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Recent progress on photoactive nonprecious transition-metal complexes

Science China Chemistry 2025年第1期 46-95页

作者： Zhong-Liang gong Hong-Jie Zhang Yan Cheng Jianxun Liu Yuhan Ai Yaqin Li Zhihui Feng Qiong Zhang Shaolong gong Yong Chen Chang-Jiang Yao Yuan-Yuan Zhu Liang-Jin Xu Yu-Wu Zhong CAS Key Laboratory of Photochemistry Institute of Chemistry Chinese Academy of Sciences State Key Laboratory of Structural Cemistry Fujian Institute of Research on the Structure of Matter Chinese Academy of Sciences School of Chemistry and Chemical Engineering Anhui Key Laboratory of Advanced Catalytic Materials and Reaction EngineeringHefei University of Technology State Key Laboratory of Explosion Science and Safety Protection School of Mechatronical Engineering Beijing Institute of Technology College of Chemistry and Molecular Sciences Hubei Key Lab on Organic and Polymeric Optoelectronic Materials Wuhan University School of Chemistry and Chemical Engineering Anhui University Key Laboratory of Photochemical Conversion and Optoelectronic Materials & CAS-HKU Joint Laboratory on New Materials Technical Institute of Physics and Chemistry Chinese Academy of Sciences

Photoactive complexes of nonprecious transition metals, mainly including those in the first-row and partially the second-row of the Periodic table of elements, have received increasing attention in view of their low cost and long-term sustainability. They are recognized as promising alternatives to noble transition metal complex congeners that have been extensively studied in optoelectronic devices, artificial photosynthesis, photocatalysis, biodiagnostics, and therapeutics, etc. This review is devoted to a comprehensive summary on the classical and recent advances on photoactive nonprecious transition metal complexes, including photoactive Zr, V, Cr, Mo, and W complexes, Mn complexes and hybrids, Fe, Co, Ni, and Cu complexes, and Zn and Cd complexes and hybrids. A particular focus is given on the molecular design, modulation of photophysical and photochemical properties, and applications of the representative and lately-developed nonprecious metal complexes. In addition, a perspective on the future development in this field is provided at the end of this review.

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黄土高原森林林下植被物种多样性及其影响因素

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东北林业大学学报 2025年第2期53卷 66-74页

作者：宫正黄河文明与可持续发展研究中心(河南大学) 开封475001

以黄土高原不同密度刺槐(Robinia pseudoacacia)林为研究对象,通过调查样地的地形及土壤理化性质,利用方差分析、线性拟合、冗余分析等方法,分析林下植被物种多样性特征,探究影响林下植被物种多样性的因素。结果表明:不同林分密度的刺... 详细信息

以黄土高原不同密度刺槐(Robinia pseudoacacia)林为研究对象,通过调查样地的地形及土壤理化性质,利用方差分析、线性拟合、冗余分析等方法,分析林下植被物种多样性特征,探究影响林下植被物种多样性的因素。结果表明:不同林分密度的刺槐林林下植被物种多样性存在显著差异(P<0.05)。刺槐林下灌木Margalef丰富度指数随坡向的增大而减小,林下草本植物Margalef丰富度指数随坡度的增加而减小。刺槐林下灌木植物物种多样性的主要影响因素是密度、坡向、土壤全氮质量分数、土壤铵态氮质量分数,草本植物物种多样性的主要影响因素是土壤速效磷质量分数。

关键词：刺槐林物种多样性影响因素冗余分析黄土高原

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The low-latitude sodium layer:comparative data from lidar observations at Hainan,China and São Paulo,Brazil

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Earth and Planetary Physics 2025年第1期9卷 39-53页

作者： Fang Wu Jing Jiao GuoTao Yang LiFang Du ZhengKuan Liu HaoRan Zheng JiXin Guo ShaoHua gong YaJun Zhu State Key Laboratory of Space Weather National Space Science CenterChinese Academy of SciencesBeijing 100190China Hainan National Field Science Observation and Research Observatory for Space Weather National Space Science CenterChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China China-Brazil Joint Laboratory for Space Weather NSSC/INPESão Josédos Campos 12227-010Brazil School of Physics and Electronics Engineering Hainan Normal UniversityHaikou 571158China

Physical and chemical processes observed in the mesosphere and thermosphere above the Earth’s low latitudes are complex and highly interrelated to activity in the low-latitude *** sodium detected by lidar can yield clues to dynamic and chemical processes in these spatial layers above the Earth’s *** paper is based on sodium layer data collected at two low-latitude stations,one in the northern hemisphere and one in the *** low-latitude sodium layer exhibits conspicuous seasonal variations in shape,density,and altitude;these variations are similar between Earth’s hemispheres:sodium layer density at both stations reaches its seasonal maximum in autumn and minimum in ***,maximal Na density over Brazil is greater than that over *** variations of Na density above the two low-latitude stations are also similar;at both,maxima are observed before *** variations of the Na layer over Brazil that differ from those observed in the northern hemisphere may be related to the South Atlantic Magnetic Anomaly(SAMA)or fountain *** suggest that low-latitude Na layer data may provide useful additional evidence that could significantly improve the low-latitude part of the WACCM-Na model.

关键词： metallic sodium layer seasonal variation nocturnal variation lidar

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西南地区某省中学生使用药物与精神活性物质的流行病学调查

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中国药物依赖性杂志 1999年第2期8卷 115-119页

作者：刘志民周伟华连智穆悦龚文林周雪石明瑛北京医科大学中国药物依赖性研究所贵州省药物滥用监测站

目的··：采用整群抽样方法对某省九个地、州、市的高二年级学生进行了中学生用药情况调查。方法··：调查内容包括８种药物／精神活性物质“一生”、“最近３０ｄ”的使用情况、用药频率（经常、偶尔）、最初使用年龄、使用原因与后... 详细信息

目的··：采用整群抽样方法对某省九个地、州、市的高二年级学生进行了中学生用药情况调查。方法··：调查内容包括８种药物／精神活性物质“一生”、“最近３０ｄ”的使用情况、用药频率（经常、偶尔）、最初使用年龄、使用原因与后果等。结果··：在２６４９例有效应答者中，一生中“经常”使用最多的物质是烟草（６．３２％），其它物质依次是非甾体抗炎止痛药（ＮＳＡＩＤｓ，２．９２％），酒（２．８９％），挥发性溶剂（０．２８％），镇静催眠药（０．２４％）和大麻（０．０４％）；“偶尔”使用最多的是酒（６６．０５％），其它物质依次是：ＮＳＡＩＤｓ（５９．２６％），烟草（２７．３６％），镇静催眠药（５．１９％），海洛因（３．１３％），挥发性溶剂（２．８１％），中枢兴奋剂（０．７３％）和大麻（０．３３％）。各种物质的初始使用年龄介于１０．７ａ至１３．４ａ。调查还对学生用药原因、后果进行了分析。结论··：少数中学生对烟草、酒和某些精神药物的使用成瘾；极个别学生有滥用违禁毒品的行为。建议加强中学生药物滥用预防教育。

关键词：中学生药物滥用预防精神活性物质流行病学

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Hypoxia-preconditioned bone marrow-derived mesenchymal stem cells protect neurons from cardiac arrest-induced pyroptosis

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Neural Regeneration Research 2025年第4期20卷 1103-1123页

作者： Xiahong Tang Nan Zheng Qingming Lin Yan You Zheng gong Yangping Zhuang Jiali Wu Yu Wang Hanlin Huang Jun Ke Feng Chen Shengli Clinical Medical College of Fujian Medical University Fujian Medical UniversityFuzhouFujian ProvinceChina Department of Emergency Fujian Provincial HospitalFuzhouFujian ProvinceChina Fujian Provincial Key Laboratory of Emergency Medicine FuzhouFujian ProvinceChina The Second Department of Intensive Care Unit Fujian Provincial Hospital South BranchFuzhouFujian ProvinceChina

Cardiac arrest can lead to severe neurological impairment as a result of inflammation,mitochondrial dysfunction,and post-cardiopulmonary resuscitation neurological *** preconditioning has been shown to improve migration and survival of bone marrow–derived mesenchymal stem cells and reduce pyroptosis after cardiac arrest,but the specific mechanisms by which hypoxia-preconditioned bone marrow–derived mesenchymal stem cells protect against brain injury after cardiac arrest are *** this end,we established an in vitro co-culture model of bone marrow–derived mesenchymal stem cells and oxygen–glucose deprived primary neurons and found that hypoxic preconditioning enhanced the protective effect of bone marrow stromal stem cells against neuronal pyroptosis,possibly through inhibition of the MAPK and nuclear factor κB ***,we transplanted hypoxia-preconditioned bone marrow–derived mesenchymal stem cells into the lateral ventricle after the return of spontaneous circulation in an 8-minute cardiac arrest rat model induced by *** results showed that hypoxia-preconditioned bone marrow–derived mesenchymal stem cells significantly reduced cardiac arrest–induced neuronal pyroptosis,oxidative stress,and mitochondrial damage,whereas knockdown of the liver isoform of phosphofructokinase in bone marrow–derived mesenchymal stem cells inhibited these *** conclude,hypoxia-preconditioned bone marrow–derived mesenchymal stem cells offer a promising therapeutic approach for neuronal injury following cardiac arrest,and their beneficial effects are potentially associated with increased expression of the liver isoform of phosphofructokinase following hypoxic preconditioning.

关键词： bone marrow–derived mesenchymal stem cells cardiac arrest cardiac resuscitation hypoxic preconditioning liver isoform of phosphofructokinase mitochondria neuroinflammation oxidative stress pyroptosis reactive oxygen species

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毛囊类器官研究:现状、问题与前景

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中国组织工程研究 2025年第31期29卷 6733-6742页

作者：王钊龚琳朴永君大连医科大学附属第一医院皮肤科辽宁省大连市116000

背景:毛囊体外重建依赖于毛乳头细胞及角质形成细胞3D共培养时的自组装行为,该过程与毛囊胚胎发育极为相似,因此,毛囊类器官可作为毛囊再生相关基础研究良好的体外模型,目前,通过仿生系统培养的全人源毛囊类器官已能成功移植到动物体内... 详细信息

背景:毛囊体外重建依赖于毛乳头细胞及角质形成细胞3D共培养时的自组装行为,该过程与毛囊胚胎发育极为相似,因此,毛囊类器官可作为毛囊再生相关基础研究良好的体外模型,目前,通过仿生系统培养的全人源毛囊类器官已能成功移植到动物体内。毛囊类器官研究使毛囊再生成为可能,但构建方法亦无统一定论,仍面临诸多挑战。目的:综述目前毛囊类器官的研究进展,总结毛囊类器官培养方法及表征,阐述应用前景,为后续研究提供可靠依据,以期促进其在组织工程及脱发治疗的临床转化。方法:应用计算机在中国知网(CNKI)及PubMed数据库中,以“毛囊再生,毛发再生,类器官”为中文检索词,“hair growth,hair loss,hair regeneration,hair follicle,dermal papilla cell,organoid”为英文检索词进行检索,查阅国内外关于毛囊类器官的相关文献,共纳入文献67篇进行后续分析。结果与结论:①不同来源的毛乳头细胞与角质形成细胞可在体外构建毛囊类器官,以获得鼠源、人-鼠嵌合及人源毛囊类器官,并成功用于啮齿动物移植模型;②多种重编程方法如电刺激、添加重组蛋白、解离细胞基因过表达等可用于促进毛囊类器官毛胚形成及毛钉伸长,同时,多种3D打印技术的应用已实现大小可控毛囊类器官的批量生产,极大提高了生产效率;③在解离细胞共培养体系中加入黑素细胞时,或可破译新生毛囊的色素缺失难题,而加入人脐静脉血管内皮细胞时,细胞聚集体内的新生血管可改善营养供给,减少中心部位坏死;④随着工程化类毛囊技术逐渐趋于成熟,患者自体细胞构建的毛囊类器官或可用于严重脱发的个体化医疗。

关键词：脱发毛囊再生毛乳头细胞毛囊类器官上皮-间充质交互作用 3D培养类器官组织工程工程化类器官

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Molecule‑Level Multiscale Design of Nonflammable Gel Polymer Electrolyte to Build Stable SEI/CEI for Lithium Metal Battery

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Nano-Micro Letters 2025年第1期17卷 404-423页

作者： Qiqi Sun Zelong gong Tao Zhang Jiafeng Li Xianli Zhu Ruixiao Zhu Lingxu Wang Leyuan Ma Xuehui Li Miaofa Yuan Zhiwei Zhang Luyuan Zhang Zhao Qian Longwei Yin Rajeev Ahuja Chengxiang Wang Key Laboratory for Liquid‑Solid Structural Evolution and Processing of Materials(Ministry of Education) School of Materials Science and EngineeringShandong UniversityJinan 250061People’s Republic of China Condensed Matter Theory Department of Physics and AstronomyUppsala UniversityUppsala 75120Sweden

The risk of flammability is an unavoidable issue for gel polymer electrolytes(GPEs).Usually,flameretardant solvents are necessary to be used,but most of them would react with anode/cathode easily and cause serious interfacial instability,which is a big challenge for design and application of nonflammable ***,a nonflammable GPE(SGPE)is developed by in situ polymerizing trifluoroethyl methacrylate(TFMA)monomers with flame-retardant triethyl phosphate(TEP)solvents and LiTFSI–LiDFOB dual lithium *** is strongly anchored to PTFMA matrix via polarity interaction between-P=O and-CH_(2)CF_(3).It reduces free TEP molecules,which obviously mitigates interfacial reactions,and enhances flame-retardant performance of TEP *** TEP molecules are also inhibited in solvation of Li^(+),leading to anion-dominated solvation sheath,which creates inorganic-rich solid electrolyte interface/cathode electrolyte interface *** coordination structure changes Li^(+)transport from sluggish vehicular to fast structural transport,raising ionic conductivity to 1.03 mS cm^(-1) and transfer number to 0.41 at 30℃.The Li|SGPE|Li cell presents highly reversible Li stripping/plating performance for over 1000 h at 0.1 mA cm^(−2),and 4.2 V LiCoO_(2)|SGPE|Li battery delivers high average specific capacity>120 mAh g^(−1) over 200 *** study paves a new way to make nonflammable GPE that is compatible with Li metal anode.

关键词： Anchoring effect Nonflammable gel electrolyte In situ cross-linked Electrode-electrolyte interface Li metal battery

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蝶阀在抽水蓄能电站尾水系统中的应用研究

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水力发电 2025年第1期51卷 81-87页

作者：龚朝晖水电水利规划设计总院有限公司北京100011

为简化抽水蓄能电站尾水系统金属结构设备布置,提高电站防水淹厂房能力,提出了采用蝶阀作为尾水系统断流设备,并对其进行了可行性分析,同时还对蝶阀与事故闸门方案进行了对比研究。结果表明,尾水系统断流设备采用蝶阀方案切实可行,可提... 详细信息

为简化抽水蓄能电站尾水系统金属结构设备布置,提高电站防水淹厂房能力,提出了采用蝶阀作为尾水系统断流设备,并对其进行了可行性分析,同时还对蝶阀与事故闸门方案进行了对比研究。结果表明,尾水系统断流设备采用蝶阀方案切实可行,可提高防水淹厂房事故扩大的能力,简化设备的安装及减少土建施工。选定规格参数的蝶阀方案可降低建设成本,提高经济效益。研究结果可为类似工程的防水淹厂房事故扩大以及设备布置提供新的思路和技术参考。

关键词：蝶阀事故闸门水淹厂房局部水头损失抽水蓄能电站

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Reconstruction characteristics of gut microbiota from patients with type 1 diabetes affect the phenotypic reproducibility of glucose metabolism in mice

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Science China Life Sciences 2025年第1期 176-188页

作者： Zhiyi Wang Mengxue gong Yuanyuan Fang Huijuan Yuan Chenhong Zhang State Key Laboratory of Microbial Metabolism School of Life Sciences and BiotechnologyShanghai Jiao Tong University Department of Endocrinology Henan Provincial People's HospitalPeople's Hospital of Zhengzhou University

The human microbiota-associated(HMA) mice model, especially the germ-free(GF)-humanized mice, has been widely used to probe the causal relationships between gut microbiota and human diseases such as type 1 diabetes(T1D). However, most studies have not clarified the extent to which the reconstruction of the human donor microbiota in recipient mice correlates with corresponding phenotypic reproducibility. In this study, we transplanted fecal microbiota from five patients with T1D and four healthy people into GF mice, and microbiota from each donor were transplanted into 10 mice. Mice with similar microbiota structure to the donor exhibited better phenotypic reproducibility. The characteristics of the microbial community assembly of donors also influenced the phenotypic reproducibility in mice, and individuals with a higher proportion of stochastic processes showed more severe disorders. Microbes enriched in patients with T1D had a stronger colonization potential in mice with impaired glucose metabolism, and microbiota functional features related to T1D were better reproduced in these mice. This indicates that assembly traits and colonization efficacy of microbiota influence phenotypic reproducibility in GF-humanized mice. Our findings provide important insights for using HMA mice models to explore links between gut microbiota and human diseases.

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Multi level cell (MLC) in 3D crosspoint phase change memory array

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Science China(Information Sciences) 2021年第6期64卷 225-226页

作者： Nanbo gong IBM T.J.Watson Research Center

The success of memory technology is of vital importance in order to handle emerging mass amount of data in our daily lives. Let us take one example here: The IBM summit is the supercomputer released in 2018 and it plays an important role to help researchers run large numbers of calculations and better understand COVID-191). To enable such powerful computing capability, the IBM summit includes250 petabytes storage capacity2). To make a fair comparison, this is larger than the total number of all the ants we can find on the earth(on the order of 10;–10;)3).

关键词： MLC Multi level cell in 3D crosspoint phase change memory array

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