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Long‐life lithium batteries enabled by a pseudo‐oversaturated electrolyte

Carbon Energy 2024年第4期6卷 115-127页

作者： Youchun Yu Simeng wang Juyan Zhang weiwei Qian Nana Zhang Guangjie Shao Haiyan Bian Yuwen Liu Lan Zhang Hebei Key Laboratory of Applied Chemistry College of Environmental and Chemical EngineeringYanshan UniversityQinhuangdaoChina Beijing Key Laboratory of Ionic Liquids Clean Process CAS Key Laboratory of Green Process and EngineeringInstitute of Process EngineeringChinese Academy of SciencesBeijingChina Haike Group Research Institute of Innovation&Technology DongyingChina Langfang Green Industrial Technology Center LangfangChina

The specific energy of Li metal batteries(LMBs)can be improved by using high‐voltage cathode materials;however,achieving long‐term stable cycling performance in the corresponding system is particularly challenging for the liquid ***,a novel pseudo‐oversaturated electrolyte(POSE)is prepared by introducing 1,1,2,2‐tetrafluoroethyl‐2,2,3,3‐tetrafluoropropyl ether(TTE)to adjust the coordination structure between diglyme(G2)and lithium bis(trifluoromethanesulfonyl)imide(LiTFSI).Surprisingly,although TTE shows little solubility to LiTFSI,the molar ratio between LiTFSI and G2 in the POSE can be increased to 1:1,which is much higher than that of the saturation state,1:*** and experimental results prove that TTE promotes closer contact of the G2 molecular with Li^(+)in the ***,it also participates in the formation of electrolyte/electrode *** electrolyte shows outstanding compatibility with both the Li metal anode and typical high‐voltage ***||Li symmetric cells show a long life of more than 2000 h at 1 mA cm^(−2),1 mAh cm^(−2).In the meantime,Li||LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2)(NCM811)cell with the POSE shows a high reversible capacity of 134.8 mAh g^(−1 )after 900 cycles at 4.5 V,1 C *** concept of POSE can provide new insight into the Li^(+)solvation structure and in the design of advanced electrolytes for LMBs.

关键词： high voltage lithium metal batteries pseudo‐oversaturated electrolyte solid electrolyte interphases(SEI) solvation structure

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Advances in Liquid Crystal Epoxy:Molecular Structures,Thermal Conductivity,and Promising Applications in Thermal Management

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Energy & Environmental Materials 2024年第4期7卷 315-343页

作者： Wenying Zhou Yun wang Fanrong Kong weiwei Peng Yandong wang Mengxue Yuan Xiaopeng Han Xiangrong Liu Bo Li School of Chemistry and Chemical Engineering Xi'an University of Science &Technology Materials Research Institute The Pennsylvania State University University Park

Traditional heat conductive epoxy composites often fall short in meeting the escalating heat dissipation demands of large-power,high-frequency,and high'voltage insulating packaging applications,due to the challenge of achieving high thermal conductivity (k),desirable dielectric performance,and robust thermomechanical properties simultaneously.

关键词： intrinsically thermal conductive epoxy liquid crystal unit ordered structure phonon transport thermal conductivity

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The role of reactive oxygen species in gastric cancer

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Cancer Biology & Medicine 2024年第9期21卷 740-753页

作者： Yuqi wang Jingli Xu Zhenjie Fu Ruolan Zhang weiwei Zhu Qianyu Zhao Ping wang Can Hu Xiangdong Cheng College of Pharmaceutical Sciences Zhejiang University of TechnologyHangzhou 310014China Department of Gastric Surgery Zhejiang Cancer HospitalHangzhou 310022China Key Laboratory of Prevention Diagnosis and Therapy of Upper Gastrointestinal Cancer of Zhejiang ProvinceHangzhou 310022China Zhejiang Provincial Research Center for Upper Gastrointestinal Tract Cancer Zhejiang Cancer HospitalHangzhou 310022China

Gastric cancer(GC)ranks fifth in cancer incidence and fourth in cancer-related mortality *** oxygen species(ROS)are highly oxidative oxygen-derived products that have crucial roles in cell signaling regulation and maintaining internal *** are closely associated with the occurrence,development,and treatment of *** review summarizes recent findings on the sources of ROS and the bidirectional regulatory effects on GC and discusses various treatment modalities for GC that are related to ROS *** addition,the regulation of ROS by natural small molecule compounds with the highest potential for development and applications in anti-GC research is *** aim of the review is to accelerate the clinical application of modulating ROS levels as a therapeutic strategy for GC.

关键词： Gastric cancer reactive oxygen species ROSantitumor therapy natural products pharmacology

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A Server Placement Algorithm for Reducing Risk and Improving Power Utilization in Data Centers

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Tsinghua Science and Technology 2024年第1期29卷 158-173页

作者： Rui Chen Huikang Huang Xiaoxuan Luo weiwei Lin School of Computer Science and Engineering South China University of TechnologyGuangzhou 510006China Peng Cheng Laboratory Shenzhen 518066China

As the power demand in data centers is increasing,the power capacity of the power supply system has become an essential resource to be *** many data centers use power oversubscription to make full use of the power capacity,there are unavoidable power supply risks associated with ***,how to improve the data center power capacity utilization while ensuring power supply security has become an important *** solve this problem,we first define it and propose a risk evaluation metric called Weighted Power Supply Risk(WPSRisk).Then,a method,named Hybrid Genetic Algorithm with Ant Colony System(HGAACS),is proposed to improve power capacity utilization and reduce power supply risks by optimizing the server placement in the power supply *** uses historical power data of each server to find a better placement solution by population *** possesses not only the remarkable local search ability of Ant Colony System(ACS),but also enhances the global search capability by incorporating genetic operators from Genetic Algorithm(GA).To verify the performance of HGAACS,we experimentally compare it with five other placement *** experimental results show that HGAACS can perform better than other algorithms in both improving power utilization and reducing the riskof powersupply system.

关键词： server placement power utilization power supply risk swarm intelligence algorithm

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Nonstoichiometric In-S group yielding efficient carrier transfer pathway in In_(2)S_(3) photoanode for solar water oxidation

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SusMat 2024年第1期4卷 154-165页

作者： Runyu Chen Linxing Meng Changda wang weiwei Xu Yulong Huang Li Song Liang Li School of Physical Science and Technology Jiangsu Key Laboratory of Thin FilmsCenter for Energy Conversion Materials&PhysicsSoochow UniversitySuzhouJiangsuP.R.China Jiangsu Key Laboratory of Advanced Negative Carbon Technologies Soochow UniversitySuzhouJiangsuP.R.China National Synchrotron Radiation Laboratory CAS Center for Excellence in NanoscienceUniversity of Science and Technology of ChinaHefeiAnhuiP.R.China School of Electronic and Information Engineering Changshu Institute of TechnologyChangshuJiangsuP.R.China

The construction of high-efficiency photoanodes is essential for developing outstanding photoelectrochemical(PEC)water splitting ***,insufficient carrier transport capabilities and sluggish surface water oxidation kinetics limit its *** a solvothermal annealing strategy,we prepared a nonstoichiometric In-S(NS)group on the surface of an In_(2)S_(3) photoanode in situ and unexpectedly formed a type II transfer path of carrier,thereby reducing the interfacial recombination and promoting the bulk *** calculations and comprehensive characterizations demonstrated NS group as an excellent oxygen evolution cocatalyst(OEC)that effectively facilitated carrier transport,lowered the surface overpotential,increased the surface active site,and accelerated the surface oxygen evolution reaction kinetics by precisely altering the rate-determining steps of*to*OH and*O to**** synergistic effects remarkably enhanced the PEC performance,with a high photocurrent density of 5.02 mA cm^(−2)at 1.23 V versus reversible hydrogen electrode and a negative shift in the onset potential by 310 *** work provides a new strategy for the in situ preparation of high-efficiency OECs and provides ideas for constructing excellent carrier transfer and transport channels.

关键词： In_(2)S_(3) photoanode water splitting

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A novel clinical data management platform for acute pancreatitis

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Journal of Zhejiang University-Science B(Biomedicine & Biotechnology) 2024年第8期25卷 711-718页

作者： Shiyin CHEN Cheng ZHANG Zhi’en wang Jian ZHANG Wenqiao YU Yanshuai wang weiwei SI Tingbo LIANG Yun ZHANG Department of Hepatobiliary and Pancreatic Surgery Zhejiang Provincial Key Laboratory of Pancreatic Diseasethe First Affiliated HospitalZhejiang University School of MedicineHangzhou 310003China Department of Rehabilitation Medicine the First Affiliated HospitalZhejiang University School of MedicineHangzhou 310003China Department of Comprehensive Intensive Care Unit the First Affiliated HospitalZhejiang University School of MedicineHangzhou 310003China

This study presents a multi-center clinical data management platform that facilitates unified and structured management of real-world data and serves as an ideal tool to enhance the quality and progress of clinical research related to severe acute pancreatitis(SAP).The use of the platform enables clinical teams to obtain safe,accurate,structurally unified,traceable,sceneclear,and fully functional real-world medical data in the diagnosis,treatment,and research of acute pancreatitis(AP).

关键词： clinical pancreatitis acute

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Microearthquake reveals the lithospheric structure at midocean ridges and oceanic transform faults

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Journal of Oceanology and Limnology 2024年第3期42卷 697-700页

作者： Zhiteng YU Jiabiao LI weiwei DING Key Laboratory of Submarine Geosciences&Second Institute of Oceanography Ministry of Natural ResourcesHangzhou 310012China

Mid-ocean ridge and oceanic transforms are among the most prominent features on the seafloor surface and are crucial for understanding seafloor spreading and plate tectonic dynamics,but the deep structure of the oceanic lithosphere remains poorly *** large number of microearthquakes occurring along ridges and transforms provide valuable information for gaining an indepth view of the underlying detailed seismic structures,contributing to understanding geodynamic processes within the oceanic *** studies have indicated that the maximum depth of microseismicity is controlled by the 600-℃***,this perspective is being challenged due to increasing observations of deep earthquakes that far exceed this suggested isotherm along mid-ocean ridges and oceanic transform *** mechanisms have been proposed to explain these deep events,and we suggest that local geodynamic processes(e.g.,magma supply,mylonite shear zone,longlived faults,hydrothermal vents,etc.)likely play a more important role than previously thought.

关键词： microearthquake mid-ocean ridge oceanic transform fault oceanic lithosphere thermal structure earthquake location

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Near-infrared double-cable conjugated polymers based on alkyl linkers with tunable length for single-component organic solar cells

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Chinese Chemical Letters 2024年第4期35卷 452-456页

作者： Yikun wang Qiaomei Chen Shijie Liang Dongdong Xia Chaowei Zhao Christopher R.McNeill weiwei Li Beijing Advanced Innovation Center for Soft Matter Science and Engineering&State Key Laboratory of Organic-Inorganic Composites Beijing University of Chemical TechnologyBeijing 100029China Institute of Applied Chemistry Jiangxi Academy of SciencesNanchang 330096China Department of Materials Science and Engineering Monash UniversityWellington RoadClaytonVictoria 3800Australia

The photovoltaic properties of double-cable conjugated polymers are significantly influenced by the length of the alkyl linkers that connect donor backbones and acceptor side units. In this study, a series of 2-(3-oxo-2,3-dihydroinden-1-ylidene)malononitrile(IC)-based double-cable polymers with alkyl linkers ranging from C_8H_(16)to C_(16)H_(32)(Px, x = 8, 10, 12, 14, 16) were synthesized for single-component organic solar cells(SCOSCs). Among these, the linker length x = 12(P12) is found to optimize the power conversion efficiencies(PCEs) in SCOSCs. Specifically, PCEs increase from P8 to P12 and then decline from P12to P16. Detailed investigations of optical absorption, charge transport, and morphology provide insights into the underlying factors contributing to these PCE variations. The findings indicate that the exceptional photovoltaic properties observed in P12 can be attributed to three key factors: A delicate balance between enhanced charge separation facilitated by the increased spacer length and reduced crystallinity resulting from longer spacers, higher charge mobilities, and well-balanced hole/electron transport characteristics. This study highlights the critical role of linker length in determining the photovoltaic properties of double-cable conjugated polymer-based SCOSCs and offers valuable guidance for the design of novel double-cable conjugated polymers.

关键词： Single-component organic solar cells Double-cable conjugated polymers Photovoltaic properties Alkyl linkers

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Three-dimensional magnetization reconstruction from electron optical phase images with physical constraints

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Science China(Physics,Mechanics & Astronomy) 2024年第11期67卷 122-132页

作者： Boyao Lyu Shihua Zhao Yibo Zhang weiwei wang Fengshan Zheng Rafal E.Dunin-Borkowski Jiadong Zang Haifeng Du Anhui Province Key Laboratory of Low-Energy Quantum Materials and Devices High Magnetic Field LaboratoryHefei Institutes of Physical ScienceChinese Academy of SciencesHefei 230031China Science Island Branch Graduate School of University of Science and Technology of ChinaHefei 230026China Department of Physics and Astronomy University of New HampshireDurham 03824USA Department of Physics The City College of New YorkNew York 10031USA Physics Program Graduate Center of the City University of New YorkNew York 10016USA Department of Chemistry University of New HampshireDurham 03824USA Institutes of Physical Science and Information Technology Anhui UniversityHefei 230601China Spin-X Institute Center for Electron MicroscopySchool of Physics and OptoelectronicsState Key Laboratory of Luminescent Materials and DevicesGuangdong-Hong Kong-Macao Joint Laboratory of Optoelectronic and Magnetic Functional MaterialsSouth China University of TechnologyGuangzhou 511442China Ernst Ruska-Centre for Microscopy and Spectroscopy with Electrons Forschungszentrum JülichJülich 52425Germany

The ability to characterize three-dimensional(3D)magnetization distributions in nanoscale magnetic materials and devices is essential to fully understand their static and dynamic magnetic *** contrast techniques in the transmission electron microscope(TEM),such as electron holography and electron ptychography,can be used to record two-dimensional(2D)projections of the in-plane magnetic induction of 3D nanoscale *** the 3D magnetic induction can in principle be reconstructed from one or more tilt series of such 2D projections,conventional tomographic reconstruction algorithms do not recover the 3D magnetization within a sample ***,we use simulations to describe the basis of an improved model-based algorithm for the tomographic reconstruction of a 3D magnetization distribution from one or more tilt series of electron optical phase images recorded in the *** algorithm allows a wide range of physical constraints,including a priori information about the sample geometry and magnetic parameters,to be *** also makes use of minimization of the micromagnetic energy in the loss *** demonstrate the reconstruction of the 3D magnetization of a localized magnetic soliton—a hopfion ring—and discuss the influence of noise,choice of magnetic constants,maximum tilt angle and number of tilt axes on the *** algorithm can in principle be adapted for other magnetic contrast imaging techniques in the TEM,as well as for other magnetic characterization techniques,such as those based on X-rays or neutrons.

关键词： three-dimensional magnetization vector field tomography differentiable programming electron holography micromagnetism

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Facile interfacial synthesis of gold micronails with adjustable length and roughness and their superior SERS properties for the detection of p-aminothiophenol Author links open overlay panel

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Particuology 2024年第8期91卷 333-340页

作者： Hang Li Kaisheng Yao Tianhang Liu weiwei Lu School of Chemistry and Chemical Engineering Henan University of Science and TechnozlogyLuoyang471023China School of Physics and Engineering Henan University of Science and TechnologyLuoyang471023China

Au hierarchical architectures with special morphology and structures are strongly desired in varied ***,a simple synthesis method was developed for the one-step preparation of Au micronails(MNs)at the planar liquid-liquid interface under mild *** well-defined Au MNs were grown and constructed at CHCl_(3)-H_(2)O interface at room temperature using aniline in CHCl_(3)as reducing agent and HAuCl_(4)in H_(2)O as precursor and no surfactant or seed is *** intriguing Au MNs with rough surface consist of big heads and thin rods,just like iron nails in ***,through simple changing the reagent concentrations,the length and surface roughness of Au MNs can be adjusted *** effects of a series of factors on the morphology and structure of the products are studied in *** p-aminothiophenol as a molecular probe,the as-obtained Au MNs all exhibit dramatically improved surface enhanced Raman scattering sensitivity and high reproducibility,the enhancement factor and limit of detection of Au MNs are 5.4×10^(5)and 1.0×10^(-10),respectively.

关键词： Au micronails Liquid-liquid interface synthesis Surface enhanced Raman scattering P-aminothiophenol

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