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Remediation mechanism of high concentrations of multiple heavy metals in contaminated soil by Sedum alfredii and native microorganisms

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Journal of Environmental Sciences 2025年第1期147卷 179-188页

作者： Zihe Wang Han Zhang Ying xiong Lieyu Zhang Jianglong Cui Guowen Li Caili Du Kaiyang Wen State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental SciencesBeijing 100012China Beijing Water Science and Technology Institute Beijing 100044China School of Architecture and Civil Engineering Chengdu UniversityChengdu 610106China

Pollution accident of nonferrous metallurgy industry often lead to serious heavy metal pollution of the surrounding *** of contaminated soil is an environmental and sustainable technology,and soil native microorganisms in the process of phytoremediation also participate in the remediation of heavy ***,the effects of high concentrations of multiple heavy metals(HCMHMs)on plants and native soil microorganisms remain ***,further clarification of themechanism of phytoremediation of HCMHMs soil by plants and native soil microorganisms is *** the plant Sedum alfredii(***)to restore HCMHM-contaminated soil,we further explored the mechanism of *** and native soil microorganisms in the remediation of HCMHM *** results showed that(i)*** can promote heavy metals from non-rhizosphere soil to rhizosphere soil,which is conducive to the effect of plants on heavy *** addition,it can also enrich the absorbed heavy metals in its roots and leaves;(ii)native soil bacteria can increase the abundance of signal molecule-synthesizing enzymes,such as trpE,trpG,bjaI,rpfF,ACSL,and yidC,and promote the expression of the pathway that converts serine to cysteine,then synthesize substances to chelate heavy *** addition,we speculated that genes such as K19703,K07891,K09711,K19703,K07891,and K09711 in native bacteria may be involved in the stabilization or absorption of heavy *** results provide scientific basis for *** to remediate heavy metals contaminated soils,and confirm the potential of phytoremediation of HCMHM contaminated soil.

关键词： Microbial remediation Phytoremediation Sedum alfredii

Influence of introducing Zr,Ti,Nb and Ce elements on externally solidified crystals and mechanical properties of high-pressure die-casting Al–Si alloy

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International Journal of Minerals,Metallurgy and Materials 2025年第1期32卷 147-153页

作者： Junjie Li Wenbo Yu Zhenyu Sun Weichen Zheng Liangwei Zhang Yanling Xue Wenning Liu Shoumei xiong Center of Materials Science and Engineering School of Mechanical and Electronic Control EngineeringBeijing Jiaotong UniversityBeijing 100044China Traffic&Transportation Engineering Central South UniversityChangsha 410075China Shanghai Synchrotron Radiation Facility Shanghai Advanced Research InstituteChinese Academy of SciencesShanghai 201204China School of Materials Science and Engineering Tsinghua UniversityBeijing 100084China

High pressure die casting(HPDC)AlSi10Mn Mg alloy castings are widely used in the automobile *** can optimize the mechanical properties of castings through heat treatment,while the release of thermal stress arouses the deformation of large integrated ***,the development of non-heat treatment Al alloys is becoming the hot *** addition,HPDC contains externally solidified crystals(ESCs),which are detrimental to the mechanical properties of *** achieve high strength and toughness of non-heat treatment die-casting Al-Si alloy,we used AlSi9Mn alloy as matrix with the introduction of Zr,Ti,Nb,and *** influences on ESCs and mechanical properties were systematically investigated through three-dimensional reconstruction and thermodynamic *** results reveal that the addition of Ti increased ESCs'size and porosity,while the introduction of Nb refined ESCs and decreased ***,large-sized Al_3(Zr,Ti)phases formed and degraded the mechanical *** introduction of Ce resulted in the poisoning effect and reduced mechanical properties.

关键词： aluminium alloy high-pressure die-casting externally solidified crystals non-heat treatment

Solar flare forecasting based on a Fusion Model

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Earth and Planetary Physics 2025年第1期9卷 171-181页

作者： YiYang Li ShiYong Huang SiBo Xu ZhiGang Yuan Kui Jiang QiYang xiong RenTong Lin School of Earth and Space Science Technology Hubei Luojia LaboratoryWuhan UniversityWuhan 430072China

Solar flare prediction is an important subject in the field of space *** learning technology has greatly promoted the development of this *** this study,we propose a novel solar flare forecasting model integrating Deep Residual Network(ResNet)and Support Vector Machine(SVM)for both≥C-class(C,M,and X classes)and≥M-class(M and X classes)*** collected samples of magnetograms from May 1,2010 to September 13,2018 from Space-weather Helioseismic and Magnetic Imager(HMI)Active Region Patches and then used a cross-validation method to obtain seven independent data *** then utilized five metrics to evaluate our fusion model,based on intermediate-output extracted by ResNet and SVM using the Gaussian kernel *** results show that the primary metric true skill statistics(TSS)achieves a value of 0.708±0.027 for≥C-class prediction,and of 0.758±0.042 for≥M-class prediction;these values indicate that our approach performs significantly better than those of previous *** metrics of our fusion model’s performance on the seven datasets indicate that the model is quite stable and robust,suggesting that fusion models that integrate an excellent baseline network with SVM can achieve improved performance in solar flare ***,we also discuss the performance impact of architectural innovation in our fusion model.

关键词： solar flare pace weather deep learning Fusion Model

CO_(2)-mediated bicarbonate conversion to concentrated formate in a CEM-based electrolyzer

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Journal of Energy Chemistry 2025年第1期100卷 605-611页

作者： Haocheng xiong Donghuan Wu Haonan Li Andrew Li Qikun Hu Siyao Song Bingjun Xu Qi Lu State Key Laboratory of Chemical Engineering Department of Chemical EngineeringTsinghua UniversityBeijing 100084China College of Chemistry and Molecular Engineering Peking UniversityBeijing 100871China Ordos Laboratory Inner Mongolia 017000China

Renewable energy-driven bicarbonate conversion to valuable chemicals presents an attractive strategy for mitigating CO_(2)emissions,as bicarbonate can be efficiently generated from the capture of atmospheric CO_(2)using alkaline solutions with reactive *** this work,we present a CO_(2)-mediated bicarbonate conversion to pure formate using a cation exchange membrane-based electrolyzer with a 25 cm^(2)electrode *** electrolysis achieved selectivities exceeding 75%for formate at a total current of 2.5 A,achieving formate concentrations up to 1.2 M and yields as high as 95%over extended *** techno-economic assessment confirmed the economic viability of the process,highlighting the potential for bicarbonate electrolysis as a sustainable method for producing valuable chemicals.

关键词： Electrocatalysis Techno-economic assessments Electrochemistry Flow electrolyzer

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数字孪生战场:概念、架构与技术

系统工程与电子技术 2025年第1期47卷 141-152页

作者：熊宇涵李雄中山大学系统科学与工程学院广东广州510275

当前作战仿真模型存在态势理解滞后、物理模型无法更新等问题,这些问题将影响后续态势推演与决策效果。为此,提出数字孪生战场的概念,并建立数字孪生战场的4层架构模型。基于这种模型,分析其在战场空间的部署方式及寿命周期运用,探讨其... 详细信息

当前作战仿真模型存在态势理解滞后、物理模型无法更新等问题,这些问题将影响后续态势推演与决策效果。为此,提出数字孪生战场的概念,并建立数字孪生战场的4层架构模型。基于这种模型,分析其在战场空间的部署方式及寿命周期运用,探讨其潜在运用价值。同时,从多源数据采集与处理、孪生战场建模、模型动态更新和态势推演与决策4个视角出发,讨论数字孪生战场建模所需的关键技术。随着作战仿真模型的运用,可以帮助指挥机构做出更高效的决策。

关键词：数字孪生战场指挥决策多源数据采集作战建模模型更新态势推演

On the ionospheric response in the Taiwan region to Typhoon Meranti in September 2016

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Geodesy and Geodynamics 2025年第1期16卷 29-41页

作者： Peng Chen Mingzhu xiong Yibin Yao Hao Chen Fucai Tang Liangcai Qiu Yuchen Zhang College of Geomatics Xi'an University of Science and Technology State Key Laboratory of Geodesy and Earth's Dynamics Innovation Academy for Precision Measurement Science and Technology Chinese Academy of Science School of Geodesy and Geomatics Wuhan University Key Laboratory of Geospace Environment and Geodesy Ministry of Education Wuhan University

Previous studies have revealed that typhoons can affect the ionosphere. This paper uses GNSS observations provided by GNSS tracking stations of Taiwan region, ERA5 gravity wave dissipation products,and Himawari-8 band 07 brightness temperature observation data to analyze the impact of Typhoon Meranti on Taiwan region's ionosphere from September 13 to 15, 2016. In addition to the daily effects of traveling ionospheric disturbances(TIDs), TIDs of various intensities caused by Meranti-induced gravity waves were observed during this period, which is inseparable from the state of the typhoon and the topographic features during its progress. The ionospheric disturbance caused by the edge of a typhoon is usually larger than that at the typhoon eye. When the typhoon approached Taiwan region with high intensity on September 14, it was observed that the gravity waves caused by the typhoon had a wavelength of about 174-293 km, a period of 13.5-23.5 min, and a propagation speed of 142-302 m/s. When the vortex structure of a typhoon interacts with complex surfaces such as mountains, it is easier to excite more medium-scale gravity waves. The origin that excites gravity waves and causes ionospheric anomalies is different from the location of the typhoon eye and changes over time. The gravity waves caused by the typhoon lasted for three days in the central mountains of Taiwan region. Still, background wind conditions restricted the propagation of gravity waves from the mesosphere to the thermosphere and led to TID predominantly concentrated between 06:00 and 13:00 UT each day.

关键词： Typhoon GNSS TEC TID Gravity waves

Insight into the activation of peroxymonosulfate by N-doped copper-based carbon for efficient degradation of organic pollutants:Synergy of nonradicals

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Chinese Chemical Letters 2025年第1期36卷 513-520页

作者： Mengmeng Ao Jian Wei Chuan-Shu He Heng Zhang Zhaokun xiong Yonghui Song Bo Lai College of Environmental Sciences Liaoning UniversityShenyang 110036China State Key Laboratory of Hydraulics and Mountain River Engineering College of Architecture and EnvironmentSichuan UniversityChengdu 610065China State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental SciencesBeijing 100012China

The contamination of water resources by phenolic compounds(PCs)presents a significant environmental hazard,necessitating the development of novel materials and methodologies for effective *** this study,a metallic copper-doped zeolitic imidazolate framework was pyrolyzed and designated as CuNC-20 for the activation of peroxymonosulfate(PMS)to degrade phenol(PE).Cu-NC-20 could effectively address the issue of metal agglomeration while simultaneously diminishing copper dissolution during the activation of PMS *** Cu-NC-20 catalyst exhibited a rapid degradation rate for PE across a broad pH range(3-9)and demonstrated high tolerance towards coexisting *** to scavenger experiments and electron paramagnetic resonance analysis,singlet oxygen(^(1)O_(2))and high-valent copperoxo(Cu(Ⅲ))were the predominant reactive oxygen species,indicating that the system was nonradicaldominated during the degradation *** quantitative structure-activity relationship(QSAR)between the oxidation rate constants of various substituted phenols and Hammett constants was *** indicated that the Cu-NC-20/PMS system had the optimal oxidation rate constant withσ^(-)correlation and exhibited a typical electrophilic reaction *** study provides a comprehensive understanding of the heterogeneous activation process for the selective removal of phenolic compounds.

关键词： N-doped copper-based carbon Phenolic compounds Peroxymonosulfate Nonradical pathway Quantitative structure-activity relationship(QSAR)

GPS: graph contrastive learning via multi-scale augmented views from adversarial pooling

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Science China(Information Sciences) 2025年第1期68卷 145-158页

作者： Wei JU Yiyang GU Zhengyang MAO Ziyue QIAO Yifang QIN Xiao LUO Hui xiong Ming ZHANG School of Computer Science National Key Laboratory for Multimedia Information ProcessingPeking University Artificial Intelligence Thrust The Hong Kong University of Science and Technology Department of Computer Science University of California

Self-supervised graph representation learning has recently shown considerable promise in a range of fields, including bioinformatics and social networks. A large number of graph contrastive learning approaches have shown promising performance for representation learning on graphs, which train models by maximizing agreement between original graphs and their augmented views(i.e., positive views). Unfortunately, these methods usually involve pre-defined augmentation strategies based on the knowledge of human experts. Moreover, these strategies may fail to generate challenging positive views to provide sufficient supervision signals. In this paper, we present a novel approach named graph pooling contrast(GPS) to address these *** by the fact that graph pooling can adaptively coarsen the graph with the removal of redundancy, we rethink graph pooling and leverage it to automatically generate multi-scale positive views with varying emphasis on providing challenging positives and preserving semantics, i.e., strongly-augmented view and weakly-augmented view. Then, we incorporate both views into a joint contrastive learning framework with similarity learning and consistency learning, where our pooling module is adversarially trained with respect to the encoder for adversarial robustness. Experiments on twelve datasets on both graph classification and transfer learning tasks verify the superiority of the proposed method over its counterparts.

关键词： graph representation learning graph neural networks graph contrastive learning graph augmentations graph pooling

AZD1775 synergizes with SLC7A11 inhibition to promote ferroptosis

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Science China(Life Sciences) 2025年第1期68卷 204-218页

作者： Chen xiong Hong Ling Yingdan Huang Hanzhi Dong Bangxiang Xie Qian Hao Xiang Zhou Fudan University Shanghai Cancer Center and Institutes of Biomedical Sciences Fudan UniversityShanghai 200032China Department of Oncology Shanghai Medical CollegeFudan UniversityShanghai 200032China Department of Breast Surgery Fudan University Shanghai Cancer CenterFudan UniversityShanghai 200032China Department of Oncology First Affiliated Hospital of Nanchang UniversityNanchang 330006China Beijing Institute of Hepatology Beijing Youan HospitalCapital Medical UniversityBeijing 100069China Beijing Engineering Research Center for Precision Medicine and Transformation of Hepatitis and Liver Cancer Beijing 100069China Key Laboratory of Breast Cancer in Shanghai Fudan University Shanghai Cancer CenterFudan UniversityShanghai 200032China Shanghai Key Laboratory of Medical Epigenetics International Co-laboratory of Medical Epigenetics and Metabolism(Ministry of Science and Technology)Institutes of Biomedical SciencesFudan UniversityShanghai 200032China

Tumor suppressor p53-mediated cell cycle arrest and DNA damage repair may exert cytoprotective effects against cancer therapies,including WEE1 *** that p53 activation can also lead to multiple types of cell death,the role of this tumor suppressor in WEE1 inhibitor-based therapies remains *** this study,we reported that nucleolar stress-mediated p53 activation enhanced the WEE1 inhibitor AZD1775-induced ferroptosis to suppress lung cancer *** findings showed that AZD1775 promoted ferroptosis by blocking cystine uptake,an action similar to that of ***,inhibition of WEE1 by the WEE1 inhibitors or siRNAs induced compensatory upregulation of SLC7A11,which conferred resistance to ***,AZD1775 prevented the enrichment of H3K9me3,a histone marker of transcriptional repression,on the SLC7A11 promoter by repressing the expression of the histone methyltransferase SETDB1,thereby enhancing NRF2-mediated SLC7A11 *** finding was also validated using the H3K9me3 inhibitor ***,we found that the nucleolar stress-inducing agent Actinomycin D(Act.D)inhibited SLC7A11 expression by activating p53,thus augmenting AZD1775-induced ***,the combination of AZD1775 and Act.D synergistically suppressed wild-type p53-harboring lung cancer cell growth both in vitro and in ***,our study demonstrates that AZD1775 promotes ferroptosis by targeting cystine uptake but also mediates the adaptive activation of SLC7A11 through the WEE1-SETDB1 cascade and NRF2-induced transcription,and inhibition of SLC7A11 by Act.D boosts the anti-tumor efficacy of AZD1775 by enhancing ferroptosis in cancers with wild-type p53.

关键词： p53 NRF2 SLC7A11 WEE1 AZD1775 ferroptosis nucleolar stress