China State Construction Engineering Corporation Beijing 100029China

China’s architecture,engineering,and construction(AEC)industry needs a clear and sustainable development *** inspiration from speeches delivered at a seminar hosted by the Chinese Academy of Engineering and extensive literature research on Chinese policies,this article presents a summary of the current trends in the AEC industry in four dimensions:industrialization as the foundation,intelligence as the enabler,lean management as the strategy,and green development as the *** four dimensions are intricately interconnected and rooted in multiple *** article provides a detailed review of the current practices,challenges,and future directions associated with each ***,ten grand challenges were proposed to stimulate discussions on the future of the AEC *** article offers an overarching understanding of the AEC industry and presents a four-dimension framework for sustainable development,which can be valuable for AEC practitioners.

关键词： green building lean construction prefabrication smart construction sustainable development

A Fluctuation Test for Structural Change Detection in Heterogeneous Panel Data Models

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Journal of Systems Science & Complexity 2024年第3期37卷 1184-1208页

作者： li Fuxiao xiao Yanting CHEN Zhanshou Department of Applied Mathematics Xi'an University of TechnologyXi'an 710048China School of Mathematics and Statistics Qinghai Normal UniversityXining 810008China Academy of Plateau Science and Sustainability Xining 810008China

Structural change in panel data is a widespread phenomena. This paper proposes a fluctuation test to detect a structural change at an unknown date in heterogeneous panel data models with or without common correlated effects. The asymptotic properties of the fluctuation statistics in two cases are developed under the null and local alternative hypothesis. Furthermore, the consistency of the change point estimator is proven. Monte Carlo simulation shows that the fluctuation test can control the probability of type i error in most cases, and the empirical power is high in case of small and moderate sample sizes. An application of the procedure to a real data is presented.

关键词： Common correlated effects fuctuation test heterogeneous panel data models structural change detection

Study on Effectiveness of Solitary-Wave-like Form Based on Overtopping Data from irregular Wave Tests

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China Ocean Engineering 2024年第4期38卷 701-710页

作者： li xiao-liang Huang Gui-biao School of Naval Architecture&Ocean Engineering Jiangsu University of Science and TechnologyZhenjiang 212100China

The previous study conducted by li(2022)demonstrates that the Goda graph can be adequately represented by a solitary-wave-like form across the entire range of relative water depth,with the exception of the extremely shallow ***,it remains uncertain whether this form is equally effective when applied to test data generated by irregular waves,as the Goda graph was initially developed based on overtopping data from regular wave ***,it is unclear whether this form is suitable for formulating overtopping discharge at composite vertical *** order to address these questions,a 2D overtopping experiment was conducted,incorporating both simple and composite types of vertical walls,with various relative water depths across the entire range,excluding the extremely shallow zone.A novel analysis procedure was developed,which proved to be highly productive and can be considered a general method for data ***,the study yielded two conclusions:(1)the solitary-wave-like form is remarkably effective in formulating overtopping test data generated by irregular waves,regardless of whether the vertical wall is simple or composite,and(2)the resulting formulas exhibit definitely better performance compared with existing formulas.

关键词： solitary-wave-like form overtopping discharge overtopping formula vertical wall

Meta label associated loss for fine-grained visual recognition

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Science China(information Sciences) 2024年第6期67卷 230-247页

作者： Yanchao li Fu xiao Hao li Qun li Shui YU School of Computer Science Nanjing University of Posts and Telecommunications School of Network Engineering Zhoukou Normal University School of Computer Science University of Technology Sydney

Recently, intensive attempts have been made to design robust models for fine-grained visual recognition, most notably are the impressive gains for training with noisy labels by incorporating a reweighting strategy into a meta-learning framework. However, it is limited to up or downweighting the contribution of an instance for label reweighting approaches in the learning process. To solve this issue, a novel noise-tolerant method with auxiliary web data is proposed. Specifically, first, the associations made from embeddings of well-labeled data with those of web data and back at the same class are measured. Next, its association probability is employed as a weighting fusion strategy into angular margin-based loss, which makes the trained model robust to noisy datasets. To reduce the influence of the gap between the well-labeled and noisy web data, a bridge schema is proposed via the corresponding loss that encourages the learned embeddings to be coherent. Lastly, the formulation is encapsulated into the meta-learning framework, which can reduce the overfitting of models and learn the network parameters to be noise-tolerant. Extensive experiments are performed on benchmark datasets, and the results clearly show the superiority of the proposed method over existing state-of-the-art approaches.

关键词： label associated loss weighting noisy samples fine-grained visual recognition noise-tolerant learning meta-learning

Crashworthiness Design and Multi-Objective Optimization of Bionic Thin-Walled Hybrid Tube Structures

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Computer Modeling in Engineering & Sciences 2024年第4期139卷 999-1016页

作者： Pingfan li Jiumei xiao Department of Applied Mechanics University of Sciences and Technology BeijingBeijing100083China

Thin-walled structures are widely used in cars due to their lightweight construction and energy-absorbing ***,issues such as high initial stress and lowenergy-absorbing efficiency *** study proposes a novel energy-absorbing structure inwhich a straight tube is combinedwith a conical tube and a bamboo-inspired bulkhead structure is *** configuration allows the conical tube to flip outward first and then fold together with the straight *** deformation mode absorbs more energy and less peak force than the conical tube sinking and flipping *** finite element numerical simulation,the specific energy absorption capacity of the structure is increased by 26%compared to that of a regular circular cross-section ***,the impact resistance of the bionic straight tapered tube structure is further improved through multi-objective optimization,promoting the engineering application and lightweight design of hybrid cross-section tubes.

关键词： Crashworthiness tube inversion multi-objective optimization energy absorption