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One-step reduction-encapsulated synthesis of Ag@polydopamine multicore-shell nanosystem for enhanced photoacoustic imaging and photothermal-chemodynamic cancer therapy

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Nano Research 2022年第9期15卷 8291-8303页

作者： xiao-Rui Li Baoli yin Lei Gao Xinhao Li Hongwen huang Guosheng Song Yi-Ge Zhou Institute of Chemical Biology and Nanomedicine State Key Laboratory of Chemo/Biosensing and ChemometricsCollege of Chemistry and Chemical EngineeringHunan UniversityChangsha 410082China State Key Laboratory of Chemo/Biosensing and Chemometrics College of Chemistry and Chemical EngineeringHunan UniversityChangsha 410082China College of Materials Science and Engineering Hunan UniversityChangsha 410082China

Though imaging-guided multimodal therapy has been demonstrated as an effective strategy to improve cancer diagnosis and therapy,challenge remains as to simplify the sophisticated synthesis procedure for the corresponding ***,an insitu one-step reduction-encapsulated method has been reported,for the first time,to synthesize multicore-shell polydopaminecoated Ag nanoparticles(AgNPs@PDA)as a cancer theranostic agent,integrating amplified photoacoustic imaging,enhanced photothermal therapy,and photothermal promoted dual tumor microenvironment-coactivated chemodynamic *** photoacoustic signal and the photothermal conversion efficiency of AgNPs@PDA nanosystem present a 6.6-and 4.2-fold enhancement compared to those of M-AgNPs-PDA(simply mixing PDA and AgNPs)derived from the increased interface heat transfer coefficient and the stronger near-infrared ***,AgNPs@PDA coactivated by dual tumor microenvironment(TME)enables controllable long-term release of hydroxyl radicals(·OH)and toxic Ag+,which can be further promoted by near-infrared light ***,the high efficiency of AgNPs@PDA nanosystem with prominent photoacoustic imaging-guided synergistic photothermal-chemodynamic cancer treatment is also found in in vitro and in vivo *** a special mention,the formation mechanism of the one-step synthesized multicore-shell nanomaterials is systematically *** work provides a much simplified one-step synthesis method for the construction of a versatile nanoplatform for cancer theranostics with high efficacy.

关键词： one-step synthesis multicore-shell nanosystem photoacoustic imaging enhanced photothermal therapy dual tumor microenvironment-coactivated chemodynamic therapy

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Online hierarchical recognition method for target tactical intention in beyond-visual-range air combat

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Defence Technology（防务技术） 2022年第8期18卷 1349-1361页

作者： Zhen Yang Zhi-xiao Sun Hai-yin Piao Ji-chuan huang De-yun Zhou Zhang Ren School of Automation Science and Electrical Engineering Beihang UniversityBeijing100191China Northwestern Polytechnical University Xi'an710072China The First Military Representative Office of the Air Force Equipment Department in Chengdu Chengdu610091China

Online accurate recognition of target tactical intention in beyond-visual-range (BVR) air combat is an important basis for deep situational awareness and autonomous air combat decision-making, which can create pre-emptive tactical opportunities for the fighter to gain air superiority. The existing methods to solve this problem have some defects such as dependence on empirical knowledge, difficulty in interpreting the recognition results, and inability to meet the requirements of actual air combat. So an online hierarchical recognition method for target tactical intention in BVR air combat based on cascaded support vector machine (CSVM) is proposed in this study. Through the mechanism analysis of BVR air combat, the instantaneous and cumulative feature information of target trajectory and relative situation information are introduced successively using online automatic decomposition of target trajectory and hierarchical progression. Then the hierarchical recognition model from target maneuver element, tactical maneuver to tactical intention is constructed. The CSVM algorithm is designed for solving this model, and the computational complexity is decomposed by the cascaded structure to overcome the problems of convergence and timeliness when the dimensions and number of training samples are large. Meanwhile, the recognition result of each layer can be used to support the composition analysis and interpretation of target tactical intention. The simulation results show that the proposed method can effectively realize multi-dimensional online accurate recognition of target tactical intention in BVR air combat.

关键词： Beyond-visual-range(BVR)air combat Tactical intention recognition Hierarchical recognition model Cascaded support vector machine(CSVM) Trajectory decomposition Maneuver element

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Dynamic modeling of a three-dimensional braided composite thin plate considering braiding directions

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Applied Mathematics and Mechanics(English Edition) 2025年第1期46卷 123-138页

作者： Chentong GAO Huiyu SUN Jianping GU W.M.huang College of Aerospace Engineering Nanjing University of Aeronautics and Astronautics School of Mechanical and Aerospace Engineering Nanyang Technological University Jiangsu Key Laboratory of Advanced Structural Materials and Application Technology School of Materials Science and EngineeringNanjing Institute of Technology

Currently, there are a limited number of dynamic models available for braided composite plates with large overall motions, despite the incorporation of three-dimensional(3D) braided composites into rotating blade components. In this paper, a dynamic model of 3D 4-directional braided composite thin plates considering braiding directions is established. Based on Kirchhoff's plate assumptions, the displacement variables of the plate are expressed. By incorporating the braiding directions into the constitutive equation of the braided composites, the dynamic model of the plate considering braiding directions is obtained. The effects of the speeds, braiding directions, and braided angles on the responses of the plate with fixed-axis rotation and translational motion, respectively, are investigated. This paper presents a dynamic theory for calculating the deformation of 3D braided composite structures undergoing both translational and rotational motions. It also provides a simulation method for investigating the dynamic behavior of non-isotropic material plates in various applications.

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Cobalamin-dependent radical S-adenosyl-L-methionine protein functions with a partner to successively methylate tricyclic indole alkaloid for chuangxinmycin maturation and derivatization

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Science China Chemistry 2025年第1期 308-316页

作者： Sili Wang Jiancheng huang Yanan Du Wei huang Yufeng Xue xiaokun Xu Guannan Zhong Yuanyuan Shi Bin Hong xiaoying Bian Wen Liu State Key Laboratory of Chemical Biology Shanghai Institute of Organic Chemistry University of Chinese Academy of SciencesChinese Academy of Sciences State Key Laboratory of Microbial Technology Shandong University National Health Commission (NHC) Key Laboratory of Biotechnology for Microbial Drugs Institute of Medicinal BiotechnologyChinese Academy of Medical Science & Peking Union Medical College

Cobalamin(Cbl)-dependent radical S-adenosyl-L-methionine(SAM) proteins constitute the largest collection of the radical SAM superfamily that has hundreds of thousands of individual members. Many of these proteins are involved in the biosynthesis of pharmaceutically important natural products to catalyze chemically demanding reactions. In the biosynthetic pathway of chuangxinmycin(CXM), a unique indole alkaloid antibiotic with potent anti-infective activity, functionalization of the characteristic thiopyrano[4,3,2-cd]indole scaffold by regio-and stereoselective C3-methylation is believed to rely on a Cbl-dependent radical process, which, however, remained to be reconstituted biochemically. We here report the dissection of this enzymatic process, which requires the incorporation of Cxm8, a Cbl-dependent radical SAM protein, with Cxm9, a DUF5825family protein that shares no homology to any proteins of known functions. Cxm8 and Cxm9 function together by forming an unexpected heterodimeric complex that selectively catalyzes C3-methylation of the tricyclic indole-S-hetero ring system in a successive manner, achieving CXM and a recently identified, C3-dimethylated congener. Detailed biochemical characterization,isotope labeling, structural simulation and bioinformatics analysis rationalized the catalysis of the Cxm8/Cxm9 complex and particularly the necessity of the DUF5825 protein for C3-methylase activity. This is the first example that a Cbl-dependent protein acts with a partner to exhibit radical SAM activity.

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Oxygen-assisted zinc recovery from electric arc furnace dust using magnesium chloride

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International Journal of Minerals,Metallurgy and Materials 2024年第10期31卷 2300-2311页

作者： Jingdong huang xiao Yang School of Materials Science and Engineering Zhejiang UniversityHangzhou 310027China School of Engineering Westlake UniversityHangzhou 310030China

Electric arc furnace(EAF)dust is an important secondary resource containing metals,such as zinc(Zn)and iron(Fe).Recover-ing Zn from EAF dust can contribute to resource recycling and reduce environmental ***,the high chemical stability of ZnFe_(2)O_(4)in EAF dust poses challenges to Zn *** address this issue,a facile approach that involves oxygen-assisted chlorination using molten MgCl_(2)is *** work focused on elucidating the role of O2 in the reaction between ZnFe_(2)O_(4)and molten MgCl_(2).The results demonstrate that MgCl_(2)effectively broke down the ZnFe_(2)O_(4)structure,and the high O2 atmosphere considerably promoted the sep-aration of Zn from other components in the form of ZnCl_(2).The presence of O2 facilitated the formation of MgFe_(2)O_(4),which stabilized Fe and prevented its ***,the excessive use of MgCl_(2)resulted in increased evaporation loss,and high temperatures pro-moted the rapid separation of *** on these findings,we successfully extracted ZnCl_(2)-enriched volatiles from practical EAF dust through oxygen-assisted *** optimized conditions,this method achieved exceptional Zn chlorination percentage of over 97%within a short period,while Fe chlorination remained below 1%.The resulting volatiles contained 85wt%of ZnCl_(2),which can be further processed to produce metallic *** findings offer guidance for the selective recovery of valuable metals,particularly from solid wastes such as EAF dust.

关键词： electric arc furnace dust zinc oxygen magnesium chloride chlorination

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Strong decays of the P_(cs)(4459) as a Ξc D^(*) molecule

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Science China(Physics,Mechanics & Astronomy) 2021年第12期64卷 104-110页

作者： Feng Yang yin huang HongQiang Zhu School of Physical Science and Technology Southwest Jiaotong UniversityChengdu 610031China College of Physics and Electronic Engineering Chongqing Normal UniversityChongqing 401331China Asia Pacific Center for Theoretical Physics Pohang University of Science and TechnologyPohang 37673Korea

In this work,we study the strong decay of the newly observed P_(cs)(4459),assuming that it is a pureΞcD^(*)molecular ***ering two possible spin-parity assignments J^(P)=1/2^(−)and J^(P)=3/2^(−),the partial decay widths of theΞcD^(*)molecular state into J/ψΛ,D^(−)_(s)Λ^(+)_(c),and DΞ^((′))_(c) final states through hadronic loops are evaluated with the help of the effective *** comparison with the LHCb data,the S-waveD^(*)Ξc molecular with J^(P)=1/2^(−)assignment for P_(cs)(4459)is supported by our study,while the P_(cs)(4459)in spin-parity J^(P)=3/2^(−)case may be explained as an S-wave coupled bound state with lagerΞcD^(*)*** addition,the calculated partial decay widths with J^(P)=1/2^(−)ΞcD^(*)molecular state picture indicate that allowed decay mode,DΞ′c,may have the biggest branching *** experimental measurements for this strong decay process could be a crucial test for the molecule interpretation of the P_(cs)(4459).

关键词： molecular state strong decay effective Lagrangians

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超碱NLi_(4)团簇修饰DHQ石墨烯的储氢性能研究

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原子与分子物理学报 2025年第5期42卷 95-101页

作者：戴小乐王允辉黄欣南京邮电大学电子与光学工程学院柔性电子(未来技术)学院南京210023 南京邮电大学理学院南京210023

基于第一性原理计算,系统研究了超碱NLi_(4)团簇修饰在DHQ石墨烯表面上的几何结构及吸附能等性质,并深入探索了其储氢性能.研究结果表明:超碱NLi_(4)团簇可以稳定均匀地吸附在DHQ石墨烯表面,Li原子与N原子的强结合能有效避免了Li原子发... 详细信息

基于第一性原理计算,系统研究了超碱NLi_(4)团簇修饰在DHQ石墨烯表面上的几何结构及吸附能等性质,并深入探索了其储氢性能.研究结果表明:超碱NLi_(4)团簇可以稳定均匀地吸附在DHQ石墨烯表面,Li原子与N原子的强结合能有效避免了Li原子发生团聚.每个NLi_(4)团簇周围最多可吸附11个氢气分子,平均吸附能为0.20 eV,最大储氢容量为12.05 wt%,达到美国能源部制定的2025年储氢目标5.5 wt%.最后,基于相对能量计算,发现当压强大于84 bar时,该储氢体系可以在室温下稳定存在.以上结果表明经超碱NLi_(4)团簇修饰的DHQ石墨烯是一种有潜力的储氢材料.

关键词：多孔材料储氢超碱NLi_(4)团簇 DHQ石墨烯第一性原理计算

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Effect of Inter-Stage Pressure on Performances of Two-Stage Transcritical CO_(2) Refrigeration Cycle with Dedicated Absorption Dual-Subcooling and Mechanical Recooling

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Journal of Thermal Science 2024年第6期33卷 2179-2189页

作者： LI Zeyu huang Caoxuheng yin Jianhui School of Electric Power South China University of TechnologyGuangzhou 510640China Guangdong Province Key Laboratory of High Efficient and Clean Energy Utilization South China University of TechnologyGuangzhou 510640China Guangdong Province Engineering Research Center of High Efficient and Low Pollution Energy Conversion Guangzhou 510640China Ningbo Jetron Technology Co.Ltd. Ningbo 315000China

The two-stage transcritical CO_(2) refrigeration cycle with dedicated dual-subcooling and mechanical recooling is *** inter-stage pressure is critical for such cycle performances;however,it has not been studied ***,the research aim is to disclose the effect of inter-stage pressure on performances of the proposed *** main work consists of four ***,the comparative study is performed to display advantages of the proposed ***,the key temperatures,heat and power consumptions as well as performance indicators for different inter-stage pressures are analyzed in detail,based on the parametric ***,the optimal inter-stage pressure for different conditions is obtained by the nonlinear direct search ***,the economic performance is *** is found that the compressor power of the proposed cycle drops by 12%,and the working temperature lower limit is reduced by 11℃.Furthermore,it is considered that the optimal inter-stage pressure is insensitive to the heat source *** novelty lies in illustrating the effect of inter-stage pressure,obtaining trends of the optimal value,and pointing out the system *** paper is favorable for design and operation optimization of the proposed system.

关键词： CO,refrigeration two-stage cycle dedicated absorption subcooling recooling thermodynamic

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Rh-Cu alloy nano-dendrites with enhanced electrocatalytic ethanol oxidation activity

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Journal of Energy Chemistry 2023年第7期82卷 343-349,I0008页

作者： Di Liu Zhejiaji Zhu Jiani Li Li-Wei Chen Hui-Zi huang xiao-Ting Jing An-Xiang yin Ministry of Education Key Laboratory of Cluster Science Beijing Key Laboratory of Photoelectronic/Electrophotonic Conversion MaterialsAdvanced Technology Research Institute(Jinan)School of Chemistry and Chemical EngineeringBeijing Institute of TechnologyBeijing 100081China

The application of direct ethanol fuel cell(DEFC)has been bottlenecked by the sluggish ethanol oxidation reaction(EOR).Efficient electrocatalysts for the C-C bond cleavage are essential to promote EOR with high efficiency and C1 ***,we prepared Rh-Cu alloy nano-dendrites(RhCu NDs)with abundant surface steps through controlled co-reduction,which exhibited significantly enhanced activity and C1 selectivity(0.47 m A cm_((ECSA))^(-2),472.4 mA mg_(Rh)^(-1),and 38.9%)than Rh NDs(0.32 mA cm((ECSA))-2,322.1 mA mgRh-1,and 21.4%)and commercially available Rh/C(0.18 mA cm_((ECSA))^(-2),265.4 mA mg_(Rh)^(-1),and 14.9%).Theoretical calculations and CO-stripping experiments revealed that alloying with Cu could modulate the surface electronic structures of Rh to resist CO-poisoning while strengthening ethanol *** situ Fourier transform infrared spectroscopy(FTIR)indicated that the surface steps on RhCu NDs further promoted the C-C bond cleavage to increase the C1 ***,optimizing the surface geometric and electronic structures of nanocrystals by rational composition and morphology control can provide a promising strategy for developing practical DEFC devices.

关键词： Rh-Cu alloy Nano-dendrites Electrocatalysis Ethanol oxidation reaction In situ FTIR

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Photoactivated organic phosphorescence by stereo-hindrance engineering for mimicking synaptic plasticity

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Light(Science & Applications) 2023年第6期12卷 972-981页

作者： He Wang Yuan Zhang Chifeng Zhou xiao Wang Huili Ma Jun yin Huifang Shi Zhongfu An Wei huang Key Laboratory of Flexible Electronics(KLoFE)&Institute of Advanced Materials(IAM) Nanjing Tech UniversityNanjing 211800China The Institute of Flexible Electronics(IFE Future Technologies)Xiamen UniversityXiamen 361005China Department of Applied Physics The Hong Kong Polytechnic UniversityKowloon 999077 Hong KongChina State Key Laboratory of Organic Electronics and Information Displays&Institute of Advanced Materials(IAM) Nanjing University of Posts&Telecommunications9 Wenyuan RoadNanjing 210023China Frontiers Science Center for Flexible Electronics(FSCFE) MIIT Key Laboratory of Flexible Electronics(KLoFE)Northwestern Polytechnical UniversityXi’an 710072China

Purely organic phosphorescent materials with dynamically tunable optical properties and persistent luminescent characteristics enable more novel applications in intelligent ***,we reported a concise and universal strategy to achieve photoactivated ultralong phosphorescence at room temperature through stereo-hindrance *** dynamically photoactivated phosphorescence behavior was ascribed to the suppression of non-radiative transitions and improvement of spin-orbit coupling(SOC)as the variation of the distorted molecular conformation by the synergistic effect of electrostatic repulsion and steric ***“trainable”phosphorescent behavior was first proposed to mimic biological synaptic plasticity,especially for unique experience-dependent plasticity,by the manipulation of pulse intensity and *** study not only outlines a principle to design newly dynamic phosphorescent materials,but also broadens their utility in intelligent sensors and robotics.

关键词： plasticity stereo electrostatic

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