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Recent progress in metal-organic frameworks(Part II—material application)

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Science China Chemistry 2025年

作者： Jiandong Pang wentao Jiang Xue-wen Zhang Hao-Long Zhou Yuxiu Sun Wei Gong Bin Wang Fuyin Ma Linwei He Long Chen Qiang Chen He-Qi Zheng Yuanjing Cui wen-jie Shi Chao Zhang Mei Wang Yue-Biao Zhang jie-Peng Zhang Chongli Zhong Yong Cui Shuao Wang Jian-Rong Li Guodong Qian Tong-Bu Lu Huan Pang Xian-He Bu Institute for New Energy Materials and Low Carbon Technologies School of Materials Science and Engineering Tianjin University of Technology School of Chemistry and Chemical Engineering Yangzhou University School of Materials Science and Engineering Nankai University School of Physical Science and Technology ShanghaiTech University MOE Key Laboratory of Bioinorganic and Synthetic Chemistry GBRCE for Functional Molecular Engineering School of Chemistry IGCMESun Yat-sen University Department of Chemistry Shantou University School of Chemical Engineering and Technology Tiangong University School of Chemistry and Chemical Engineering Shanghai Jiao Tong University State Key Laboratory of Radiation Medicine and Protection School for Radiological and Interdisciplinary Sciences Soochow University College of Materials Science & Engineering Beijing University of Technology State Key Laboratory of Silicon and Advanced Semiconductor Materials Cyrus Tang Center for Sensor Materials and ApplicationsSchool of Materials Science & Engineering Zhejiang University

As a class of functional crystalline porous materials, metal-organic frameworks(MOFs) gained rapid development in the past three decades and a large number of MOFs with ordered structures, high surface areas, and functionalized channels have been investigated. MOFs and MOF-derived/composite materials show great potential in many application fields. In this review, we discussed the main applications of MOFs and MOF-derived/composite materials in small molecule storage, separation, luminescence, sensing, multitype catalysis, and energy storage. In addition, challenges and problems in the future research of MOFsrelated fields are also discussed.

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Ordered proposition fusion based on consistency and uncertainty measurements

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Science China(Information Sciences) 2017年第8期60卷 117-135页

作者： Dayou LIU Yungang ZHU ni ni jie LIU College of Computer Science and Technology Jilin University Key Laboratory of Symbolic Computation and Knowledge Engineering of Ministry of Education Jilin University Beijing Entry-Exit Inspection and Quarantine Bureau

The fusion of ordered propositions is an important and widespread problem in artificial intelligence,but existing fusion methods have difficulty handling the fusion of ordered propositions. In this paper, we propose a solution based on consistency and uncertainty measurements. The main contributions of this paper are as follows. First, we propose the concept of convexity degree, mean, and center of basic support function to comprehensively describe the basic support function of ordered propositions. Second, we introduce entropy as a measure of uncertainty in the basic support function of ordered propositions. Third, we generalize the indeterminacy of the basic support function and propose a novel method to measure the consistency between two basic support functions. Finally, based on the above researches, we propose a novel algorithm for fusing ordered propositions. Theoretical analysis and experimental results demonstrate that the proposed method outperforms state-of-the-art methods.

关键词： uncertainty processing ordered proposition evidence theory dempster rule of combination information fusion

Regional features of pollen R-values in China

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Science China Earth Sciences 2024年第1期67卷 295-308页

作者： jie XIA Jian ni College of Life Sciences Zhejiang Normal UniversityJinhua 321004China Jinhua Mountain Observation and Research Station for Subtropical Forest Ecosystems Jinhua 321004China

Establishing a quantitative relationship between modern pollen and vegetation remains a pivotal but intricate pursuit within the field of Quaternary *** R-value,a well-established and traditional metric characterized by its simplicity and direct applicability,serves to calibrate the nonlinear disparities between surface pollen and modern *** study entails the construction of a comprehensive pollen R-value dataset for China derived from R-values published between 1987 and *** dataset,compiled after rigorous screening,calibration,and standardization processes,encompasses 898 modern pollen sampling sites and 2115 pollen R-value data entries,encapsulating 152 pollen taxa spanning 65 families and 113 *** the extracted R-values yielded the following insights:(1)A macrospatial analysis validates previously established knowledge at a site-specific ***,pollen R-value variations across China are statistically *** two-thirds of pollen taxa exhibit underrepresentation(e.g.,Taxodiaceae,Corylus,nitraria,Tamarix,Cyperaceae,Poaceae,and Fabaceae),while the remaining one-third display overrepresentation(e.g.,Pinus,Picea,Betula,Ephedra,Chenopodiaceae,and Artemisia).The degree of underrepresentation surpasses that of overrepresentation,and the representation patterns of Castanea,Quercus,Polygonaceae,and Asteraceae are contingent upon vegetation types.(2)Pollen R-values follow distinct spatial distribution patterns within *** the woody vegetation region of eastern China,R-values progressively decline from north to south,correlating with rising temperatures and ***,in herbaceous vegetation regions of northern and western China,R-values decrease from east to west and from northeast to southwest,corresponding to increased ***,pollen R-values manifest variation contingent on pollen taxa,vegetation types,and climatic regions,even differing for the same taxa across varying

关键词： Pollen R-value Modern pollen-vegetation relationship Regional pattern Variability Paleovegetation reconstruction

Catalyst–Support Interaction in Polyaniline‑Supported ni_(3)Fe Oxide to Boost Oxygen Evolution Activities for Rechargeable Zn‑Air Batteries

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Nano-Micro Letters 2025年第1期17卷 176-190页

作者： Xiaohong Zou Qian Lu Mingcong Tang jie Wu Kouer Zhang wenzhi Li Yunxia Hu Xiaomin Xu Xiao Zhang Zongping Shao Liang An Department of Mechanical Engineering The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong SARPeople’s Republic of China Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment TechnologySchool of Environmental Science and TechnologyNanjing University of Information Science and TechnologyNanjing 210044People’s Republic of China Department of Chemistry The Chinese University of Hong KongMa Lin BuildingShatinHong Kong SAR 999077People’s Republic of China WA School of Mines:Minerals Energy and Chemical Engineering(WASM‑MECE)Curtin UniversityPerthWA 6102Australia Research Institute for Advanced Manufacturing The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong SARPeople’s Republic of China Research Institute for Smart Energy The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong SARPeople’s Republic of China

Catalyst–support interaction plays a crucial role in improving the catalytic activity of oxygen evolution reaction(OER).Here we modulate the catalyst–support interaction in polyaniline-supported ni_(3)Fe oxide(ni_(3)Fe oxide/PAni)with a robust hetero-interface,which significantly improves oxygen evolution activities with an overpotential of 270 mV at 10 mA cm^(-2)and specific activity of 2.08 mA cm_(ECSA)^(-2)at overpotential of 300 mV,3.84-fold that of ni_(3)Fe *** is revealed that the catalyst–support interaction between ni_(3)Fe oxide and PAni support enhances the ni–O covalency via the interfacial ni–N bond,thus promoting the charge and mass transfer on ni_(3)Fe *** the excellent activity and stability,rechargeable Zn-air batteries with optimum ni_(3)Fe oxide/PAni are assembled,delivering a low charge voltage of 1.95 V to cycle for 400 h at 10 mA cm^(-2).The regulation of the effect of catalyst–support interaction on catalytic activity provides new possibilities for the future design of highly efficient OER catalysts.

关键词： Catalyst-support interaction Supported catalysts Heterointerface Oxygen evolution reaction Zn-air batteries

Spin polarization and production rate studies of surface muons in a novel solenoid capture system based on CSNS

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Nuclear Science and Techniques 2017年第8期28卷 61-68页

作者： Ran Xiao Yan-Fen Liu Xiao-jie ni Zi-wen Pan Bang-Jiao Ye State Key Laboratory of Particle Detection and Electronics University of Science and Technology of China Hefei 230026 China Department of Modern Physics University of Science and Technology of China Hefei 230026 China Institute of High Energy Physics Chinese Academy ofSciences Beijing 100049 China

A novel surface muon capture system with a large acceptance was proposed based on the China spallation neutron source(CSNS).This system was designed using a superconducting solenoid where a long graphite target was put inside ***,the spin polarization evolution was studied in a constant uniform magnetic *** the magnetic field can interact with the spin of the surface muon,both the spin polarization and production rate of the surface muons collected by the new capture system were calculated by the *** results showed that the surface muons could still keep a high spin polarization([90%)with different magnetic fields(0–10 T),and the larger magnetic field is,the more surface muons can be ***,the proton phase space,Courant–Snyder parameters,and intensities of surface muons of different beam fractions were given with magnetic fields of 0 and *** solenoid capture system can focus proton and surface muon beams and collect p?and l?*** can also provide an intense energetic positron source.

关键词：自旋极化率采集系统 μ介子表面电磁生产均匀磁场自旋相互作用

Crystallization characteristics of iron-rich glass ceramics prepared from nickel slag and blast furnace slag

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International Journal of Minerals,Metallurgy and Materials 2011年第4期18卷 455-459页

作者： Zhong-jie Wang wen ni Ke-qing Li Xiao-yan Huang Li-ping Zhu School of Civil and Environmental Engineering University of Science and Technology Beijing Beijing 100083 China

The crystallization process of iron-rich glass-ceramics prepared from the mixture of nickel slag（NS） and blast furnace slag（BFS） with a small amount of quartz sand was investigated.A modified melting method which was more energy-saving than the traditional methods was used to control the crystallization *** results show that the iron-rich system has much lower melting temperature,glass transition temperature（Tg）,and glass crystallization temperature（Tc）,which can result in a further energy-saving *** results also show that the system has a quick but controllable crystallization process with its peak crystallization temperature at 918°*** crystallization of augite crystals begins from the edge of the sample and invades into the whole *** crystallization process can be completed in a few minutes.A distinct boundary between the crystallized part and the non-crystallized part exists during the *** the non-crystallized part showing a black colour,some sphere-shaped augite crystals already exist in the glass matrix before samples are heated to *** the crystallized part showing a khaki colour,a compact structure is formed by augite crystals.

关键词： glass ceramics grain growth crystallization slag

Ultrasound Imaging of Pipeline Crack Based on Composite Transducer Array

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Chinese Journal of Mechanical Engineering 2018年第5期31卷 25-34页

作者： Shou-Peng Song Ying-jie ni Department of Instrument Science and Engineering School of Mechanical Engineering Jiangsu University

Cracks, especially small cracks are di cult to be detected in oil and gas transportation pipelines buried underground or covered with layers of material by using the traditional ultrasonic inspection techniques. Therefore, a new com?posite ultrasonic transducer array with three acoustic beam incidence modes is developed. The space model of the array is also established to obtain the defect reflection point location. And the crack ultrasound image is thus formed through a series of small cubical elements expanded around the point locations by using the projection of binariza?tion values extracted from the received ultrasonic echo signals. Laboratory experiments are performed on a pipeline sample with di erent types of cracks to verify the e ectiveness and performance of the proposed technique. From the image, the presence of small cracks can be clearly observed, in addition to the sizes and orientations of the cracks. The proposed technique can not only inspect common flaws, but also detect cracks with various orientations, which is helpful for defect evaluation in pipeline testing.

关键词： Composite transducer array Ultrasound imaging Crack NDT&E

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环糊精聚合物在食品分析样品前处理中的应用

分析测试学报 2025年第1期44卷 34-42页

作者：王楠王媛宗帅赵文杰河南工业大学化学化工学院河南郑州450001 宁夏计量质量检验检测研究院宁夏银川750411

环糊精聚合物(CDPs)是由环糊精(CD)分子以化学键合等手段构筑的含有多个环糊精单元的高分子衍生物,不仅很好地保留了环糊精的包络识别性能,还兼具聚合物优良的机械强度、稳定性和化学可调性等优点。CDPs在样品前处理中具有广泛的应用潜... 详细信息

环糊精聚合物(CDPs)是由环糊精(CD)分子以化学键合等手段构筑的含有多个环糊精单元的高分子衍生物,不仅很好地保留了环糊精的包络识别性能,还兼具聚合物优良的机械强度、稳定性和化学可调性等优点。CDPs在样品前处理中具有广泛的应用潜力,选择性吸附与分离、高效去除污染物、可再生性与环保性等特性为其在环境保护、食品安全等领域的应用提供了有力支持。该文概括了不同的CDPs的合成方法及其在食品分析样品前处理领域的重要作用,通过与固相微萃取、磁性固相萃取、搅拌棒萃取等技术结合,CDPs能够有效地分离和富集食品中的目标分析物(如农药残留、食品添加剂和天然香味成分等)。并总结与展望了CDPs的发展现状和未来发展趋势。

关键词：环糊精环糊精聚合物样品前处理食品分析选择性吸附

Numerical simulation of base flow with hot base bleed for two jet models

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Defence Technology（防务技术） 2014年第3期10卷 279-284页

作者： wen-jie YU Yong-gang YU Bin ni School of Energy and Power Engineering Nanjing University of Science & Technology North Information Control Group Ltd

In order to improve the benefits of base bleed in base flow field,the base flow with hot base bleed for two jet models is *** axisymmetric Navier-Stokes equations are computed by using a finite volume *** base flow of a cylinder afterbody with base bleed is *** simulation results are validated with the experimental data,and the experimental results are well *** this basis,the base flow fields with base bleed for a circular jet model and an annulus jet model are investigated by selecting the injection temperature from 830 K to 2200 *** results show that the base pressure of the annular jet model is higher than that of the circular jet model with the changes of the injection parameter and the injection *** the circular jet model,the hot gases are concentrated in the vicinity of the *** the annular jet model,the bleed gases flow into the shear layer directly so that the hot gases are concentrated in the shear *** latter temperature distribution is better for the increase of base pressure.

关键词： Fluid mechanics Base bleed Base flow Numerical simulation Annulus jet