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Rare Metals 2024年第1期43卷 225-235页

作者： Feng-Xia Wu Feng-Hua Li Xia-Li Lv Qi-Xian Zhang Guo-Bao xu Wen-Xin Niu State Key Laboratory of Electroanalytical Chemistry Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China Shaoxing Institute of Technology Shanghai UniversityShaoxing 312000China University of Science and Technology of china Hefei 230026China school of Materials Science and Engineering Shanghai UniversityShanghai 200436China Zhejiang Institute of Advanced Materials Shanghai UniversityJiashan 314113China University of chinese academy of sciences Beijing 100039China

Noble metal surfaces with intrinsic chirality serve as an ideal candidate for investigating enantioselective chemistry due to their superior chemical durability and high catalytic ***,significant advance has been made in synthesizing metal nanocrystals with intrinsic ***,the majority reports are limited to ***,through a heteroepitaxial growth strategy,the synthesis of metal nanocrystals with intrinsic chirality to palladium was extended for the first time and their application in enantioselective recognition was *** heteroepitaxial growth strategy allows for transferring the chirality of homochiral Au nanocrystals to Au@Pd core–shell *** employing the chiral Au@Pd nanocrystals as enantiomeric recognizing elements,a series of electrochemical sensors for chiral discrimination were *** optimal conditions,the peak potential between D-dihydroxyphenylalanine(D-DOPA)and L-dihydroxyphenylalanine(L-DOPA)is about 80 m V,and the peak current of D-DOPA is 2 times as much as that of L-DOPA,which enables the determination of the enantiomeric excess(EE,%)of ***,this report not only introduces a heteroepitaxial growth strategy to synthesize metal nanocrystals with intrinsic chirality,but also demonstrates the superior capability of integrating intrinsic chirality and catalytic properties into metal nanocrystals for chiral recognition.

关键词： Core–shell nanostructures Chirality transfer Electrochemical sensors Chiral recognition Chiroplasmonics

Nonlinear compression of picosecond chirped pulse from thin-disk amplifier system through a gas-filled hollow-core fiber

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chinese Physics B 2016年第12期25卷 277-282页

作者：陆俊黄志远王丁许毅刘彦祺郭晓杨黎文开吴分翔刘征征冷雨欣 school of Physics Science and Engineering Tongji University Shanghai 200092 China State Key Laboratory of High Field Laser Physics Institute of Optics and Fine Mechanics Chinese Academy of Sciences Shanghai 201800 China University of chinese academy of sciences Beijing 100049 China department of Physics Shanghai University Shanghai 200444 China

We theoretically study the nonlinear compression of a 20-rnJ, 1030-nm picosecond chirped pulse from the thin-disk amplifier in a krypton gas-filled hollow-core fiber. The chirp from the thin-disk amplifier system has little influence on the initial pulse, however, it shows an effect on the nonlinear compression in hollow-core fiber. We use a large diameter hollow waveguide to restrict undesirable nonlinear effects such as ionization; on the other hand, we employ suitable gas pressure and fiber length to promise enough spectral broadening; with 600-μm, 6-bar （1 bar = 105 Pa）, 1.8-m hollow fiber, we obtain 31.5-fs pulse. Moreover, we calculate and discuss the optimal fiber lengths and gas pressures with different initial durations induced by different grating compression angles for reaching a given bandwidth. These results are meaningful for a compression scheme from picoseconds to femtoseconds.

关键词： picosecond pulse hollow-core fiber thin-disk amplifier spectrum broadening

High-Pressure Behavior of Ferromagnesite(Mg_(0.81)Fe_(0.19))CO_(3)by Synchrotron X-Ray Diffraction and Raman Spectroscopy up to 53 GPa

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Journal of Earth Science 2024年第2期35卷 525-535页

作者： Lin Liang Guibin Zhang Shengxuan Huang Jingjing Niu Dongzhou Zhang Jingui xu Wen Liang Shan Qin Key Laboratory of Orogenic Belts and Crustal Evolution MOEand School of Earth and Space SciencesPeking UniversityBeijing100871China CAS Center of Excellence in Tibetan Plateau Earth sciences and Key Laboratory of Continental Collision and Plateau Uplift Institute of Tibetan Plateau ResearchChinese Academy of SciencesBeijing100101China Hawai’i Institute of Geophysics and Planetology School of Ocean and Earth Science and TechnologyUniversity of Hawai’i at ManoaHawai’i96822USA Key Laboratory of High Temperature and High Pressure Study of the Earth’s Interior Institute of GeochemistryChinese Academy of SciencesGuiyang550081China

Ferromagnesite(Mg,Fe)CO_(3)with 20 mol%iron is a potential host mineral for carbon transport and storage in the Earth *** high-pressure behavior of synthetic ferromagnesite(Mg_(0.81)Fe_(0.19))CO_(3)up to 53 GPa was investigated by synchrotron X-ray diffraction(XRD)and Raman *** iron bearing carbonate underwent spin transition at around 44–46 GPa accompanied by a volume collapse of 1.8%,which also demonstrated a variation in the dνi/dP slope of the Raman *** pressure-volume data was fitted by a third-order Birch-Murnaghan equation of state(BM-EoS)for the high spin *** best-fit K_(0)=108(1)GPa and K_(0)'=4.2(1).Combining the dνi/dP and the K_(0),the mode Grüneisen parameters of each vibrational mode(T,L,ν4 andν1)were *** effects of iron concentration on the Mg_(1−x)Fe_(x)CO_(3)system related to high-pressure compressibility and vibrational properties are *** results expand the knowledge of the physical properties of carbonates and provide insights to the potential deep carbon host.

关键词： ferromagnesite synchrotron XRD Raman spectroscopy high pressure geochemistry mineral

A survey on causal inference for recommendation

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The Innovation 2024年第2期5卷 130-144页

作者： Huishi Luo Fuzhen Zhuang Ruobing Xie Hengshu Zhu Deqing Wang Zhulin An Yongjun xu Institute of Artificial Intelligence Beihang UniversityBeijing 100191China Zhongguancun Laboratory Beijing 100094China WeChat Search Application department TencentBeijing 100080China The Career Science Laboratory BOSS ZhipinBeijing 100028China SKLSDE School of Computer ScienceBeihang UniversityBeijing 100191China Institute of Computing Technology Chinese Academy of SciencesBeijing 100190China

Causal inference has recently garnered significant interest among recommender system(RS)researchers due to its ability to dissect cause-and-effect relationships and its broad applicability across multiple *** offers a framework to model the causality in RSs such as confounding effects and deal with counterfactual problems such as offline policy evaluation and data *** there are already some valuable surveys on causal recommendations,they typically classify approaches based on the practical issues faced in RS,a classification that may disperse and fragment the uni-fied causal *** RS researchers’unfamiliarity with causality,it is necessary yet challenging to comprehensively review relevant studies from a coherent causal theoretical perspective,thereby facilitating a deeper integration of causal inference in *** survey provides a systematic review of up-to-date papers in this area from a causal theory standpoint and traces the evolutionary development of RS methods within the same causal ***,we introduce the fundamental concepts of causal inference as the basis of the following ***,we propose a novel theory-driven taxonomy,categorizing existing methods based on the causal theory employed,namely those based on the potential outcome framework,the structural causal model,and general *** review then delves into the technical details of how existing methods apply causal inference to address particular recommender ***,we highlight some promising directions for future research in this *** papers and open-source resources will be progressively available at https://***/Chrissie-Law/Causal-Inference-forRecommendation.

关键词： survey details causal

CMN: a co-designed neural architecture search for efficient computing-in-memory-based mixture-of-experts

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Science china(Information sciences) 2024年第10期67卷 100-114页

作者： Shihao HAN Sishuo LIU Shucheng DU Mingzi LI Zijian YE Xiaoxin xu Yi LI Zhongrui WANG Dashan SHANG department of Electrical and Electronic Engineering The University of Hong Kong ACCESS-AI Chip Center for Emerging Smart Systems InnoHK Centers Key Lab of Fabrication Technologies for Integrated Circuits Chinese Academy of Sciences Laboratory of Microelectronics Devices and Integrated Technology Institute of MicroelectronicsChinese Academy of Sciences University of chinese academy of sciences school of Microelectronics Southern University of Science and Technology

Artificial intelligence(AI) has experienced substantial advancements recently, notably with the advent of large-scale language models(LLMs) employing mixture-of-experts(MoE) techniques, exhibiting human-like cognitive skills. As a promising hardware solution for edge MoE implementations, the computing-in-memory(CIM) architecture collocates memory and computing within a single device, significantly reducing the data movement and the associated energy consumption. However, due to diverse edge application scenarios and constraints, determining the optimal network structures for MoE, such as the expert's location,quantity, and dimension on CIM systems remains elusive. To this end, we introduce a software-hardware co-designed neural architecture search(NAS) framework, CIM-based MoE NAS(CMN), focusing on identifying a high-performing MoE structure under specific hardware constraints. The results of the NYUD-v2 dataset segmentation on the RRAM(SRAM) CIM system reveal that CMN can discover optimized MoE configurations under energy, latency, and performance constraints, achieving 29.67×(43.10×) energy savings,175.44×(109.89×) speedup, and 12.24× smaller model size compared to the baseline MoE-enabled Visual Transformer, respectively. This co-design opens up an avenue toward high-performance MoE deployments in edge CIM systems.

关键词： mixture-of-experts computing-in-memory neural architecture search resistive random-access memory static random-access memory

Astrometric Observations of NEA 1998 HH49 Using the Daocheng 50 cm Telescope

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Research in Astronomy and Astrophysics 2024年第7期24卷 71-78页

作者： Huan xu Xiang-Ming Cheng Yi-Gong Zhang Teng-Fei Song Zhen-Jun Zhang Qing-Yu Peng Yunnan Observatories Chinese Academy of SciencesKunming 650216China University of chinese academy of sciences Beijing 100049China Key Laboratory of the Structure and Evolution of Celestial Objects Chinese Academy of SciencesKunming 650216China Engineering Laboratory on Applied Astronomical Technology of Yunnan Kunming 650216China school of Information Engineering Kunming UniversityKunming 650214China school of Computer Science and Information Engineering Anyang Institute of TechnologyAnyang 455000China department of Computer Science Jinan UniversityGuangzhou 510632China Sino-French Joint Laboratory for Astrometry Dynamics and Space ScienceJinan UniversityGuangzhou 510632China

This study details an astrometric observation campaign of the Near-Earth Asteroid 1998 HH49,conducted with the aim of refining our understanding of its physical *** the 50 cm telescope located at the Wumingshan Mountain in Daocheng,Sichuan,images were obtained over four nights,from 2023 October 19 to October *** observations were processed using Astrometrica software,facilitating the precise determination of the asteroid's *** observational results were compared with the ephemerides from three distinct sources to verify accuracy:the Jet Propulsion Laboratory(JPL)Horizons System,the Institut de Mécanique Céleste et de Calcul deséphémérides(IMCCE)Miriade,and the Near-Earth Objects Dynamic Site(NEODyS-2).When compared with the JPL ephemeris,a mean observed-minus-calculated(O-C)result of 0.″07 in the *** and-0.″35 in the *** was ***,the comparison with the IMCCE ephemeris yielded mean O-C results of 0.″08 in the *** and-0.″06 in the *** comparison with the NEODyS-2 ephemeris yielded the mean O-C results of 0.″06 in ***-0.″49 in *** study's findings demonstrate a general consistency between the observed data and the ephemeris predictions,with minor discrepancies observed across the data ***,both the JPL and NEODyS-2 ephemerides show that the residuals in the *** exceed those in the *** disparities may result from atmospheric differential color refraction,ephemeris discrepancies,observational errors,and other ***,it is worth noting that further investigation is required due to the potential influence of additional ***,the Daocheng 50 cm Telescope exhibits the ability to conduct high-precision positional measurements.

关键词： astrometry ephemerides time

GPS TEC response to the 22 July 2009 total solar eclipse in East Asia

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GPS TEC response to the 22 July 2009 total solar eclipse in ...

Associations between remnant cholesterol levels and mortality in patients with diabetes

中国科学院地质与地球物理研究所第十届(2010年度)学术年会

作者： Feng Ding,Weixing Wan,Baiqi ning,Libo Liu,Huijun Le,Guirong xu, Min Wang,Guozhu Li,Yiding Chen,Zhipeng Ren,Bo Xiong,Lianhuan Hu, Xinan Yue,Biqiang Zhao,Fengqin Li,and Min Yang 1 beijing National Observatory of Space Environment,Institute of Geology and Geophysics,chinese academy of sciences,beijing,china. 2 Institute of Heavy Rain,china Meteorological Administration, Wuhan,china. 3 Institute of Earthquake Science,china Earthquake Administration, beijing,china. 4 graduate school of the chinese academy of sciences,beijing,china. 5 University Corporation for Atmospheric Research,Boulder,Colorado, USA.

[1]The longest total solar eclipse of this century occurred in East and South Asia on 22 July *** eclipse was accompanied with a medium magnetic storm,whose main phase onset occurred～27 min after the passage of the Moon’s umbral *** TEC data from 60 GPS stations,we construct differential TEC maps to investigate the ionosphere response to the solar eclipse in central china in the range of 26°N-36°N, 108°E-118°E(i.e.,the magnetic latitude 15°N-25°N).During the eclipse’s totality,a "shadow" in the ionosphere shown as TEC depletion area was formed～100 km south of the Moon’s umbral path with a maximum decrease of 5 *** TEC depletion area moved eastward,following the movement of the totality area with a time lag of～10 min. Enhancements of TEC due to the storm are observed after the main phase *** relative drop of TEC due to the solar eclipse is evidently larger at lower latitudes than that at higher ones and around noontime than that in the *** modeling work,we find that the latitudinal dependence of the TEC response may result from latitudinal variation of magnetic inclination,which influences the diffusion of ionization among different ***,the local time dependence of TEC response is closely related to the local time variation of background atmosphere density,which affects the electron loss efficiency in the ionosphere.

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World Journal of Diabetes 2024年第4期15卷 712-723页

作者： Deng Pan Lin xu Li-Xiao Zhang Da-Zhuo Shi Ming Guo department of Cardiovascular Xiyuan Hospital of China Academy of Chinese Medical SciencesBeijing 100091China graduate school Beijing University of Chinese MedicineBeijing 100020China National Clinical Research Center for chinese Medicine Cardiology Xiyuan Hospital of China Academy of Chinese Medical SciencesBeijing 100091China Gynecological department of Traditional chinese Medicine China-Japan Friendship HospitalBeijing 100020China

BACKGROUND Dyslipidemia is frequently present in patients with *** associations of remnant cholesterol and mortality remains unclear in patients with *** To explore the associations of remnant cholesterol with all-cause and cardiovas-cular mortality in patients with *** This prospective cohort study included 4740 patients with diabetes who par-ticipated in the National Health and Nutrition Examination Survey from 1999 through *** cholesterol was used as the exposure variable,and all-cause and cardiovascular mortality were considered outcome *** data were obtained from the National Death Index,and all participants were followed from the interview date until death or December 31,*** proportional Cox regression models were used to explore the associations between exposure and outcomes,in which remnant cholesterol was modeled as both a categorical and a continuous *** cubic splines(RCSs)were calculated to assess the nonlinearity of ***(stratified by sex,age,body mass index,and duration of diabetes)and a series of sensitivity analyses were performed to evaluate the robustness of the *** During a median follow-up duration of 83 months,1370 all-cause deaths and 389 cardiovascular deaths were *** with remnant cholesterol levels in the third quartile had a reduced risk of all-cause mortality[hazard ratio(HR)95%confidence interval(CI):0.66(0.52-0.85)];however,when remnant cholesterol was modeled as a continuous variable,it was associated with increased risks of all-cause[HR(95%CI):1.12(1.02-1.21)per SD]and cardiovascular[HR(95%CI):1.16(1.01-1.32),per SD]*** RCS demonstrated nonlinear associations of remnant cholesterol with all-cause and cardiovascular *** and sensitivity analyses did not reveal significant differences from the above *** In patients with diabetes,higher remnant cholesterol was associated wi

关键词： Diabetes Remnant cholesterol Mortality Cardiovascular National Health and Nutrition Examination Survey

Dynamic Characteristic Analysis of HIV Mother to Child Transmission in china

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Biomedical and Environmental sciences 2010年第5期23卷 402-408页

作者： JUN-JIE WANG KATHLEEN HEATHER REILLY HUA HAN ZHI-HANG PENG ning WANG National Center for AIDS/STD Control and Prevention Chinese Center for Disease Control and PreventionBeijing 100050China Tulane University Health sciences Center School of Public Health and Tropical MedicineNew OrleansLAUSA National ASIC Design Engineering Center Institute of AutomationChinese Academy of SciencesBeijing 100190China department of Epidemiology and Biostatistics Nanjing Medical UniversityNanjing 210029China

Objective to explore dynamic characteristics of the HIV mother to child transmission （MTCT） epidemic in *** A deterministic dynamic transmission model was used to determine the effect of key parameters on the likely long-term trends of the HIV MTCT epidemic in *** 7.0 was used to develop the *** The number of the susceptibles （S）,the transmission rate （β）,and the screening proportion （α） of HIV positive pregnant women have the greatest impact on the HIV MTCT epidemic in *** growth of the MTCT epidemic in china could not be controlled only by decreasing the MTCT transmission *** prevalence of HIV positive women should be reduced and more pregnant women should be tested for *** Prevention of MTCT （PMTCT） should focus not only on the reduction of HIV transmission rates and incidences of HIV among women but also on the increase of HIV testing for pregnant *** most cost-effective PMTCT means for china should be investigated in future studies.

关键词： mother to child transmission dynamic model HIV china