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Ionic liquid derived electrocatalysts for electrochemical water splitting

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Green Energy & Environment 2024年第4期9卷 604-622页

作者： Tianhao Li weihua Hu Chongqing Key Laboratory for Advanced Materials and Technologies of Clean Energy School of Materials and EnergySouthwest UniversityChongqing400715China Yibin Academy of Southwest University University RoadYibinSichuan644005China

Hydrogen production from electrochemical water splitting is a promising strategy to generate green energy,which requires the development of efficient and stable electrocatalysts for the hydrogen evolution reaction and the oxygen evolution reaction(HER and OER).Ionic liquids(ILs)or poly(ionic liquids)(PILs),containing heteroatoms,metal-based anions,and various structures,have been frequently involved as precursors to prepare electrocatalysts for water ***,ILs/PILs possess high conductivity,wide electrochemical windows,and high thermal and chemical stability,which can be directly applied in the electrocatalysis process with high *** this review,we focus on the studies of ILs/PILs-derived electrocatalysts for HER and OER,where ILs/PILs are applied as heteroatom dopants and metal precursors to prepare catalysts or are directly utilized as the *** to those attractive properties,IL/PIL-derived electrocatalysts exhibit excellent performance for electrochemical water *** these accomplishments and developments are systematically summarized and thoughtfully ***,the overall perspectives for the current challenges and future developments of ILs/PILs-derived electrocatalysts are provided.

关键词： Ionic liquid Electrochemical water splitting Hydrogen evolution reaction Oxygen evolution reaction

Red Emitting Phosphor (Y, Gd) Bx Vi - x O4- x :Eu3 + with High Color Purity for Plasma display Panels

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Journal of Rare Earths 2004年第Z2期22卷 107-109页

作者： Lai Huasheng Chen Baojiu Wang Linsheng Xu Wu Wang Xiaojun Xie Yihua Ren Xinguang di weihua JiangXi South Rare Earth High-Tech. Co. Ltd.Ganzhou 341000China Key Laboratory of Excited State Processes Changchun Institute of OpticsFine Mechanics and PhysicsChinese Academy of SciencesChangchun 130033China Key Laboratory of Excited State ProcessesChangchun Institute of OpticsFine Mechanics and PhysicsChinese Academy of SciencesChangchun 130033China JiangXi South Rare Earth High-Tech. Co.Ltd.Ganzhou 341000China Key Laboratory of Excited State ProcessesChangchun Institute of OpticsFine Mechanics and PhysicsChinese Academy of SciencesChangchun 130033China University of Science and Technology of China Hefei 230026China Key Laboratory of Excited State ProcessesChangchun Institute of OpticsFine Mechanics and PhysicsChinese Academy of SciencesChangchun 130033China Key Laboratory of Excited State ProcessesChangchun Institute of OpticsFine Mechanics and PhysicsChinese Academy of SciencesChangchun 130033China Key Laboratory of Excited State ProcessesChangchun Institute of OpticsFine Mechanics and PhysicsChinese Academy of SciencesChangchun 130033China Key Laboratory of Excited State ProcessesChangchun Institute of OpticsFine Mechanics and PhysicsChinese Academy of SciencesChangchun 130033China

(Y, Gd)BxV1- xO4-x :Eu3 + phosphors were prepared by solid state reaction. The red emission color purity of (Y, Gd)Bx V1 - x O4-x :Eu3 + phosphor is much better than that of the recent widely-used commercial red emitting phosphor (Y,Gd)BO3:Eu3+ and its relative emission intensity is 84% of the commercial phosphor (Y, Gd)BO3 :Eu3+. It is expected that (Y, Gd) Bx V1 -x O4: Eu3 + phosphor will be a promising candidate for PDP (plasma display panels) application.

关键词： PDP (Y, Gd)BxVi-xO4-x:Eu3+ phosphor photoluminescence rare earths

Robust Feedback Set Stabilization of Logic Networks with State-Dependent Uncertain Switching and Control Constraints

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Journal of Systems Science & Complexity 2024年第2期37卷 629-646页

作者： DAI Chaoqun GUO Yuqian GUI weihua School of Automation Central South UniversityChangsha 410083China

This study investigates the robust feedback set stabilization of switched logic control networks(SLCNs)with state-dependent uncertain switching and control ***,based on the properties of the semi-tensor product of matrices and the vector representation of logic,an SLCN with state-dependent uncertain switching and control constraints is expressed in algebraic ***,an input transformation and a switching model are constructed to transfer the original SLCN into one with a free control input and arbitrary *** equivalence between the set stabilizability of the original SLCN and that of the resulting SLCN is *** on such equivalence,the authors propose a necessary and sufficient condition for robust feedback set ***,an example is presented to demonstrate the application of the results obtained.

关键词： Input transformation robust control invariant subset robust feedback set stabilizability semi-tensor product state-dependent constraints switched logic control network

Fully distributed dynamic event-triggered formation-containment tracking for multiagent systems with multiple types of disturbances

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Science China(Information Sciences) 2024年第1期67卷 168-186页

作者： weihua LI Huaguang ZHANG Juan ZHANG Rui WANG College of Information Science and Engineering Northeastern University State Key Laboratory of Synthetical Automation for Process Industries Northeastern University

This paper is dedicated to addressing the time-varying output formation-containment tracking(TVOFCT) problem for heterogeneous linear multiagent systems(MASs) with multiple types of disturbances under directed communication *** agents are divided into tracking leaders,formation leaders,and *** the output space,the formation leaders are required to form an expected geometric formation while tracking the tracking leader,and the followers are required to enter the convex hull spanned by formation ***,a disturbance observer is designed to observe the disturbance with deterministic ***,by combining adaptive technology with event-triggered technology,an independent fully distributed dynamic event-triggered(FDDET) compensator is designed to estimate the state of the tracking *** main advantages of this compensator lie in the following three aspects:(1) the adaptive weight does not increase unboundedly;(2) the interval time between events is expanded;(3) the design does not rely on any global *** to the design of this compensator,an independent FDDET convex hull observer is further designed to observe the convex hull spanned by formation ***,based on the designed disturbance observer,compensator,and convex hull observer,the adaptive disturbance rejection control input which can make the MASs achieve TVOFCT is ***,a numerical simulation is provided to clearly verify the validity of the theoretical results.

关键词： formation-containment tracking disturbance rejection multiagent systems fully distributed control dynamic event-triggered control

An Efficient Method to Estimate Admittance of Black-boxed Inverter-based Resources for Varying Operating Points

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CSEE Journal of Power and Energy Systems 2024年第1期10卷 421-426页

作者： weihua Zhou Bin Liu Nabil Mohammed Behrooz Bahrani Department of Electrical and Computer Systems Engineering Monash UniversityMelbourne 3800Australia Energy Centre Commonwealth Scientific and Industrial Research Organisation(CSIRO)Newcastle 2300Australia.He is now with the Network Planning DivisionTransgridSydney 2000Australia

Traditional analytical approaches for stability assessment of inverter-based resources(IBRs),often requiring detailed knowledge of IBR internals,become impractical due to IBRs’proprietary *** measurements,relying on electromagnetic transient simulation or laboratory settings,are not only time-intensive but also operationally inflexible,since various non-linear control loops make IBRs’admittance models operating-point ***,such admittance measurements must be performed repeatedly when operating point *** avoid time-consuming and cumbersome measurements,admittance estimation for arbitrary operating points is highly ***,existing admittance estimation algorithms usually face challenges in versatility,data demands,and *** this challenge,this letter presents a simple and efficient admittance estimation method for blackboxed IBRs,by utilizing a minimal set of seven operating points to solve a homogeneous linear equation *** studies demonstrate this proposed method ensures high accuracy across various types of *** accuracy is satisfying even when non-negligible measurement errors exist.

关键词： Admittance estimation black box inverterbased resource measurement error operating point

Iodine enrichment in the groundwater in South China and its hydrogeochemical control

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Journal of Environmental Sciences 2024年第8期142卷 226-235页

作者： Fengping Zhou Qianting Xu Yuyun Chen weihua Zhang Rongliang Qiu Guangdong Provincial Key Laboratory of Environmental Pollution and Remediation Technology Guangdong Provincial Engineering Research Center for Heavy Metal Contaminated Soil RemediationSchool of Environmental Science and EngineeringSun Yat-sen UniversityGuangzhou 510275China Shenzhen Research Institute Sun Yat-sen UniversityShenzhen 518057China Guangdong Provincial Key Laboratory of Agricultural&Rural Pollution Abatement and Environmental Safety School of Natural Resources and EnvironmentSouth China Agricultural UniversityGuangzhou 510642China Guangdong Laboratory for Lingnan Modern Agriculture Guangzhou 510642China

In North China,iodine-rich groundwater has been extensively studied,but few in South *** study aimed to investigate the characteristics of iodine-rich groundwater in South China and identify potential contamination *** results revealed that the average concentration of iodine in groundwater was 890μg/L,with a maximumconcentration of 6350μg/L,exceeding the permitted levels recommended by the World Health Organization(5–300μg/L).Notably,the enrichment of iodide occurred in acidic conditions(pH=6.6)and a relatively low Eh environment(Eh=198.4 mV).Pearson correlation and cluster analyses suggested that the enrichment of iodide could be attributed to the intensified redox process involving Mn(II),iodine(I_(2)),or iodate(IO_(3)^(−))in the *** strong affinity between Mn(II)and I_(2)/IO_(3)^(−)facilitated their interaction,resulting in the formation and mobilization of I^(−)from the soil to the *** experiments further confirmed that reducing substances(such as sodium sulfides,ascorbic acids,and fulvic acids)in the soil with low dissolved oxygen(DO)levels(dissolution of iodine ***,higher DO content(>3.8 mg/L)promoted the oxidation of I^(−)into I_(2)or IO_(3)^(−),leading to its *** research provides new insights into the characteristics and mechanisms of I^(−)enrichment in groundwater in South China,and emphasizes the significance of the redox reactions involving Mn(II)and I_(2)/IO_(3)^(−),as well as the influence of soil properties in regulating the occurrence and transportation of iodine species within groundwater systems.

关键词： Iodine enrichment Acid environment Groundwater South China Manganese

Multimodal Data-Driven Reinforcement Learning for Operational Decision-Making in Industrial Processes

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IEEE/CAA Journal of Automatica Sinica 2024年第1期11卷 252-254页

作者： Chenliang Liu Yalin Wang Chunhua Yang weihua Gui the School of Automation Central South UniversityChangsha 410083China IEEE

Dear Editor, This letter proposes a multimodal data-driven reinforcement learning-based method for operational decision-making in industrial processes. Due to the frequent fluctuations of feedstock properties and operating conditions in the industrial processes, existing data-driven methods cannot effectively adjust the operational variables. In addition, multimodal data such as images, audio.

关键词： processes modal adjust

Asynchronous Learning-Based Output Feedback Sliding Mode Control for Semi-Markov Jump Systems: A Descriptor Approach

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IEEE/CAA Journal of Automatica Sinica 2024年第6期11卷 1358-1369页

作者： Zheng Wu Yiyun Zhao Fanbiao Li Tao Yang Yang Shi weihua Gui School of Automation Central South UniversityChangsha 410083China Power Electronics Machines and Control GroupThe University of NottinghamNottingham NG72RDUK Department of Mechanical Engineering University of VictoriaVictoria BC V8W 3P6Canada IEEE

This paper presents an asynchronous output-feed-back control strategy of semi-Markovian systems via sliding mode-based learning *** with most literature results that require exact prior knowledge of system state and mode information,an asynchronous output-feedback sliding sur-face is adopted in the case of incompletely available state and non-synchronization *** holonomic dynamics of the sliding mode are characterized by a descriptor system in which the switching surface is regarded as the fast subsystem and the system dynamics are viewed as the slow *** upon the co-occurrence of two subsystems,the sufficient stochastic admissibility criterion of the holonomic dynamics is derived by utilizing the characteristics of cumulative distribution ***,a recursive learning controller is formulated to guarantee the reachability of the sliding manifold and realize the chattering reduction of the asynchronous switching and sliding ***,the proposed theoretical method is substantia-ted through two numerical simulations with the practical contin-uous stirred tank reactor and F-404 aircraft engine model,respectively.

关键词： Asynchronous switching learning-based control output feedback semi-Markovian jump systems sliding mode con-trol(SMC).

A Deep Residual PLS for Data-Driven Quality Prediction Modeling in Industrial Process

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IEEE/CAA Journal of Automatica Sinica 2024年第8期11卷 1777-1785页

作者： Xiaofeng Yuan Weiwei Xu Yalin Wang Chunhua Yang weihua Gui School of Automation Central South UniversityChangsha 410083China She is now with Guangzhou Electromechanical Technician College Guangzhou 510000China

Partial least squares(PLS)model is the most typical data-driven method for quality-related industrial tasks like soft ***,only linear relations are captured between the input and output data in the *** is difficult to obtain the remaining nonlinear information in the residual subspaces,which may deteriorate the prediction performance in complex industrial *** fully utilize data information in PLS residual subspaces,a deep residual PLS(DRPLS)framework is proposed for quality prediction in this *** by deep learning,DRPLS is designed by stacking a number of PLSs successively,in which the input residuals of the previous PLS are used as the layer *** enhance representation,nonlinear function is applied to the input residuals before using them for stacking highlevel *** each PLS,the output parts are just the output residuals from its previous ***,the output prediction is obtained by adding the results of each *** effectiveness of the proposed DRPLS is validated on an industrial hydrocracking process.

关键词： Deep residual partial least squares(DRPLS) nonlinear function quality prediction soft sensor