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Fertilization practices affect biological nitrogen fixation by modulating diazotrophic communities in an acidic soil in southern China

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Pedosphere 2023年第2期33卷 301-311页

作者： Long GUO Chao WANG Manman ZHENG wenxing li Zejiang CAI Boren WANG Juan CHEN Ren Fang SHEN State Key Laboratory of Soil and Sustainable Agriculture Institute of Soil ScienceChinese Academy of SciencesNanjing 210008(China) University of Chinese Academy of Sciences Beijing 100049(China) Qiyang Red Soil Experimental Station Chinese Academy of Agricultural SciencesQiyang 426182(China) Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes of Ministry of Education Hohai UniversityNanjing 210098(China)

Biological nitrogen(N)fixation(BNF)driven by diazotrophs is an important pathway for N input in agricultural ***,free-living BNF and its associated diazotrophic communities under different fertilization practices in acidic soils are poorly ***,we conducted a long-term(29 years)fertilization experiment to explore how fertilization affected free-living BNF via changing biotic and abiotic *** fertilization treatments included an unfertilized control(CK),chemical N,phosphorus(P),and potassium(K)fertilizers(NPK),NPK plus lime(NPKL),NPK plus straw(NPKS),NPK plus straw and lime(NPKSL),and NPK plus manure(NPKM).Compared with CK(1.51 nmol C_(2)H_(2)g^(-1)d^(-1)),BNF rate was significantly(Plization treatments without manure reduced the gene abundance(0.71×10^(8)-1.18×10^(8)copies g^(-1))andα-diversity(Shannon index,1.11-2.43)of diazotrophic communities,whereas the treatment with manure had a positive effect on diazotrophic abundance(3.23×10^(8)copies g^(-1))and Shannon index(3.36).Non-parametric multivariate analysis of variance(PERMANOVA)suggested that manure application(R^(2)=0.212,P=0.001)had a stronger influence on diazotrophic community composition than the addition of lime(R^(2)=0.115,P=0.019)or straw(R^(2)=0.064,P=0.161).Random forest modeling revealed that BNF rates can be significantly(Pling(PLS-PM)suggested that the diazotrophic community attributes and soil properties mainly provided direct and indirect contributions to the variations in BNF rates,*** dominant genera,Pelomonas,Azospirillum,and Dechloromonas,were positiv

关键词： chemical fertilizer community composition free-living N fixation long-term fertilization practices manure application soil pH

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Electrochemical Oxygen Evolution Performance of Nitrogen-Doped Ultra-Thin Carbon Nanosheets Composite Ru1Co Single Atom Alloy Catalysts

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Chinese Journal of Chemistry 2024年第9期42卷 973-979页

作者： Ziwei Deng Zhiyi Sun Yaqiong li Jiajing Pei wenxing Chen Energy&Catalysis Center Schoolof Materials Science and EngineeringBeijing Institute of TechnologyBeijing 100081China Beijing Synchrotron Radiation Facility Institute of High Energy PhysicsChinese Academy of SciencesBeijing 00049China

Energy transformation is imminent,and hydrogen energy is one of the important new energy *** of the keys to increasing the rate of hydrogen evolution during electrolysis is the use of high-performance catalysts for oxygen evolution reactions(OER).Single-atom alloys(SAAs)have garnered significant attention because they partially reduce costs and combine the advantages of both single-atom catalysts(SACs)and alloy ***,an efficient pyrolysis strategy based on a mixing and drying process is designed to anchor ultra-small Co cluster particles,combined with Ru single atoms dispersed on nitrogen-doped ultra-thin carbon nanosheets(Ru_(1)Co SAA/NC).The prepared electrocatalyst exhibits superior OER activity and superb stability,demonstrating an overpotential of 238 mV for OER with a current density of 10 mA·cm^(-2) in 0.5 mol/L H_(2)SO_(4).And we also utilized in-situ XAS to detect the oxidation state of Ru sites during *** in all,this method achieves cost reductions and efficiency improvements through the design of SAAs,offering new prospects for the structural transformation of clean energy.

关键词： Oxygen evolution reaction Single alloy catalyst Ultra-thin carbon nanosheets Electrocatalyst Pyrolysis RuiCo SAA/NC

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Portable hydrogel-based tri-channel fluorescence sensor array for visual detection of multiple explosives

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Nano Research 2024年第7期17卷 6483-6492页

作者： wenxing Gao Wenfeng liu Saijin Huang lin Wang Yingying Jian Yutong li Weiwei Wu li Shang State Key Laboratory of Solidification Processing School of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi'an 710072China School of Advanced Materials and Nanotechnology Xidian UniversityXi'an 710126China Honors College Northwestern Polytechnical UniversityXi'an 710119China

The identification and detection of various types of explosives are essential for human health and environmental ***-based sensing approach offers significant advantages in detecting multi-analytes simultaneously,thereby holding great potential in identifying multiple ***,we report a tri-channel fluorescence array composed of three distinct fluorescence probes based on gold nanoclusters and nicotinamide adenine dinucleotide with well-separated emission *** the specific interactions of explosives with different fluorescent probes and the yielded response patterns,seven explosives can be successfully distinguished with 100%*** particular,the sensor array exhibits excellent performance in the quantitative analysis of individual explosive and the differentiation of multiple explosive *** facilitate the field detection towards practical application,the tri-channel fluorescence array was further integrated with polymer *** fabricated portable hydrogel-based array sensors can not only visually identify seven different explosives by their distinct fluorescence color change,but also enable quantitative detection based on linear discriminant analysis(LDA)together with a *** study illustrates the great potential of hydrogel-based fluorescence sensor array as robust sensors for explosives,which also holds significant promise for the development of portable explosive devices towards practical application.

关键词： sensor array gold nanoclusters explosives fluorescence hydrogels

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Atomic interface regulation of rare-marth metal single atom catalysts for energy conversion

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Nano Research 2024年第5期17卷 3493-3515页

作者： Ziheng Zhan Zhiyi Sun Zihao Wei Yaqiong li wenxing Chen Shenghua li Siping Pang School of Materials Science and Engineering Beijing Institute of TechnologyBeijing 100081China

Efficient photocatalysis and electrocatalysis in energy conversion have been important strategies to alleviate energy crises and environmental *** recent years,with the rapid development of emerging catalysts,significant progress has been made in photocatalysis for converting solar energy into chemical energy and electrocatalysis for converting electrical energy into chemical ***,their selectivity and efficiency of the products are *** earth(RE)can achieve atomic level fine regulation of catalysts and play an crucial role in optimizing catalyst performance by their unique electronic and orbital ***,there is a lack of systematic review on the atomic interface regulation mechanism of RE and their role in energy conversion *** atom catalysts(SACs)provide clear active sites and 100%atomic utilization,which is conducive to exploring the regulatory mechanisms of ***,this review mainly takes atomic level doped RE as an example to review and discuss the atomic interface regulation role of RE elements in energy ***,a brief introduction was given to the synthesis strategies that can effectively exert the atomic interface regulation effect of RE,with a focus on the atomic interface regulation mechanism of ***,the regulatory mechanisms of RE atoms have been systematically summarized in various energy conversion ***,the challenges faced by RE in energy conversion,as well as future research directions and prospects,were pointed out.

关键词： rare earth elements interface regulation effect single-atom catalyst energy conversion

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以计算思维为导向的计算机信息技术教学改革分析

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移动信息 2024年第1期46卷 115-117页

作者：李文星中共新安县委党校河南洛阳471800

在数字化时代,信息技术已成为人们生活和工作中不可或缺的重要部分。为了更好地使用信息技术,人们不仅需要掌握相关基础知识,还需培养计算思维能力。计算思维不仅是解决计算机相关问题的方法,更是在面对复杂问题时进行抽象表示和自动化... 详细信息

在数字化时代,信息技术已成为人们生活和工作中不可或缺的重要部分。为了更好地使用信息技术,人们不仅需要掌握相关基础知识,还需培养计算思维能力。计算思维不仅是解决计算机相关问题的方法,更是在面对复杂问题时进行抽象表示和自动化处理的重要思考方式。文中深入分析了以计算思维为导向的计算机信息技术教学改革策略,探讨了如何将计算思维更好地融入教学中,以适应当前社会的发展需要。

关键词：计算思维计算机信息技术教学改革策略分析

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湖北秭归鱼泉洞泉域系统中六六六(HCHs)和滴滴涕(DDTs)的分布、来源与迁移

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地质科技通报 2024年第3期43卷 311-322页

作者：杨秀雯魏志莹易佳佩李雯星景一鸣秦超杰熊俊武刘伟周宏祁士华陈伟中国地质大学(武汉)环境学院武汉430074 中国地质大学(武汉)地质调查研究院武汉430074 中国地质大学(武汉)生物地质与环境地质国家重点实验室武汉430074 中国地质大学(武汉)长江流域环境水科学湖北省重点实验室武汉430074

岩溶区特殊的地形地貌,使得地表环境中的有机氯农药(OCPs)很容易进入地下环境,对地下水的安全构成威胁。采用气相色谱-电子捕获检测器(GC-ECD)对湖北秭归鱼泉洞泉域系统中的典型OCPs——六六六(HCHs)和滴滴涕(DDTs)进行了检测,探究了其... 详细信息

岩溶区特殊的地形地貌,使得地表环境中的有机氯农药(OCPs)很容易进入地下环境,对地下水的安全构成威胁。采用气相色谱-电子捕获检测器(GC-ECD)对湖北秭归鱼泉洞泉域系统中的典型OCPs——六六六(HCHs)和滴滴涕(DDTs)进行了检测,探究了其时空分布特征、潜在污染来源和迁移特征。结果表明:水体中HCHs质量浓度范围为0.09~5.17 ng/L,土壤和泉沉积物中HCHs质量分数范围分别为0.36~3.67,0.11~2.53 ng/g;水体中DDTs质量浓度范围为0.13~7.16 ng/L,土壤和泉沉积物中DDTs质量分数范围分别为0.22~19.13,0.73~11.53 ng/g,呈现出以DDTs为主的污染特征。水体中HCHs和DDTs质量浓度在冬季最高;土壤中HCHs和DDTs质量分数分别在夏季和冬季达到最高;泉沉积物中HCHs和DDTs质量分数分别在夏季和春季达到峰值。特征比值结果显示,水体、土壤和泉沉积物中HCHs主要源于林丹的使用;水体中DDTs主要源于历史残留,而土壤和泉沉积物中DDTs主要来源于近期使用。相关性分析结果表明,HCHs和DDTs可从补给区地表水和补给区土壤分别向排泄区泉水和泉沉积物中迁移。HCHs和DDTs在介质中的快速迁移证实了岩溶区地下水的脆弱性。本研究成果可以为岩溶地下水资源和环境的保护提供参考。

关键词：岩溶区六六六(HCHs) 滴滴涕(DDTs) 来源迁移有机氯农药(OCPs) 鱼泉洞泉域湖北秭归

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Enhanced recovery of high-purity Fe powder from iron-rich electrolytic manganese residue by slurry electrolysis

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International Journal of Minerals,Metallurgy and Materials 2024年第3期31卷 531-538页

作者： wenxing Cao Jiancheng Shu Jiaming Chen Zihan li Songshan Zhou Shushu liao Mengjun Chen Yong Yang Key Laboratory of Solid Waste Treatment and Resource Recycle(SWUST) Ministry of EducationSouthwest University of Science and TechnologyMianyang 621010China School of Chemistry and Chemical Engineering Chongqing UniversityChongqing 400044China Daxin Manganese Mining Branch of South Manganese Group limited Chongzuo 532315China

Iron-rich electrolytic manganese residue(IREMR)is an industrial waste produced during the processing of electrolytic metal manganese,and it contains certain amounts of Fe and Mn resources and other heavy *** this study,the slurry electrolysis technique was used to recover high-purity Fe powder from *** effects of IREMR and H2SO4 mass ratio,current density,reaction temper-ature,and electrolytic time on the leaching and current efficiencies of Fe were *** to the results,high-purity Fe powder can be recovered from the cathode plate,and the slurry electrolyte can be *** leaching efficiency,current efficiency,and purity of Fe reached 92.58%,80.65%,and 98.72wt%,respectively,at a 1:2.5 mass ratio of H2SO4 and IREMR,reaction temperature of 60℃,electric current density of 30 mA/cm^(2),and reaction time of 8 *** addition,vibrating sample magnetometer(VSM)analysis showed that the coercivity of electrolytic iron powder was 54.5 A/m,which reached the advanced magnetic grade of electrical pure-iron powder(DT4A coercivity standard).The slurry electrolytic method provides fundamental support for the industrial application of Fe resource recovery in IRMER.

关键词： iron-rich electrolytic manganese residue slurry electrolysis high-purity iron powder leaching efficiency current efficiency

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Novel Long Non-coding RNA Markers for Prognostic Prediction of Patients with Bladder Cancer

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Chinese Medical Sciences Journal 2020年第3期35卷 239-247页

作者： wenxing li Yanli Zhang Department of Diagnosis Heze Medical CollegeHezeShandong 274000China Department of Urology Affiliated Hospital of Heze Medical CollegeHezeShandong 274000China School of life Sciences Tsinghua UniversityBeijing 100084China School of Veterinary Medicine Huazhong Agricultural UniversityWuhan 430072China

Objective To explore novel long non-coding RNA(lncRNA)molecular markers related to bladder cancer prognosis and to construct a prognostic prediction model for bladder cancer *** LncRNA expression data of patients with bladder cancer were downloaded from TCGA *** Cox regression and likelihood-based survival analysis were used to discover prognosis related *** studies of prognosis related lncRNAs were conducted by co-expression analysis and pathway enrichment *** Cox regression analysis was used to establish risk score model,and Receiver Operating Characteristic analysis was used to determine the optimal cut-off point of the *** risk score model was validated through Kaplan Meier estimation method and log-rank *** Seven prognosis related lncRNAs(OCIAD1-AS1,RP11-111 J6.2,AC079354.3,RP11-553 A21.3,RP11-598 F7.3,CYP4 F35 P and RP11-113 K21.4)which can predict survival of bladder cancer patient were ***-expression analysis and pathway analysis of these novel lncRNA signature and their target genes further revealed that these lncRNAs play important roles in the occurrence and development of bladder ***,a seven-lncRNA signature based risk score model for prognostic prediction of bladder cancer patients was established and ***,we identified the potential significance of two tumor-related antisense lncRNAs(OCIAD1-AS1 and RP11-553 A21.3)in the prognosis of bladder *** Our results suggest that these lncRNA markers may serve as potential prognosis predictors for bladder cancer and deserve further functional verification studies.

关键词： bladder cancer long non-coding RNA prognosis survival prediction

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Room-temperature and atmospheric-pressure hydrogenation of lignin-derived phenol to KA oil by Pt/NiO@MOFs

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Nano Research 2024年第8期17卷 7053-7060页

作者： Fengbin Zheng Kun Wang Yifei Ren Bohua Wang wenxing Chen Caoyu Yang Shengxian Shao Yinglong Wang Zhiyong Tang Guodong li College of Chemical Engineering Qingdao University of Science and TechnologyQingdao 266042China CAS Key Laboratory of Nanosystem and Hierarchical Fabrication CAS Center for Excellence in NanoscienceNational Center for Nanoscience and TechnologyBeijing 100190China School of Materials Science and Engineering Beijing Institute of TechnologyBeijing 100181China School of Nanoscience and Technology University of Chinese Academy of SciencesBeijing 100049China

Hydrogenation of lignin-derived phenol to KA oil(the mixture of cyclohexanone(K)and cyclohexanol(A))is attractive yet challenging in the sustainable upgrading of biomass derivatives under mild *** supported metal catalysts have been widely studied but the active components on supports often exhibit low recyclability due to their instability under experimental *** we show fabricating ultrasmall Pt/NiO in the pores of chromium terephthalate MIL-101 as catalysts for hydrogenation of ***,Pt/NiO@MIL-101 achieves catalytic phenol hydrogenation to KA oils of tunable K/A ratios and good reusability under room temperature and atmospheric hydrogen pressure,superior to contrast Pt@MIL-101 and Pt/NiO *** excellent performance mainly originates from the effective adsorption and activation of phenol by coordinatively unsaturated Cr sites and H2 activation on ultrasmall Pt/NiO as well as its effective spillover to the adsorbed phenol over Cr sites for hydrogenation ***,such catalyst also displays the excellent performances for hydrogenation of phenol’s derivatives under mild conditions.

关键词： ultrasmall Pt/NiO MIL-101 phenol hydrogenation KA oil

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A general and facile calcination method to synthesize single-site catalysts for highly efficient electrochemical CO_(2) reduction

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Nano Research 2024年第5期17卷 3895-3901页

作者： Rui Sui Bingyan Wang Yongsheng Wang Jiajing Pei Wei Zhu wenxing Chen Chunhui li Ailing Sun Zhongbin Zhuang Engineering Research Center of Advanced Rare Earth Materials Department of ChemistryTsinghua UniversityBeijing 100084China College of Chemistry and Green Catalysis Center Zhengzhou UniversityZhengzhou 450001China State Key Lab of Organic-Inorganic Composites and Beijing Advanced Innovation Center for Soft Matter Science and Engineering Beijing University of Chemical TechnologyBeijing 100029China Beijing Synchrotron Radiation Facility Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China Energy&Catalysis Center School of Materials Science and EngineeringBeijing Institute of TechnologyBeijing 100081China

The electrochemical CO_(2) reduction reaction(CO_(2)RR)has received widespread attention as a promising method for producing sustainable chemicals and mitigating the global ***,we demonstrate a general and facile synthetic route for the metal-nitrogen-carbon(M-N-C)type catalyst by simply calcinating metal acetate and urea with commercial carbon black,which have potential application in CO_(2)*** synthesized Ni-NC-600 catalyst has the structure of single Ni atom coordinated with one N atom and three C atoms(Ni-N_(1)C_(3)),which is suggested by X-ray absorption *** Ni-NC-600 catalyst exhibits high CO_(2)RR catalytic performance and a high CO Faraday efficiency above 98%in a wide potential range from-0.7 to-1.3 V(*** hydrogen electrode(RHE)),superior to most of the reported Ni-N-C *** work has developed a facile strategy to synthesize high performance CO_(2)RR catalyst.

关键词： nickel single atom catalyst CO_(2)reduction reaction CO production electrocatalyst

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