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Journal of Magnesium and Alloys 2024年第3期12卷 1170-1185页

作者： Junping Shen tao Lai zheng Yin Yang Chen Kun Wang Hong Yan Honggun Song Ruiliang Liu Chao Luo Zhi Hu School of Advanced Manufacturing Nanchang UniversityNanchang 330031China Institute for Advanced Study Nanchang UniversityNanchang 330031China Singapore Centre for Environmental Life Sciences Engineering Nanyang Technological University60 Nanyang Drive 637751Singapore

Revealing the localized corrosion process of Mg alloy is considered as one of the most significant ways for improving its corrosion *** reliable monitor should be high distinguishability and real-time in liquid ***,Mg-9Al-1Fe and Mg-9Al-1Fe-1Gd alloys were designed to highlight the impact of intermetallic on the corrosion ***-situ AFM with a special electrolyte circulation system and quasi-in-situ SEM observation were used to monitor the corrosion process of the designed ***-EDS and TEM-SAED were applied to identify the intermetallic in the designed alloys,and their volta potentials were measured by *** to the real-time and real-space in-situ AFM monitor,the corrosion process consisted of dissolution of anodicα-Mg phase,accumulation of corrosion products around cathodic phase and shedding of some fine cathodic ***,the localized corrosion process of Mg alloy was revealed combined with the results of the monitor of corrosion process and Volta potential difference.

关键词： Magnesium Localized corrosion In-situ AFM SKPFM Corrosion behaviour.

A solubility limited pyrene-4,5,9,10-tetraone-based covalent organic framework for high-performance aqueous zinc-organic batteries

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Nano Research 2024年第6期17卷 5095-5103页

作者： Min Cheng Shibing zheng Tianjiang Sun Diantao Li Weijia Zhang zhengtai Zha Qiong Sun Jing Tian Kai Zhang Zhanliang tao Frontiers Science Center for New Organic Matter State Key Laboratory of Advanced Chemical Power SourcesKey Laboratory of Advanced Energy Materials Chemistry(Ministry of Education)Collaborative Innovation Center of Chemical Science and Engineering(Tianjin)Renewable Energy Conversion and Storage CentreNankai UniversityTianjin 300071China Haihe Laboratory of Sustainable Chemical Transformations Tianjin 300192China

Pyrene-4,5,9,10-tetraone(PTO),with a high theoretical capacity of 408 mAh·g^(−1),is a promising candidate for rechargeable aqueous zinc-ion batteries(RAZIBs),but its zincated products during discharge process suffer from high solubility in ***,aβ-ketoenamine-linked two-dimensional(2D)covalent organic framework(COF)based on a 2,7-diaminopyrene-4,5,9,10-tetraone(4KT-BD)monomer and a 2,4,6-trihydroxy-benzene-1,3,5-tricarbaldehyde(Tp)node(4KT-Tp-COF)is synthesized to address the above *** well-designed 4KT-Tp-COF displays low solubility in 3 M Zn(CF3SO3)2 owing to the favorableπ-πstacking as well as extended ***,the ingenious structural design of the active molecule and the long-range ordered nano-channels alter the intramolecular electron distribution,which facilitates the ionic ***,the 4KT-Tp-COF cathode exhibits a stable capacity of 181 mAh·g^(−1)at 0.2 A·g^(−1),superior rate capability of 139 mAh·g^(−1)at 20 A·g^(−1),and a long lifetime of 1000 cycles without capacity loss at 30 A·g^(−1).Even at a low temperature of−20°C,the electrode also performs an ultralong cycling life of 9000 cycles with a capacity of 106 mAh·g^(−1)at 5 A·g^(−1).The comprehensive characterizations of ex-situ analyses together with the theoretical calculations validate that the groups of C=O can contribute highly accessible redox-active sites for Zn^(2+)*** ultra-stable 4KT-Tp-COF cathode provides important insights for designing robust organic electrodes for sustainable and large-scale electrochemical energy storage.

关键词： pyrene-4,5,9,10-tetraone solubility limited covalent organic framework zinc batteries

Layered niobium carbide enabling excellent kinetics and cycling stability of Li-Mg-B-H hydrogen storage material Layered niobium carbide enabling excellent kinetics

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Rare Metals 2024年第3期43卷 1153-1166页

作者： Li-wen Lu Hui Luo Guang-Xu Li Yun Li Xin-Hua Wang Cun-Ke Huang Zhi-QiangLan wen-zheng Zhou Jin Guo Mohammad Ismail Hai-Zhen Liu Guangxi Novel Battery Materials Research Center of Engineering Technology Guangxi Colleges and Universities Key Laboratory of Blue Energy and Systems IntegrationSchool of Physical Science and TechnologyGuangxi UniversityNanning530004China State Key Laboratory of Featured Metal Materials and Life-Cycle Safety for Composite Structures Nanning530004China School of Mechanical and Electrical Engineering Quzhou College of TechnologyQuzhou324000China Department of Materials Science and Engineering Zhejiang UniversityHangzhou310027China Faculty of Ocean Engineering Technology and Informatics Universiti Malaysia Terengganu21030Kuala NerusTerengganuMalaysia Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education) Nankai UniversityTianjin300071China

The Li-Mg-B-H composite(2LiBH_(4)+MgH_(2))has a high capacity of 11.4 wt%as a hydrogen storage ***,the slow kinetics and poor cycling stability severely restrict its practical *** this work,a layered Nb_(2)C MXene was first synthesized and then introduced to tailor the kinetics and cycling stability of the Li-Mg-B-H *** milled 2LiH+MgB_(2)composites were initially hydrogenated to obtain the 2LiBH_(4)+MgH_(2)*** 2LiBH_(4)+MgH_(2)+5wt%Nb_(2)C can release 9.0 wt%H_(2)in 30 min at 400℃,while it is only 2.7 wt%for the undoped 2LiBH_(4)+MgH_(2).The dehydrogenation activation energies of MgH_(2)and LiBH_(4)are 123 and 154 kJ·mol^(-1)respectively for the 5 wt%Nb_(2)C-doped composite,lower than the undoped composite(164 and 165 kJ·mol^(-1)).The 2LiBH_(4)+MgH_(2)+5 wt%Nb_(2)C possesses excellent cycling stability,with the reversible capacity only slightly reduced from 9.4 wt%for the 1st cycle to 9.3 wt%for the 20th ***_(2)C keeps stable in the composite and acts as an efficient catalyst for the Li-Mg-B-H *** is believed that both the layered structure and the active Nb element contribu te to the enhanced hydrogen storage performances of the Li-Mg-B-H *** work confirms that the Nb_(2)C MXene with layered stru cture has a significant enhancing impact on the Li-Mg-B-H hydrogen storage materials,which is different from the bulk NbC.

关键词： Hydrogen storage Lithium borohydride Magnesium hydride Nb_(2)C MXene

An efficient online histogram publication method for data streams with local differential privacy

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Frontiers of Information Technology & Electronic Engineering 2024年第8期25卷 1096-1109页

作者： tao tao Funan ZHANG Xiujun WANG Xiao zheng Xin ZHAO School of Computer Science and Technology Anhui University of TechnologyMaanshan 243032China Anhui Engineering Research Center for Intelligent Applications and Security of Industrial Internet Maanshan 243032China Engineering Research Institute Anhui University of TechnologyMaanshan 243032China Shengli No.1 Middle School of Dongying City Dongying 257000China

Many areas are now experiencing data streams that contain privacy-sensitive *** the sharing and release of these data are of great commercial value,if these data are released directly,the private user information in the data will be ***,how to continuously generate publishable histograms(meeting privacy protection requirements)based on sliding data stream windows has become a critical issue,especially when sending data to an untrusted third *** histogram publication methods are unsatisfactory in terms of time and storage costs,because they must cache all elements in the current sliding window(sW).Our work addresses this drawback by designing an efficient online histogram publication(EOHP)method for local differential privacy data ***,in the EOHP method,the data collector first crafts a histogram of the current SW using an approximate counting ***,the data collector reduces the privacy budget by using the optimized budget absorption mechanism and adds appropriate noise to the approximate histogram,making it possible to publish the histogram while retaining satisfactory data *** experimental results on two different real datasets show that the EOHP algorithm significantly reduces the time and storage costs and improves data utility compared to other existing algorithms.

关键词： Data stream Differential privacy Sliding windows Approximate counting

Global Marine Cold Seep Metagenomes Reveal Diversity of Taxonomy,Metabolic Function,and Natural Products

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Genomics, Proteomics & Bioinformatics 2024年第2期22卷 121-134页

作者： tao Yu Yingfeng Luo Xinyu Tan Dahe Zhao Xiaochun Bi Chenji Li Yanning zheng Hua Xiang Songnian Hu State Key Laboratory of Microbial Resources Institute of MicrobiologyChinese Academy of SciencesBeijing 100101China University of Chinese Academy of Sciences Beijing 100049China

Cold seeps in the deep sea are closely linked to energy exploration as well as global climate *** alkane-dominated chemical energy-driven model makes cold seeps an oasis of deep-sea life,showcasing an unparalleled reservoir of microbial genetic ***,by analyzing 113 metagenomes collected from 14 global sites across 5 cold seep types,we present a comprehensive Cold Seep Microbiomic Database(CSMD)to archive the genomic and functional diversity of cold seep *** CSMD includes over 49 million non-redundant genes and 3175 metagenome-assembled genomes,which represent 1895 species spanning 105 *** addition,beta diversity analysis indicates that both the sampling site and cold seep type have a substantial impact on the prokaryotic microbiome community *** and anaerobic metabolisms are prevalent in microbial communities,accompanied by considerable mixotrophs and facultative anaerobes,highlighting the versatile metabolic potential in cold ***,secondary metabolic gene cluster analysis indicates that at least 98.81%of the sequences potentially encode novel natural products,with ribosomally synthesized and post-translationally modified peptides being the predominant type widely distributed in archaea and ***,the CSMD represents a valuable resource that would enhance the understanding and utilization of global cold seep microbiomes.

关键词： Global marine cold seep Metagenome Prokaryotic microbiome Metabolic function Natural product

Demonstration of acousto-optical modulation based on a thin-film AlScN photonic platform

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Photonics Research 2024年第6期12卷 1138-1149页

作者： KEWEI BIAN ZHENYU LI YUSHUAI LIU SUMEI XU XINGYAN ZHAO YANG QIU YUAN DONG QIZE ZHONG tao WU SHAONAN zheng TING HU School of Microelectronics Shanghai UniversityShanghai 201800China School of Information Science and Technology ShanghaiTech UniversityShanghai 201210China Shanghai Institute of Microsystem and Information Technology Chinese Academy of SciencesShanghai 200050China University of Chinese Academy of Sciences Beijing 100049China

Acousto-optic(AO)modulation technology holds significant promise for applications in microwave and optical signal ***-film scandium-doped aluminum nitride(AlScN),with excellent piezoelectric properties and a wide transparency window,is a promising candidate for achieving on-chip AO modulation with a fabri-cation process compatible with complementary metal-oxide-semiconductor(CMOS)*** study presents,to the best of our knowledge,the first demonstration of AO modulators with surface acoustic wave generation and photonic waveguides monolithically integrated on a 400-nm-thick film of AlScN on an *** intramodal AO modulation is realized based on an AlScN straight waveguide,and the modulation efficiency is significantly enhanced by 12.3 dB through the extension of the AO interaction length and the utilization of bidirectional acoustic *** intermodal AO modulation and non-reciprocity are further demonstrated based on a multi-mode spiral waveguide,achieving a high non-reciprocal contrast(>10 dB)across an optical bandwidth of 0.48 *** research marks a significant stride forward,representing an advancement in the realization of microwave photonic filters,magnet-free isolators,and circulators based on the thin-film AlScN photonic platform.

关键词： waveguide film microwave

3D vertically aligned microchannel structure to enhance piezoelectric energy harvesting performance of PZT/PVDF&CNTs piezoelectric composites

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Journal of Materiomics 2024年第5期10卷 1063-1070页

作者： Limin Hou Yu Huan Mupeng zheng Yilong Liu Chuilei Wang Xinjian Wang Changxiao Li Zhenxing Wang tao Wei School of Materials Science and Engineering University of JinanJinan250022China Key Laboratory of Advanced Functional Materials Faculty of Materials and ManufacturingBeijing University of TechnologyBeijing100124China Electronic Materials Research Laboratory Key Laboratory of the Ministry of Education and International Center for Dielectric ResearchXi'an Jiaotong UniversityXi'an710049China SICC Co. LtdJinan250000China

Piezoelectric energy harvesters(PEHs)have attracted significant attention with the ability of converting mechanical energy into electrical energy and power the self-powered microelectronic ***,material's superior energy harvesting performance is closely related to its high transduction coefficient(d_(33)×g_(33)),which is dependent on higher piezoelectric coefficient d33 and lower dielectric constantεr of ***,the high d33 and lowεr are difficult to be simultaneously achieved in piezoelectric ***,lead zirconate titanate(PZT)based piezoelectric composites with vertically aligned microchannel structure are constructed by phase-inversion *** polyvinylidene fluoride(PVDF)and carbon nanotubes(CNTs)are mixed as fillers to fabricate PZT/PVDF&CNTs *** unique structure and uniformly distributed CNTs network enhance the polarization and thus improve the *** PVDF filler effectively reduce theε*** a consequence,the excellent piezoelectric coefficient(d_(33)=595 pC/N)and relatively low dielectric constant(ε_(r)=1,603)were obtained in PZT/PVDF&CNTs composites,which generated an ultra-high d_(33)×g_(33) of 24,942×10^(−15) m^(2)/***,the PZT/PVDF&CNTs piezoelectric composites achieve excellent energy harvesting performance(output voltage:66 V,short current:39.22μA,and power density:1.25μW/mm^(2)).Our strategy effectively boosts the performance of piezoelectric-polymer composites,which has certain guiding significance for design of energy harvesters.

关键词： Piezoelectric-polymer composites Phase-inversion method 3D vertically aligned microchannel structure Piezoelectric energy harvester Carbon nanotubes

Theta Oscillations Support Prefrontal-hippocampal Interactions in Sequential Working Memory

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Neuroscience Bulletin 2024年第2期40卷 147-156页

作者： Minghong Su Kejia Hu Wei Liu Yunhao Wu tao Wang Chunyan Cao Bomin Sun Shikun Zhan zheng Ye Institute of Psychology Chinese Academy of SciencesBeijing 100101China Department of Psychology University of Chinese Academy of SciencesBeijing 100049China Department of Neurosurgery Center for Functional NeurosurgeryRuijin HospitalShanghai Jiao Tong University School of MedicineShanghai 200025China Institute of Neuroscience Center for Excellence in Brain Science and Intelligence TechnologyChinese Academy of SciencesShanghai 200031China

The prefrontal cortex and hippocampus may support sequential working memory beyond episodic memory and spatial *** stereoelectroencephalography(SEEG)study investigated how the dorsolateral prefrontal cortex(DLPFC)interacts with the hippocampus in the online processing of sequential *** patients with epilepsy(eight women,age 27.6±8.2 years)completed a line ordering task with SEEG recordings over the DLPFC and the *** showed longer thinking times and more recall errors when asked to arrange random lines clockwise(random trials)than to maintain ordered lines(ordered trials)before recalling the orientation of a particular ***,the ordering-related increase in thinking time and recall error was associated with a transient theta power increase in the hippocampus and a sustained theta power increase in the DLPFC(3–10 Hz).In particular,the hippocampal theta power increase correlated with the memory precision of line ***,theta phase coherences between the DLPFC and hippocampus were enhanced for ordering,especially for more precisely memorized ***,the theta band DLPFC→hippocampus influence was selectively enhanced for ordering,especially for more precisely memorized *** study suggests that theta oscillations may support DLPFC-hippocampal interactions in the online processing of sequential information.

关键词： Sequential working memory Hippocampus Dorsolateral prefrontal cortex Theta oscillations Stereoelectroencephalography(SEEG) Phase coherence Granger causality

Self-templating synthesis of biomass-based porous carbon nanotubes for energy storage and catalytic degradation applications

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Green Energy & Environment 2024年第3期9卷 584-595页

作者： Manman Xu Shiqi Fu Yukai wen Wei Li Qiongfang Zhuo Haida Zhu Zhikeng zheng Yuwen Chen Anqi Wang Kai Yan Research Centre for Eco-Environmental Engineering School of Environment and Civil EngineeringDongguan University of TechnologyDongguan523808China School of Environmental Science and Engineering Sun Yat-sen UniversityGuangzhou510275China

Dwindling energy sources and a worsening environment are huge global problems,and biomass wastes are an under-exploited source of material for both energy and material ***,self-template decoction dregs of Ganoderma lucidum-derived porous carbon nanotubes(ST-DDLGCs)were synthesized via a facile and scalable strategy in response to these ***-DDLGCs exhibited a large surface area(1731.51 m^(2)g^(-1))and high pore volume(0.76 cm^(3)g^(-1)),due to the interlacing tubular structures of precursors and extra-hierarchical porous structures on tube *** the ST-DDLGC/PMS system,the degradation efficiency of capecitabine(CAP)reached~97.3%within 120 ***,ST-DDLGCs displayed high catalytic activity over a wide pH range of 3–9,and strong anti-interference to these typical and ubiquitous anions in wastewater and natural water bodies(i.e.,H_(2)PO_(4)^(-),NO_(3)^(-),Cl^(-) and HCO_(3)^(-)),in which a ^(1)O_(2)-dominated oxidation was identified and non-radical mechanisms were ***,ST-DDLGC-based coin-type symmetrical supercapacitors exhibited outstanding electrochemical performance,with specific capacitances of up to 328.1 F g^(-1)at 0.5 A g^(-1),and cycling stability of up to 98.6%after 10,000 cycles at a current density of 2 A g^(-1).The superior properties of ST-DDLGCs could be attributed to the unique porous tubular structure,which facilitated mass transfer and presented numerous active *** results highlight ST-DDLGCs as a potential candidate for constructing inexpensive and advanced environmentally functional materials and energy storage devices.

关键词： Ganoderma lucidum residue Porous carbon nanotubes Self-template method Wastewater treatment Supercapacitor electrode

Evaluation of Resistance of Different Kiwifruit Varieties (Lines) to Canker Disease and Brown Spot Disease

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Phyton-International Journal of Experimental Botany 2024年第6期93卷 1249-1261页

作者： wenwen Su Chongpei zheng Zhencheng Han Chunguang Ren Di Wu tao Li Yi Yang Weijie Li Institute of Mountain Resources of Guizhou Province Guizhou Academy of SciencesGuiyang550001China Guizhou Botanical Garden Guizhou Academy of SciencesGuiyang550001China Key Laboratory of Plant Resource Conservation and Germplasm Innovation in Mountainous Region(Ministry of Education) Institute of Agro-Bioengineering/College of Life SciencesGuizhou UniversityGuiyang550025China

Kiwifruit canker and brown spot are signiﬁcant diseases affecting kiwis,caused by Pseudomonas syringae patho-genic variations(Pseudomonas syringae ***(Psa))and Corynesporapolytica(Corynespora cassiicola).At present,the research on canker disease and brown spot disease mainly focuses on the isolation and identiﬁcation of pathogenic bacteria,drug control,resistance gene mining and functional veriﬁ*** has proved that breeding disease resistant varieties are an effective method to control canker disease and brown spot ***,most existing cultivars lack genes for canker and brown spot *** kiwifruit resources in nat-ure exhibit extensive genetic diversity due to prolonged natural selection,containing numerous resistance ***,due to insufﬁcient understanding of the resistance of most kiwifruit varieties(lines)to canker disease and brown spot disease,some high-quality resources have not been fully *** incidence of canker and brown spot of 18 kiwifruit cultivars(lines)was measured by inoculating isolated branches and leaves,and their resistance to canker and brown spot was analyzed according to the length,disease index,mean diameter,and systematic *** results were as follows:Among 18 different kiwifruit varieties(lines)for canker disease,there were two highly resistant materials,eight disease-resistant materials,four disease-susceptible materials,and two highly susceptible ***,regarding brown spot disease,there were one highly resistant material,ﬁve dis-ease-resistant materials,four susceptible materials,and three highly susceptible ***,four resources were resistant to both *** outcomes provided a theoretical basis for breeding kiwifruit against canker and brown spot.

关键词： Kiwifruit canker disease brown spot resistance evaluation