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Uncertainty and disturbance estimator-based model predictive control for wet flue gas desulphurization system

Chinese Journal of Chemical Engineering 2024年第3期67卷 182-194页

作者： Shan Liu wenqi zhong Li Sun Xi Chen Rafal Madonski School of Energy and Environment Key Laboratory of Energy Thermal Conversion and Control of Ministry of EducationSoutheast UniversityNanjing 210096China Faculty of Automatic Control Electronics and Computer ScienceSilesian University of TechnologyGliwise 44-100Poland

Wet flue gas desulphurization technology is widely used in the industrial process for its capability of efficient pollution removal.The desulphurization control system,however,is subjected to complex reaction mechanisms and severe disturbances,which make for it difficult to achieve certain practically relevant control goals including emission and economic performances as well as system robustness.To address these challenges,a new robust control scheme based on uncertainty and disturbance estimator(UDE)and model predictive control(MPC)is proposed in this paper.The UDE is used to estimate and dynamically compensate acting disturbances,whereas MPC is deployed for optimal feedback regulation of the resultant dynamics.By viewing the system nonlinearities and unknown dynamics as disturbances,the proposed control framework allows to locally treat the considered nonlinear plant as a linear one.The obtained simulation results confirm that the utilization of UDE makes the tracking error negligibly small,even in the presence of unmodeled dynamics.In the conducted comparison study,the introduced control scheme outperforms both the standard MPC and PID(proportional-integral-derivative)control strategies in terms of transient performance and robustness.Furthermore,the results reveal that a lowpass-filter time constant has a significant effect on the robustness and the convergence range of the tracking error.

关键词： Desulphurization system Disturbance rejection Model predictive control Uncertainty and disturbance estimator Nonlinear system

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Supercritical CO_(2) Cycles for Nuclear-Powered Marine Propulsion:Preliminary Conceptual Design and Off-Design Performance Assessment

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Journal of Thermal Science 2024年第1期33卷 328-347页

作者： LI Zhaozhi SHI Mingzhu SHAO Yingjuan zhong wenqi Key Laboratory of Energy Thermal Conversion and Control of Ministry of Education School of Energy and EnvironmentSoutheast UniversityNanjing 210096China

Using the efficient,space-saving,and flexible supercritical carbon dioxide(sCO_(2)) Brayton cycle is a promising approach for improving the performance of nuclear-powered ships.The purpose of this paper is to design and compare sCO_(2) cycle power systems suitable for nuclear-powered ships.Considering the characteristics of nuclear-powered ships,this paper uses different indicators to comprehensively evaluate the efficiency,cost,volume,and partial load performance of several nuclear-powered sCO_(2) cycles.Four load-following strategies are also designed and compared.The results show that the partial cooling cycle is most suitable for nuclear-powered ships because it offers both high thermal efficiency and low volume and cost,and can maintain relatively high thermal efficiency at partial loads.Additionally,the new load-following strategy that adjusts the turbine speed can keep the compressor away from the surge line,making the cycle more flexible and efficient compared to traditional inventory and turbine bypass strategies.

关键词： supercritical CO_(2)cycle nuclear marine propulsion off-design performance

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Multiobjective economic model predictive control using utopia-tracking for the wet flue gas desulphurization system

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Chinese Journal of Chemical Engineering 2023年第2期54卷 343-352页

作者： Shan Liu wenqi zhong Xi Chen Li Sun Lukuan Yang Key Laboratory of Energy Thermal Conversion and Control of Ministry of Education School of Energy and EnvironmentSoutheast UniversityNanjing 210096China

Efficient control of the desulphurization system is challenging in maximizing the economic objective while reducing the SO_(2) emission concentration. The conventional optimization method is generally based on a hierarchical structure in which the upper optimization layer calculates the steady-state results and the lower control layer is responsible to drive the process to the target point. However, the conventional hierarchical structure does not take the economic performance of the dynamic tracking process into account. To this end, multi-objective economic model predictive control(MOEMPC) is introduced in this paper, which unifies the optimization and control layers in a single stage. The objective functions are formulated in terms of a dynamic horizon and to balance the stability and economic performance. In the MOEMPC scheme, economic performance and SO_(2) emission performance are guaranteed by tracking a set of utopia points during dynamic transitions. The terminal penalty function and stabilizing constraint conditions are designed to ensure the stability of the system. Finally, an optimized control method for the stable operation of the complex desulfurization system has been established. Simulation results demonstrate that MOEMPC is superior over another control strategy in terms of economic performance and emission reduction, especially when the desulphurization system suffers from frequent flue gas disturbances.

关键词： Desulphurization system Economics Economic model predictive control Flue gas Optimization Utopia point

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Simultaneous desulfurization and denitrification of sintering flue gas via composite absorbent

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Chinese Journal of Chemical Engineering 2016年第8期24卷 1104-1111页

作者： Jie Wang wenqi zhong Key Laboratory of Energy Thermal Conversion and Control of Ministry of Education School of Energy and Environment Southeast University Centre for Simulation and Modelling of Particulate Systems Southeast University–Monash University Joint Research School

Experiments on simultaneous absorption of SO_2 and NO_X from sintering flue gas via a composite absorbent NaClO_2/NaClO were carried out. The effects of various operating parameters such as NaClO_2 concentration(ms), NaClO concentration(mp), molar ratio of NaClO_2/NaClO(M), solution temperature(TR), initial solution pH, gas flow(Vg) and inlet concentration of SO_2(CS) and NO(CN) on the removal efficiencies of SO_2 and NO were discussed. The optimal experimental conditions were determined to be initial solution pH = 6, TR=55 °C and M = 1.3 under which the average efficiencies of desulfurization and denitrification could reach99.7% and 90.8%, respectively. Moreover, according to the analysis of reaction products, it was found that adding NaClO to NaClO_2 aqueous solution is favorable for the generation of ClO_2 and Cl_2 which have significant effect on desulfurization and denitrification. Finally, engineering experiments were performed and obtained good results demonstrating that this method is practicable and promising.

关键词： Simultaneous desulfurization and denitrification Sintering flue gas Composite absorbent

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污泥/煤泥混合燃烧过程中N和S污染物迁移规律

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东南大学学报（自然科学版） 2024年第2期54卷 456-464页

作者：时振翔钟文琪周冠文东南大学能源热转换及其过程测控教育部重点实验室南京210096

为探究污泥/煤泥混合燃烧过程中N、S污染物的排放机理,开展N、S污染物迁移规律研究.基于热重-质谱分析仪获得的污泥/煤泥混合燃烧时气态污染物的基础生成规律,建立污泥/煤泥混合燃烧实验系统,研究不同污泥质量分数、温度下污泥/煤泥混... 详细信息

为探究污泥/煤泥混合燃烧过程中N、S污染物的排放机理,开展N、S污染物迁移规律研究.基于热重-质谱分析仪获得的污泥/煤泥混合燃烧时气态污染物的基础生成规律,建立污泥/煤泥混合燃烧实验系统,研究不同污泥质量分数、温度下污泥/煤泥混合燃烧的SO_(2)、NO的排放规律,并通过对4个不同阶段燃烧产物的X射线光电子能谱(XPS)检测,研究N、S官能团在燃烧过程中的转化规律.结果表明,污泥质量分数为40%时固硫固氮效果最明显;随污泥质量分数增加,吡啶类氮更多转化为吡咯类氮,使HCN产量增加以及胺类和腈类生成量增加,导致总NO排放量随污泥质量分数增加先增加后减少;有机硫类释放更为完全,燃烧产生的含S污染物增多,灰分中硫酸盐含量同步增长,因此总SO_(2)的释放量随污泥质量分数增加变化较小.

关键词：污泥/煤泥混合燃烧污染物迁移 X射线光电子能谱(XPS)

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Co-firing of coal and biomass in oxy-fuel fluidized bed for CO2 capture: A review of recent advances

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Chinese Journal of Chemical Engineering 2019年第10期27卷 2261-2272页

作者： Qinwen Liu Yan Shi wenqi zhong Aibing Yu Key Laboratory of Energy Thermal Conversion and Control of the Ministry of Education School of Energy and EnvironmentSoutheast UniversityNanjing 210096China Center for Simulation and Modelling of Particulate Systems Southeast University-Monash University Joint Research InstituteSuzhou 215000China 3 ARC Research Hub for Computational Particle TechnologyDepartment of Chemical EngineeringMonash UniversityClaytonVIC 3800Australia

The co-firing of coal and biomass in oxy-fuel fluidized beds is one of the most promising technologies for capturing CO2.This technology has attracted wide attention from academia and industry in recent years as a negative emission method to capture CO2 produced by carbon contained in biomass.In the past decades,many studies have been carried out regarding experiments and numerical simulations under oxy-fuel combustion conditions.This paper firstly briefly discusses the techno-economic viability of the biomass and coal co-firing with oxycombustion and then presents a review of recent advancements involving experimental research and computational fluid dynamics(CFD)simulations in this field.Experimental studies on mechanism research,such as thermogravimetric analysis and tube furnace experiments,and fluidized bed experiments based on oxy-fuel fluidized beds with different sizes as well as the main findings,are summarized as a part of this review.It has been recognized that CFD is a useful approach for understanding the behaviors of the co-firing of coal and biomass in oxyfuel fluidized beds.We summarize a recent survey of published CFD research on oxy-fuel fluidized bed combustion,which categorized into Eulerian and Lagrangian methods.Finally,we discuss the challenges and interests for future research.

关键词： Oxy-fuel combustion Co-firing of coal and biomass Oxy-fuel fluidized bed CFD simulation

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石英砂颗粒流化磨损特性和机制实验研究

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东南大学学报（自然科学版） 2024年第2期54卷 503-512页

作者：王簪庞磊邵应娟钟文琪东南大学能源与环境学院南京210096

针对颗粒磨损过程中的体相断裂和表面剥层2种主要机制,设计流化床冷态实验系统,并开展石英砂颗粒磨损实验,探究操作参数、颗粒性质等因素对颗粒流化磨损的影响规律.结果表明:在快速磨损阶段,体相断裂和表面剥层均对石英砂颗粒磨损有明... 详细信息

针对颗粒磨损过程中的体相断裂和表面剥层2种主要机制,设计流化床冷态实验系统,并开展石英砂颗粒磨损实验,探究操作参数、颗粒性质等因素对颗粒流化磨损的影响规律.结果表明:在快速磨损阶段,体相断裂和表面剥层均对石英砂颗粒磨损有明显影响,粒度变化速率大且产生大量细粉,体相断裂产生颗粒的质量分数明显小于表面剥层产生细粉的质量分数,因而表面剥层在快速磨损阶段是主导机制;粒度变化速率随表观气速的增加而增大,与初始粒径的关系不明显.进入稳态磨损阶段后,石英砂磨损的主导机制仍为表面剥层,体相断裂机制对颗粒流化磨损几乎没有贡献,粒度变化速率不再随表观气速、初始粒径而发生变化.基于实验数据结果,提出了适用于预测石英砂颗粒流化磨损的数学模型.

关键词：磨损表面剥层体相断裂磨损机制数学模型

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基于Aspen Plus的煤部分气化氢电联产系统模拟

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东南大学学报（自然科学版） 2024年第2期54卷 475-486页

作者：张泽祎李照志邵应娟钟文琪东南大学能源热转换及其过程测控教育部重点实验室南京210096

为了提高煤制氢系统的能源利用效率,减少碳排放,构建了4种以煤部分气化为基础的新型氢电联产系统.基于Aspen Plus软件,采用系统效率、制氢效率作为评价标准,对各系统进行模拟与对比分析.结果表明:存在不同氧煤比与碳转化率使得系统效率... 详细信息

为了提高煤制氢系统的能源利用效率,减少碳排放,构建了4种以煤部分气化为基础的新型氢电联产系统.基于Aspen Plus软件,采用系统效率、制氢效率作为评价标准,对各系统进行模拟与对比分析.结果表明:存在不同氧煤比与碳转化率使得系统效率达到最高,系统1~4分别在碳转化率为60%、85%、65%、60%时达到最高系统效率;各系统效率与气化效率随着气化温度的提高,呈先迅速增长后趋于平稳趋势;各系统效率与气化效率随着气化压力的提高,呈先迅速减少后趋于平稳趋势;在氧煤比为0.33,气化压力为2 MPa,气化温度为1000℃工况下系统1~4效率分别为59.12%、66.13%、62.21%和58.57%;采用CO_(2)与O_(2)作为气化剂,且CO_(2)与O_(2)的质量比为4∶1的煤部分气化加压富氧燃烧循环系统(系统2)在各项标准下具有优势,为最佳氢电联产系统.

关键词：煤炭部分气化半焦加压富氧燃烧系统建模热力学分析

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Dynamic optimization oriented modeling and nonlinear model predictive control of the wet limestone FGD system

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Chinese Journal of Chemical Engineering 2020年第3期28卷 832-845页

作者： Lukuan Yang wenqi zhong Li Sun Xi Chen Yingjuan Shao Key Laboratory of Energy Conversion and Process Measurement and Control Ministry of Education School of Energy and EnvironmentSoutheast UniversityNanjing 210096China

Nonlinear model predictive control(NMPC)scheme is an effective method of multi-objective optimization control in complex industrial systems.In this paper,a NMPC scheme for the wet limestone flue gas desulphurization(WFGD)system is proposed which provides a more flexible framework of optimal control and decision-making compared with PID scheme.At first,a mathematical model of the FGD process is deduced which is suitable for NMPC structure.To equipoise the model’s accuracy and conciseness,the wet limestone FGD system is separated into several modules.Based on the conservation laws,a model with reasonable simplification is developed to describe dynamics of different modules for the purpose of controller design.Then,by addressing economic objectives directly into the NMPC scheme,the NMPC controller can minimize economic cost and track the set-point simultaneously.The accuracy of model is validated by the field data of a 1000 MW thermal power plant in Henan Province,China.The simulation results show that the NMPC strategy improves the economic performance and ensures the emission requirement at the same time.In the meantime,the control scheme satisfies the multiobjective control requirements under complex operation conditions(e.g.,boiler load fluctuation and set point variation).The mathematical model and NMPC structure provides the basic work for the future development of advanced optimized control algorithms in the wet limestone FGD systems.

关键词： Wet limestone flue gas desulphurization(WFGD)system Modeling Nonlinear model predictive control(NMPC) Multi-objective optimization

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Experiments on particle cluster behaviors in a fast fluidized bed

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Chinese Journal of Chemical Engineering 2017年第9期25卷 1153-1162页

作者： Dailin Chen Xuejiao Liu Ziwen Sun wenqi zhong Baosheng Jin School of Energy & Environment Southeast University

A three-dimensional(3D) fast fluidized bed with the riser of 3.0 m in height and 0.1 m in inner diameter was established to experimentally study the cluster behaviors of Geldart B particles. Five kinds of quartz sand particles(dp= 0.100, 0.139, 0.177, 0.250 and 0.375 mm and ρp= 2480 kg·m^(-3)) were respectively investigated, with the total mass of the bed material kept as 10 kg. The superficial gas velocity in the riser ranges from 2.486 to 5.594 m·s^(-1) and the solid mass flux alters from 30 to 70 kg·((m^(-2)·s))^(-1). Cluster characteristics and evolutionary processes in the different positions of the riser were captured by the cluster visualization systems and analyzed by the self-developed binary image processing. The results found four typical cluster structures in the riser,i.e., the macro stripe-shaped cluster, saddle-shaped cluster, U-shaped cluster and the micro cluster. The increasing superficial gas velocity and particle sizes result in the increasing average cluster size and the decreasing cluster time fraction, while the solid mass flux in the riser have the reverse influences on the cluster size and time fraction. Additionally, clusters in the upper region of the riser often have the larger size and time fraction than that in the lower region. All these effects of operating conditions on clusters become less obvious when particle size is less than 0.100 mm.

关键词： Gas–solid flow Cluster Fast fluidized bed Geldart B particle

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