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Alternative Strategy for Development of Dielectric Calcium Copper Titanate‑Based Electrolytes for Low‑Temperature Solid Oxide Fuel Cells

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Nano-Micro Letters 2025年第1期17卷 310-332页

作者： Sajid Rauf Muhammad Bilal Hanif Zuhra Tayyab Matej Veis MAKYousaf Shah Naveed Mushtaq Dmitry Medvedev Yibin Tian chen xia Martin Motola Bin Zhu College of Mechatronics and Control Engineering Shenzhen UniversityShenzhen 518060People’s Republic of China Department of Inorganic Chemistry Faculty of Natural SciencesComenius University BratislavaIlkovicova684215 BratislavaSlovakia Energy Storage Joint Research Center School of Energy and EnvironmentSoutheast UniversityNanjing 210096People’s Republic of China Hydrogen Energy Laboratory Ural Federal University620002 EkaterinburgRussia Laboratory of Electrochemical Devices Based on Solid Oxide Proton Electrolytes Institute of High Temperature Electrochemistry620066 EkaterinburgRussia School of Microelectronics Hubei UniversityWuhan 430062People’s Republic of China

The development of low-temperature solid oxide fuel cells(LT-SOFCs)is of significant importance for realizing the widespread application of *** has stimulated a substantial materials research effort in developing high oxide-ion conductivity in the electrolyte layer of *** this context,for the first time,a dielectric material,CaCu_(3)Ti_(4)O_(12)(CCTO)is designed for LT-SOFCs electrolyte application in this *** individual CCTO and its heterostructure materials with a p-type Ni_(0.8)Co_(0.15)Al_(0.05)LiO_(2−δ)(NCAL)semiconductor are evaluated as alternative electrolytes in LT-SOFC at 450–550℃.The single cell with the individual CCTO electrolyte exhibits a power output of approximately 263 mW cm^(-2) and an open-circuit voltage(OCV)of 0.95 V at 550℃,while the cell with the CCTO–NCAL heterostructure electrolyte capably delivers an improved power output of approximately 605 mW cm^(-2) along with a higher OCV over 1.0 V,which indicates the introduction of high hole-conducting NCAL into the CCTO could enhance the cell performance rather than inducing any potential short-circuiting *** is found that these promising outcomes are due to the interplay of the dielectric material,its structure,and overall properties that led to improve electrochemical mechanism in CCTO–***,density functional theory calculations provide the detailed information about the electronic and structural properties of the CCTO and NCAL and their heterostructure CCTO–*** study thus provides a new approach for developing new advanced electrolytes for LT-SOFCs.

关键词： LT-SOFCs Dielectric CaCu_(3)Ti_(4)O_(12) Semiconductor Ni_(0.8)Co_(0.15)Al_(0.05)LiO_(2−δ) Ionic conductivity Heterostructure electrolyte

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Global robust optimal sliding mode control for uncertain affine nonlinear systems

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Journal of Systems Engineering and Electronics 2009年第4期20卷 838-843页

作者： Pang Haiping chen xia Coll. of Automation and Electronic Engineering Qingdao Univ. of Science and Technology Qingdao 266042 P. R. China

The problem of robustifying linear quadratic regulators （LQRs） for a class of uncertain affine nonlinear systems is considered. First, the exact linearization technique is used to transform an uncertain nonlinear system into a linear one and an optimal LQR is designed for the corresponding nominal system. Then, based on the integral sliding mode, a design approach to robustifying the optimal regulator is studied. As a result, the system exhibits global robustness to uncertainties and the ideal sliding mode dynamics is the same as that of the optimal LQR for the nominal system. A global robust optimal sliding mode control （GROSMC） is realized. Finally, a numerical simulation is demonstrated to show the effectiveness and superiority of the proposed algorithm compared with the conventional optimal LQR.

关键词： robust control optimal control sliding mode control nonlinear systems uncertain systems exact linearization.

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“Buckets effect”in the kinetics of electrocatalytic reactions

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Journal of Energy Chemistry 2024年第2期89卷 388-396,I0010页

作者： Haowen Cui Yan-xia chen Hefei National Laboratory for Physical Sciences at Microscale Department of Chemical PhysicsUniversity of Science and Technology of ChinaHefei 230026AnhuiChina

In this study,we systematically investigated the effect of proton concentration on the kinetics of the oxygen reduction reaction(ORR)on Pt(111)in acidic *** results demonstrate a rectangular hyperbolic relationship,i.e.,the ORR current excluding the effect of other variables increases with proton concentration and then tends to a constant *** consider that this is caused by the limitation of ORR kinetics by the trace oxygen concentration in the solution,which determines the upper limit of ORR kinetics.A model of effective concentration is further proposed for rectangular hyperbolic relationships:when the reactant concentration is high enough to reach a critical saturation concentration,the effective reactant concentration will become a constant *** could be due to the limited concentration of a certain reactant for reactions involving more than one reactant or the limited number of active sites available on the *** study provides new insights into the kinetics of electrocatalytic reactions,and it is important for the proper evaluation of catalyst activity and the study of structureperformance relationships.

关键词： Oxygen reduction reaction Kinetics Zero order Rectangular hyperbolic relationship pH effect

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Deciphering the linear relationship in the activity of the oxygen reduction reaction on Pt electrodes:A decisive role of adsorbates

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Journal of Energy Chemistry 2024年第7期94卷 70-77页

作者： Haowen Cui Yan-xia chen Hefei National Research Center for Physical Sciences at Microscale and Department of Chemical Physics University of Science and Technology of ChinaHefei 230026AnhuiChina

Despite substantial efforts in developing high-performance catalysts for the oxygen reduction reaction(ORR),the persistent challenge lies in the high onset overpotential of the ORR,and the effect of the elec-trolyte solution cannot be ***,we have systematically investigated the impact of adsorbate species and concentration,as well as solution pH,on the ORR activity on Pt(111)and Pt(poly)*** results all tend to establish a linear quantitative relationship between the onset potential for ORR and the adsorption equilibrium potential of the *** finding indicates the decisive role of adsorbates in the onset potential for ORR,suggesting that the adsorption potential of adsorbates can serve as an intuitive criterion for ORR *** support for this conclusion is derived from experimental results obtained from the oxygen evolution reaction on Pt(poly)with different adsorbate species and from the hydrogen evolution reaction on Pt(111)with iodine *** further propose both an empirical equation for the onset potential for ORR and the concept of a potential-regulated adsor-bate shielding effect to elucidate the influence of adsorbates on ORR *** study provides new insights into the high onset overpotential of the ORR and offers potential strategies for predicting and enhancingORRactivity inthefuture.

关键词： Oxygen reduction reaction Activity Adsorbate Equilibrium potential Pt(111)

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A Model Predictive Control Method for Hybrid Energy Storage Systems

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CSEE Journal of Power and Energy Systems 2021年第2期7卷 329-338页

作者： Siyuan chen Qiufan Yang Jianyu Zhou xia chen State Key Laboratory of Advanced Electromagnetic Engineering and Technology and School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074China

The traditional PI controller for a hybrid energy storage system(HESS)has certain drawbacks,such as difficult tuning of the controller parameters and the additional filters to allocate high-and low-frequency power *** paper proposes a model predictive control(MPC)method to control three-level bidirectional DC/DC converters for grid-connections to a HESS in a DC ***,the mathematical model of a HESS consisting of a battery and ultra capacitor(UC)is established and the neutral point voltage imbalance of a three-level converter is solved by analyzing the operating modes of the ***,for the control of the grid-connected converters,an MPC method is proposed for calculating steady-state reference values in the outer layer and the dynamic rolling optimization in the inner *** outer layer ensures the voltage regulation and establishes the current predictive model,while the inner layer,using the model predictive current control,makes the current follow the predictive value,thus reducing the system current *** cascaded topology has two independent controllers and is free of filters to realize the high-and low-frequency power allocation for a ***,it allows two types of energy storage devices to independently regulate the voltage and realizes the power allocation of the battery and ***,simulation studies are conducted in PSCAD/EMTDC,and the effectiveness of the proposed HESS control strategy is verified in a case,such as a controller comparison and fault scenario.

关键词： Double layer control method hybrid energy storage system(HESS) model predictive control(MPC) three-level DC/DC converter

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The Effectiveness of Structural Monetary Policy and Macro-Prudential Policies——Based on the DSGE Model That Includes Bank Heterogeneous Credit

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Journal of Systems Science & Complexity 2021年第6期34卷 2267-2290页

作者： KUANG Xiong WANG Qian chen xia School of Economics Hainan UniversityHaikou 570228China International Economics and Finance Institute Beijing 100820China

Structural monetary policy and macro-prudential policies are important parts of the policy system of the People’s Bank of *** constructing a dynamic stochastic general equilibrium model that includes the heterogeneity of corporate and bank credit,the authors divide the policies of the People’s Bank of China into seven categories,and explores the policy effectiveness of structural monetary policy,macro-prudential policy and traditional aggregate monetary *** simulation of the model,it is found that whether facing technical shocks,interest rate shocks or credit shocks,the structural two-pillar policy tool that uses the deposit reserve interest rate as the target of operation is most conducive to economic *** progress has the most positive and lasting impact on *** rates and credit policies will leave follow-up problems in the adjustment of the economy,and structural two-pillar policies can alleviate the impact of these problems.

关键词： Heterogeneous bank credit macro-prudential policy structural monetary policy two-pillar policy

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Selective catalytic oxidation of NO over iron and manganese oxides supported on mesoporous silica

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Journal of Natural Gas Chemistry 2008年第3期17卷 273-277页

作者： Junfeng Zhang Yan Huang xia chen Department of Environmental Science and Engineering Xiangtan University Xiangtan 411105 Hunan China

The selective catalytic oxidation （SCO） of NO was studied on a catalyst consisting of iron-manganese oxide supported on mesoporous silica （MPS） with different Mn/Fe ratios. Effects of the amount of manganese and iron, oxygen, and calcination temperature on NO conversion were also investigated. It was found that the Mn-Fe/MPS catalyst with a Mn/Fe molar ratio of 1 showed the highest activity at the calcination temperature of 400 °C. The results showed that over this catalyst, NO conversion reached 70% under the condition of 280 °C and a space velocity of 5000 h-1. SO2 and H2O had no adverse impact on the reaction activity when the SCO reaction temperature was above 240 °C. In addition, the SCO activity was suppressed gradually in the presence of SO2 and H2O below 240 °C, and such an effect was reversible after heating treatment.

关键词： selective catalytic oxidation of NO nitrogen monoxide mesoporous silica iron manganese

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Wireless Network Architecture for Evacuated Tube Transportation System

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China Communications 2020年第10期17卷 206-217页

作者： Li Han Hao Wu xia chen the State Key Laboratory of Rail Traffic Control and Safety School of Electronic and Information EngineeringBeijing Jiaotong UniversityHaidian DistrictBeijing 100044China Beijing Engineering Research Center of High-speed Railway Broadband Mobile Communications School of Electronic and Information EngineeringBeijing Jiaotong UniversityHaidian DistrictBeijing 100044China

Evacuated Tube Transportation(ETT)systems have been claimed to have considerable strengths,including ultra-highspeed,safety,and ***,the frequent handover caused by the high-speed brings a challenge for ETT mobile wireless communication to preserve steady link ***,in such a special scenario,the wireless link between the base station and the passengers on the train needs to experience fading from both metal pipe and train,thus the free-wave coverage with antennas in traditional high-speed rail wireless communication systems is not suitable for *** on the characteristics of ETT,an improved architecture of wireless communication network is proposed,using distributed base stations with remote radio units(RRUs)and baseband units(BBUs)and leaky waveguides to form stable *** a redundant BBUs or RRUs structure is designed for coverage *** on this redundant architecture,a fast handover scheme is proposed to resolve the handover *** analytical and simulation results show that the proposed scheme is capable of reducing communication outage probability and handover failure probability remarkably.

关键词： evacuated tube transportation network architecture coverage enhancement handover

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PRECISE MOMENT ASYMPTOTICS FOR THE STOCHASTIC HEAT EQUATION OF A TIME-DERIVATIVE GAUSSIAN NOISE

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Acta Mathematica Scientia 2019年第3期39卷 629-644页

作者： Heyu LI xia chen School of Mathematics Jilin UniversityChangchun 130012China Department of Mathematics University of TennesseeKnoxville TN 37996USA

This article establishes the precise asymptotics Eu^m(t, x)(t → ∞ or m → ∞) for the stochastic heat equation ?u/?t(t, x) =1/2?u(t, x) + u(t, x)(t, x)?W/?t(t, x) with the time-derivative Gaussian noise W?/?t(t, x) ... 详细信息

关键词： Sto chastic hea t equation t ime-deriva tive Gaussian noise Brownian mot ion Feynman-Kac representation Schilder's large deviation

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Research on windmill starting characteristics of MTE-D micro turbine engine

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Chinese Journal of Aeronautics 2013年第4期26卷 858-867页

作者： xia chen Fu Xin Wan Zhaoyun Huang Guoping chen Jie College of Energy and Power Engineering Nanjing University of Aeronautics and Astronautics

Micro turbine engine （MTE） is an important kind of propulsion system for miniature unmanned aircraft or missiles, because of its better high-speed performance （than propeller propulsion） and higher propulsion efficiency （obviously than rockets）. Windmill start is a common air-starting mode used in micro turbine engine. The windmill starting characteristics are important to the practical use of micro turbine engine. In this paper, the windmill starting characteristics research for a 12 cm diameter （MTE-D） micro turbine engine is carried out by experiment and numerical simulation. The characteristic of rotor mechanical losses at low-speed condition is stud- ied, and the engine common working line of windmill starting process is obtained. Based on the engine windmill characteristics, the propane ignition characteristics under different inflow conditions are researched, and the envelope of propane ignition and propane flameout is determined. The experimental research of fuel supply and ignition characteristics is completed, and the envelope of fuel supply and ignition is obtained. The windmill stage, propane ignition stage, fuel ignition stage and acceleration process from idling-speed to 80% full speed of MTE-D micro turbine engine is optimized, and the optimization windmill starting parameters are collected. The successful wind-mill starting experiment under this condition with engine speed up to 80% full speed indicates that these starting parameters are reasonable. All the starting parameters of MTE-D micro turbine engine obtained in this work are dimensionless parameters, and the conclusions obtained in this study have some reference to other micro turbine engines with the similar structural form and starting process.

关键词： Flameout boundary Ignition characteristics Low speed characteristics Micro turbine engine Windmill starting

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