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Experimental and theoretical investigation of sulfur-doped g-C_(3)N_(4)nanosheets/FeCo_(2)O_(4)nanorods S-scheme heterojunction for photocatalytic H_(2)evolution

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Nano Research 2024年第9期17卷 8007-8016页

作者： Haitao Wang Lianglang Yu Jiahe Peng Jing zou Weiping Gong Jizhou Jiang School of Chemistry and Environmental Engineering School of Environmental Ecology and Biological EngineeringKey Laboratory of Green Chemical Engineering Process of Ministry of EducationEngineering Research Center of Phosphorus Resources Development and Utilization of Ministry of EducationNovel Catalytic Materials of Hubei Engineering Research CenterWuhan Institute of TechnologyWuhan 430205China Guangdong Provincial Key Laboratory for Electronic Functional Materials and Devices Huizhou UniversityHuizhou 516007China

g-C_(3)N_(4)emerges as a promising metal-free semiconductor photocatalyst due to its cost-effectiveness,facile synthesis,suitable visible light response,and robust thermal ***,its practical application in photocatalytic hydrogen evolution reaction(HER)is impeded by rapid carrier recombination and limited light absorption *** this study,we successfully develop a novel g-C_(3)N_(4)-based step-scheme(S-scheme)heterojunction comprising two-dimensional(2D)sulfur-doped g-C_(3)N_(4)nanosheets(SCN)and one-dimensional(1D)FeCo_(2)O_(4)nanorods(FeCo_(2)O_(4)),demonstrating enhanced photocatalytic HER *** engineered SCN/FeCo_(2)O_(4)S-scheme heterojunction features a well-defined 2D/1D heterogeneous interface facilitating directed interfacial electron transfer from FeCo_(2)O_(4)to SCN,driven by the lower Fermi level of SCN compared to FeCo_(2)O_(4).This establishment of electron-interacting 2D/1D S-scheme heterojunction not only facilitates the separation and migration of photogenerated carriers,but also enhances visible-light absorption and mitigates electron-hole pair *** structure analysis and density functional theory calculations corroborate that the carrier migration in the SCN/FeCo_(2)O_(4)photocatalyst adheres to a typical S-scheme heterojunction mechanism,effectively retaining highly reactive photogenerated ***,the optimized SCN/FeCo_(2)O_(4)heterojunction exhibits a substantially high hydrogen production rate of 6303.5μmol·g^(-1)·h^(-1)under visible light excitation,which is 2.4 times higher than that of the ***,the conjecture of the S-scheme mechanism is confirmed by in situ XPS *** 2D/1D S-scheme heterojunction established in this study provides valuable insights into the development of high-efficiency carbon-based catalysts for diverse energy conversion and storage applications.

关键词： g-C_(3)N_(4) FeCo_(2)O_(4) S-scheme heterojunction photocatalytic hydrogen evolution reaction(HER)

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Commentary on “Why people should run after positive affective experiences instead of health benefits”

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Journal of Sport and Health Science 2024年第4期13卷 451-452页

作者： Ting Wang Jinghua Chen Robert Schinke Liye zou Body-Brain-Mind Laboratory School of PsychologyShenzhen UniversityShenzhen 518060China School of Kinesiology and Health Sciences Laurentian UniversitySudburyON P3E 2C6Canada

Maltagliati et al.1 recently highlighted the vital role of affective experiences in promoting physical activity(PA).The authors suggested that positive affective experiences,rather than health benefits,can tip the balance in favor of PA over sedentary *** authors proposed a new formal decision model between PA and sedentary alternatives and reported that when health benefits are the unique reason to action,the costs of PA(e.g.,effort)and the subjective value(SV)of sedentary alternatives(V_(sed))are the main drivers of decision-making processes.

关键词： benefits formal decision

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Parameter sensitivity analysis of the axial stability for a marine flexible pipe

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Petroleum 2024年第3期10卷 548-556页

作者： Liping Tang Jiaxin zou Kenan Song Yongheng Shi Li Liu School of Mechatronic Engineering Southwest Petroleum UniversityChengdu610500China School of Engineering University of AberdeenAberdeenAB243UEUK Oil&Gas Control Center National Petroleum and Natural Gas Pipeline Network Group Co.Ltd.Beijing100020China

Marine unbonded flexible pipes serve as the most essential equipment in offshore oil and gas exploration and *** compressive loads during installation or in service in the complex marine environment usually lead to buckling failure.A flexible pipe is a composite structure with multiple functional layers,of which the tensile armor layer plays a key role with regard to the response of the pipe subjected to axial *** this paper,a simplified three-dimensional finite element model is developed,focusing on the tensile layer and replacing the carcass layer,pressure sheath layer,and pressure armor layer by a cylindrical rigid body to reduce computational *** using this model,the buckling failure modes of the tensile armor layer(in particular the birdcaging phenomenon)are *** key parameters that affect the stability of the flexible pipe under axial compression and torsion are emphasized,and their effects on its axial and torsional stiffness are compared and *** results show that both the lay angle of the steel wires and the interlayer friction coefficient have a significant influence on the axial and torsional stiffness of the pipe,whereas the damaged length of the outer sheath has virtually no effect.

关键词： Flexible pipe Tensile armor Buckling failure Key parameters Stiffness

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Construction of flower-like MoS_(2)decorated on Cu doped CoZn-ZIF derived N-doped carbon as superior microwave absorber

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Nano Research 2024年第9期17卷 8250-8260页

作者： Yun Han Di Lan Mengjun Han Zihao Xia Jiaxiao zou Zirui Jia College of Chemistry and Chemical Engineering Qingdao UniversityQingdao 266071China School of Materials Science and Engineering Hubei University of Automotive TechnologyShiyan 442002China

The rational design of composition nanostructures and morphologies of the carbon-based composites materials has a significant potential for tuning electromagnetic parameters and thereby improving their performance as electromagnetic wave(EMW)*** this work,the flower-like Cu/Co-NC/MoS_(2)(NC=N-doped carbon skeleton)composites were successfully prepared by employing CuCoZn-ZIF(ZIF=zeolitic imidazolate framework)as precursor with subsequent annealing and hydrothermal *** unique flower-like morphology and electromagnetic synergy strategy between components enable the as-obtained Cu/Co-NC/MoS_(2)composites to exhibit outstanding microwave absorption ***,the minimum reflection loss of Cu/Co-NC/MoS_(2)reaches-54.36 dB at 2.7 *** the thickness reduces to 2.2 mm,the maximum effective absorption bandwidth can be achieved as large as 6.72 *** research develops useful ideas for optimizing multicomponent microwave absorbing materials.

关键词： ternary metal-organic frameworks(MOFs) MoS_(2) flower-like morphology microwave absorption

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Functional thermal fluids and their applications in battery thermal management:A comprehensive review

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Journal of Energy Chemistry 2024年第7期94卷 78-101页

作者： Xinyue Xu Keyu Weng Xitao Lu Yuanqiang Zhang Shuyan Zhu Deqiu zou Faculty of Maritime and Transportation Ningbo UniversityNingbo 315211ZhejiangChina

With the increasing requirements for fast charging and discharging,higher requirements have been put forward for the thermal management of power ***,there is an urgent need to develop efficient heat transfer *** a new type of heat transfer fluids,functional thermal fluids mainly includ-ing nanofluids(NFs)and phase change fluids(PCFs),have the advantages of high heat carrying density,high heat transfer rate,and broad operational temperature ***,challenges that hinder their practical applications *** this paper,we firstly overview the classification,thermophysical prop-erties,drawbacks,and corresponding modifications of functional thermal *** NFs,the high ther-mal conductivity and high convective heat transfer performance were mainly elaborated,while the stability and viscosity issues were also *** then for PCFs,the high heat carrying density was mainly elaborated,while the problems of supercooling,stability,and viscosity were also *** this basis,the composite fluids combined NFs and PCFs technology,has been ***,the thermal properties of traditional fluids,NFs,PCFs,and composite fluids are compared,which proves that functional thermal fluids are a good choice to replace traditional fluids as ***,battery thermal management system(BTMS)based on functional thermal fluids is summarized in detail,and the thermal management effects and pump consumption are compared with that of water-based ***,the current technical challenges that parameters optimization of functional thermal fluids and structures optimization of BTMS systematically are *** the future,it is necessary to pay more attention to using machine learning to predict thermophysical properties of functional thermal fluids and their applications for BTMS under actual vehicle conditions.

关键词： Functionalthermal fluids Nanofluids Phase change fluids Battery thermal management system Thermophysical properties

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Bilateral effect of acupuncture on cerebrum and cerebellum in ischaemic stroke patients with hemiparesis:a randomised clinical and neuroimaging trial

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Stroke & Vascular Neurology 2024年第3期9卷 306-317,I0264-I0273页

作者： Tianzhu Chen Tianyan Chen Yong Zhang Kang Wu Yihuai zou Department of Neurology Dongzhimen HospitalBeijing University of Chinese MedicineBeijingChina School of Journalism and Communication Renmin University of ChinaBeijingChina Department of Rehabilitation Dongzhimen HospitalBeijing University of Chinese MedicineBeijingChina

Background Acupuncture involving the limb region may be effective for stroke rehabilitation clinically,but the visualised and explanatory evidence is *** objectives were to assess the specific effects of acupuncture for ischaemic stroke(IS)patients with hemiparesis and investigate its therapy-driven modification in functional *** IS patients were randomly assigned(2:1)to receive 10 sessions of hand-foot 12 needles acupuncture(HA,n=30)or non-acupoint(NA)acupuncture(n=16),enrolling gender-matched and age-matched healthy controls(HCs,n=34).The clinical outcomes were the improved Fugl-Meyer Assessment scores including upper and lower extremity(ΔFM,ΔFM-UE,ΔFM-LE).The neuroimaging outcome was voxel-mirrored homotopic connectivity(VMHC).Static and dynamic functional connectivity(sFC,DFC)analyses were used to study the neuroplasticity *** 46 ISs(mean(SD)age,59.37(11.36)years)and 34 HCs(mean(SD)age,52.88(9.69)years)were included in the per-protocol analysis of clinical and *** clinical,ΔFM scores were 5.00 in HA group and 2.50 in NA group,with a dual correlation betweenΔFM andΔVMHC(angular:r=0.696,p=0.000;cerebellum:r=-0.716,p=0.000)fitting the linear regression model(R2=0.828).In neuroimaging,ISs demonstrated decreased VMHC in bilateral postcentral gyrus and cerebellum(Gaussian random field,GRF corrected,voxel p<0.001,cluster p<0.05),which fitted the logistic regression model(AUC=0.8413,accuracy=0.7500).Following acupuncture,VMHC in bilateral superior frontal gyrus orbital part was increased with cerebro-cerebellar changes,involving higher sFC between ipsilesional superior frontal gyrus orbital part and the contralesional orbitofrontal cortex as well as cerebellum(GRF corrected,voxel p<0.001,cluster p<0.05).The coefficient of variation of VMHC was decreased in bilateral posterior cingulate gyrus(PPC)locally(GRF corrected,voxel p<0.001,cluster p<0.05),with integration states transforming into segregation states overall(

关键词： acupuncture Acupuncture random

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Parameter Estimation of Sub-/Super-synchronous Oscillation Based on Interpolated All-phase Fast Fourier Transform with Optimized Window Function

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Journal of Modern Power Systems and Clean Energy 2024年第4期12卷 1031-1041页

作者： Bo Sun Xi Wu Xi Chen Zixiao zou Qiang Li Bixing Ren School of Electrical Engineering Southeast UniversityNanjingChina State Grid Jiangsu Electric Power Company Limited Research Institute NanjingChina

In recent years,with increasing amounts of renew-able energy sources connecting to power grids,sub-/super-syn-chronous oscillations(SSOs)occurred more *** to the time-variant nature of SsO magnitudes and frequencies,as well as the mutual interferences among SsO modes with close frequencies,the accurate parameter estimation of SsO has be-come a particularly challenging *** solve this issue,this paper proposes an improved spectrum analysis method by im-proving the window function and a spectrum correction method to achieve higher ***,by aiming at the sidelobe characteristics of the window function as evaluation criteria,a combined cosine function is optimized using a genetic algorithm(GA).Furthermore,the obtained window function is self-con-volved to extend its excellent characteristics,which have better performance in reducing mutual interference from other SSO ***,a new form of interpolated all-phase fast Fourier transform(IpApFFT)using the optimized window func-tion is proposed to estimate the parameters of *** meth-od allows for phase-unbiased estimation while maintaining algo-rithmic simplicity and *** performance of the pro-posed method is demonstrated under various conditions,com-pared with other estimation *** results vali-date the effectiveness and superiority of the proposed method.

关键词： Sub-/Super-synchronous oscillation(SSO) window function parameter estimation interpolated all-phase fast Fourier transform(ApFFT)

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Double stimulus-responsive palladium catalysts for ethylene polymerization and copolymerization

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Chinese Chemical Letters 2024年第7期35卷 407-411页

作者： Hailong He Wenbing Wang Wenmin Pang Chen zou Dan Peng CAS Key Laboratory of Soft Matter Chemistry Department of Polymer Science and EngineeringUniversity of Science and Technology of ChinaHefei National Laboratory for Physical Sciences at the MicroscaleHefei 230026China

The external stimulus response strategy has been evolved rapidly in the field of olefin *** this work,we modularly synthesized three types of double stimulus responsiveα-diimine palladium catalysts,combining redox regulation and other regulation together,such as light,Lewis acid and alkali *** catalytic activities and the molecular weight of polyethylene products can be regulated for 4 times in ethylene *** palladium complexes were also used for the copolymerization reaction of ethylene and polar monomers,such as methyl 10-undecylenate and methyl acrylate,effectively regulating the catalytic activities,the molecular weight and polar monomer incorporation of the prepared *** research on these dual-regulated palladium complexes makes full use of prepared catalysts and provides new inspirations for regulating olefin polymerization.

关键词： Dual-regulated Stimulus-responsive Palladium Ethylene polymerization Polar monomer

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Genome mining of multi-substituted alkylresorcinols from a hybrid highly reducing-and typeⅢ-polyketide pathway

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Chinese Chemical Letters 2024年第7期35卷 345-349页

作者： Huaran Zhang Yuting Huang Yingjie Tang Dekun Kong Yi zou College of Pharmaceutical Sciences Southwest UniversityChongqing 400715China

Fungal alkylresorcinols are a class of polyketides,which are commonly synthesized by the hybridization of highly reducing polyketide synthase(hrPKS)with non-reducing polyketide synthase(nrPKS).In this study,we identified and demonstrated a new assembly model for synthesizing alkylresorcinol(scirpilin A,1),which was accomplished by collaboration of a hrPKS(FscA)and a typeⅢPKS(FscB).Furthermore,three post-tailoring enzymes(FscC,FscD,and FscE)act iteratively on 1 skeleton,including successive 14e-oxidation of inert carbons,di-halogenation,and di-methylation,to form highly oxidized and multisubstituted *** work presents an unusual synthesis manner of alkylresorcinols,sheds light on the collaborative mechanism between hrPKS and typeⅢPKS and provides three valuable enzymatic catalysts for the tailoring of alkylresorcinol family natural products in future.

关键词： Genome mining Alkylresorcinol hrPKS TypeⅢPKS Iterative catalysis

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Enhancing hydrolytic stability of dynamic imine bonds and polymers in acidic media with internal protecting groups

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Chinese Chemical Letters 2024年第5期35卷 161-165页

作者： Hang Chen Chengzhi Cui Hebo Ye Hanxun zou Lei You College of Environmental and Biological Engineering Fujian Provincial Key Laboratory of Ecology-Toxicological Effects&Control for Emerging ContaminantsPutian UniversityPutian 351100China State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China College of Chemistry and Material Science Fujian Normal UniversityFuzhou 350007China Fujian Science&Technology Innovation Laboratory for Optoelectronic Information of China Fuzhou 350108China

Imine bonds are among the most explored building motifs in dynamic chemistry,polymers,and materials,and yet,their acid-resistance remains a longstanding *** we demonstrate a concept of internal protecting groups for improving the kinetic stability of dynamic imine bonds and *** examination of structure-reactivity relationship of a series of aldehydes/imines bearing a neighboring carboxyl allowed uncovering of required structural features for dynamically masking imine bonds with cyclic *** studies indicated that noncovalent interactions along with sterics control the ringchain equilibrium and the stability of imine *** incorporation of internal protecting groups into imine polymers further enabled their controlled stability in acidic ***,a combination of dynamic covalent network and coordination supramolecular network provided a facile means for the modulation of luminescent and mechanical properties of *** strategies and results reported should be beneficial to molecular assemblies,dynamic polymers,biological delivery,and intelligent materials.

关键词： Dynamic covalent chemistry Internal protecting group Kinetic stability Imine bond Dynamic polymer

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