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Elaborating strengthen mechanism of Pt-Ir solid solution superalloy at finite temperature

Rare Metals 2024年第3期43卷 1243-1256页

作者： Wei yu xiao-yu chong yun-Xuan Zhou Meng-Di Gan Ying-Xue Liang Yan Wei Ai-Min Zhang Chang-Yi Hu Xing-yu Gao Li Chen Hai-Feng Song Jing Feng Faculty of Materials Science and Engineering Kunming University of Science and TechnologyKunming650093China yunnan Precious Metals Laboratory Co.LTD Kunming650106China Laboratory of Computational Physics Institute of Applied Physics and Computational MathematicsBeijing100088China

Pt-Ir alloy is potential superalloys used above 1300℃because of their high strength and creep ***,the ductility of Pt-Ir alloy has rapidly deteriorated with the increase of Ir,resulting in poor *** work quantitatively evaluated the solid solution strengthening(SSS)and grain refinement strengthening(GRS)of Pt-Ir alloy using first-principles calculations combined with experimental ***,the stretching force constants in the second nearest neighbor region(SFC^(2nd))of pure Ir(193.7 eV·nm^(-2))are 3.40 times that of pure Pt(57.0 eV·nm^(-2)),i.e.,the interatomic interaction is greatly enhanced with the increase of Ir content,which leads to the decrease of ductility,and modulus misfit plays a dominant role in ***,the physical mechanisms responsible for the hardness(H_(V))of Pt-Ir alloy,using the power-law-scaled function of electron work function coupled SSS and GRS,are attributed to the electron redistribution caused by different Ir ***,a thorough assessment of the thermodynamic characteristics of Pt-Ir binary alloy was conducted,culminating in development of a mapping model that effectively relates enmposition,temperature and *** results revealed that the compressive strength incrcases with the Ir content,and the highest strength was observed in Pt_(0.25)Ir_(0.75).This study provides valuable insights into the Pt-Ir alloy system.

关键词： Elastic properties Phonon Solid solution strengthen Force constants CALPHAD

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Properties of Fe-Mn-Al alloys with different Mn contents using density functional theory

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Rare Metals 2023年第4期42卷 1387-1397页

作者： Xiang Luo Jing Feng Ya-Hui Liu Ming-yu Hu xiao-yu chong Ye-Hua Jiang Faculty of Materials Science and Engineering Kunming University of Science and TechnologyKunming650093China

The chemical stability,electronic structures,mechanical properties and Debye temperature of Fe-MnAl alloys were investigated using first-principles *** formation enthalpy and cohesive energy are negative for Fe-Mn-Al alloys,showing that they are thermodynamically *** has the lowest formation enthalpy,indicating that FeAl is the most stable alloy in the Fe-Mn-Al *** partial density of states,total density of states and electron density distribution maps were used to analyze the physical properties of the Fe-MnAl alloys.A combination of mainly covalent and metallic bonds exists in these Fe-Mn-Al alloys,resulting in good electronic conductivity,high melting points,and high *** alloys display disparate anisotropy due to the calculated different shapes of the 3D curved surface of the Young's modulus and anisotropic *** has the highest bulk modulus,shear modulus and Yong's modulus of 187.1,119.8 and 296.2 GPa,***,the Debye temperatures and sound velocity of these Fe-Mn-Al compounds were explored.

关键词： Fe-Mn-Al alloys Electronic structures Stability Mechanical properties Debye temperature First-principles calculation

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Changes of alloying elements on elasticity and solid solution strengthening ofα-Ti alloys:a comprehensive high-throughput first-principles calculations

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Rare Metals 2022年第8期41卷 2719-2731页

作者： Tao Liu xiao-yu chong Wei yu yun-Xuan Zhou Hai-Guang Huang Rong-Feng Zhou Jing Feng Faculty of Material Science and Engineering Kunming University of Science and TechnologyKunming650093China yunnan Titanium Industry Co.Ltd Chuxiong675000China City College Kunming University of Science and TechnologyKunming650051China

Herein,the effects of 33 alloying elements on the elastic properties and solid solution strengthening(SSS)of a-Ti alloys were systematically studied via first-principles calculations based on a dilute solid *** alloying elements in these calculations were thermodynamically favorable,which indicated that these elements could be dissolved inα-Ti ***_(35)Os had the highest elastic modulus as compared to those of other dilute Tibased solid ***,Co,and Pt were found to be promising candidates for improving the ductilities ofα-Ti solid solution *** solution strengthening was analyzed using Cottrell's and Labush's *** on the solid solubility,Ir,Rh,Ni,and Pt were found to possess the best solid solution hardening effects in the following order:Ir>Rh>Ni>*** bonding state between Ti and the impurity atom was visually characterized owing to the difference between their charge *** integrating the calculations of mean bond length and mean population,the results showed that Ti-Os had the largest mean population and degree of delocalization of the electron cloud around the solute atom,implying ionic characteristics of Os and ***,after analyzing the alloying elements of each group,we found thatⅧ-group elements(Ru,Rh,Pd,Os,Ir,Pt)had good potentials for improving the comprehensive mechanical properties of Ti alloys.

关键词： Thermodynamics First-principles calculations Mechanical properties Titanium alloys Electronic structure

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Numerical and experimental study on the falling film flow characteristics with the effect of co-current gas flow in hydrogen liquefaction process

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Petroleum Science 2024年第2期21卷 1369-1384页

作者： chong-Zheng Sun yu-Xing Li Hui Han xiao-Yi Geng xiao Lu College of Energy Storage Technology Shandong University of Science and TechnologyQingdao 266590ShandongChina College of Pipeline and Civil Engineering/Shandong Provincial Key Laboratory of Oil&Gas Storage and Transportation Safety China University of PetroleumQingdao 266580ShandongChina

Liquid hydrogen storage and transportation is an effective method for large-scale transportation and utilization of hydrogen energy. Revealing the flow mechanism of cryogenic working fluid is the key to optimize heat exchanger structure and hydrogen liquefaction process(LH2). The methods of cryogenic visualization experiment, theoretical analysis and numerical simulation are conducted to study the falling film flow characteristics with the effect of co-current gas flow in LH2spiral wound heat *** results show that the flow rate of mixed refrigerant has a great influence on liquid film spreading process, falling film flow pattern and heat transfer performance. The liquid film of LH2mixed refrigerant with column flow pattern can not uniformly and completely cover the tube wall surface. As liquid flow rate increases, the falling film flow pattern evolves into sheet-column flow and sheet flow, and liquid film completely covers the surface of tube wall. With the increase of shear effect of gas-phase mixed refrigerant in the same direction, the liquid film gradually becomes unstable, and the flow pattern eventually evolves into a mist flow.

关键词： Hydrogen liquefaction Spiral wound heat exchanger Flow pattern transition Falling film flow

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Metal-organic frameworks on 3D interconnected macroporous sponge foams for large-scale water decontamination:A mini review

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Chinese Chemical Letters 2024年第5期35卷 77-84页

作者： xiao-Hong Yi chong-Chen Wang Beijing Key Laboratory of Functional Materials for Building Structure and Environment Remediation School of Environment and Energy EngineeringBeijing University of Civil Engineering and ArchitectureBeijing 100044China

Water pollution caused by global population growth,urban expansion and industrialization development is one of the urgent issues that need to be addressed in the 21st *** to now,it was challenging for metal-organic frameworks(MOFs)to be used in the actual water treatment due to that the powder MOFs suffered from difficult reuse,poor water stability and easy *** is an effective strategy to immobilize MOFs powder onto porous sponge foam carriers for accomplishing large flux,facile recycling,easy processing water treatment *** this review article,the fabrication approaches and applications of different MOFs/sponge composites were highlighted,in which the fluorescence detection of pollutants,adsorption and separation of pollutants,catalytic reduction and oxidation of pollutants were ***,the future challenges and opportunities of MOF/sponge for water treatment are proposed,aiming to provide in-depth guidance for the future design and manufacture of the immobilized MOFs onto sponge foams.

关键词： Metal-organic frameworks Sponge foam Water decontamination Adsorption Catalysis

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Deciphering dynamic surface of PtRu alloy nanocatalysts to revisit their synergistic effects during the electrooxidation

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Science China Chemistry 2024年第7期67卷 2224-2233页

作者： xiao-chong Li Bo Wang Zhou yu Qiang Wan Ju-Fang Zheng Emmanuel Maisonhaute xiao-Shun Zhou Ya-Hao Wang Key Laboratory of the Ministry of Education for Advanced Catalysis Materials Institute of Physical ChemistryZhejiang Normal UniversityJinhua 321004China Laboratoire Interface et Systèmes Electrochimiques CNRS UMR 8235Sorbonne UniversitéF-75252 Paris cedex 5France

Correlating dynamic structural transformation of catalysts with the surface intermediate species under operating conditions is critical for updating the understanding of structure–performance ***,we probe the electrochemical potentialdependent surface structures and adsorbed intermediates on PtRu binary alloy nanocatalysts to revisit its synergistic mechanisms for CO electrooxidation enhanced ***-situ spectral characteristics by using modified shell-isolated nanoparticle-enhanced Raman spectroscopy,show that in acidic solution,when the potential is positively scanned from 0.1 V to 1.5 V relative to reversible hydrogen electrode(RHE),the surface of the alloy catalyst evolves from metallic PtRu to adsorbed oxygen gradually covering and accumulating on Ru sites(denoted as PtRuO_(x),x≤2),forming segregated RuO_(2),and finally forming a threedimensional oxide layer(denoted as 3D PtRuO_(4)).Moreover,molecular evidence associated with periodic density functional theory calculations reveals that electronic effects promote ruthenium to become more oxidizable and *** particular,we found here that ^(*)O and ^(*)OH at surface RuO_(x) sites are highly efficient CO oxidation active species in comparison to the same entities adsorbed on metallic Ru *** work sheds light on the complex surface dynamic process of practical Pt-based binary nanocatalysts and improves the understanding of synergistic mechanism for the development of fuel cell devices.

关键词： in-situ Raman spectroscopy surface evolution bifunctional mechanism PtRu electrooxidation

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Oxidation behavior of Ni-based superalloy GH4738 under tensile stress

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Rare Metals 2024年第8期43卷 3913-3920页

作者： Ji-chong Hu Hai-Liang Huang chong-chong Wu xiao-yu Sun Jie Wang Yan-Hong Yang Jing-Long Qu Liang Jiang Jin-He Dou Yang Chen Institute for Advanced Studies in Precision Materials Yantai University Department of Management and Engineering Link?ping University Shi-Changxu Innovation Center for Advanced Materials Institute of Metal ResearchChinese Academy of Sciences Gaona Aero Material Co. Ltd College of Artificial Intelligence and Big Data Shandong First Medical University and Shandong Academy of Medical Sciences

Revealing the oxidation behavior of superalloys is crucial for optimizing material properties and extending service *** study investigated the oxidation behavior of superalloy GH4738 under stress states at 850℃.High-throughput specimens were fabricated to withstand different stresses at the same *** oxidation s amples were analyzed using the mass gain method to obtain oxidation kinetic *** results show that the external stress below 200 MPa could improve the oxidation resistance of the *** tensile stress increasing,the oxide layer becomes thinner,denser and more complete,while internal oxidation *** tensile stress alters the structure of the external oxide layer from a two-layer to a threelayer *** Cr2O3oxide layer inhibits the outward diffusion of Ti,leading to Ti enrichment at the oxide-matrix interface and altering the oxidation mechanism of GH4738.

关键词： Ni-based Superalloy Oxidation behavior Tensile stress Oxide layer

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Study of the Lift Force Induced by An Interceptor on A High-Speed Mono-Hull:The Affecting Factors and Estimation Formula

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China Ocean Engineering 2024年第4期38卷 557-571页

作者： DENG Rui HU yu-xiao HUANG Si-chong SONG Zhi-jie WANG Shi-gang WU Tie-cheng School of Ocean Engineering and Technology Sun Yat-sen Universityand Southern Marine Science and Engineering Guangdong Laboratory(Zhuhai)Zhuhai 519082China

To find a better way to estimate the lift force induced by an interceptor on a high-speed mono-hull ship,a series of high-speed mono-hull ship models are designed and investigated under different *** lift forces are obtained by numerical calculations and validated by a model test in a towing *** factors that influence the force are the interceptor height,velocity,draft,and deadrise *** relationship between each factor and the induced lift force is investigated and *** found that the induced lift mainly depends on the interceptor height and advancing velocity,and is proportional to the square of the interceptor height and *** results also showed that the effects of the draft and deadrise angle are relatively less important,and the relationship between the induced lift and these two factors is generally *** on the results,a formula including the combined effect of all factors used to estimate the lift force induced by the interceptor is developed based on systematic *** proposed formula could be used to estimate the lift force induced by interceptors,especially under high-speed condition.

关键词： high-speed mono-hull ship interceptor lift force formula lift force towing tank test computational fluid dynamics

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State-of-the-art on the anchorage performance of rock bolts subjected to shear load

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International Journal of Coal Science & Technology 2024年第1期11卷 1-30页

作者： yu Chen Haodong xiao School of Civil Engineering Sun Yat-sen UniversityZhuhai519082China

Rock bolts are extensively utilized in underground engineering as a means of offering support and stability to rock masses in tunnels,mines,and other underground *** environments of high ground stress,faults or weak zones can frequently arise in rock formations,presenting a significant challenge for engineering and potentially leading to underground engineering *** bolts serve as a crucial structural element for the transmission of tensile stress and are capable of withstanding shear loads to prevent sliding of weak zones within rock ***,a complete understanding of the behavior of rock bolts subjected to shear loads is *** paper presents a state-of-the-art review of the research progress of rock bolts subjected to shear load in three categories:experiment,numerical simulation,and analytical *** review focuses on the research studies and developments in this area since the 1970s,providing a comprehensive overview of numerous factors that influence the anchorage performance of rock *** factors include the diameter and angle of the rock bolt installation,rock strength,grouting material,bolt material,borehole diameter,rock bolt preload,normal stress,joint surface roughness and joint expansion *** paper reviews the improvement of mechanical parameter setting in numerical simulation of rock bolt ***,it delves into the optimization of the analytical model concerning rock bolt shear theory,approached from the perspectives of both Elastic foundation beam theory coupled with Elastoplasticity theory and Structural mechanic *** significance of this review lies in its ability to provide insights into the mechanical behavior of rock *** paper also highlights the limitations of current research and guidelines for further research of rock bolts.

关键词： Rock bolt Shear load Shear test Numerical simulation Analytical model

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Real-time monitoring of hydrogel phase transition in an ultrahigh Q microbubble resonator

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Photonics Research 2020年第4期8卷 497-502页

作者： DAQUAN YANG AIQIANG WANG JIN-HUI CHEN xiao-chong yu CHUWEN LAN yuEFENG JI yuN-FENG xiao State Key Laboratory of Information Photonics and Optical Communications School of Information and Communication EngineeringBeijing University of Posts and TelecommunicationsBeijing 100876China State Key Laboratory for Artificial Microstructure and Mesoscopic Physics School of PhysicsPeking UniversityBeijing 100871China Frontiers Science Center for Nano-optoelectronics&Collaborative Innovation Center of Quantum Matter Beijing 100871China Collaborative Innovation Center of Extreme Optics Shanxi UniversityTaiyuan 030006China Beijing Academy of Quantum Information Sciences Beijing 100193China

The ability to sense dynamic biochemical reactions and material processes is particularly crucial for a wide range of applications,such as early-stage disease diagnosis and biomedicine *** microcavities-based label-free biosensors are renowned for ultrahigh sensitivities,and the detection limit has reached a single nanoparticle/molecule *** particular,a microbubble resonator combined with an ultrahigh quality factor(Q)and inherent microfluidic channel is an intriguing platform for optical biosensing in an aqueous *** this work,an ultrahigh Q microbubble resonator-based sensor is used to characterize dynamic phase transition of a thermosensitive ***,by monitoring resonance wavelength shift and linewidth broadening,we(for the first time to our knowledge)reveal that the refractive index is increased and light scattering is enhanced simultaneously during the hydrogel hydrophobic transition *** platform demonstrated here paves the way to microfluidical biochemical dynamic detection and can be further adapted to investigating single-molecule kinetics.

关键词： Real-time monitoring hydrogel phase transition an ultrahigh Q microbubble resonator

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