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Development review and the prospect of oil shale in-situ catalysis conversion technology

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Petroleum Science 2024年第2期21卷 1385-1395页

作者： Li Wang Chen-Hao Gao Rui-Ying xiong Xiao-jun Zhang ji-Xiang Guo The Unconventional Oil and Gas Institute China University of Petroleum-BeijingBeijing102200China

As an unconventional resource, oil shale possesses abundant reserves and significant potential for industrial applications. The rational and efficient development of oil shale resources holds immense importance in reducing national energy demand. In-situ catalytic technology, characterized by its high efficiency, low pollution, and minimal energy consumption, represents a key direction for future oil shale development. This paper provides a comprehensive review of research progress in in-situ oil shale mining technology, oil shale pyrolysis catalysts, the pyrolysis mechanism of kerogen, and the compatibility of different heating processes and catalysts. Furthermore, the paper proposes future research directions and prospects for oil shale in-situ catalytic technology, including reservoir modification, highefficiency catalyst synthesis, injection processes, and high-efficiency heating technology. These insights serve as valuable technical references for the advancement of oil shale in-situ catalytic technology.

关键词： Oil shale In-situ catalytic technology Pyrolysis catalyst Kerogen pyrolysis mechanism

Human movement monitoring and behavior recognition for intelligent sports using customizable and flexible triboelectric nanogenerator

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Science China(Technological Sciences) 2022年第4期65卷 826-836页

作者： YANG Yun HOU XiaoJuan GENG WenPing MU jiLiang ZHANG Le WANG XiangDong HE jian xiong ji jun CHOU Xiujian Science and Technology on Electronic Test and Measurement Laboratory North University of ChinaTaiyuan 030051China Department of Mining Engineering Luliang UniversityLvliang 033000China Physical Education Institute Jimei UniversityXiamen 361021China

Effective collection,recognition,and analysis of sports information is the key to intelligent sports,which can help athletes to improve their skills and formulate scientific training plans and competition *** present,wearable electronic devices used for movement monitoring still have some limitations,such as high cost and energy consumption,incompatibility of suitable flexibility and personalized spatial structure,dissatisfactory data analysis methods,*** this work,a novel three-dimensionalprinted thermoplastic polyurethane is introduced as the elastic shell and friction layer,and it endows the proposed customizable and flexible triboelectric nanogenerator(CF-TENG)with personalized spatial structure and robust correlation to external *** practical application,it exhibits highly sensitive responses to the joint-bending motion of the finger,wrist,or ***,a pressure-sensing insole and smart ski pole based on CF-TENG are manufactured to build a comprehensive sports monitoring system to transmit the athletes’motion information from feet and hands through the plantar pressure distribution and ski pole *** recognize the movement status,the self-developed automatic peak recognition algorithm(P-Find)and machine learning algorithm(subspace K-Nearest Neighbors)were introduced to accurately distinguish the four typical motion behaviors and three primary sub-techniques of cross-country skiing,with accuracy rates of 98.2%and 100%.This work provides a novel strategy to promote the personalized applications of TENGs in intelligent sports.

关键词： triboelectric nanogenerator flexible movement monitoring behavior recognition intelligent sports

In situ modification of heavy oil catalyzed by nanosized metal-organic framework at mild temperature and its mechanism

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Chinese Journal of Chemical Engineering 2024年第3期67卷 166-173页

作者： Li Wang ji-Xiang Guo Rui-Ying xiong Chen-Hao Gao Xiao-jun Zhang Dan Luo The Unconventional Oil and Gas Institute China University of Petroleum-BeijingBeijing 102200China Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of SciencesBeijing 101400China

Two catalysts, nano-sized cobalt-metal-organic framework(Co-MOF) and nickel(Ni)-MOF, were successfully prepared by the modification method. Tetralin(C10H12) was used as the hydrogen donor for the catalytic cracking and hydrogenation modification study of the dehydrated crude oil from the Shengli Oilfield. The optimal reaction conditions were determined through orthogonal experiments, and the components of the crude oil and modified oil samples were analyzed. The results revealed that the nanoMOF catalysts were successfully prepared and exhibited high catalytic activity. They could catalyze the cracking of large molecules in heavy oil at mild temperatures(<300°C), leading to the decomposition of the hydrogen donor. When the mass fraction of the catalyst was 0.2%, the mass fraction of the hydrogen donor was 1%, and the reaction temperature was 280°C, the Ni-MOF showed the best catalytic viscosity reduction effect. It could reduce the viscosity of heavy oil at 50°C from 15761.9 m Pa.s to 1266.2 m Pa.s,with a viscosity reduction rate of 91.97%. The modification effect of Co-MOF was the next best, which could reduce the viscosity of heavy oil to 2500.1 m Pa.s with a viscosity reduction rate of 84.14%. Molecular dynamics simulations revealed a strong interaction force between the MOF surface and asphaltene molecules. In the process of heavy-oil catalytic hydrogenation, the nano-MOF catalyst exhibited high catalytic activity. On the one hand, the empty d orbitals outside the metal atoms in the catalyst could polarize the carbon atoms in the organic matter, accelerating the breaking of long chains. On the other hand, the metal atoms in the catalyst could bond with the carbon σ bonds, breaking the carbon-carbon bonds. This disrupted the structure of the recombined components in the crude oil, irreversibly reducing the viscosity of the heavy oil and improving its fluidity.

关键词： Nano-sized MOF Petroleum Viscosity reduction Catalyst Nanomaterials

Multiple exciton generation effect in photocatalytic overall water splitting

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Science China Chemistry 2024年第2期67卷 424-425页

作者： Xiaolei Guo ji-jun Zou Key Laboratory for Green Chemical Technology of Ministry of Education School of Chemical Engineering and TechnologyTianjin UniversityTianjin300072China

This highlight is based on recent research published in Nature Energy by Li and co-workers [1] from Northwestern Polytechnology University, reporting an exceeding 100% internal quantum efficiency(IQE) in photocatalytic overall water splitting. This breakthrough promises a bright future for efficient photocatalyst design by utilizing the multiple exciton effect(MEG).

关键词： splitting effect utilizing

Unlocking T cell exhaustion:Insights and implications for CAR-T cell therapy

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Acta Pharmaceutica Sinica B 2024年第8期14卷 3416-3431页

作者： Dian xiong Haijun Yu Zhi-jun Sun State Key Laboratory of Oral&Maxillofacial Reconstruction and Regeneration Key Laboratory of Oral Biomedicine Ministry of EducationHubei Key Laboratory of StomatologySchool&Hospital of StomatologyFrontier Science Center for Immunology and MetabolismTaikang Center for Life and Medical ScienceWuhan UniversityWuhan 430079China Department of Radiation and Medical Oncology Hubei Province Cancer Clinical Study CenterHubei Key Laboratory of Tumor Biological BehaviorsZhongnan Hospital of Wuhan UniversityWuhan 430071China

Chimeric antigen receptor T(CAR-T)cell therapy as a form of adoptive cell therapy(ACT)has shown significant promise in cancer treatment,demonstrated by the FDA-approved CAR-T cell therapies targeting CD19 or B cell maturation antigen(BCMA)for hematological malignancies,albeit with moderate outcomes in solid ***,despite these advancements,the efficacy of CAR-T therapy is often compromised by T cell exhaustion,a phenomenon that impedes the persistence and effector function of CAR-T cells,leading to a relapse rate of up to 75%in patients treated with CD19 or CD22 CAR-T cells for hematological *** to overcome CAR-T exhaustion employ state-of-the-art genomic engineering tools and single-cell sequencing *** this review,we provide a comprehensive understanding of the latest mechanistic insights into T cell exhaustion and their implications for the current efforts to optimize CAR-T cell *** insights,combined with lessons learned from benchmarking CAR-T based products in recent clinical trials,aim to address the challenges posed by T cell exhaustion,potentially setting the stage for the development of tailored next-generation approaches to cancer treatment.

关键词： Cancer immunotherapy CAR-T therapy T cell exhaustion Tumor immune microenvironment Spatial immune contexture Single-cell technologies CAR-T engineering Combination therapy

A review on reinforcement learning-based highway autonomous vehicle control

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Green Energy and Intelligent Transportation 2024年第4期3卷 72-90页

作者： Ali Irshayyid jun Chen Guojiang xiong Oakland University USA Guizhou UniversityChina

Autonomous driving is an active area of research in artificial intelligence and *** advances in deep reinforcement learning(DRL)show promise for training autonomous vehicles to handle complex real-world driving *** paper reviews recent advancement on the application of DRL to highway lane change,ramp merge,and platoon *** particular,similarities,differences,limitations,and best practices regarding the DRL formulations,DRL training algorithms,simulations,and metrics are reviewed and *** paper starts by reviewing different traffic scenarios that are discussed by the literature,followed by a thorough review on the DRL technology such as the state representation methods that capture interactive dynamics critical for safe and efficient merging and the reward formulations that manage key metrics like safety,efficiency,comfort,and *** from this review can guide future research toward realizing the potential of DRL for automated driving in complex traffic under uncertainty.

关键词： Autonomous vehicles Connected and automated vehicles Deep reinforcement learning Platoon

Restricted Arc-Connectivity of Harary Digraphs

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Journal of the Operations Research Society of China 2024年第2期12卷 540-547页

作者： jun-Hao Zhang ji-Xiang Meng College of Mathematics and System Science Xinjiang UniversityUrumqi 830046XinJiangChina

The h-restricted arc-connectivity of a digraph is an important parameter to measure fault-tolerance of interconnection *** paper determines that the h-restricted arc-connectivity of the Harary digraph D=G(n;1,2,.:,k)i... 详细信息

关键词： Restricted arc-connectivity λ_(h)(D) Super-λ_(h) λ_(h)-Atom λ_(h)-Superatom

Two-way shape memory effect in a Ti-Zr-Nb-Ta high-temperature shape memory alloy

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Rare Metals 2024年第3期43卷 1257-1262页

作者： Cheng-Yang xiong Tuo Li jun Wang Yan Li School of Materials Science and Engineering Beihang UniversityBeijing100191China

The two-way shape memory effect in a Ti-18.5Zr-10Nb-3.5Ta high-temperature shape memory alloy was investigated.X-ray diffraction measurem ent shows that the alloy is composed of orthorhombicα"-martensite.ωphase is not found in Ti-18.5Zr-10Nb-3.5Ta alloy due to the suppressing effect of Ta ***α"-martensite laths are found in the transmission electron microscope observation;after the bending deformation,there appear a lot of *** alloy exhibits a shape memory strain of 3.8%aud a high reverse martensite transformation start temperature of 464 *** maximum two-way shape memory strain of 1.2%is obtained in the alloy with the prebending training strain of 10%.The mechanism can be ascribed to the effect of internal stress field caused by dislocations.

关键词： Ti-Zr Shape memory alloys Two-way shape memory effect

Event-triggered adaptive output feedback control for hyperbolic PDEs: swapping-based design

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Science China(Information Sciences) 2024年第5期67卷 327-328页

作者： Chunting ji Zhengqiang ZHANG Xue-jun XIE School of Engineering Qufu Normal University Institute of Automation Qufu Normal University

Partial differential equations(PDEs) characterize transport phenomena and fluid flow, and common cases include heat exchangers and road traffic [1]. Recently, scholars have become enthusiastic about event-triggered control(ETC) of hyperbolic PDEs, primarily because it can help conserve computing and communication resources. For example,Ref. [2] presented an output feedback ETC scheme for 2 × 2hyperbolic PDEs.

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