检索结果-南通市图书馆

Insight into the sorption and desorption pattern of pyrrolizidine alkaloids and their N-oxides in acidic tea(Camellia sinensis)plantation soils

引用

journal of Environmental Sciences 2025年第2期148卷 350-363页

作者： Yuting Lu Haolei han Yuexing Yi Yunfeng Chai ChenWang xiangchun Zhang xiangde Yang Hongping Chen Tea Research Institute Chinese Academy of Agricultural SciencesHangzhou 310008China Graduate School of Chinese Academy of Agricultural Sciences Beijing 100081China School of Chemical Engineering and Materials Zhejiang University of TechnologyHangzhou 310008China Key Laboratory of Tea Quality and Safety&Risk Assessment Ministry of AgricultureHangzhou 310008China Key Laboratory of Tea Quality and Safety Control Ministry of Agriculture and Rural AffairsHangzhou 310000China

Pyrrolizidine alkaloids(PAs)and their N-oxides(PANOs)are phytotoxins produced by various plant species and have been emerged as environmental *** sorption/desorption behaviors of PAs/PANOs in soil are crucial due to the horizontal transfer of these natural products from PA-producing plants to soil and subsequently absorbed by plant *** study firstly investigated the sorption/desorption behaviors of PAs/PANOs in tea plantation soils with distinct *** amounts for seneciphylline(Sp)and seneciphylline-N-oxide(SpNO)in three acidic soils ranged from 2.9 to 5.9μg/g and 1.7 to 2.8μg/g,*** percentages for Sp and SpNO were from 22.2%to 30.5%and 36.1%to 43.9%.In the mixed PAs/PANOs systems,stronger sorption of PAs over PANOs was occurred in tested ***,the Freundlich models more precisely described the sorption/desorption *** exchange capacity,sand content and total nitrogen were identified as major influencing factors by linear regression ***,the soils exhibiting higher sorption capacities for compounds with greater *** were more likely to migrate within soils and be absorbed by tea *** contributes to the understanding of environmental fate of PAs/PANOs in tea plantations and provides basic data and clues for the development of PAs/PANOs reduction technology.

关键词： Pyrrolizidine alkaloids Sorption-desorption behavior Tea plantation system Acidic soil Linear regression model

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Remediation mechanism of high concentrations of multiple heavy metals in contaminated soil by Sedum alfredii and native microorganisms

引用

journal of Environmental Sciences 2025年第1期147卷 179-188页

作者： Zihe Wang han Zhang Ying xiong Lieyu Zhang jianglong Cui Guowen Li Caili Du Kaiyang Wen State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental SciencesBeijing 100012China Beijing Water Science and Technology Institute Beijing 100044China School of Architecture and Civil Engineering Chengdu UniversityChengdu 610106China

Pollution accident of nonferrous metallurgy industry often lead to serious heavy metal pollution of the surrounding *** of contaminated soil is an environmental and sustainable technology,and soil native microorganisms in the process of phytoremediation also participate in the remediation of heavy ***,the effects of high concentrations of multiple heavy metals(HCMHMs)on plants and native soil microorganisms remain ***,further clarification of themechanism of phytoremediation of HCMHMs soil by plants and native soil microorganisms is *** the plant Sedum alfredii(***)to restore HCMHM-contaminated soil,we further explored the mechanism of *** and native soil microorganisms in the remediation of HCMHM *** results showed that(i)*** can promote heavy metals from non-rhizosphere soil to rhizosphere soil,which is conducive to the effect of plants on heavy *** addition,it can also enrich the absorbed heavy metals in its roots and leaves;(ii)native soil bacteria can increase the abundance of signal molecule-synthesizing enzymes,such as trpE,trpG,bjaI,rpfF,ACSL,and yidC,and promote the expression of the pathway that converts serine to cysteine,then synthesize substances to chelate heavy *** addition,we speculated that genes such as K19703,K07891,K09711,K19703,K07891,and K09711 in native bacteria may be involved in the stabilization or absorption of heavy *** results provide scientific basis for *** to remediate heavy metals contaminated soils,and confirm the potential of phytoremediation of HCMHM contaminated soil.

关键词： Microbial remediation Phytoremediation Sedum alfredii

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Effect of lanthanum on microstructure of a nickel-based single crystal superalloy

引用

China Foundry 2025年第1期22卷 55-64页

作者： Hong Gao Kai Guan Ren-jie Cui jian-chao Qin Zi-han Zhao Zhao-hui Huang Science and Technology on Advanced High Temperature Structural Materials Laboratory Beijing Institute of Aeronautical MaterialsBeijing 100095China

To enhance the high-temperature oxidation resistance and mechanical properties of a secondgeneration nickel-based superalloy,various concentrations of lanthanum(La)ranging from 5.0×10^(-5)wt.%to 3.4×10^(-4)wt.%are added to the *** microstructure of the nickel-based single crystal superalloy with trace of La was examined by means of SEM,EDS and *** show the addition of La decreases the segregation of elements and increases the amount ofγ/γ′eutectics of the as-cast alloy,and in the interdendritic region,the growth of eutectics is accompanied by the growth of strip clusters composed of Ni_(5)La and Ni_(3)*** the La content in the alloy increases,the proportion of Ni_(5)La in the cluster *** heat treatment,incipient melting occurs in the cluster regions,leading to an increase in microporosity compared to the original as-cast ***,the heat treatment alters the shape of the clusters from a strip morphology to an elliptical one,and it changes their composition from Ni_(5)La and Ni_(3)Ta to a combination of Ni_(5)La,Ni_(3)Ta,and MC carbides.

关键词： single crystal superalloy lanthanum microstructure heat-treatment precipitate phase

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Synthesis ofδ-MnO_(2)via ozonation routine for low temperature formaldehyde removal

引用

journal of Environmental Sciences 2025年第1期147卷 642-651页

作者： Guijun Fan Yacong Guo Shaohua Chai Le Zhang jian Guan Guojun Ma Ning han Yunfa Chen State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China College of Chemical Engineering University of Chinese Academy of SciencesBeijing 100049China Key Laboratory of Science and Technology on Particle Materials Institute of Process EngineeringChinese Academy of SciencesBeijing 361021China Key Laboratory for Mechanics in Fluid Solid Coupling Systems Institute of MechanicsChinese Academy of SciencesBeijing 100190China School of Petrochemical Engineering&Environment Zhejiang Ocean UniversityZhoushan 316022China

Nowadays,it is still a challenge to prepared high efficiency and low cost formaldehyde(HCHO)removal catalysts in order to tackle the long-living indoor air ***,δ-MnO_(2)is successfully synthesized by a facile ozonation strategy,where Mn^(2+)is oxidized by ozone(O_(3))bubble in an alkaline *** presents one of the best catalytic properties with a low 100%conversion temperature of 85℃for 50 ppm of HCHO under a GHSV of 48,000 mL/(g·hr).As a comparison,more than 6 times far longer oxidation time is needed if O3 is replaced by O_(2).Characterizations show that ozonation process generates a different intermediate of tetragonalβ-HMnO_(2),which would favor the quick transformation into the final productδ-MnO_(2),as compared with the relatively more thermodynamically stable monoclinicγ-HMnO_(2)in the O_(2)***,HCHO is found to be decomposed into CO_(2)via formate,dioxymethylene and carbonate species as identified by room temperature insitu diffuse reflectance infrared fourier transform *** these results show great potency of this facile ozonation routine for the highly activeδ-MnO_(2)synthesis in order to remove the HCHO contamination.

关键词： δ-MnO_(2) Ozone oxidation HCHO oxidation In-situ DRIFTS

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Organic pollutant sensing for human health based on carbon dots

引用

Chinese Chemical Letters 2025年第1期36卷 147-157页

作者： Quan Zhang Shunjie xing jingqian han Li Feng jianchun Li Zhaosheng Qian jin Zhou Affiliated Hospital of Shandong Second Medical University(261031 School of Clinical Medicine)School of PharmacyShandong Second Medical UniversityWeifang 261053China Shandong Botai Measurement and Testing Co.Ltd. Weifang 261000China College of Chemistry and Materials Science Zhejiang Normal UniversityJinhua 321004China

Organic pollutants are harmful and toxic chemical substances that adversely threaten human health and the living environment all over the *** and more studies have been investigating the relationship between low level of human exposure of organic compounds and various internal *** the sake of assessing disease risk due to organic compounds contact in a particular location,it is imperative for relevant government departments to make a human health risk assessment in view of the organic pollutants'bioavailability and their dosage-response *** is inevitable to make use of an efficient method to detect organic pollutants,which is significant for public health and *** assays based on carbon dots thus would provide a very plausible candidate *** consulting a large number of literatures,we offer a comprehensive review of the sensing applications of carbon dots for organic pollutants.

关键词： Fluorescent probe Human health Organic pollutants Carbon dots Detection and sensing

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Organic fertilizer enhances soil aggregate stability by altering greenhouse soil content of iron oxide and organic carbon

引用

journal of Integrative Agriculture 2025年第1期24卷 306-321页

作者： Lijun Ren han Yang jin Li Nan Zhang Yanyu han Hongtao Zou Yulong Zhang College of Land and Environment Shenyang Agricultural University/National Engineering Research Center for Efficient Utilization of Soil and Fertilizer Resources/Key Laboratory of Arable Land Conservation in Northeast ChinaMinistry of Agriculture and Rural AffairsShenyang 110866China

Both soil organic carbon (SOC) and iron (Fe) oxide content, among other factors, drive the formation and stability of soil ***, the mechanism of these drivers in greenhouse soil fertilized with organic fertilizer is not well *** a 3-year field experiment, we aimed to investigate the factors which drive the stability of soil aggregates in greenhouse *** explore the impact of organic fertilizer on soil aggregates, we established four treatments:no fertilization (CK);inorganic fertilizer (CF);organic fertilizer (OF);and combined application of inorganic and organic fertilizers(COF).The application of organic fertilizer significantly enhanced the stability of aggregates, that is it enhanced the mean weight diameter, geometric mean diameter and aggregate content (%) of>0.25 mm aggregate *** and COF treatments increased the concentration of SOC, especially the aliphatic-C, aromatic-C and polysaccharide-C components of SOC, particularly in>0.25 mm *** fertilizer application significantly increased the content of free Fe(Fed), reactive Fe (Feo), and non-crystalline Fe in both bulk soil and ***, non-crystalline Fe showed a positive correlation with SOC content in both bulk soil and *** non-crystalline Fe and SOC were significantly positively correlated with>2 mm mean weight ***, we believe that the increase of SOC, aromatic-C, and non-crystal ine Fe concentrations in soil after the application of organic fertilizer is the reason for improving soil aggregate stability.

关键词： organic fertilizer soil aggregates soil organic carbon iron oxides greenhouse soil

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

ARF4 acting upstream of LBD16 promotes adventitious root formation in peach

引用

Horticultural Plant journal 2025年第1期11卷 145-161页

作者： jingjing Liu Lingling Gao Ruoxi Zhang Anqi Gao Zamith Kerubo Oginga Beibei Zheng Yuepeng han CAS Key Laboratory of Plant Germplasm Enhancement and Specialty Agriculture Wuhan Botanical GardenThe Innovative Academy of Seed Design of Chinese Academy of SciencesWuhanHubei 430074China Hubei Hongshan Laboratory WuhanHubei 430070China University of Chinese Academy of Sciences Beijing 100049China

Although class A auxin response factors(ARFs)are known to regulate adventitious root(AR)development through the canonical SCFTIR1-Aux/IAA-ARF signaling pathway,the regulatory role of class B ARFs in AR development remains largely ***,this research focused on the role of class B ARF transcription factors in peach(Prunus persica‘Shengli')adventitious root ***,we report the role of a class B ARF gene Pp ARF4 in adventitious root formation in *** transcriptome and q RT-PCR analyses showed that the transcription of Pp ARF4 was significantly up-regulated in auxin-treated stem explants.Y2H assay showed that Pp ARF4 had no interaction with Pp IAAs(AUxIN/INDOLE ACETIC ACIDs).Pp ARF4 could bind the promoters of lateral root development gene Pp LBD16 and auxin transport gene Pp PIN1 to activate their *** overexpression of Pp ARF4 and Pp LBD16 in Arabidopsis promoted AR ***,Pp ARF4 could act as a negative regulator of flavone synthesis and thus prevent the explants from *** results not only provide novel insights into the functions of ARFs in regulating plant growth and development,but will also be useful for fulfilling asexual propagation by stem cuttings in peach.

关键词： Prunus persica Adventitious root Auxin Pp ARF4 Pp LBD16

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

An electrically activable nanochip to intensify gas-ionic-immunotherapy

引用

Science Bulletin 2025年第3期70卷 390-406页

作者： Gang Wang jingrui Li Shumin Sun Yuqi Yang Zhihui han Zifan Pei Liang Cheng Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesSoochow UniversitySuzhou 215123China

Excess intracellular H_(2)S induces destructive mitochondrial toxicity,while overload of Zn^(2+)results in cell pyroptosis and potentiates the tumor immunogenicity for ***,the precise delivery of both therapeutics remains a great ***,an electrically activable ZnS nanochip for the controlled release of H_(2)S and Zn^(2+)was developed for enhanced gas-ionic-immunotherapy(GIIT).Under an electric field,a locality with particularly high concentrations of H_(2)S and Zn^(2+)was established by the voltage-controlled degradation of the ZnS nanoparticles(NPs).Consequently,the ZnS nanochip-mediated gas-ionic therapy(GIT)resulted in mitochondrial membrane potential depolarization,energy generation inhibition,and oxidative stress imbalance in tumor ***,the cyclic guanosine monophosphate-adenosine monophosphate synthase-stimulator of interferon genes(cGAS-STING)signaling pathway was activated due to the mitochondrial ***,the released Zn^(2+)resulted in the increase of the intracellular Zn levels and cell pyroptosis,which enhanced the immunogenicity via the release of damage-associated molecular patterns(DAMPs).In vitro and in vivo studies revealed that the ZnS nanochip-based GIT effectively eliminated the tumors under an electric field and mobilized the cytotoxic T lymphocytes for *** combination withαCTLA-4 further promoted the adaptive immune response and inhibited tumor metastasis and long-term tumor *** work presented an electrically activable ZnS nanochip for combined immunotherapy,which might inspire the development of electric stimulation therapy.

关键词： H_(2)S gas therapy lonic interference therapy Electrically controll eddelivery Cell pyroptosis CGAS-STING pathway

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Pore-scale investigation of forced imbibition in porous rocks through interface curvature and pore topology analysis

引用

journal of Rock Mechanics and Geotechnical Engineering 2025年第1期17卷 245-257页

作者： jianchao Cai xiangjie Qin han Wang Yuxuan xia Shuangmei Zou State Key Laboratory of Petroleum Resources and Engineering China University of PetroleumBeijing102249China Hubei Key Laboratory of Oil and Gas Exploration and Development Theory and Technology China University of GeosciencesWuhan430074China

Forced imbibition,the invasion of a wetting fluid into porous rocks,plays an important role in the effective exploitation of hydrocarbon resources and the geological sequestration of carbon ***,the interface dynamics influenced by complex topology commonly leads to non-wetting fluid ***,the underlying mechanisms under viscously unfavorable conditions remain *** study employs a direct numerical simulation method to simulate forced imbibition through the reconstructed digital rocks of *** interface dynamics and fluid–fluid interactions are investigated through transient simulations,while the pore topology metrics are introduced to analyze the impact on steady-state residual fluid distribution obtained by a pseudo-transient *** results show that the cooperative pore-filling process promoted by corner flow is dominant at low capillary *** leads to unstable inlet pressure,mass flow,and interface curvature,which correspond to complicated interface dynamics and higher residual fluid *** forced imbibition,the interface curvature gradually increases,with the pore-filling mechanisms involving the cooperation of main terminal meniscus movement and arc menisci *** topology with small diameter pores may result in the destabilization of interface *** residual fluid saturation is negatively correlated with porosity and pore throat size,and positively correlated with tortuosity and aspect ratio.A large mean coordination number characterizing global connectivity promotes ***,high connectivity characterized by the standardized Euler number corresponding to small pores is associated with a high probability of non-wetting fluid trapping.

关键词： Forced imbibition Porous rocks Interface dynamics Pore topology Residual fluid distribution

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Unraveling the reaction mechanism of high reversible capacity CuP_(2)/C anode with native oxidation PO_(x) component for sodium-ion batteries

引用

Chinese Chemical Letters 2025年第1期36卷 574-578页

作者： Huixin Chen Chen Zhao Hongjun Yue Guiming Zhong xiang han Liang Yin Ding Chen State Key Laboratory of Advanced Design and Manufacturing for Vehicle Body College of Mechanical and Vehicle EngineeringHunan UniversityChangsha 410082China CAS key Laboratory of Design and Assembly of Functional Nanostructures and Fujian Provincial Key Laboratory of NanomaterialsFujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China College of Materials Science and Engineering Co-Innovation Center of Efficient Processing and Utilization of Forest ResourcesNanjing Forestry UniversityNanjing 210037China Laboratory of Advanced Spectro-electrochemistry and Li-ion Batteries Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023China Institute of Physics Chinese Academy of SciencesBeijing 100190China xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials Xiamen Institute of Rare Earth MaterialsHaixi institutesChinese Academy of SciencesXiamen 361021China

Phosphorus-based anode is a promising anode for sodium-ion batteries(SIBs)due to its high specific capacity,however,suffers from poor electronic conductivity and unfavorable electrochemical *** metals such as copper(Cu)into phosphorus has been demonstrated to not only improve the electronic conductivity but also accommodate the volume change during cycling,yet the underline sodiation mechanism is not ***,take a copper phosphide and reduced graphene oxide(CuP_(2)/C)composite as an example,which delivers a high reversible capacity of>900 mAh/***,it is revealed that the native oxidation PO_(x)components of the CuP_(2)/C composite show higher electrochemical reversibility than the bulk Cu P_(2),based on a quantitative analysis of high-resolution solid-state^(31)P NMR,ex-situ xPS and synchrotron x-ray diffraction characterization *** sodiation products Na_(3)PO_(4) and Na_(4)P_(2)O_(7) derived from PO_(x) could react with Na-P alloys and regenerate to PO_(x) during charge process,which probably accounts for the high reversible capacity of the Cu P_(2)/C *** findings also illustrate that the phosphorus transforms into nanocrystalline Na_(3)P and Na_(x)P alloys,which laterally shows crystallization-amorphization evolution process during cycling.

关键词： CuP_(2)/C composite POx component Reaction mechanism Solid-state NMR Sodium-ion batteries

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

欢迎您,

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案：

请选择收藏分类：

通借通还

欢迎您,

建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案： 新增检索档案 确定 取消

请选择收藏分类： 新增自定义分类 确定 取消

通借通还

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

请选择保存的检索档案：

请选择收藏分类：