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Effect of background electrolytes on the adsorption of nitroaromatic compounds onto bentonite

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Journal of environmental sciences 2009年第8期21卷 1044-1052页

作者： chen baoliang, {2. wenhai department of environmental science, zhejiang university, Hangzhou 31002., zhejiang, china. department of environmental {2. Zhejiang University Hangzhou 310028 Zhejiang China

To further elucidate interaction of nitroaromatic compounds with mineral surface, the sorption of m-dinitrobenzene （m-DNB） and nitrobenzene to original bentonite in aqueous solution containing different electrolytes （i.e., KCl, NH4Cl, CaCl2.and Tetramethylammonium bromide （TMAB）） was studied. The sorption of m-DNB was greatly enhanced with the presence of KCl and NH4Cl, while little influence was observed with CaCl2.and TMAB, following the order of KCl 〉 NH4Cl 〉〉 TMAB, CaCl2. or DI water. For nitrobenzene, sorption enhancement only occurred at high nitrobenzene concentrations in the presence of KCl, and the solute equilibrium concentration at inflexion point was lowered with increasing KCl concentration. These sorption enhancements were significantly promoted with the increase of electrolyte concentration. The salting-out effect is insufficient to account for the sorption enhancement by original bentonite with increasing KCI or NH4Cl concentration. X-ray diffraction patterns of bentonite suspensions indicated that the sorption enhancement of m-DNB was attributed to the intercalation of K^＋ or NH4^＋ into bentonite interlayer and then dehydration with m-DNB to form inner-sphere complexes, which caused previously expanded bentonite interlayers to collapse in aqueous suspension, thus further enhanced the interaction of phenyl with siloxane surface. In comparison, the sorption enhancement of NB is attributed to the formation of outer-sphere complexes with K^＋ at high solute-loadings （〉 2.（0-400 mg/kg）. The sorption of m-DNB to initially modified TMA^＋-bentonite and K^＋-bentonite was almost the same as respective sorption to original bentonite in solution containing TMA^＋ and K^＋.

关键词： sorption nitroaromatic compound bentonite cation type wastewater treatment

ATP as anindicator of biomass activity in thermophilic upflow anaerobic sludge blanket reactor

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Journal of environmental sciences 2000年第3期12卷 380-384页

作者： chen Hong (department of {2. science and Engineering ,zhejiang university ,Hangzhou 31 0 0 2.7,china) 浙江大学浙江杭州 3 1 0 0 2

Thisworkinvestigatedthebiomassactivityinathermophilicupflowanaerobicsludgeblanket (UASB )reactorof wastewatertreatment .SynthetictextilewastewaterwithpH 1 0— 1 1 ,CODlevelof2.0 0 0— 30 0 0mg/Lwastested .Cellularadenosine triphosphate (ATP)involatilesolids (VS ;mgATP/gVS)wasmeasuredandexpressedasspecificATPcontenttocomparethe biomassactivityinupzoneandlowerzoneinUASBreactor .TheresultshowsthatthespecificATPcontentbasedontotalvolatile solids (VS)inlowerzone ( 0 .0 4 6mgATP/gVSaverage)ismuchlowerthanthatinupzone ( 0 .62.gATP/gVSaverage)duetohighcontentofinactivebiomassandhighpHinlowerzone .TheSATPinupzoneincreasesasHRTincreasesandapproachestoa maximumvalueof 0 .85mgATP/gVSatHRTof 7h ,thendecreases .ItshowsmostofthetotalVSinupzonerepresentactive bacterialbiomassatHRTof 7h .Rateofsubtractutiliz*** effectofHRTonSATPinlowerzoneisnotassignificantasonSATPinupzone .ThebuffercapacityofthethermophilicUASB reactorisverygood .ItistheactivityofsludgegranulesinlowerzonethatgivetheUASBreactorsuchagoodbuffercapacitytotheinlethighpH .

关键词： ATP biomassactivity UASBreactor

Tumor-derived exosomes induce initial activation by exosomal CD19 antigen but impair the function of CD19-specific CAR T-cells via TGF-βsignaling

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Frontiers of Medicine 2024年第1期18卷 128-146页

作者： Yuanyuan Hao Panpan chen Shanshan Guo Mengyuan Li Xueli Jin Minghuan Zhang wenhai Deng Ping Li Wen Lei Aibin Liang Wenbin Qian department of Hematology The Second Affiliated HospitalCollege of MedicineZhejiang UniversityHangzhou310009China department of Hematology Henan Provincial People’s HospitalZhengzhou University People’s HospitalZhengzhou450003China Key Laboratory of Laboratory Medicine Ministry of EducationSchool of Laboratory Medicine and Life SciencesWenzhou Medical UniversityWenzhou325000China department of Hematology Tongji Hospital of Tongji UniversityShanghai200065China

Tumor-derived exosomes (TEXs) enriched in immune suppressive molecules predominantly drive T-cell dysfunction and impair antitumor immunity. Chimeric antigen receptor (CAR) T-cell therapy has emerged as a promising treatment for refractory and relapsed hematological malignancies, but whether lymphoma TEXs have the same impact on CAR T-cell remains unclear. Here, we demonstrated that B-cell lymphoma-derived exosomes induce the initial activation of CD19-CAR T-cells upon stimulation with exosomal CD19. However, lymphoma TEXs might subsequently induce CAR T-cell apoptosis and impair the tumor cytotoxicity of the cells because of the upregulated expression of the inhibitory receptors PD-1, TIM3, and LAG3 upon prolonged exposure. Similar results were observed in the CAR T-cells exposed to plasma exosomes from patients with lymphoma. More importantly, single-cell RNA sequencing revealed that CAR T-cells typically showed differentiated phenotypes and regulatory T-cell (Treg) phenotype conversion. By blocking transforming growth factor β (TGF-β)-Smad3 signaling with TGF-β inhibitor LY2.09761, the negative effects of TEXs on Treg conversion, terminal differentiation, and immune checkpoint expression were rescued. Collectively, although TEXs lead to the initial activation of CAR T-cells, the effect of TEXs suppressed CAR T-cells, which can be rescued by LY2.09761. A treatment regimen combining CAR T-cell therapy and TGF-β inhibitors might be a novel therapeutic strategy for refractory and relapsed B-cell lymphoma.

关键词： tumor-derived exosome chimeric antigen receptor T-cell lymphoma TGF-β

Improved Efficiency and Stability of Organic Solar Cells by Interface Modification Using Atomic Layer Deposition of Ultrathin Aluminum Oxide

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Energy & environmental Materials 2024年第3期7卷 282-290页

作者： Ai Lan Yiqun Li Huiwen Zhu Jintao Zhu Hong Lu Hainam Do Yifan Lv Yonghua chen Zhikuan chen Fei chen Wei huang School of Flexible Electronics(Future Technologies)and Key Laboratory of Flexible Electronics(KLOFE)and Institute of Advanced Materials(IAM) Jiangsu National Synergetic Innovation Center for Advanced Materials(SICAM)Nanjing Tech UniversityNanjing 210009China department of Chemical and environmental Engineering University of Nottingham Ningbo ChinaNingbo 315000China Key Laboratory of Flexible Electronics of zhejiang Province Ningbo Institute of Northwestern Polytechnical UniversityNingbo 315103China Frontiers science Center for Flexible Electronics Xi'an Institute of Flexible Electronics(IFE)and Xi'an Institute of Biomedical Materials&EngineeringNorthwestern Polytechnical UniversityXi'an 710072China

The interfacial contacts between the electron transporting layers(ETLs)and the photoactive layers are crucial to device performance and stability for OSCs with inverted ***,atomic layer deposition(ALD)fabricated ultrathin Al_(2.O_(3)layers are applied to modify the ETLs/active blends(PM6:BTP-BO-4F)interfaces of OSCs,thus improving device *** ALD-Al_(2.O_(3)thin layers on ZnO significantly improved its surface morphology,which led to the decreased work function of ZnO and reduced recombination losses in *** simultaneous increase in open-circuit voltage(V_(OC)),short-circuit current density(J_(SC))and fill factor(FF)were achieved for the OSCs incorporated with ALD-Al_(2.O_(3)interlayers of a certain thickness,which produced a maximum PCE of 16.61%.Moreover,the ALD-Al_(2.O_(3)interlayers had significantly enhanced device stability by suppressing degradation of the photoactive layers induced by the photocatalytic activity of ZnO and passivating surface defects of ZnO that may play the role of active sites for the adsorption of oxygen and moisture.

关键词： atomic layer deposition interface modification organic solar cells stability

Global convergence in terrestrial gross primary production response to atmospheric vapor pressure deficit

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science china(Life sciences) 2024年第9期67卷 2016-2025页

作者： Chao huang Jingfeng huang Jingfeng Xiao Xing Li Hong SHe Yu Liang Fusheng {2. Hanqin Tian Key Laboratory of National Forestry and Grassland Administration on Forest Ecosystem Protection and Restoration of Poyang Lake Watershed College of ForestryJiangxi Agricultural UniversityNanchang 330045China CAS Key Laboratory of Forest Ecology and Management Institute of Applied EcologyChinese Academy of SciencesShenyang 110016China Institute of Applied Remote Sensing&Information Technology College of Environmental and Resource SciencesZhejiang UniversityHangzhou 310058China Key Laboratory of Agricultural Remote Sensing and Information Systems Zhejiang ProvinceZhejiang UniversityHangzhou 310058China Earth Systems Research Center Institute for the Study of EarthOceansand SpaceUniversity of New HampshireDurham NH 03824USA Research Institute of Agriculture and Life sciences Seoul National UniversitySeoul 08826South Korea School of Natural Resources University of Missouri203 ABNR BuildingColumbiaMO 65211USA Schiller Institute for Integrated science and Society Department of Earth and Environmental SciencesBoston CollegeChestnut HillMA 02467USA

Atmospheric vapor pressure deficit(VPD)increases with climate warming and may limit plant ***,gross primary production(GPP)responses to VPD remain a mystery,offering a significant source of uncertainty in the estimation of global terrestrial ecosystems carbon *** this study,in-situ measurements,satellite-derived data,and Earth System Models(ESMs)simulations were analysed to show that the GPP of most ecosystems has a similar threshold in response to VPD:first increasing and then *** VPD exceeds these thresholds,atmospheric drought stress reduces soil moisture and stomatal conductance,thereby decreasing the productivity of terrestrial *** ESMs underscore CO_(2. fertilization effects but predict significant GPP decline in low-latitude ecosystems when VPD exceeds the *** results emphasize the impacts of climate warming on VPD and propose limitations to future ecosystems productivity caused by increased atmospheric water *** VPD,soil moisture,and canopy conductance interactions into ESMs enhances the prediction of terrestrial ecosystem responses to climate change.

关键词： atmospheric water demands soil moisture stomatal conductance photosynthesis climate warming

Calibration of KEC Value in Acidic Red Soils with Fumigation-Extraction Method

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Pedosphere 2002年第1期12卷 33-40页

作者： chen GUOCHAO and HE ZHENLI department of Resource {2., College of environmental and Resource {2.s, Huajiachi Campus, zhejiang university, Hangzhou 31002. (china) department of Resource science College of Environmental and Resource Sciences Huajiachi Campus Zhejiang University Hangzhou 310029

Commonly used KEC value (0.45) of the fumigation-extraction (FE) method was obtained on the basis of temperate neutral soils. To ascertain its applicability to acidic red soils widespread in southern china and other subtropical regions, the KEC value was investigated based on 8 acidic red soils by in situ labelling of native soil microorganisms using 14C-labelled glucose. Realistic KEC value for red soils could be obtained by in situ 14C-labelling as long as an incubation period of 72.h is adopted after addition of 14C glucose to soil. The single KEC values for the eight red soils ranged from 0.2. to 0.35 and averaged 0.31. Lower KEC value obtained in red soils probably resulted from different soil quality, compared with other types of soil, which causes possible changes in microbial community structure and extractability of cellular component. Microbial biomass C contents of the eight red soils measured using a unique and constant KEC value of 0.45 decreased by 2..2.~40% in comparison to those usin g variable KEC values. The results suggest that microbial biomass C would be significantly underestimated using the present KEC value and a calibration of the KEC value is necessary for red soils.

关键词： calibration in situ 14C-labelling KEC value red soils

First wetland mapping at 10-m spatial resolution in South America using multi-source and multi-feature remote sensing data

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science china Earth sciences 2024年第10期67卷 3252-3269页

作者： Weiwei SUN Gang YANG Yuling huang Dehua MAO Ke huang Lin ZHU Xiangchao MENG Tian FENG Chao {2. Yong GE department of Geography and Spatial Information Techniques Ningbo UniversityNingbo 315211China State Key Laboratory of Resources and environmental Information System Institute of Geographic Sciences&Natural Resources ResearchChinese Academy of SciencesBeijing 100101China Natural Resources and Planning Bureau Shanghai Pudong New DistrictShanghai 200100China Key Laboratory of Wetland Ecology and Environment Northeast Institute of Geography and AgroecologyChinese Academy of SciencesChangchun 130102China Faculty of Electrical Engineering and Computer science Ningbo UniversityNingbo 315211China School of Geography science and Geomatics Engineering Suzhou University of Science and TechnologySuzhou 215009China

Wetland degradation has been accelerating in recent years globally. Accurate information on the geographic distribution and categories of wetlands is essential for their conservation and management. Despite being the world′s fourth largest continent, South America has limited research on wetland mapping, and there is currently no available map that provides comprehensive information on wetland distribution and categories in the region. To address this issue, we used Sentinel-1, Sentinel-2.and SRTM data, developed a sample collection method and a wetland mapping method with a collection of multi-source features such as optical features, polarization features and shape features for South American wetlands. We produced a 10-m resolution wetland map based on the Google Earth Engine(GEE) platform. Our Level-1 wetland cover map accurately captured six wetland sub-categories with an overall accuracy of 96.2.% and a kappa coefficient of 0.8649, while our Level-2.water cover map included five sub-categories with an overall accuracy of 97.2.% and a kappa coefficient of0.9368. The results show that the total area of existing wetlands in South America is approximately 1,737,000 km~2. which is6.8% of the total land area. Among the ten wetland categories, shallow sea had the largest area(960,52..4 km~2., while aquaculture ponds had the smallest area 1513.6 km~2. Swamp had the second largest area(306,2.0.1 km~2.. Brazil, Argentina,Venezuela, Bolivia, and Colombia were found to have the largest wetland areas, with Brazil and Colombia having the most diverse wetland categories. This product can serve as baseline data for subsequent monitoring, management, and conservation of South American wetlands.

关键词： Wetland mapping Google Earth Engine Sentinel imagery South America

Response of Stream Pollution Characteristics to Catchment Land Cover in Cao-E River Basin, china

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Pedosphere 2011年第1期21卷 115-123页

作者： SHEN Ye-Na LUE Jun chen Ding-Jiang SHI Yi-Ming department of Natural Resources College of Environmental Science and Natural Resources Zhejiang University Hangzhou 310029 (China) china Ministry of Education Key Lab of environmental Remediation and Ecological Health Zhejiang University Hangzhou 310029 (China) zhejiang Provincial Key Laboratory of Subtropical Soil and Plant Nutrition Zhejiang University Hangzhou 310029 (China)

This study addressed the relationship of river water pollution characteristics to land covers and human activities in the catchments in a complete river system named Cao-E River in eastern *** on the hydrogeochemical data collected monthly over a period of 3 years,cluster analysis(CA) and principal component analysis(PCA) were adopted to categorize the river reaches and reveal their pollution *** to the differences of water quality in the river reaches and land use patterns and average population densities in their catchments,the whole river system could be categorized into three groups of river reaches,i.e.,non-point sources pollution reaches(NPSPR),urban reaches(UR) and mixed sources pollution reaches(MSPR).In UR and MSPR,the water quality was mainly impacted by nutrient and organic pollution,while in NPSPR nutrient pollution was the main *** nitrate was the main nitrogen form in NPSPR and particulate phosphorus was the main phosphorus form in *** were no apparent trends for the variations of pollutant concentrations with increasing river flows in NPSPR and MSPR,while in UR the pollutant concentrations decreased with increasing river *** dry season was the critical period for water pollution control in ***,catchment land covers and human activities had significant impact on river reach water pollution type,nutrient forms and water quality responses to hydrological conditions,which might be crucial for developing strategies to combat water pollution in watershed scale.

关键词： cluster analysis hydrological conditions pollution factors principle component analysis water quality

Effects of Heavy Metals on Ammonification, Nitrification and Denitrification in Maize Rhizosphere

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Pedosphere 2001年第2期11卷 115-122页

作者： chenYINGXU YANGYE 等 DpartmentofEnivronmentalEngineering ZhejiangUniversityHangzhou310029（China） DpartmentofEnivronmentalEngineering ZhejiangUniversityofTechnologyHangzhou310032（China）

The ammonification, nitrification and denitrification in maize rhizosphere of alluvial soils were compared with those in the bulk soil after exposure to different kinds of heavy metals. The addition of cadmium at low levels (2.mg kg-1 and 5 mg kg-1) could stimulate the ammonification and nitrification in the soils, while inhibition influences were found at high levels of Cd addition (10 mg kg-1 and 2. mg kg-1). The relationship between microbial activity and cadmium concentration varied with the kind of microorganisms. The nitrifying bacteria were more sensitive to cadmium pollution than the ammonifying bacteria. When Cd(II), Cu(II) and Cr(VI) were compared at the same addition concentration of 2. mg kg-1 soil, Cd(II) was the most effective inhibitor of ammonification and denitrification among the three investigated heavy metals, and Cr(VI) had the most strong inhibitory influence on the nitrifying bacteria. The microbial activities in rhizosphere were higher than those in the bulk soil for most of the treatments. Cr(VI) proved to be the most effective in enhancing the microbial activities in rhizosphere, and this could be caused by the positive reduction of Cr(VI) to Cr(III) in rhizosphere, and the relatively sufficient existence of organic matter which intensified the adsorption of the metal. It seemed that the rhizosphere had some mitigation effect on heavy metal toxicity.

关键词： ammonification denitrification heavy metal pollution nitrification rhizosphere