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A bipolar modified separator using TiO2 nanosheets anchored on N-doped carbon scaffold for high-performance Li–S batteries

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Journal of Materials Science & Technology 2020年第20期52卷 152-158页

作者： Na Li Fei chen xiangtao chen Zhongxu chen Yang Qi Xiaodong Li Xudong Sun Key Laboratory for Anisotropy and Texture of Materials(Ministry of Education) School of Materials Science and EngineeringNortheastern UniversityShenyang 110819China College of Environmental and Chemical Engineering Dalian UniversityDalian 116622China

Lithium-sulfur batteries hold promise for next generation batteries due to their high theoretical energy density and low ***,the rapid capacity fading caused by the shuttle of polysulfide between two electrodes severely hinders the practical application of Li-S *** address the issue,we reported a three-dimensional heterostructured TiO2 nanosheets/N-doped carbon(TO/NC),which is coated on a commercial polypro pylene(PP) separator,as an efficient barrier for Li-S *** TO/NC coating layer provides a bipolar chemical adsorption of lithium polysulfides(LiPSs) via TiO2 nanosheets with exposed(001) facets and N-doped carbon,showing high trapping capacity and remarkable electrocatalytic activity for *** slurry-bladed carbon black/sulfur cathode with 64 wt% sulfur offers outstanding performance with an initial capacity of 1314 mAh g^-1 at 0.2 *** 900 cycles,the cell still maintains the capacity of 448 mA h g^-1 at a 1 C rate with a degradation rate of only 0.055% per *** separator reported in this work holds great promise for the development of high-energy Li-S batteries.

关键词： Lithium-sulfur batteries N-doped carbon Separator TiO2 Nanosheets

Target Gap of Emission Reduction for China:Analysis based on Elastic Decoupling

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Chinese Journal of Population,Resources and Environment 2012年第2期10卷 84-93页

作者： Li Zhongmin chen xiangtao Yao Yu International Business School Shaanxi Normal UniversityXi'an Shaanxi 710062China

The present paper analyzes historically the relationship between carbon emission and economic development by different stages through adopting elastic decoupling methods and Tapio evaluation criteria along with a comparison with the national Five Year Plans. The analysis shows that the influencing factors to the relationship between carbon emission and economy in China are different, and economic development and carbon emission have less connection in the recent 30 years of reform and opening-up in China. It is a difficult task to realize the promise that we will reduce carbon emission by 40%-50% in 2020 based on the data from historical experience and different expectations for economic development from economists. Through constructing the calcula- tion model of carbon emission intensity gap according to different development scenarios, the analysis shows that economic growth, infrastructure investment and further development of industrial-ization are the main drivers to the increase of carbon emission, technological progress, and particularly, the reduction of energy consumption is the primary means to reduce carbon emission in China. It is imperative to transform the economic growth pattern, and it is a grand task to perform and there is a long way to go for China to maintain economic growth and reduce carbon intensity.

关键词： low-carbon economy emission reduction promise target gap elastic decoupling

β-细辛醚通过抑制TRPV4的表达缓解谷氨酸诱导的Ca^(2+)超载

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合肥工业大学学报（自然科学版） 2024年第2期47卷 263-269页

作者：蒋兰兰陈向涛储涛蔡静雯刘浩宇尹兰香安徽医科大学药学院安徽合肥230022 中国科学技术大学附属第一医院(安徽省立医院)药剂科安徽合肥230001

谷氨酸处理会导致Ca^(2+)超载,瞬时受体电位香草素受体4(transient receptor potential vanilloid 4,TRPV4)在其中的作用及可能机制尚不清楚。β-细辛醚能快速透过血脑屏障,对兴奋性毒性具有较强的神经保护作用。文章以高分化的PC12细... 详细信息

谷氨酸处理会导致Ca^(2+)超载,瞬时受体电位香草素受体4(transient receptor potential vanilloid 4,TRPV4)在其中的作用及可能机制尚不清楚。β-细辛醚能快速透过血脑屏障,对兴奋性毒性具有较强的神经保护作用。文章以高分化的PC12细胞为研究对象,探究β-细辛醚(15、30、60μmol/L)预处理4 h,40 mmol/L谷氨酸处理实时记录对PC12细胞Ca^(2+)浓度的影响,采用钙成像技术检测Ca^(2+)浓度的变化;采用实时荧光定量聚合酶链式反应(polymerase chain reaction,PCR)、Western Blot及免疫荧光技术检测TRPV4的mRNA和蛋白的表达;采用Lipofectiamine 2000脂质体实验转染TRPV4-siRNA和pEX-3-TRPV4,观察沉默和过表达TRPV4对谷氨酸引起Ca^(2+)超载的影响。结果表明:与正常对照组相比,谷氨酸处理5 min可诱导Ca^(2+)超载,显著提高TRPV4的mRNA和蛋白的表达;与模型组相比,β-细辛醚能够剂量依赖性地降低谷氨酸诱导的Ca^(2+)超载和TRPV4的表达;沉默TRPV4抑制细胞Ca^(2+)超载;过表达TRPV4则部分逆转β-细辛醚抑制谷氨酸诱导的Ca^(2+)超载。该研究证明,谷氨酸处理PC12细胞5 min通过上调TRPV4的表达诱导Ca^(2+)超载,β-细辛醚作为TRPV4的拮抗剂,是一种潜在的抑制兴奋性毒性的药物。

关键词：谷氨酸兴奋性毒性 β-细辛醚瞬时受体电位香草素受体4(TRPV4) Ca^(2+)超载

Patterning alternate TiO_(2) and Cu_(2)O strips on a conductive substrate as film photocatalyst for Z-scheme photocatalytic water splitting

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Science Bulletin 2022年第23期67卷 2420-2427,M0004页

作者： Honglei Zhu Chao Zhen xiangtao chen Shun Feng Bo Li Yufei Du Gang Liu Hui-Ming cheng Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China School of Materials Science and Engineering University of Science and Technology of ChinaShenyang 110016China School of Material Science&Engineering Northeastern UniversityShenyang 110819China Institute of Technology for Carbon Neutrality Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China

Semiconductor heterostructures mediated by electrical conductors are very promising for Z-scheme photocatalytic water *** contrast to conventional particulate heterostructures,alternate TiO_(2)and Cu_(2)O film stripes patterned parallel on a fluorine-doped tin oxide(FTO) conductive substrate was fabricated as a model film photocatalyst to study the characteristics of the photogenerated charge transfer *** Z-scheme transfer process with an effective transport distance of up to 5 μm occurs only in regions distant from the TiO_(2)/Cu_(2)O strip edges through the FTO substrate from the *** contrast,the transfer of charge around their contact regions follows the conventional transfer process through the TiO_(2)/Cu_(2)O strip *** results indicate that the Z-scheme transfer process occurring in such a large region dominates the charge transfer processes in the TiO_(2)/FTO/Cu_(2)O pattern film ***,unlike the single component film,which is inactive for photocatalytic overall water splitting,the modified TiO_(2)/Cu_(2)O pattern film can induce photocatalytic overall water splitting at a stoichiometric H_(2)/O_(2) ratio close to 2:*** findings have significant implications in designing efficient heterostructures by employing a Z-scheme charge transfer process.

关键词： Photocatalyst Pattern film Heterostructure Z-scheme Water splitting

Breaking the Fe_(3)O_(4)-wrapped copper microstructure to enhance copper-slag separation

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International Journal of Minerals,Metallurgy and Materials 2024年第10期31卷 2312-2325页

作者： Xiaopeng Chi Haoyu Liu Jun Xia Hang chen xiangtao Yu Wei Weng Shuiping Zhong Zijin School of Geology and Mining Fuzhou UniversityFuzhou 350108China Fujian Key Laboratory of Green Extraction and High-Value Utilization of New Energy Metals Fuzhou UniversityFuzhou 350108China Zijin Mining Group Co. Ltd.Longyan 364200China Collaborative Innovation Center of Steel Technology University of Science and Technology BeijingBeijing 100083China

The precipitation of Fe_(3)O_(4)particles and the accompanied formation of Fe_(3)O_(4)-wrapped copper structure are the main obstacles to copper recovery from the molten slag during the pyrometallurgical smelting of copper ***,the commercial powdery pyrite or anthracite is replaced with pyrite-anthracite pellets as the reductants to remove a large amount of Fe_(3)O_(4)particles in the molten slag,resulting in a deep fracture in the Fe_(3)O_(4)-wrapped copper microstructure and the full exposure of the copper matte *** 1wt%composite pellet is used as the reductant,the copper matte droplets are enlarged greatly from 25μm to a size observable by the naked eye,with the copper content being enriched remarkably from 1.2wt%to 4.5wt%.Density functional theory calculation results imply that the formation of the Fe_(3)O_(4)-wrapped copper structure is due to the preferential adhesion of Cu_(2)S on the Fe_(3)O_(4)particles.X-ray photoelectron spectroscopy,Fourier transform infrared spectrometer(FTIR),and Raman spectroscopy results all reveal that the high-efficiency conver-sion of Fe_(3)O_(4)to FeO can decrease the volume fraction of the solid phase and promote the depolymerization of silicate network *** a consequence,the settling of copper matte droplets is enhanced due to the lowered slag viscosity,contributing to the high efficiency of copper-slag separation for copper *** results provide new insights into the enhanced in-situ enrichment of copper from mol-ten slag.

关键词： pyrometallurgical smelting process slag cleaning reductants copper matte

A Fast Method for Community Detection Based on the Contribution of Nodes

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A Fast Method for Community Detection Based on the Contribut...

Evaluation and Hotspots Identification of Shallow Groundwater Contamination Risk in the Lower Reaches of the Liaohe River Plain

2011 International Conference on Computer Science and Information Technology(ICCSIT 2011)

作者： xiangtao chen Houwang Xing School of Information Science and Engineering Hunan University

ISBN: (纸本)9781612848334

Communities exist in complex network of different areas, and there have been some methods to identify the communities in networks. However, the high computationally demanding limits their applications. In this paper, we propose a measurement of relationship between node and community, and then give a new comparative definition for community in complex networks. Based on these definitions we put forward the corresponding detecting algorithm. The effectiveness of our algorithm is demonstrated by extensive experiments on lots of computer generated graphs and public available real-world graphs. The result shows our algorithm is fast and accuracy in detecting communities.

关键词： Comparative Definition Community Structure Contribution Complex Network

来源： cnki会议评论

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Journal of Resources and Ecology 2016年第1期7卷 51-60页

作者：孙才志陈相涛陈雪姣辽宁师范大学城市与环境学院大连116029

As a prerequisite for groundwater protection and contamination control, evaluation of groundwater con- tamination risk was the extension of groundwater vulnerability assessment. Based on disaster theory and using shallow groundwater of the lower reaches of Liaohe River Plain as the study area, we built an evaluation index system and a contamination index model for groundwater contamination risks from the perspectives of intrinsic vulnerability, external stresses, and functional value. We used data acquisition technology （remote sensing） and spatial analysis technology （GIS） to calculate the value of groundwater contamination risks. The spatial distribution of hotspots was obtained by calculating G index. Results show that groundwater contamination is above a mid-level risk in most of the study area. Areas with extreme high risk account for 37.86%, areas with high risk 32.47%, areas with moderate risk 12.07%, areas with light risk 3.17%, and areas with slight risk 14.43%. Hotspots areas are mainly located in central Shenyang City, northwest of Xinmin City, Beizhen City and Liaozhong County. Coldspots are mainly in Panjin City, Yingkou City, Dashiqiao City, Dawa County and Panshan County. The results reflect the spatial distribution and mechanism of groundwater contamination risk in the study area and provide relative references for land use planning and groundwater resource protection in the lower reaches of the Liaohe River Plain.

关键词： lower reaches of the Liaohe River Plain groundwater contamination risk evaluation index system spatial hotspot analysis

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基于SCAD-ESN的时间序列预测模型

工程科学与技术 2017年第6期49卷 129-134页

作者：张各各徐珍曾波陈祥涛河南科技大学网络与通信技术研究所河南洛阳471023 河南科技大学网络信息中心河南洛阳471023 河南科技大学数学与统计学院河南洛阳471023

回声状态网络(ESN)是一种重要的时间序列预测方法,但在训练数据存在噪声或野点情况下,ESN将会出现过拟合问题。针对该问题,提出基于平滑消边绝对偏离罚函数的回声状态网络(SCAD-ESN)模型。不同于在模型中加入岭回归、L1范数罚函数及小... 详细信息

回声状态网络(ESN)是一种重要的时间序列预测方法,但在训练数据存在噪声或野点情况下,ESN将会出现过拟合问题。针对该问题,提出基于平滑消边绝对偏离罚函数的回声状态网络(SCAD-ESN)模型。不同于在模型中加入岭回归、L1范数罚函数及小波降噪等常规方法,该模型利用SCAD罚函数对变量进行选择,将小变量置为零以满足变量稀疏性,将大变量直接置为常数,从而能够很好地解决ESN过拟合问题并满足近似无偏估计。对于SCAD罚函数的非凸函数优化问题,提出基于局部二次近似(LQA)的求解方法,将最小角回归(LQR)方法用于SCAD罚函数求解,避免了计算量巨大的问题。使用基于粒子群优化(PSO)的超参数选取方法快速确定平滑消边绝对偏离–回声状态网络模型的超参数,克服利用经验选取超参数时存在的盲目性较大且难以确定整体最优的超参数问题。混沌系统数值仿真和网络流量仿真结果表明,相对于常规模型,该模型能有效地降低测试误差,从而克服过拟合问题。

关键词：混沌时间序列预测回声状态网络平滑消边绝对偏离罚函数粒子群算法

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下辽河平原浅层地下水脆弱性评价

地球信息科学学报 2016年第2期18卷 238-247页

作者：孙才志陈雪姣陈相涛辽宁师范大学城市与环境学院大连116029

以下辽河平原为研究对象,在DRASTIC模型基础上,结合RS技术建立了DRASTICL(DRASTIC land use type)模型。利用Arc GIS的水文分析工具对DEM影像进行子流域划分与数据提取。通过对参数进行不确定性表征,对三角模糊参数设定不同α截集,在此... 详细信息

以下辽河平原为研究对象,在DRASTIC模型基础上,结合RS技术建立了DRASTICL(DRASTIC land use type)模型。利用Arc GIS的水文分析工具对DEM影像进行子流域划分与数据提取。通过对参数进行不确定性表征,对三角模糊参数设定不同α截集,在此基础上将随机参数和模糊参数进行蒙特卡罗模拟。将不同α截集下模拟结果代入模糊模式识别模型,根据累积分布规律,选取不同百分位,从而得出不同α截集与不同百分位地下水脆弱性取值。结合Arc GIS数据可视化表达,得出不同α截集下下辽河平原浅层地下水脆弱性分布图,以此辨析下辽河平原浅层地下水不确定性与脆弱性程度。最后运用灵敏度分析辨别各参数对模拟结果的实际贡献程度。结果表明:(1)模糊模式识别模型用非线性的形式充分反映参数连续性变化对模拟结果产生的影响。(2)加入土地利用类型参数,结果更能反映人类活动影响下地下水脆弱程度。(3)不同α水平、不同百分位、与不同灵敏度系数3个层次的分析有效处理了参数不确定性问题,为制定相关政策提供更加准确的参考依据,对今后本地区的地下水环境开发利用和保护具有重要意义。

关键词：下辽河平原地下水脆弱性不确定性灵敏度系数