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Enhancing the Performance of Perovskite Light-Emitting Diodes via Synergistic Effect of Defect Passivation and Dielectric Screening

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Nano-Micro Letters 2024年第10期16卷 244-256页

作者： Xuanchi Yu Jia guo Yulin mao Chengwei Shan Fengshou Tian Bingheng Meng Zhaojin Wang Tianqi Zhang Aung Ko Ko Kyaw Shuming Chen Xiaowei Sun Kai Wang Rui Chen Guichuan xing institute of Applied Physics and Materials Engineering University of MacaoAvenida da UniversidadeTaipaMacao 999078People's Republic of China Department of Electrical and Electronic Engineering Southern University of Science and TechnologyShenzhen 518055People's Republic of China

Metal halide perovskites,particularly the quasi-two-dimensional perovskite subclass,have exhibited considerable potential for next-generation electroluminescent materials for lighting and ***,the presence of defects within these perovskites has a substantial influence on the emission efficiency and durability of the *** this study,we revealed a synergistic passivation mechanism on perovskite films by using a dual-functional compound of potassium *** dual functional potassium bromide on the one hand can passivate the defects of halide vacancies with bromine anions and,on the other hand,can screen the charged defects at the grain boundaries with potassium *** approach effectively reduces the probability of carriers quenching resulting from charged defects capture and consequently enhances the radiative recombination efficiency of perovskite thin films,leading to a significant enhancement of photoluminescence quantum yield to near-unity values(95%).Meanwhile,the potassium bromide treatment promoted the growth of homogeneous and smooth film,facilitating the charge carrier injection in the ***,the perovskite light-emitting diodes based on this strategy achieve a maximum external quantum efficiency of~21%and maximum luminance of~60,000 cd m^(-2).This work provides a deeper insight into the passivation mechanism of ionic compound additives in perovskite with the solution method.

关键词： Synergistic passivation strategy Defects passivation Dielectric screening Perovskite light-emitting diodes

High-sensitivity photovoltage based on the interfacial photoelectric effect in the SrTiO_(3-δ)/Si heterojunction

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Science china(Physics,Mechanics & Astronomy) 2010年第11期53卷 2080-2083页

作者： WEN Juan 1,guo HaiZhong 1,xing Jie 2,Lü HuiBin 1,JIN Kui-Juan 1,HE Meng 1 & YANG guoZhen 1 1 Beijing National Laboratory for Condensed Matter Physics,institute of Physics,Chinese Academy of Sciences,Beijing 100190,china 2 School of Materials Sciences and technology,china university of Geosciences,Beijing 100083,china 1. Beijing National Laboratory for Condensed Matter Physics Institute of Physics Chinese Academy of Sciences Beijing 100190 China2. School of Materials Sciences and Technology China University of Geosciences Beijing 100083 China

A high sensitivity photovoltaic effect has been observed in a heterojunction composed of n-type wide bandgap oxide SrTiO 3-δ and p-type Si fabricated by laser molecular beam *** responsivity of open-circuit photovoltage can reach 10 4 V/W without any amplification under zero bias for the wavelength range from visible to near infrared light in nW-μW *** attribute the high performance of the photovoltage responsivity to the interfacial photoelectric effects in the SrTiO 3-δ /Si *** the experimental results,some ideas can be generalized to improve photovoltaic efficiency and develop high sensitivity photodetectors with wide bandgap oxide materials and Si.

关键词： SrTiO 3-δ/Si heterojunction interfacial photoelectric effect photovoltage

Distribution and bioavailability of mercury in size-fractioned atmospheric particles around an ultra-low emission power plant in Southwest china

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Journal of Environmental Sciences 2024年第4期138卷 141-152页

作者： Wei Zhang Jinjuan Li Hao Qiu xingqiang guo Zhijun Fei Yi xing Deliang Yin College of Resources and Environmental Engineering Guizhou UniversityGuiyang 550025China College of Resources and Environmental Engineering Guizhou Institute of TechnologyGuiyang 550003China Key Laboratory of Karst Georesources and Environment(Guizhou university) Ministry of EducationGuiyang 550025China School of Energy and Environmental Engineering University of Science&Technology BeijingBeijing 100083China

Ultra-low emission(ULE)technology retrofits significantly impact the particulate-bound mercury(Hg)emissions from coal-fired power plants(CFPPs);however,the distribution and bioavailability of Hg in size-fractioned particulate matter(PM)around the ULE-retrofitted CF-PPs are less ***,total Hg and its chemical speciation in TSP(total suspended particles),PM_(10)(aerodynamic particle diameter≤10μm)and PM_(2.5)(aerodynamic particle diameter≤2.5μm)around a ULE-retrofitted CFPP in Guizhou Province were *** PM_(2.5)concentration was higher around this ULE-retrofitted CFPP than that in the intra-regional urban cities,and it had higher mass Hg concentration than other sizefractioned *** Hg concentrations in PM had multifarious sources including CFPP,vehicle exhaust and biomass combustion,while they were significantly higher in autumn and winter than those in other seasons(P21%)while higher HCl-soluble fractions(>40%).Mass concentrations of exchangeable,HCl-soluble,elemental,and residual Hg in PM_(2.5)were higher than those in other size-fractioned PM,and were markedly elevated in autumn and winter(P2.5),HCl-soluble Hg presented a significantly positive relationship with elemental Hg(P1).Overall,these results suggested that atmospheric PM-bound Hg around the ULE-retrofitted CFPP tends to accumulate in finer PM,and has higher bioavailable fractions,while has potential transformation between chemical speciation.

关键词： Size-fractioned particles Mercury Chemical speciation Coal-fired power plant Ultra-low emission

HDPairFinder:A data processing platform for hydrogen/deuterium isotopic labeling-based nontargeted analysis of trace-level amino-containing chemicals in environmental water

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Journal of Environmental Sciences 2024年第2期136卷 583-593页

作者： Tingting Zhao Kristin Carroll Caley B.Craven Nicholas J.P.Wawryk Shipei xing Jian guo xing-Fang Li Tao Huan Department of Chemistry Faculty of ScienceUniversity of British ColumbiaVancouver Campus2036 Main MallVancouverBritish ColumbiaV6T 1Z1Canada Division of Analytical and Environmental Toxicology Department of Laboratory Medicine and PathologyFaculty of Medicine and DentistryUniversity of AlbertaEdmontonAlberta T6G 2G3Canada

The combination of hydrogen/deuterium(H/D)formaldehyde-based isotopic methyl labeling with solid-phase extraction and high-performance liquid chromatography–high resolution mass spectrometry(HPLC-HRMS)is a powerful analytical solution for nontargeted analysis of trace-level amino-containing chemicals in water *** the huge amount of chemical information generated in HPLC-HRMS analysis,identifying all possible H/Dlabeled amino chemicals presents a significant challenge in data *** address this,we designed a streamlined data processing pipeline that can automatically extract H/D-labeled amino chemicals from the raw HPLC-HRMS data with high accuracy and ***,we developed a cross-correlation algorithm to correct the retention time shift resulting from deuterium isotopic effects,which enables reliable pairing of H-and D-labeled ***,we implemented several bioinformatic solutions to remove false chemical features generated by in-source fragmentation,salt adduction,and natural13C ***,we used a data mining strategy to construct the AMINES library that consists of over 38,000 structure-disjointed primary and secondary amines to facilitate putative compound ***,we integrated these modules into a freely available R program,*** rationale of each module was justified and its performance tested using experimental H/D-labeled chemical standards and authentic water *** further demonstrated the application of HDPairFinder to effectively extract N-containing contaminants,thus enabling the monitoring of changes of primary and secondary N-compounds in authentic water *** is a reliable bioinformatic tool for rapid processing of H/D isotopic methyl labeling-based nontargeted analysis of water samples,and will facilitate a better understanding of N-containing chemical compounds in water.

关键词： Isotope labeling Nontargeted analysis Reactive N-compounds HPLC-HRMS Source water

A fiducial argument for generalized p-value

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Science china Mathematics 2007年第7期50卷 957-966页

作者： Xin-min LI~(1+) xing-zhong XU~2 guo-ying LI~3 1 institute of Applied Mathematics,Shandong university of technology,Zibo 255049,china 2 Department of Mathematics,Beijing institute of technology,Beijing 100801,china 3 Academy of Mathematics and Systems Science,Chinese Academy of Sciences,Beijing 100800,china institute of Applied Mathematics Shandong University of Technology Zibo 255049 China Department of Mathematics Beijing Institute of Technology Beijing 100801 China Academy of Mathemtics Systems Science Chinese Academy of Sciences Beijing 100800 China

This paper provides a general method for constructing generalized p-value via the fiducial ***,the power properties of the generalized test are *** illustrations, the two-parameter exponential distribution and unbalan... 详细信息

关键词： fiducial distribution generalized p-value frequency property two-parameter exponential distribution variance component 62F03 62E15

Finite groups in which elements of the same order outside the center are conjugate

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Science china Mathematics 2007年第10期50卷 1493-1500页

作者： xing-zhong YOU~1 guo-hua QIAN~2 Wu-jie SHI~(3+) ~1 School of Mathematics and Computing Science,Changsha university of Science and technology,Changsha 410076,china ~2 Department of Mathematics,Changshu institute of technology,Changshu 215500,china ~3 School of Mathematics,Suzhou university,Suzhou 215006,china 1. School of Mathematics and Computing Science Changsha University of Science and Technology Changsha 410076 China 2. Department of Mathematics Changshu Institute of Technology Changshu 215500 China 3. School of Mathematics Suzhou University Suzhou 215006 China

We prove that if G is a finite group in which the elements of the same order outside the center are conjugate, then either G is abelian or G ≌ S3.

关键词： finite group, rational group, conjugacy class

Impaired pericyte-Müller glia interaction via PDGFRβsuppression aggravates photoreceptor loss in a rodent model of light-induced retinal injury

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International Journal of Ophthalmology(English edition) 2024年第10期17卷 1800-1808页

作者： Wei Xu Li-Jin Cui Xiao-Ying Yang Xiao-Yuan Cui Jian guo guo-xing Xu Department of Ophthalmology the First Affiliated Hospital of Fujian Medical UniversityFuzhou 350001Fujian ProvinceChina Department of Ophthalmology National Regional Medical CenterBinhai Campus of the First Affiliated Hospital of Fujian Medical UniversityFuzhou 350212Fujian ProvinceChina Fujian institute of Ophthalmology Fuzhou 350001Fujian ProvinceChina

AIM:To investigate the involvement of pericyte-Müller glia interaction in retinal damage repair and assess the influence of suppressing the platelet-derived growth factor receptorβ(PDGFRβ)signaling pathway in retinal pericytes on photoreceptor loss and Müller glial ***:Sprague-Dawley rats were exposed to intense light to induce retinal *** antibody against PDGFRβwere deployed to block the signaling pathway in retinal pericytes through intravitreal *** histology and Müller glial reaction were assessed following light *** vitro,normal and PDGFRβ-blocked retinal pericytes were cocultured with Müller cell line(rMC-1)to examine morphological and protein expression changes upon supplementation with light-injured supernatants of homogenized retinas(SHRs).RESULTS:PDGFRβblockage 24h prior to intense light exposure resulted in a significant exacerbation of photoreceptor *** upregulation of GFAP and p-STAT3,observed after intense light exposure,was significantly inhibited in the PDGFRβblockage *** ther upregulation of cytokines monocyte chemoattractant protein 1(MCP-1)and interleukin-1β(IL-1β)was also observed following PDGFRβ*** the in vitro coculture system,the addition of light-injured SHRs induced pericyte deformation and upregulation of proliferating cell nuclear antigen(PCNA)expression,while Müller cells exhibited neuron-like morphology and expressed ***,PDGFRβblockage in retinal pericytes abolished these cellular responses to light-induced damage,consistent with the in vivo PDGFRβblockage ***:Pericyte-Müller glia interaction plays a potential role in the endogenous repair process of retinal *** of this interaction exacerbates photoreceptor degeneration in light-induced retinal injury.

关键词： pericyte Müller glia light-induced retinal injury platelet-derived growth factor receptorβ signal pathway

Techniques of mining under buildings in deep-lying seams

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中国有色金属学会会刊：英文版 2005年第S1期15卷 315-318页

作者： guo Zeng-zhang~(1,2), XIE He-ping~2, WANG Jin-zhuang~2 (1. Jiaozuo institute of technology, Jiaozuo 454000, china 2. china university of mining and technology, Beijing 100083, china) Jiaozuo Inst Technol Jiaozuo 454000 Peoples R China china Univ Min & Technol Beijing 100083 Peoples R China

The features of the surface subsidence basin caused by mining in the deep-lying seams are associated with the width of the coal pillar between two working faces. If the pillar is wide, a waved subsidence basin will occur on the surface. If the pillar is narrow, the maximum surface subsidence value will be very great. The influence of the interval pillar to the stress distribution caused by mining in the deep-lying seam was specially studied by using a three-dimensional finite-difference FLAC3D program. The techniques mining in the deep-lying seams under buildings were presented.

关键词： mining subsidence numerical simulation extraction under buildings

Fe-N-C core-shell catalysts with single low-spin Fe(Ⅱ)-N_(4)species for oxygen reduction reaction and high-performance proton exchange membrane fuel cells

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Journal of Energy Chemistry 2024年第6期93卷 538-546,I0013页

作者： Yan Wan Linhui Yu Bingxin Yang Caihong Li Chen Fang Wei guo Fang-xing Xiao Yangming Lin Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials Xiamen Institute of Rare Earth MaterialsHaixi InstituteChinese Academy of SciencesXiamen 361021FujianChina CAS Key Laboratory of Urban Pollutant Conversion Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021FujianChina Fujian institute of Research on the Structure of Matter Chinese Academy of SciencesFuzhou 350002FujianChina College of Materials Science and Engineering Fuzhou UniversityNew CampusMinhou 350108FujianChina College of Chemistry and Materials Science Fujian Normal UniversityFuzhou 350117FujianChina

Fe-N-doped carbon materials(Fe-N-C)are promising candidates for oxygen reduction reaction(ORR)relative to Pt-based catalysts in proton exchange membrane fuel cells(PEMFCs).However,the intrinsic contributions of Fe-N_(4)moiety with different chemical/spin states(e.g.D1,D2,D3)to ORR are unclear since various states coexist *** the present work,Fe-N-C core-shell nanocatalyst with single lowspin Fe(Ⅱ)-N_(4)species(D1)is synthesized and identified with ex-situ ultralow temperature Mossbauer spectroscopy(T=1.6 K)that could essentially differentiate various Fe-N_(4)states and invisible Fe-O *** quantifying with CO-pulse chemisorption,site density and turnover frequency of Fe-N-C catalysts reach 2.4×10^(-9)site g^(-1)and 23 e site~(-1)s^(-1)during the ORR,***-wave potential(0.915V_(RHE))of the Fe-N-C catalyst is more positive(approximately 54 mV)than that of Pt/***,we observe that the performance of PEMFCs on Fe-N-C almost achieves the 2025 target of the US Department of Energy by demonstrating a current density of 1.037 A cm^(-2)combined with the peak power density of 0,685 W cm^(-2),suggesting the critical role of Fe(Ⅱ)-N_(4)site(D1).After 500 h of running,PEMFCs still deliver a power density of 1.26 W cm^(-2)at 1.0 bar H_(2)-O_(2),An unexpected rate-determining step is figured out by isotopic labelling experiment and theoretical *** work not only offers valuable insights regarding the intrinsic contribution of Fe-N_(4)with a single spin state to alkaline/acidic ORR,but also provides great opportunities for developing high-performance stable PEMFCs.

关键词： Fuel cells Oxygen reduction reaction Non-platinum group metals(PGMs) Isotopic labelling Active site TOF