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Journal of Materials Science & Technology 2024年第3期170卷 122-128页

作者： Songsong Xu Ying Han Jiapeng sun Guoqing Zu Mingkun Jiang weiwei Zhu Xu Ran Key Laboratory of Advanced Structural Materials Ministry of EducationChangchun University of TechnologyChangchun 130012China School of Materials Science and engineering Changchun University of TechnologyChangchun 130012China Provincial Key Laboratory of Advanced Materials Processing and Application for Rail Transit Changchun University of TechnologyChangchun 130012China college of Mechanics and Materials Hohai UniversityNanjing 211100China

Similar to other metallic materials,duplex stainless steel dramatically loses its advantage of high ductility as they are ***,we produce a gradient nanograined dual-phase structure in the 2101 duplex stainless steel,thus facilitating a superior strength-ductility synergy:a yield strength of 1009.5 MPa being two times higher than that of the as-received sample,a total elongation of 23.4%and a uniform elongation of 5.9%.This novel structure is produced through a processing route of ultrasonic severe surface rolling and annealing,which realizes a superposition of gradient nanostructure and lamellar dual-phase structure with austenite and *** the tension deformation of gradi-ent nanograined dual-phase structured duplex stainless steel,a significant accumulation of geometrically necessary dislocations *** dislocations are formed to accommodate the deformation incompat-ibility caused by the layer-by-layer difference in strength and hardness of individual phase domains,as well as the inherent difference in properties between the austenite and ferrite *** results in a stronger hetero-deformation induced strengthening and hardening significantly contributing to superior mechanical *** study provides a new avenue to develop advanced steels with high strength and ductility.

关键词： Gradient structure Duplex stainless steel Synergetic strengthening Strength Ductility

Vanadyl Sulfate Based Hole-Transporting Layer Enables Efficient Organic Solar Cells

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Chinese Journal of Chemistry 2024年第14期42卷 1644-1650页

作者： Mengdi Li Yuqing sun Yang Cheng Chaowei Zhao Jicai Zhang weiwei Li Research Center for Optoelectronic Materials and Devices School of Physical Science and TechnologyGuangxi UniversityNanningGuangxi530004 China Institute of Applied Chemistry Jiangxi Academy of SciencesNanchangJiangxi330096 China Beijing Advanced Innovation Center for Soft Matter Science and engineering&State Key Laboratory of Organic-Inorganic Composites Beijing University of Chemical TechnologyBeijing100029 China

It remains an urgent task to develop alternative hole-transporting layer(HTL)materials beyond commonly used PEDOT:PSS to increase the shelf-life of organic solar cells(OSCs).Inorganic metal oxide type materials,such as NiO_(x),CoO_(x)and VO_(x),with suitable work functions have attracted numerous research attention *** this work,more abundant and easily accessible oxygenated salt,vanadyl sulfate(VOSO_(4))has been demonstrated to be excellent choice as HTL for *** VOSO_(4)-based HTL can be readily processed by spin-coating from the precursor solution with subsequent thermal annealing and UVO *** a consequence,a high power conversion efficiency(PCE)of 18.72%can be achieved for PM8:L8-BO based OSCs with the VOSO_(4)-based *** transmittance,smooth film surface,suitable energy level and high conductivity were revealed to contribute to the high OSC *** importantly,compared to device with PEDOT:PSS,VOSO_(4)-based OSCs exhibit improved stability when stored in the N_(2)filled glove *** being stored for 600 h,VOSO_(4)-based device can retain 89%of its initial ***,VOSO_(4)can be used as general HTL in PM6:BTP-BO-4Cl and PM6:IT-4F based OSCs,yielding high PCEs of 17.87%and 13.85%,respectively.

关键词： Organic solar cells Semiconductors Hole-transporting layers Vanadyl sulfate Power output Efficiency Vanadium Interfacial modification

Multifunctional SnO_(2) QDs/MXene Heterostructures as Laminar Interlayers for Improved Polysulfide Conversion and Lithium Plating Behavior

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Nano-Micro Letters 2024年第11期16卷 156-169页

作者： Shungui Deng weiwei sun Jiawei Tang Mohammad Jafarpour Frank Nüesch Jakob Heier Chuanfang Zhang college of Materials Science and engineering Sichuan UniversityChengdu 610065People’s Republic of China Laboratory for Functional Polymers Swiss Federal Laboratories for Materials Science and Technology(EMPA)Überlandstrasse 1298600 DübendorfSwitzerland Institute of Materials Science and engineering Ecole Polytechnique Fédérale de Lausanne(EPFL)Station 121015 LausanneSwitzerland Key Laboratory of Quantum Materials and Devices of Ministry of Education School of PhysicsSoutheast UniversityNanjing 211189People’s Republic of China SEU‑FEI Nano‑Pico Center Key Laboratory of MEMS of Ministry of EducationSoutheast UniversityNanjing 210096People’s Republic of China

Poor cycling stability in lithium–sulfur(Li–S)batteries necessitates advanced electrode/electrolyte design and innovative interlayer *** catalysis has emerged as a promising approach,leveraging the adsorption and catalytic performance on lithium polysulfides(LiPSs)to inhibit LiPSs shuttling and improve redox *** this study,we report an ultrathin and laminar SnO_(2)@MXene heterostructure interlayer(SnO_(2)@MX),where SnO_(2) quantum dots(QDs)are uniformly distributed across the MXene *** combined structure of SnO_(2) QDs and MXene,along with the creation of numerous active boundary sites with coordination electron environments,plays a critical role in manipulating the catalytic kinetics of sulfur *** Li–S cell with the SnO_(2)@MX-modified separator not only demonstrates superior electrochemical performance compared to cells with a bare separator but also induces homogeneous Li deposition during *** a result,an areal capacity of 7.6 mAh cm^(-2) under a sulfur loading of 7.5 mg cm^(-2) and a high stability over 500 cycles are *** work demonstrates a feasible strategy of utilizing a laminar separator interlayer for advanced Li–S batteries awaiting commercialization and may shed light on the understanding of heterostructure catalysis with enhanced reaction kinetics.

关键词： Lithium-sulfur battery Heterogeneous catalysis Heterostructure Redox kinetics Lithium dendrites

A chromosome-level genome assembly of the miiuy croaker(Miichthys miiuy)using nanopore sequencing and Hi-C

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Aquaculture and Fisheries 2024年第2期9卷 218-225页

作者： Tianjun Xu Ye Li weiwei Zheng Yuena sun Laboratory of Fish Molecular Immunology College of Fisheries and Life ScienceShanghai Ocean UniversityShanghai201306China Laboratory of Marine Biology and Biotechnology Qingdao National Laboratory for Marine Science and TechnologyQingdao266200China Key Laboratory of Exploration and Utilization of Aquatic Genetic Resources(Shanghai Ocean University) Ministry of EducationShanghai201306China National Pathogen Collection Center for Aquatic Animals Shanghai Ocean UniversityShanghai201306China

Miiuy croaker,Miichthys miiuy is an ecologically important teleost species which is widely distributed in southeast coast of *** this study,we present a chromosomal-scale genome assembly of the miiuy croaker which is an important Sciaenidae fish and economical *** adopted Oxford Nanopore and Hi-C sequencing techniques to achieve an assembly with high accuracy and *** investigation of genome characteristic and functional features may provide insights into the study of phylogenetic diversity of miiuy *** study can also be beneficial to improve molecular assisted breeding ***,it can be a great resource to better conduct further study of other sciaenids.

关键词： Miiuy croaker Chromosomal assembly Genome annotation Genome evolution Phylogenetic

Observation of the failure mechanism in Ag_(10)Ge_(15)Te_(75)-based memristor induced by ion transport

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Nano Research 2024年第9期17卷 8431-8437页

作者： Yuwei Xiong Kuibo Yin weiwei sun Jingcang Li Shangyang Shang Lei Xin Qiyun Wu Xiaoran Gong Yidong Xia Litao sun SEU-FEI Nano-Pico Center Key Laboratory of MEMS of Ministry of EducationSoutheast UniversityNanjing 210096China college of engineering and Applied Sciences Nanjing UniversityNanjing 210093China

The solid-electrolyte-based memristors have attracted tremendous attention for the next-generation nonvolatile memory for both logic and neuromorphic ***,they encounter variability performance challenges which originated from the random ionic transport and conductive filaments ***,the electrochemical metallized mechanism associated with ion transport has been ***,the failure mechanism caused by ion transport during cycles is rarely ***,the five stages of failure in the Ag/Ag_(10)Ge_(15)Te_(75)/W memristor are elucidated through ex-situ current-voltage measurements combined with in-situ transmission electron microscopy *** investigation reveals that the migration and enrichment of Ag ions result in the precipitation of Ag_(2)*** formation of Ag_(2)Te hinders the device's ability to maintain its bipolar characteristics and also decreases the resistance value of the high resistance state,thereby reducing the device's switching *** promising results provide important guidance for the future design of structures and the manipulation of ion transport for high-performance memristors.

关键词： Ag10Ge15Te75 in-situ transmission electron microscopy(TEM) failure mechanism

A novel Tb^(3+) and Eu^(3+) co-doped dual-emitting phosphate K_(3)SrBi(P_(2)O_(7))_(2) phosphor for application in FIR thermometers

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Journal of Rare Earths 2024年第3期42卷 455-463,I0001页

作者： Baochen Wang Shifeng sun Zeqi Li Zongwang Li weiwei Lin Chao Zeng Yan-gai Liu Ruiyu Mi School of Chemical and Environmental engineering Anhui Polytechnic UniversityWuhu241000China State-Province Joint engineering Laboratory of Zeolite Membrane Materials Key Lab of Fluorine and Silicon for Energy Materials and Chemistry of Ministry of EducationInstitute of Advanced MaterialsCollege of Chemistry and Chemical EngineeringJiangxi Normal UniversityNanchang330022China Beijing Key Laboratory of Materials Utilization of Nonmetallic Minerals and Solid Wastes National Laboratory of Mineral MaterialsSchool of Materials Science and TechnologyChina University of GeosciencesBeijing100083China

Rare earth co-doped phosphor for fluorescence intensity ratio(FIR) thermometer has gained increasing attention in recent years. Herein, the novel Tb^(3+)and Eu^(3+)co-doped K_(3)SrBi(P_(2)O_(7))_(2)(KSBP) phosphate phosphors were reported. The crystal structure of the title phosphor was determined using Rietveld refinement and proved to have a three-dimensional structure. The time-resolved spectroscopy reveals that there is almost no energy transfer between Tb^(3+)and Eu^(3+). More importantly, Tb^(3+)and Eu^(3+)emissions show different thermal quenching behaviors, which claims the potential of this material for application in optical thermometer. The FIR of the typical KSBP:0.02Tb^(3+),0.04Eu^(3+)sample demonstrates a polynomial relationship as a function of temperature and the absolute and relative sensitivity are0.025 K^(-1) and 0.59%/K, respectively. In general, our study reports a novel and potential KSBP:Tb^(3+),Eu^(3+)phosphate phosphor that is promising for use in high-sensitive FIR thermometers.

关键词： Phosphor Thermometer Fluorescence intensity ratio Thermal stability Rare earths

Modeling Reynolds stress anisotropy invariants via machine learning

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Acta Mechanica Sinica 2024年第6期40卷 50-63页

作者： Xianglin Shan Xuxiang sun Wenbo Cao weiwei Zhang Zhenhua Xia School of Aeronautics Northwestern Polytechnical UniversityXi’an710072China Department of engineering Mechanics Zhejiang UniversityHangzhou310027China

The presentation and modeling of turbulence anisotropy are crucial for studying large-scale turbulence structures and constructing turbulence ***,accurately capturing anisotropic Reynolds stresses often relies on expensive direct numerical simulations(DNS).Recently,a hot topic in data-driven turbulence modeling is how to acquire accurate Reynolds stresses by the Reynolds-averaged Navier-Stokes(RANS)simulation and a limited amount of data from *** existing studies use mean flow characteristics as the input features of machine learning models to predict high-fidelity Reynolds stresses,but these approaches still lack robust generalization *** this paper,a deep neural network(DNN)is employed to build a model,mapping from tensor invariants of RANS mean flow features to the anisotropy invariants of high-fidelity Reynolds *** the aspects of tensor analysis and input-output feature design,we try to enhance the generalization of the model while preserving invariance.A functional framework of Reynolds stress anisotropy invariants is derived *** irreducible invariants are then constructed from a tensor group,serving as alternative input features for ***,we propose a feature selection method based on the Fourier transform of periodic *** results demonstrate that the data-driven model achieves a high level of accuracy in predicting turbulence anisotropy of flows over periodic hills and converging-diverging ***,the well-trained model exhibits strong generalization capabilities concerning various shapes and higher Reynolds *** approach can also provide valuable insights for feature selection and data generation for data-driven turbulence models.

关键词： Reynolds stress Anisotropy invariant Tensor analysis Machine learning

Design and preparation of a crosslinkable,oil-resistant,and bio-based elastomer from fumarate

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Science China Chemistry 2024年第2期67卷 622-631页

作者： Hui Yang Haijun Ji Xinxin Zhou Shihan Yang Liwei Li Chaoying sun weiwei Lei Runguo Wang Liqun Zhang Beijing State Key Laboratory of Organic-Inorganic Composites&Beijing Laboratory of Biomedical Materials Beijing University of Chemical TechnologyBeijing100029China Hubei Key Laboratory of Polymer Materials Faculty of Materials Science and EngineeringHubei UniversityWuhan430062China

Poly(diethyl fumarate-co-methoxyethyl acrylate-co-vinyl chloroacetate)(PDEFMV),a novel bio-based elastomer with a saturated structure,was synthesized via redox emulsion *** glass-transition temperatures of PDEFMV,adjusted through the variation of the diethyl fumarate-to-methoxyethyl acrylate feeding ratio,ranged from-36.1 to-14.8 ℃.The number-average molecular weights of PDEFMV ranged from 384,000 to 46,000 g/*** designing the molecular structure,vinyl chloroacetate was used to provide active sites for subsequent vulcanization and *** active chlorine groups within the PDEFMV chain reacted with the crosslinking agent trithiocyanuric acid under high temperature and pressure to form a nonsulfur crosslinked three-dimensional network *** achieve the desired properties,carbon black(CB,N330) was incorporated to reinforce PDEFMV,leading to the formation of PDEFMV/CB composites.A comprehensive study was conducted on the high-temperature oil resistance of PDEFMV/CB *** immersion in IRM903 oil at temperatures of 150 and 200 ℃ for 72 h,the mass and volume changes in PDEFMV/CB were lower than those observed in commercially available acrylate rubber(AR)/CB,indicating that PDEFMV exhibited superior oil ***,the aging characteristics and mechanisms of oil resistance in the PDEFMV/CB and AR/CB composites were investigated at different temperatures(150,200,and 250 ℃).The results provide insights into the operational temperature ranges suitable for PDEFMV/CB and offer valuable guidance for potential industrial applications.

关键词： diethyl fumarate molecular design bio-based elastomer solvent-free synthetic route high-temperature oil resistance

First wetland mapping at 10-m spatial resolution in South America using multi-source and multi-feature remote sensing data

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Science China Earth Sciences 2024年第10期67卷 3252-3269页

作者： weiwei sun Gang YANG Yuling HUANG Dehua MAO Ke HUANG Lin ZHU Xiangchao MENG Tian FENG Chao CHEN Yong GE Department of Geography and Spatial Information Techniques Ningbo UniversityNingbo 315211China State Key Laboratory of Resources and Environmental Information System Institute of Geographic Sciences&Natural Resources ResearchChinese Academy of SciencesBeijing 100101China Natural Resources and Planning Bureau Shanghai Pudong New DistrictShanghai 200100China Key Laboratory of Wetland Ecology and Environment Northeast Institute of Geography and AgroecologyChinese Academy of SciencesChangchun 130102China Faculty of Electrical engineering and Computer Science Ningbo UniversityNingbo 315211China School of Geography Science and Geomatics engineering Suzhou University of Science and TechnologySuzhou 215009China

Wetland degradation has been accelerating in recent years globally. Accurate information on the geographic distribution and categories of wetlands is essential for their conservation and management. Despite being the world′s fourth largest continent, South America has limited research on wetland mapping, and there is currently no available map that provides comprehensive information on wetland distribution and categories in the region. To address this issue, we used Sentinel-1, Sentinel-2 and SRTM data, developed a sample collection method and a wetland mapping method with a collection of multi-source features such as optical features, polarization features and shape features for South American wetlands. We produced a 10-m resolution wetland map based on the Google Earth Engine(GEE) platform. Our Level-1 wetland cover map accurately captured six wetland sub-categories with an overall accuracy of 96.24% and a kappa coefficient of 0.8649, while our Level-2 water cover map included five sub-categories with an overall accuracy of 97.23% and a kappa coefficient of0.9368. The results show that the total area of existing wetlands in South America is approximately 1,737,000 km~2, which is6.8% of the total land area. Among the ten wetland categories, shallow sea had the largest area(960,527.4 km~2), while aquaculture ponds had the smallest area 1513.6 km~2. Swamp had the second largest area(306,240.1 km~2). Brazil, Argentina,Venezuela, Bolivia, and Colombia were found to have the largest wetland areas, with Brazil and Colombia having the most diverse wetland categories. This product can serve as baseline data for subsequent monitoring, management, and conservation of South American wetlands.

关键词： Wetland mapping Google Earth Engine Sentinel imagery South America

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