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Super-high bed sintering for iron ores:variation and optimization of bed resistance

Journal of Iron and Steel Research International 2025年第1期32卷 40-51页

作者： Liang-ping xu Lin Xiong Hui-bo Liu Xi-duan Yang Ai-xiang Mao Pei-dun Chen Guang-hui Li School of Minerals Processing and Bioengineering Central South UniversityChangsha410083HunanChina Central Research Institute Baosteel Group Co.Ltd.Shanghai201900China Manufacturing Management Department Guangdong Zhongnan Iron and Steel Co.Ltd.Shaoguan512123GuangdongChina Technology and Development Center Shandong Taishan Iron and Steel Group Co.Ltd.Jinan271100ShandongChina

As the bed depth increases,sintering yield increases,but the productivity *** reveal the reasons for the decrease in productivity and explore targeted solutions,the bed resistance of mixtures,wet zone,and combustion zone was analyzed in the *** results showed that the decreased porosity of mixture resulted in the increased bed resistance by 160.56%when the bed depth increased from 600 to 1000 *** improving porosity of 1%by adding loosening bars with optimized size and distribution,the bed resistance decreased,and the productivity increased by 5%.The increase in bed depth increased the thickness of the wet zone from 120 to 680 mm and the resistance from 1.56 to 8.83 *** using a three-stage intensive mixer and pre-adding water for granulation,the moisture of mixture was reduced by 0.6%,and the sintering productivity increased by 4%.Besides,the high bed resistance is mainly caused by the increase in the thickness of the combustion zone from 31.9 to 132.7 mm,and the bed resistance increased from 0.70 to 5.62 *** bed resistance of the combustion zone at 900 mm was increased by 90.51%compared to 700 *** optimization of the distribution of coke breeze,the thickness of combustion zone at the lower layer decreased from 132.7 to 106.84 mm and permeability improved significantly.

关键词： Super-high bed sintering Bed resistance Permeability Productivity Wet zone Combustion zone

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Microplastics enhance the adsorption capacity of zinc oxide nanoparticles:Interactive mechanisms and influence factors

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Journal of Environmental Sciences 2025年第1期147卷 665-676页

作者： Weiping Xiong Min Hu Siying He yuhang Ye Yinping xiang Haihao Peng Zhaomeng Chen Zhengyong xu Honglin Zhang Weixiang Li Shudian Peng College of Environmental Science and Engineering Hunan University and Key Laboratory of Environmental Biology and Pollution Control(Hunan University)Ministry of EducationChangsha 410082China Hunan Boke Environmental Engineering Co.Ltd. Hengyang 421099China College of Environmental Protection and Safety Engineering University of South ChinaHengyang 421001China Hunan Modern Environmental Technology Co.Ltd. Changsha 410004China

Microplastics(MPs)are of particular concern due to their ubiquitous occurrence and propensity to interact and concentrate various waterborne contaminants from aqueous *** on the interaction and joint toxicity of MPs on engineered nanoparticles(ENPs)are exhaustive,but limited research on the effect of MPs on the properties of ENPs in multisolute ***,the effect of MPs on adsorption ability of ENPs to antibiotics was investigated for the first *** results demonstrated that MPs enhanced the adsorption affinity of ENPs to antibiotics and MPs before and after aging showed different effects on *** polyamide prevented aggregation of ZnONPs by introducing negative charges,whereas virgin polyamide affected ZnONPs with the help of electrostatic ***-IR and XPS analyses were used to probe the physicochemical interactions between ENPs and *** results showed no chemical interaction and electrostatic interactionwas the dominant force between ***,the adsorption rate of antibiotics positively correlated with pH and humic acid but exhibited a negative correlation with ionic *** study highlights that ENPs are highly capable of accumulating and transporting antibiotics in the presence of MPs,which could result in a widespread distribution of antibiotics and an expansion of their environmental risks and toxic effects on *** also improves our understanding of the mutual interaction of various co-existing contaminants in aqueous environments.

关键词： Microplastics Engineered nanoparticles Adsorption Tetracycline

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Direct seawater splitting for hydrogen production:Recent advances in materials synthesis and technological innovation

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Green Energy & Environment 2025年第1期10卷 11-33页

作者： Yilin Zhao Zhipeng yu Aimin Ge Lujia Liu Joaquim Luis Faria Guiyin xu Meifang Zhu State Key Laboratory for Modification of Chemical Fibers and Polymer Materials Center for Advanced Low-dimension MaterialsCollege of Materials Science and EngineeringDonghua UniversityShanghai201620China International Iberian Nanotechnology Laboratory(INL) Avenida Mestre Jose VeigaBraga4715-330Portugal The MacDiarmid Institute for Advanced Materials and Nanotechnology School of Chemical and Physical SciencesVictoria University of WellingtonWellington6012New Zealand LSRE-LCM-Laboratory of Separation and Reaction Engineering-Laboratory of Catalysis and Materials Faculty of EngineeringUniversity of PortoRua Dr.Roberto Frias s/nPorto4200-465Portugal ALiCE-Associate Laboratory in Chemical Engineering Faculty of EngineeringUniversity of PortoRua Dr.Roberto Frias s/nPorto4200-465Portugal

Direct seawater splitting has emerged as a popular and promising research direction for synthesising clean,green,non-polluting,and sustainable hydrogen energy without depending on high-purity water in the face of the world’s shortage of fossil ***,efficient seawater splitting is hindered by slow kinetics caused by the ultra-low conductivity and the presence of bacteria,microorganisms,and stray ions in ***,producing hydrogen on an industrial scale is challenging due to the high production *** present review addresses these challenges from the catalyst point of view,namely,that designing catalysts with high catalytic activity and stability can directly affect the rate and effect of seawater *** the ion transfer perspective,designing membranes can block harmful ions,improving the stability of seawater *** the energy point of view,mixed seawater systems and self-powered systems also provide new and low-energy research systems for seawater ***,ideas and directions for further research on direct seawater splitting in the future are pointed out,with the aim of achieving low-cost and high-efficiency hydrogen production.

关键词： Seawater splitting Catalyst Membranes Mixed seawater systems Self-powered systems

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Recent progress in exploring heterogeneous catalyst surface chemistry with near ambient pressure XPS

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Science China Chemistry 2025年

作者： yuanjie xu Zemin An yu Tang Institute of Molecular Engineering Plus Institute of Molecule Catalysis and In Situ/Operando Studies College of Chemistry Fuzhou University

X-ray photoelectron spectroscopy(XPS) is a crucial surface analysis technique that has become a key tool in the study of heterogeneous catalysis. Detecting surface chemistry under conditions that closely mimic actual industrial catalytic processes is essential for understanding the mechanisms involved. In the past decade, near ambient pressure X-ray photoelectron spectroscopy(NAP-XPS) has been increasingly utilized to study the surface chemistry of catalysts during heterogeneous catalytic processes, offering insights into structure-performance correlations. This review begins with a brief overview of NAP-XPS instrumentation. Next, we discuss the application of NAP-XPS in the study of thermal catalysis reactions, followed by a summary of the research on catalyst restructuring under reaction conditions. Additionally, we address the challenges and future perspectives for the development and application of NAP-XPS. Catalysis is inherently dynamic, requiring an understanding of the real-time behavior of catalysts under varying conditions. Therefore, future improvements in the ability to probe reaction intermediates with higher spatial and temporal resolution under conditions that closely mimic industrial environments are needed.

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SDG space: Revealing the structure and complementarities among sustainable development goals in China

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Fundamental Research 2025年第1期5卷 360-369页

作者： Gong, Mimi yu, Ke Zhou, Changchang Liu, Zhouyi xu, Zhenci xu, Ming Qu, Shen Center for Systems Integration and Sustainability Department of Fisheries and Wildlife Michigan State University East Lansing 48824 MI United States Center for Energy and Environmental Policy Research Beijing Institute of Technology Haidian District Beijing 100081 China School of Geography Nanjing Normal University 1 Wenyuan Road Qixia Nanjing 210023 China Department of Geography The University of Hong Kong 999077 Hong Kong School of Environment Tsinghua University Beijing 100084 China

To achieve the United Nations Sustainable Development Goals (SDGs) by 2030, it is essential to understand the interlinkages between the goals. Previous research has investigated these interactions by focusing on their correlations. However, few studies have systematically prioritized them from a structural perspective through the complementarity measurements and empirically validated their policy effectiveness, such as which goals and indicators impact other SDGs most, especially in China. This study introduces a new concept known as the ‘SDG space’ by employing the “Product Space” approach in network science and economics. It measures the complementarities between SDGs and indicators through their network structures in investigating effective policy design. Using the most recent available but unpublished data for 31 Chinese provinces, the SDG space was constructed at the 17 SDG and 118 indicator levels by analyzing the probability of comparative advantage between each SDG or indicator pair co-occurring in the same place. Historical data confirm that in the ‘SDG Space’ network, a goal connected to other well-developed goals would enjoy better future growth and vice versa. The structure reveals that SDG 4 (Quality Education), 15 (Life on Land), and 1 (No Poverty) are critical goals with transformative synergies to other SDGs. Furthermore, we identified strong complementarities between land-based ecosystems and clean water and climate actions using the finer-grained indicator-level space. These findings help pave the way for China toward a sustainable future by providing science-based policy recommendations for decision-makers. They can be generally applied to other countries and regions to assist in navigating toward sustainable development. © 2024

关键词： China Network analysis Product space SDG space Sustainable development goals

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Advances in the Development of Gradient Scaffolds Made of Nano‑Micromaterials for Musculoskeletal Tissue Regeneration

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Nano-Micro Letters 2025年第3期17卷 455-500页

作者： Lei Fang Xiaoqi Lin Ruian xu Lu Liu yu Zhang Feng Tian Jiao Jiao Li Jiajia xue Beijing Laboratory of Biomedical Materials Beijing University of Chemical TechnologyBeijing 100029People’s Republic of China State Key Laboratory of Organic‑Inorganic Composites Beijing University of Chemical TechnologyBeijing 100029People’s Republic of China School of Biomedical Engineering Faculty of Engineering and ITUniversity of Technology SydneySydneyNSW 2007Australia

The intricate hierarchical structure of musculoskeletal tissues,including bone and interface tissues,necessitates the use of complex scaffold designs and material structures to serve as tissue-engineered *** has led to growing interest in the development of gradient bone scaffolds with hierarchical structures mimicking the extracellular matrix of native tissues to achieve improved therapeutic *** on the anatomical characteristics of bone and interfacial tissues,this review provides a summary of current strategies used to design and fabricate biomimetic gradient scaffolds for repairing musculoskeletal tissues,specifically focusing on methods used to construct compositional and structural gradients within the *** latest applications of gradient scaffolds for the regeneration of bone,osteochondral,and tendon-to-bone interfaces are ***,the current progress of testing gradient scaffolds in physiologically relevant animal models of skeletal repair is discussed,as well as the challenges and prospects of moving these scaffolds into clinical application for treating musculoskeletal injuries.

关键词： Gradient scaffolds Musculoskeletal tissues Advanced manufacturing Biomaterials Tissue regeneration

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Visualization of the protective role of estrogen against female liver fibrosis via an ER viscosity NIR fluorescent probe

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Science China Chemistry 2025年第1期68卷 360-368页

作者： Zheng Liu Changyu Zhang Zipeng Li Wanying Ma Jia Liu xiang Xia Ning xu Wen Sun Jianjun Du Jiangli Fan Xiaojun Peng State Key Laboratory of Fine Chemicals Dalian University of TechnologyDalian 116024China Ningbo Institute of Dalian University of Technology Ningbo 315016China

Endoplasmic reticulum(ER)viscosity has emerged as a new potential biomarker for hepatic fibrosis(HF).Herein,we report the first ER-targeting viscosity-responsive near-infrared(NIR)fluorescent probe HBT-PP for investigations of HF *** twisted intramolecular charge transfer(TICT)and the excited state intramolecular proton transfer(ESIPT)are combined to endow HBT-PP with the selective response towards viscosity(~62-fold)and a super large stokes shift(~320 nm).HBT-PP mainly targets organelle ER and is able to image the drug-or alcohol-induced viscosity elevation in living ***,HBT-PP was successfully applied to visualize the gender difference in HF and the protective role of estrogen in restraining HF *** note,after 10 min of stain with HBT-PP,HF lesions showed a stage-based response,indicating the potential of this probe in fast and early diagnosis of *** results clearly demonstrated the promising application of HBT-PP as a new tool for exploring ER viscosity-involved physiological and pathological processes.

关键词： NIR fluorescent probe ER viscosity hepatic fibrosis gender difference estrogen

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Characteristics and phytotoxicity of hydrochar-derived dissolved organic matter:Effects of feedstock type and hydrothermal temperature

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Journal of Environmental Sciences 2025年第3期149卷 139-148页

作者： Qianqian Lang xuan Guo Chao Wang Lingyao Li yufei Li Junxiang xu xiang Zhao Jijin Li Bensheng Liu Qinping Sun Guoyuan Zou Institute of Plant Nutrition and Resources Beijing Academy of Agriculture and Forestry SciencesBeijing 100097China

The dissolved organic matter(DOM)with high mobility and reactivity plays a crucial role in *** this study,the characteristics and phytotoxicity ofDOMreleased fromthe hydrochars prepared from different feedstocks(cowmanure,corn stalk and Myriophyllum aquaticum)under three hydrothermal carbonization(HTC)temperatures(180,200 and 220°C)were *** results showed that the hydrochars had high dissolved organic carbon content(20.15 to 37.65 mg/g)and its content showed a gradual reduction as HTC temperature *** fluorescent components including mixed substance of fulvic acid-like and humic acid-like substances(C1,30.92%-58.32%),UVA humic acid-like substance(C2,25.27%-29.94%)and protein-like substance(C3,11.74%-41.92%)were identified in hydrochar DOM by excitation emission matrix spectra coupled with parallel factor *** HTC temperature increased the relative proportion of aromatic substances(C1+C2)and humification degree of hydrochar DOM from cow manure,while it presented adverse effects on the hydrochar DOM from corn stalk and *** principal component analysis suggested that feedstock type and HTC temperature posed significant effects on the characteristics of hydrochar ***,seed germination test of all hydrochar DOM demonstrated that the root length was reduced by 8.88%-26.43%in contrast with control,and the germination index values were 73.57%-91.12%.These findings provided new insights into the potential environmental effects for hydrochar application in soil.

关键词： Hydrochar Hydrothermal temperature Dissolved organic matter Excitation emission matrix Parallel factor analysis Phytotoxicity

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Galileo multi-day precise orbit determination using L-band and SLR data

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Geodesy and Geodynamics 2025年第1期16卷 99-110页

作者： Tianhe xu Honglei Yang Song Li Zhenlong Fang Wenfeng Nie Min Li Baoguo yu Shandong Key Laboratory of Optical Astronomy and Solar-Terrestrial Environment Institute of Space Sciences Shandong University Navigation Laboratory of the 54th Research Institute of China Electronics Technology Group Corporation

The continuously available satellites of European Galileo currently reach more than 25. To explore the rationality and reliability of the L-band and satellite laser ranging(SLR) data processing strategies, we design the Galileo L-band, the SLR-only, and the combined L-band/SLR dynamic precise orbit determination(POD) strategies by using the normal equations(NEQs) stacking, and investigate their continuity and stability by employing the Galileo L-band data and SLR observations for the time span of the whole year of 2023, based on the Bei Dou/GNSS analysis center platform of Shandong University by using the modified Bernese GNSS Software Version 5.4. The orbital consistency of the L-band 1-day solution is the best with the Three-dimensional Root-Mean-Square(3D-RMS) values of 3.6 cm compared with the Center for Orbit Determination in Europe Multi-GNSS Experiment(COM) orbits, the corresponding values is 1.4 cm, 2.5 cm, and 2.3 cm in Radial, the Tangential, and the Normal(RTN) direction, respectively. While the SLR-only 9-day arc length is optimal with the RTN values of 5.3 cm, 30 cm, and 38.2 cm,as well as the 3D-RMS values of 48.9 cm. Encouragingly, the difference of the orbital accuracy between the combined L-band/SLR multi-day solution and the COM orbits is reduced by 0.5 cm and 0.9 cm, 0.6 cm and 1.2 cm in T-, and N-direction for the 3-and 5-day solution respectively. The corresponding values improve 0.7 cm and 0.9 cm, 1.4 cm and 1.8 cm for the 3-and 5-day orbital overlaps difference between the combined L-band/SLR and the L-band solution. Take the E09 satellite as a case study, the SLR-only orbital accuracy is regularly optimized as the multi-day arc lengthens and with the sites ***, the SLR residuals of its three types of orbits further demonstrate the positive contribution of SLR to the combination of the GNSS and SLR techniques.

关键词： Galileo POD SLR L-band NEQs stacking

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Resting-state brain network remodeling after different nerve reconstruction surgeries:a functional magnetic resonance imaging study in brachial plexus injury rats

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Neural Regeneration Research 2025年第5期20卷 1495-1504页

作者： yunting xiang xiangxin Xing xuyun Hua yuwen Zhang Xin xue Jiajia Wu Mouxiong Zheng He Wang Jianguang xu School of Rehabilitation Science Shanghai University of Traditional Chinese MedicineShanghaiChina Engineering Research Center of Traditional Chinese Medicine Intelligent Rehabilitation Ministry of EducationShanghaiChina Department of Rehabilitation Medicine Yueyang Hospital of Integrated Traditional Chinese and Western MedicineShanghai University of Traditional Chinese MedicineShanghaiChina Department of Traumatology and Orthopedics Yueyang Hospital of Integrated Traditional Chinese and Western MedicineShanghai University of Traditional Chinese MedicineShanghaiChina Institute of Science and Technology for Brain-Inspired Intelligence Fudan UniversityShanghaiChina Key Laboratory of Computational Neuroscience and Brain-Inspired Intelligence(Fudan University) Ministry of EducationShanghaiChina Human Phenome Institute Fudan UniversityShanghaiChina

Distinct brain remodeling has been found after different nerve reconstruction strategies,including motor representation of the affected ***,differences among reconstruction strategies at the brain network level have not been *** study aimed to explore intranetwork changes related to altered peripheral neural pathways after different nerve reconstruction surgeries,including nerve repair,endto-end nerve transfer,and end-to-side nerve ***–Dawley rats underwent complete left brachial plexus transection and were divided into four equal groups of eight:no nerve repair,grafted nerve repair,phrenic nerve end-to-end transfer,and end-to-side transfer with a graft sutured to the anterior upper ***-state brain functional magnetic resonance imaging was obtained 7 months after *** independent component analysis algorithm was utilized to identify group-level network components of interest and extract resting-state functional connectivity values of each voxel within the *** in intra-network resting-state functional connectivity were compared among the *** muscle reinnervation was assessed by behavioral observation(elbow flexion)and *** results showed that alterations in the sensorimotor and interoception networks were mostly related to changes in the peripheral neural *** repair was related to enhanced connectivity within the sensorimotor network,while end-to-side nerve transfer might be more beneficial for restoring control over the affected limb by the original motor *** thalamic-cortical pathway was enhanced within the interoception network after nerve repair and end-to-end nerve *** areas related to cognition and emotion were enhanced after end-to-side nerve *** study revealed important brain networks related to different nerve *** networks may be potential targets for enhancing motor recovery.

关键词： brain functional networks end-to-end nerve transfer end-to-side nerve transfer independent component analysis nerve repair peripheral plexus injury resting-state functional connectivity

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