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Dynamic mechanical properties,deformation and damage mechanisms of eutectic high-entropy alloy AlCoCrFeNi_(2.1)under plate impact

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journal of Materials Science & Technology 2023年第3期134卷 178-188页

作者： S.P.zhao Z.D.Feng L.x.Li x.j.zhao L.Lu S.Chen N.B.Zhang Y.Cai S.N.Luo The Peac Institute of Multiscale Sciences ChengduChina Key Laboratory of Advanced Technologies of Materials Ministry of EducationSouthwest Jiaotong UniversityChengduChina

Shock compression and spallation of a eutectic high-entropy alloy(HEA)AlCoCrFeNi_(2.1)with lamellar structure are investigated via plate impact loading with free-surface velocity measurements.The as-cast and postmortem samples are characterized with transmission electron microscopy,electron back-scatter diffraction and scanning electron microscopy.An accurate Hugoniot equation of state is determined.Af-ter shock compression to∼12 GPa,both the L1_(2)and B_(2)phases retain their ordered structures.Dense dislocations in the{111}slip planes,stacking faults and deformation twins are found in the L1_(2)phase,along with fewer dislocations in the{110}slip bands in the B(2)phase.Shock-induced deformation twin-ning within the L1_(2)phase of this HEA is observed as a new deformation mechanism under various load-ing conditions.For spallation,both ductile and brittle damage modes are observed.The micro voids and cracks prefer to nucleate at the phase boundaries chiefly,then in the B(2)phase.Under similar shock stress,the spall strength of AlCoCrFeNi_(2.1)HEA is about 40%higher than those of other reported dual-phase HEAs due to the high stability of its semi-coherent phase boundaries.

关键词： High-entropy alloy Hugoniot Spall damage Microstructure

Shock compression and spallation damage of high-entropy alloy Al_(0.1)CoCrFeNi

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journal of Materials Science & Technology 2022年第33期128卷 1-9页

作者： N.B.Zhang j.xu Z.D.Feng Y.F.Sun j.Y.Huang x.j.zhao x.H.Yao S.Chen L.Lu S.N.Luo Key Laboratory of Advanced Technologies of Materials Ministry of EducationSouthwest Jiaotong UniversityChengdu 610031China The Peac Institute of Multiscale Sciences Chengdu 610031China Department of Engineering Mechanics South China University of TechnologyGuangzhou 510641China

Shock compression and spallation damage of a face-center cubic phase high-entropy alloy(HEA)Al_(0.1)CoCrFeNi were investigated via plate impact experiments along with free surface velocity measurements.Postmortem samples were characterized with transmission electron microscopy and electron backscatter diffraction.The Hugoniot equation of state and spall strength at different impact strengths were determined.There exists a power-law relation between spall strength and strain rate.The spall strength of Al_(0.1)CoCrFeNi HEA is about 50%higher than those of previously studied HEAs and comparable to those widely applied structural stainless steels at the same shock stress.Dislocation glide and stacking faults are the important deformation mechanisms in the Al_(0.1)CoCrFeNi HEA.Nanotwins are only observed at high shock stress.Damage in the Al_(0.1)CoCrFeNi HEA is ductile in nature.Voids are nucleated preferentially in grain interiors,and the intragranular voids show a strong dependence on grain boundary misorientation and peak stress.

关键词： Al_(0.1)CoCrFeNi High-entropy alloy Hugoniot Spall damage Microstructure

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Study on Flower Bud Morphological Differentiation of ’Tianxiang’ Strawberry

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Study on Flower Bud Morphological Differentiation of ’Tianx...

Characteristics of concentrations and chemical compositions for PM2.5 in the region of Beijing, Tianjin, and Hebei, China

第七届世界草莓大会

作者： H.j.Lei x.j.zhao x.j.Shen Y.T.Zhang T.H.Li Department of Fruit Science College of Agriculture and Biotechnology/Key Laboratory of Stress Physiology and Molecular Biology for Fruit Trees of BeijingChina Agricultural University Forestry and Pomology Institute Beijing Academy of Agriculture and Forestry Sciences

Flower bud differentiation is very important for the yield and quality of strawberry fruit.In order to identify flower bud development,the paraffin section method was adopted to observe the morphological differentiation of apical meristems of ’Tianxiang’ strawberry（Fragaria × ananassa Duch.） runner plants in Beijing,2009.The results showed that top flower bud differentiation lasted for about44 days,might be divided into seven stages.On 15 September,the buds came into the primary differentiation stage,the apical points became semi-circular,broader,and nearly 70%of the buds started differentiation on 20 September.Then the inflorescence primordia were visible on the apical points,and about 60%of the buds went into the inflorescence primordium differentiation stage on 25 September.Thereafter,the sepal primordia appeared at the base of inflorescence primordia,60%of the buds were in the sepal primordium differentiation stage by 1 October.On 6 October,in about 90%of the buds the petal primordia could be seen inside of sepal primordial.About 10 d later,the stamen primordia developed in around 80%of the buds.On 22 October,the pistil primordia appeared on the surface of the receptacles.The main pistil primordium differentiation stage was from 22 to 29 October,and about 70%of the buds had finished their pistil primordium differentiation on 29 October.At the end of sampling on 29 October,the secondary buds were mainly in the stamen primordium differentiation stage,and the tertiary buds were mainly in the petal primordium differentiation stage.Our results provided the details of flower bud development in ’Tianxiang’strawberry in Beijing,which will contribute to its production and management.

关键词： strawberry flower bud morphological differentiation paraffin section

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Characteristics of concentrations and chemical compositions ...

深度学习在脑出血及向脑室内扩张和外周水肿的自动分割和体积测量方面显示出良好的可靠性

创新驱动发展提高气象灾害防御能力——第30届中国气象...

作者： P.S.zhao F.Dong D.He x.j.zhao x.L.Zhang W.Z.Zhang Q.Yao H.Y.Liu Institute of Urban Meteorology China Meteorological Administration Meteorological Science Institute of Hebei Meteorological Science Institute of Tianjin Chengde Meteorological Bureau

In order to study the temporal and spatial variations of PM 2.5 and its chemical compositions in the region of Beijing, Tianjin, and Hebei （BTH）, PM 2.5 samples were collected at four urban sites in Beijing （Bj）, Tianjin （Tj）, Shijiazhuang （SjZ）, and Chengde （CD）, and also one site at Shangdianzi （SDZ） regional background station over four seasons from 2009 to 2010. The samples were weighted for mass concentrations and analyzed in the laboratory for chemical profiles of 19 elements （Al, As, Ba, Ca, Cd, Co, Cr, Cu, Fe, K, Mg, Mn, Ni, P, Pb, Sr, Ti, V, and Zn）, eight water-soluble inorganic ions （Na+ , NH4+ , K+ , Mg2+ , Ca2+ , Cl- , NO3- , and SO42- ）, and carbon fractions （OC and EC）. The concentrations of PM 2.5 and its major chemical species were season dependent and showed spatially similar characteristics in the plain area of BTH. The average annual concentrations of PM 2.5 were 71.8-191.2 μgm -3 at the five sites, with more than 90% of sampling days exceeding 50 μg m -3 at Bj, Tj, and SjZ. PM 2.5 pollution was most serious at SjZ, and the annual concentrations of PM 2.5 , secondary inorganic ions, OC, EC, and most crustal elements were all highest. Due to stronger photochemical oxidation, the sum of concentrations of secondary inorganic ions （NH4+ , NO3- , and SO42- ） was highest in the summer at SDZ, Bj, Tj, and CD. Analysis of electric charges of water-soluble inorganic ions indicated the existence of nitric acid or hydrochloric acid in PM 2.5 . For all five sites, the concentrations of OC, EC and also secondary organic carbon （SOC） in the spring and summer were lower than those in the autumn and winter. SOC had more percentages of increase than primary organic carbon （POC） during the winter. The sums of crustal elements （Al, Ca, Fe, Mg, Ti, Ba, and Sr） were higher in the spring and autumn owing to more days with blowing or floating dust. The concentrations of heavy metals were at higher levels in the BTH area by comparison with other studies. In Shijiazhuang and Chengde, the PM 2.5 pollution was dominated

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国际医学放射学杂志 2021年第5期 609-609页

作者： x.j.zhao K.x.Chen G.Wu G.Y.Zhang x.Zhou C.F.Lv 欧静

摘要目的首次评价基于无新网络的深度学习方法在CT上对原发性脑出血(ICH)、脑出血向脑室内扩张(IVH)和血肿周围水肿(PHE)的全自动分割和体积测量的性能。方法

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H-and j-aggregation of conjugated small molecules in organic solar cells

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journal of Energy Chemistry 2024年第6期93卷 174-192,I0005页

作者： Qiaoqiao zhao Feng He State Key Laboratory of Biobased Material and Green Papermaking Qilu University of TechnologyShandong Academy of SciencesJinan 250353ShangdongChina Shenzhen Grubbs Institute and Department of Chemistry Southern University of Science and TechnologyShenzhen 518055GuangdongChina Guangdong Provincial Key Laboratory of Catalysis Southern University of Science and TechnologyShenzhen 518055GuangdongChina

As H-and j-aggregation receive more and more attention in the research of organic solar cells(OSCs),especially in small molecular systems,deep understanding of aggregation behavior is needed to guide the design of conjugated small molecular structure and the fabrication process of OSC device.For this end,this review is written.Here,the review firstly introduced the basic information about H-and j-aggregation of conjugated small molecules in OSCs.Then,the characteristics of H-and j-aggregation and the methods to identify them were summarized.Next,it reviewed the research progress of H-and j-aggregation of conjugated small molecules in OSCs,including the factors influencing H-and j-aggregation in thin film and the effects of H-and j-aggregation on OPV performance.

关键词： H-aggregation j-aggregation Organic solar cells Small molecules Efficiency Stability

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STCF conceptual design report (Volume 1): Physics & detector

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Frontiers of physics 2024年第1期19卷 1-154页

作者： M.Achasov x.C.Ai L.P.An R.Aliberti Q.An x.Z.Bai Y.Bai O.Bakina A.Barnyakov V.Blinov V.Bobrovnikov D.Bodrov A.Bogomyagkov A.Bondar I.Boyko Z.H.Bu F.M.Cai H.Cai j.j.Cao Q.H.Cao x.Cao Z.Cao Q.Chang K.T.Chao D.Y.Chen H.Chen H.x.Chen j.F.Chen K.Chen L.L.Chen P.Chen S.L.Chen S.M.Chen S.Chen S.P.Chen W.Chen x.Chen x.F.Chen x.R.Chen Y.Chen Y.Q.Chen H.Y.Cheng j.Cheng S.Cheng T.G.Cheng j.P.Dai L.Y.Dai x.C.Dai D.Dedovich A.Denig I.Denisenko j.M.Dias D.Z.Ding L.Y.Dong W.H.Dong V.Druzhinin D.S.Du Y.j.Du Z.G.Du L.M.Duan D.Epifanov Y.L.Fan S.S.Fang Z.j.Fang G.Fedotovich C.Q.Feng x.Feng Y.T.Feng j.L.Fu j.Gao Y.N.Gao P.S.Ge C.Q.Geng L.S.Geng A.Gilman L.Gong T.Gong B.Gou W.Gradl j.L.Gu A.Guevara L.C.Gui A.Q.Guo F.K.Guo j.C.Guo j.Guo Y.P.Guo Z.H.Guo A.Guskov K.L.Han L.Han M.Han x.Q.Hao j.B.He S.Q.He x.G.He Y.L.He Z.B.He Z.x.Heng B.L.Hou T.j.Hou Y.R.Hou C.Y.Hu H.M.Hu K.Hu R.j.Hu W.H.Hu x.H.Hu Y.C.Hu j.Hua G.S.Huang j.S.Huang M.Huang Q.Y.Huang W.Q.Huang x.T.Huang x.j.Huang Y.B.Huang Y.S.Huang N.Hüsken V.Ivanov Q.P.ji j.j.jia S.jia Z.K.jia H.B.jiang j.jiang S.Z.jiang j.B.jiao Z.jiao H.j.jing x.L.Kang x.S.Kang B.C.Ke M.Kenzie A.Khoukaz I.Koop E.Kravchenko A.Kuzmin Y.Lei E.Levichev C.H.Li C.Li D.Y.Li F.Li G.Li G.Li H.B.Li H.Li H.N.Li H.j.Li H.L.Li j.M.Li j.Li L.Li L.Li L.Y.Li N.Li P.R.Li R.H.Li S.Li T.Li W.j.Li x.Li x.H.Li x.Q.Li x.H.Li Y.Li Y.Y.Li Z.j.Li H.Liang j.H.Liang Y.T.Liang G.R.Liao L.Z.Liao Y.Liao C.x.Lin D.x.Lin x.S.Lin B.j.Liu C.W.Liu D.Liu F.Liu G.M.Liu H.B.Liu j.Liu j.j.Liu j.B.Liu K.Liu K.Y.Liu K.Liu L.Liu Q.Liu S.B.Liu T.Liu x.Liu Y.W.Liu Y.Liu Y.L.Liu Z.Q.Liu Z.Y.Liu Z.W.Liu I.Logashenko Y.Long C.G.Lu j.x.Lu N.Lu Q.F.Lü Y.Lu Y.Lu Z.Lu P.Lukin F.j.Luo T.Luo x.F.Luo Y.H.Luo H.j.Lyu x.R.Lyu j.P.Ma P.Ma Y.Ma Y.M.Ma F.Maas S.Malde D.Matvienko Z.x.Meng R.Mitchell A.Nefediev Y.Nefedov S.L.Olsen Q.Ouyang P.Pakhlov G.Pakhlova x.Pan Y.Pan E.Passemar Y.P.Pei H.P.Peng L.Peng x.Y.Peng x.j.Peng K.Peters S.Pivovarov E.Pyata B.B.Qi Y.Q.Qi W.B.Qian Y.Qian C.F.Qiao j.j.Qin j.j.Qin L.Q.Qin x.S.Qin T.L.Qiu j.Rademacker C.F.Redmer H.Y.Sang Anhui University Hefei 230039China Beihang University Beijing 100191China Budker Institute of Nuclear Physics Novosibirsk 630090Russia CAS Key Laboratory of Theoretical Physics Institute of Theoretical PhysicsChinese Academy of SciencesBeijing 100190China Cavendish Laboratory University of CambridgeJJ Thomson AveCambridge CB30HEUnited Kingdom Central China Normal University Wuhan 430079China Central South University Changsha 410083China China University of Geosciences Wuhan 430074China China University of Mining and Technology Xuzhou 221116China École Polytechnique Fédérale de Lausanne(EPFL) LausanneSwitzerland Fudan University Shanghai 200433China Goethe University Frankfurt D-60325 Frankfurt am MainGermany Guangxi Normal University Guilin 541004China Guangxi Uninversity Nanning 530004China Hangzhou Institute for Advanced Study UCASHangzhou 310024China Hebei Normal University Shijiazhuang 050024China Hebei University Baoding 071002China Hefei University of Technology Hefei 230601China Helmholtz Institute Mainz Staudinger Weg 18D-55099 MainzGermany Henan Normal University Xinxiang 453007China Henan University Kaifeng 475004China High Energy Physics Center Chung-Ang UniversitySeoul 06974Korea Higher School of Economy 11 Pokrovsky Bulvar Moscow 109028Russia Huangshan University Huangshan 245000China Hubei University of Automotive Technology Shiyan 442002China Hunan Normal University Changsha 410081China Hunan University of Science and Technology Xiangtan 411201China Hunan University Changsha 410082China Indiana University BloomingtonIndiana 47405USA Inner Mongolia University Hohhot 010021China Institute of Advanced Science Facilities Shenzhen 518107China Institute of High Energy Physics Chinese Academy of SciencesBeijing 100049China Institute of Modern Physics Chinese Academy of SciencesLanzhou 730000China Institute of Physics Academia SinicaTaipeiTaiwan 11529China Institute of Theoretical Physics Chinese Academy of SciencesBeijing 100190China jilin University Changch

The superτ-charm facility(STCF)is an electron–positron collider proposed by the Chinese particle physics community.It is designed to operate in a center-of-mass energy range from 2 to 7 GeV with a peak luminosity of 0.5×10^(35) cm^(–2)·s^(–1) or higher.The STCF will produce a data sample about a factor of 100 larger than that of the presentτ-charm factory—the BEPCII,providing a unique platform for exploring the asymmetry of matter-antimatter(charge-parity violation),in-depth studies of the internal structure of hadrons and the nature of non-perturbative strong interactions,as well as searching for exotic hadrons and physics beyond the Standard Model.The STCF project in China is under development with an extensive R&D program.This document presents the physics opportunities at the STCF,describes conceptual designs of the STCF detector system,and discusses future plans for detector R&D and physics case studies.

关键词： electron–positron collider tau-charm region high luminosity STCF detector conceptual design

HDPairFinder:A data processing platform for hydrogen/deuterium isotopic labeling-based nontargeted analysis of trace-level amino-containing chemicals in environmental water

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journal of Environmental Sciences 2024年第2期136卷 583-593页

作者： Tingting zhao Kristin Carroll Caley B.Craven Nicholas j.P.Wawryk Shipei xing jian Guo xing-Fang Li Tao Huan Department of Chemistry Faculty of ScienceUniversity of British ColumbiaVancouver Campus2036 Main MallVancouverBritish ColumbiaV6T 1Z1Canada Division of Analytical and Environmental Toxicology Department of Laboratory Medicine and PathologyFaculty of Medicine and DentistryUniversity of AlbertaEdmontonAlberta T6G 2G3Canada

The combination of hydrogen/deuterium(H/D)formaldehyde-based isotopic methyl labeling with solid-phase extraction and high-performance liquid chromatography–high resolution mass spectrometry(HPLC-HRMS)is a powerful analytical solution for nontargeted analysis of trace-level amino-containing chemicals in water samples.Given the huge amount of chemical information generated in HPLC-HRMS analysis,identifying all possible H/Dlabeled amino chemicals presents a significant challenge in data processing.To address this,we designed a streamlined data processing pipeline that can automatically extract H/D-labeled amino chemicals from the raw HPLC-HRMS data with high accuracy and efficiency.First,we developed a cross-correlation algorithm to correct the retention time shift resulting from deuterium isotopic effects,which enables reliable pairing of H-and D-labeled peaks.Second,we implemented several bioinformatic solutions to remove false chemical features generated by in-source fragmentation,salt adduction,and natural13C isotopes.Third,we used a data mining strategy to construct the AMINES library that consists of over 38,000 structure-disjointed primary and secondary amines to facilitate putative compound annotation.Finally,we integrated these modules into a freely available R program,HDPairFinder.R.The rationale of each module was justified and its performance tested using experimental H/D-labeled chemical standards and authentic water samples.We further demonstrated the application of HDPairFinder to effectively extract N-containing contaminants,thus enabling the monitoring of changes of primary and secondary N-compounds in authentic water samples.HDPairFinder is a reliable bioinformatic tool for rapid processing of H/D isotopic methyl labeling-based nontargeted analysis of water samples,and will facilitate a better understanding of N-containing chemical compounds in water.

关键词： Isotope labeling Nontargeted analysis Reactive N-compounds HPLC-HRMS Source water

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Remarkable enhancement of gas selectivity on organosilica hybrid membranes using urea-modulated metal-organic framework nanoparticles

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Frontiers of Chemical Science and Engineering 2024年第2期18卷 83-92页

作者： Yayun zhao Dechuan zhao Chunlong Kong Yichao Lin xuezhen Wang Liang Chen Key Laboratory of Advanced Fuel Cells and Electrolyzers Technology of Zhejiang Province Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo 315201China University of Chinese Academy of Sciences Beijing 100049China Collaboration Innovation Center for Tissue Repair Material Engineering Technology China West Normal UniversityNanchong 637009China

Metal-organic framework/organosilica hybrid membranes on tubular ceramic substrates have shown great potential for the implementation of membrane technology in practical gas separation projects due to their higher permeance compared to commercial polymers.However,the selectivities of the reported membranes are moderate.Here,we have incorporated urea-modulated metal-organic frameworks into organosilica membranes to greatly enhance its separation performance.The urea-modulated metal-organic frameworks exhibit less-defined edges of crystallographic facets and high defect density.They can be well-dispersed in the organosilica layer,which substantially suppresses the interfacial defects between metal-organic frameworks and organosilica,which is beneficial for improving the selectivity of membranes for gas separation.The results have shown that the enhanced ideal selectivity of H_(2)/CH_(4) was 165 and that of CO_(2)/CH_(4) was 43,with H_(2) permeance of about 1.25×10^(−6) mol·m^(−2)·s^(−1)·Pa^(−1) and CO_(2) permeance of 3.27×10^(−7) mol·m^(−2)·s^(−1)·Pa^(−1) at 0.2 MPa and 25℃.In conclusion,the high level of hybrid membranes can be used to separate H_(2)(or CO_(2))from the binary gas mixture H_(2)/CH_(4)(or CO_(2)/CH_(4)),which is important for gas separation in practical applications.Moreover,the simple and feasible modulation of metal-organic framework is a promising strategy to tune different metal-organic frameworks for membranes according to the actual demands.

关键词： ZIF-8 nanocrystals urea organosilica hybrid membrane enhanced separation performance