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Dielectric genetic tailoring strategy dominating MoSe_(2)@rGO assembled architecture with electromagnetic functions

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Journal of Advanced Ceramics 2024年第9期13卷 1461-1472页

作者： wen-qiang cao Qi Zheng Lin Li Chuan-Bao cao Mao-Sheng cao School of Materials Science and Engineering Beijing Institute of TechnologyBeijing 100081China Key Laboratory for Photonic and Electronic Bandgap Materials Ministry of EducationSchool of Physics&Electron EngineeringHarbin Normal UniversityHarbin 150025China

The intensification of electromagnetic(EM)pollution and the development of military detection technology have increased the requirements for EM functional *** this study,a molybdenum diselenide@reduced graphene oxide(MoSe_(2)@rGO)-assembled architecture is constructed,where the MoSe_(2) nanosheets grow uniformly on the rGO *** regulating the contributions of conduction genes and polarization genes,adjustable EM functions of MoSe_(2)@rGO hybrids can be *** reflection loss(RL)of the sample can reach−68.7 dB at a thickness of 2.32 mm,and the maximum effective absorption bandwidth can reach 5.04 *** conduction genes dominate,the MoSe_(2)@rGO hybrids exhibit a 98.7%electromagnetic interference(EMI)shielding *** design of the EM energy conversion device and the results of the radar cross section(RCS)simulation demonstrate the practical application potential of the *** work provides inspiration for designing multifunctional EM materials.

关键词： MoSe_(2) graphene hybrids dielectric gene microwave absorption(MA) electromagnetic interference(EMI)shielding

A multifunctional stealthy material for wireless sensing and active camouflage driven by configurable polarization

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Journal of Materials Science & Technology 2023年第1期132卷 42-49页

作者： Min Zhang Mao-Sheng cao qiang-qiang Wang Xi-Xi Wang wen-qiang cao Hui-Jing Yang Jie Yuan School of Materials Science and Engineering Beijing Institute of TechnologyBeijing 100081China Department of Physics Beijing Technology and Business UniversityBeijing 100048China School of Electrical and Electronic Engineering Nanyang Technological University639798Singapore Department of Physics Tangshan Normal UniversityTangshan 063000China School of Information Engineering Minzu University of ChinaBeijing 100081China

The dipole species transformation and polarization relaxation configuration are achieved by changing the cobalt ion stoichiometry,which precisely tailors the electromagnetic attenuation performance of bismuth iron cobalt *** the stoichiometric ratio of Fe:Co is 19:1,the optimal reflection loss reaches-60 *** high electromagnetic attenuation performance significantly improve the linear sensitivity of the strain response and active customized stealth capability of the designed multifunctional capacitor-like ***,the wireless multifunctional design integrates energy attenuaten of electromagnetic wave with the wireless sensing and active camouflage functions for the first *** work provides an important step for the realization of electromagnetical multifunctional applications including electromag-netic protection and electromagnetic sensing in artificial beings,medical health and even space travel.

关键词： Electromagnetic absorption Polarization relaxation Electromagnetic sensing Active camouflage

A Nano-Micro Engineering Nanofiber for Electromagnetic Absorber,Green Shielding and Sensor

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Nano-Micro Letters 2021年第2期13卷 112-123页

作者： Min Zhang Chen Han wen-qiang cao Mao-Sheng cao Hui-Jing Yang Jie Yuan School of Materials Science and Engineering Beijing Institute of TechnologyBeijing 100081People’s Republic of China Department of Physics Tangshan Normal UniversityTangshan 063000People’s Republic of China School of Information Engineering Minzu University of ChinaBeijing 100081People’s Republic of China

It is extremely unattainable for a material to simultaneously obtain efficient electromagnetic(EM)absorption and green shielding performance,which has not been reported due to the competition between conduction loss and ***,by tailoring the internal structure through nano-micro engineering,a NiCo2O4 nanofiber with integrated EM absorbing and green shielding as well as strain sensing functions is *** the improvement of charge transport capability of the nanofiber,the performance can be converted from EM absorption to shielding,or even ***,as the conductivity rising,the reflection loss declines from −52.72 to −10.5 dB,while the EM interference shielding effectiveness increases to 13.4 dB,suggesting the coexistence of the two EM ***,based on the high EM absorption,a strain sensor is designed through the resonance coupling of the patterned NiCo2O4 *** strategies for tuning EM performance and constructing devices can be extended to other EM functional materials to promote the development of electromagnetic driven devices.

关键词： Electromagnetic absorber Electromagnetic shielding NiCo2O4 nanofiber Sensor

Multidimensional hollow SiO_(2)/C nanofibers modified by magnetic nanocrystals for electromagnetic energy conversion and lithium battery storage

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Nano Research 2024年第8期17卷 7301-7314页

作者： Chen Han Qi Zheng Juncheng Jin Jiajia Zhang wen-qiang cao Kun Xiang Min Zhang Mao-Sheng cao Anhui Provincial Laboratory of Biomimetic Sensor and Detecting Technology College of Materials and Chemical EngineeringWest Anhui UniversityLu’an 237012China School of Materials Science and Engineering Beijing Institute of TechnologyBeijing 100081China Department of Physics Beijing Technology and Business UniversityBeijing 100048China

Multifunctional materials are powerful tools to support the advancement of energy conversion *** with prominent electromagnetic and electrochemical properties can realize the conversion of electromagnetic energy and solve the subsequent storage ***,an electrospinning-thermal reduction method is employed to construct ultrafine nickel nanoparticle modified porous SiO_(2)/C(Ni-SiO_(2)/C)hollow nanofibers as promising materials for applications in both electromagnetic wave absorption(EMA)and lithium-ion ***,when used as an EMA material,the reflection loss(RL)of Ni-SiO_(2)/C can reach−47.8 dB at 15.8 GHz with a matching thickness of 2.2 *** excellent microwave absorption performance can be attributed to the enhanced conduction loss,polarization relaxation,synergistic magnetic loss,and preferred impedance matching,which result from multi-component magnetic/dielectric synergy and the unique interconnected multidimensional hollow ***,the electronic conductivity and electrochemical activity of the samples are significantly enhanced due to the uniform distribution of ultrafine Ni nanoparticles in the amorphous SiO_(2)/C ***,the hierarchical hollow porous structure provides sufficient free space for volume change during lithiation/delithiation ***,the Ni-SiO_(2)/C nanocomposite exhibits a high reversible capacity of 917.6 mAh·g^(−1)at 0.1 A·g^(−1).At a high current density of 2 A·g^(−1),a capacity of 563.9 mAh·g^(−1)can be maintained after 300 *** energy conversion-storage device is designed to store waste electromagnetic energy in the form of useful electrical *** work inspires the development of high-performance bifunctional materials.

关键词： Ni-SiO_(2)/C nanofiber electromagnetic absorption lithium-ion storage electrospinning multidimensional structure

In Situ Atomic Reconstruction Engineering Modulating Graphene-Like MXene-Based Multifunctional Electromagnetic Devices Covering Multi-Spectrum

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Nano-Micro Letters 2024年第9期16卷 247-261页

作者： Ting‑Ting Liu Qi Zheng wen‑qiang cao Yu‑Ze Wang Min Zhang Quan‑Liang Zhao Mao‑Sheng cao School of Materials Science and Engineering Beijing Institute of TechnologyBeijing 100081People’s Republic of China Department of Physics Beijing Technology and Business UniversityBeijing 100048People’s Republic of China School of Mechanical and Materials Engineering North China University of TechnologyBeijing 100144People’s Republic of China

With the diversified development of big data,detection and precision guidance technologies,electromagnetic(EM)functional materials and devices serving multiple spectrums have become a hot *** the multispectral response of materials is a challenging and meaningful scientific *** this study,MXene/TiO_(2)hybrids with tunable conduction loss and polarization relaxation are fabricated by in situ atomic reconstruction *** importantly,MXene/TiO_(2)hybrids exhibit adjustable spectral responses in the GHz,infrared and visible spectrums,and several EM devices are constructed based on *** antenna array provides excellent EM energy harvesting in multiple microwave bands,with|S11|up to−63.2 dB,and can be tuned by the degree of *** ultra-wideband bandpass filter realizes a passband of about 5.4 GHz and effectively suppresses the transmission of EM signals in the *** infrared stealth device has an emissivity of less than 0.2 in the infrared spectrum at wavelengths of 6-14μ*** work can provide new inspiration for the design and development of multifunctional,multi-spectrum EM devices.

关键词： Graphene-like MXene hybrids Multi-spectral response Multi-function antenna Ultra-wideband bandpass filter Electromagnetic device

Optimizing the key parameter to accelerate the recovery of AMOC under a rapid increase of greenhouse gas forcing

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Atmospheric and Oceanic Science Letters 2025年第1期18卷 39-45页

作者： Haolan Ren Fei Zheng Tingwei cao qiang Wang International Center for Climate and Environment Science(ICCES) Institute of Atmospheric PhysicsChinese Academy of SciencesBeijingChina University of Chinese Academy of Sciences BeijingChina College of Oceanography Hohai UniversityNanjingChina CAS Key Laboratory of Ocean Circulation and Waves Institute of OceanologyChinese Academy of Sciences and Pilot National Laboratory for Marine Science and Technology(Qingdao)QingdaoChina

Atlantic Meridional Overturning Circulation(AMOC)plays a central role in long-term climate variations through its heat and freshwater transports,which can collapse under a rapid increase of greenhouse gas forcing in climate *** studies have suggested that the deviation of model parameters is one of the major factors in inducing inaccurate AMOC *** this work,with a low-resolution earth system model,the authors try to explore whether a reasonable adjustment of the key model parameter can help to re-establish the AMOC after its *** a new optimization strategy,the extra freshwater flux(FWF)parameter is determined to be the dominant one affecting the AMOC’s *** traditional ensemble optimal interpolation(EnOI)data assimilation and new machine learning methods are adopted to optimize the FWF parameter in an abrupt 4×CO_(2) forcing experiment to improve the adaptability of model parameters and accelerate the recovery of *** results show that,under an abrupt 4×CO_(2) forcing in millennial simulations,the AMOC will first collapse and then re-establish by the default FWF parameter ***,during the parameter adjustment process,the saltier and colder sea water over the North Atlantic region are the dominant factors in usefully improving the adaptability of the FWF parameter and accelerating the recovery of AMOC,according to their physical relationship with FWF on the interdecadal timescale.

关键词： Recovery of AMOC 4×CO_(2)forcing Key parameter Parameter estimation Data assimilation Machine learning

基于近缘种微卫星引物的栓皮栎SSR标记开发及群体检测

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分子植物育种 2017年第2期15卷 633-639页

作者：石晓蒙温强曹牧郭鑫徐立安南京林业大学南方现代林业协同创新中心南京210037 江西省林业科学院省植物生物技术重点实验室南昌330013

SSR标记是研究栓皮栎在天然资源锐减下群体遗传变异与进化的有效工具。为解决栓皮栎未建立DNA序列库而使得现有SSR标记数量相对不足的问题,本研究通过比较无梗花栎、蒙古栎、夏栎、麻栎、辽东栎5个栎属近缘种的62对微卫星引物在栓皮栎... 详细信息

SSR标记是研究栓皮栎在天然资源锐减下群体遗传变异与进化的有效工具。为解决栓皮栎未建立DNA序列库而使得现有SSR标记数量相对不足的问题,本研究通过比较无梗花栎、蒙古栎、夏栎、麻栎、辽东栎5个栎属近缘种的62对微卫星引物在栓皮栎的扩增通用性,从而进一步获得新的栓皮栎SSR标记。62对SSR引物中有41对在栓皮栎中有稳定的PCR扩增,总的通用性比例占66.1%。其中,仅比较各物种基因组开发SSR引物,夏栎的微卫星引物通用性最高,占80%。随后,采用3个栓皮栎群体138个个体开展引物多态性检测,最终获得17对具有较高多态性SSR引物。各引物检测的等位基因数(Na)为4~14个,平均7.8个;17个位点中有15个为高度多态性位点(PIC>0.5),其中多态位点大于0.8的5对引物来自夏栎(2p24,FIR053)、辽东栎(E11~12)、蒙古栎(DN726,DN717)。本研究可为开展栓皮栎群体遗传学的深入研究提供了更多的SSR标记选择。

关键词：栓皮栎 SSR标记通用性遗传多样性

Deciphering fungal metabolon coupling tandem inverse-electrondemand Diels-Alder reaction and semipinacol rearrangement for the biosynthesis of spiro polycyclic alkaloids

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Science China Chemistry 2025年第01期 288-296页

作者： Shuai Liu wen-qiang Xu Ying-Tong Di Man-Cheng Tang Ding-Kang Chen Ming-Ming cao Yao-wen Chang Hong-Yu Tang Chun-Mao Yuan Jun-Bo Yang Zhi-Li Zuo Han Guo Zi-Fei Xu Ying Zeng Yun-Dong Wu Xiao-Jiang Hao Key Laboratory of Phytochemistry and Natural Medicines (Chinese Academy of Sciences) Kunming Institute of Botany Chinese Academy of Sciences University of Chinese Academy of Sciences Lab of Computational Chemistry and Drug Design State Key Laboratory of Chemical Oncogenomics Peking University Shenzhen Graduate School Shenzhen Bay Laboratory State Key Laboratory of Microbial Metabolism School of Life Sciences & Biotechnology Shanghai Jiao Tong University State Key Laboratory of Functions and Applications of Medicinal Plants Guizhou Medical University Molecular Biology Experimental Center Germplasm Bank of Wild Species in Southwest China Kunming Institute of Botany Chinese Academy of Sciences Yunnan Key Laboratory for Wild Plant Resources Kunming Institute of Botany Chinese Academy of Sciences Research Unit of Chemical Biology of Natural Anti-Virus Products Chinese Academy of Medical Sciences

In the intricate process of natural product biosynthesis, a metabolon can enhance metabolic flux by associating sequential enzymes. A fungal metabolon, comprising of flavin-dependent monooxygenase Spe F and P450 monooxygenase Spe G, is identified in the biosynthesis of spiro polycyclic alkaloids(+)-notoamide B and its diastereomer(+)-versicolamide B. Using notoamide E as a substance, Spe F/Spe G metabolon can control the stereoselectivity of its 2,3-epoxidation, followed by hydrogen atom ion at C-17 to generate reactive epoxide tau-m A with dienyl iminium unit. Subsequently,(+)-notoamide B and(+)-versicolamide B are produced via tandem nonenzymatic inverse-electron-demand Diels-Alder reaction and semipinacol rearrangement. This provides the first example of metabolon in the biosynthesis of spiro-prenylated indole alkaloids.

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一种新型开槽结构减缩微带天线RCS

微波学报 2011年第4期27卷 9-12页

作者：李文强曹祥玉高军姚旭空军工程大学电讯工程学院西安710077

现有开槽技术减缩微带天线RCS是以牺牲辐射性能为代价,文中提出了一种圆形槽与矩形槽相结合的开槽方式,这种方式可以实现RCS的有效减缩。理论分析和仿真、实测结果表明,该方法设计的微带天线在辐射性能没有变化的同时,在4～8GHz频率范... 详细信息

现有开槽技术减缩微带天线RCS是以牺牲辐射性能为代价,文中提出了一种圆形槽与矩形槽相结合的开槽方式,这种方式可以实现RCS的有效减缩。理论分析和仿真、实测结果表明,该方法设计的微带天线在辐射性能没有变化的同时,在4～8GHz频率范围内单站RCS有了较大幅度的减缩,最大减缩量达到了22dBsm。

关键词：微带天线雷达散射截面减缩开槽