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Frontiers of Materials Science 2024年第1期18卷 29-43页

作者： wei Xiao wei yang Shantang Liu Hubei Key Lab of Novel Reactor&Green Chemical Technology School of Chemistry and Environmental EngineeringWuhan Institute of TechnologyWuhan 430073China Hubei Key Laboratory of Wudang Local Chinese Medicine Research Department of ChemistrySchool of Pharmaceutical SciencesHubei University of MedicineShiyan 442000China

Metal-organic frameworks(MOFs)have attracted widespread attention due to their regular structures,multiple material centers,and various *** are always considered as one kind of ideal templates for developing highly sensitive and selective gas *** this study,the advantages of MOFs with the high specific surface area(71.9891 m^(2)·g^(-1))and uniform morphology were fully utilized,and urchin-like SnO_(2) nanowires were obtained by the hydrothermal method followed by the calcination using Sn-MOFs consisting of the ligand of C_(9)H_(6)O_(6)(H_(3)BTC)and Sn/Ce center ions as sacrificial *** unique urchin-like nanowire structure facilitated gas diffusion and adsorption,resulting in superior gas sensitivity.A series of Ce-doped SnO_(2) nanowires with different doping ratios were synthesized,and their gas sensing properties towards formaldehyde were *** resulted Ce-SnO_(2) was revealed to have high sensitivity(201.2 at 250℃),rapid response(4 s),long-term stability,and good repeatability for formaldehyde sensing,and the gas sensing mechanism of Ce-SnO_(2) exposed to formaldehyde was also systematically discussed.

关键词： Ce-SnO_(2) SnO_(2) gas sensor formaldehyde Sn-MOF

Adaptive multi-channel Bayesian graph attention network for IoT transaction security

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Digital Communications and Networks 2024年第3期10卷 631-644页

作者： Zhaowei Liu Dong yang Shenqiang Wang Hang su School of Computer and Control Engineering Yantai UniversityYantai264005China Department of Electronics Information and BioengineeringPolitecnico di MilanoMilan20133Italy

With the rapid advancement of 5G technology,the Internet of Things(IoT)has entered a new phase of appli-cations and is rapidly becoming a significant force in promoting economic *** to the vast amounts of data created by numerous 5G IoT devices,the Ethereum platform has become a tool for the storage and sharing of IoT device data,thanks to its open and tamper-resistant ***,Ethereum account security is necessary for the Internet of Things to grow quickly and improve people's *** modeling Ethereum trans-action records as a transaction network,the account types are well identified by the Ethereum account classifi-cation system established based on Graph Neural Networks(GNNs).This work first investigates the Ethereum transaction ***,experimental metrics reveal that the Ethereum transaction network is neither optimal nor even satisfactory in terms of accurately representing transactions per *** flaw may significantly impede the classification capability of GNNs,which is mostly governed by their *** work proposes an Adaptive Multi-channel Bayesian Graph Attention Network(AMBGAT)for Ethereum account clas-sification to address this *** uses attention to enhance node features,estimate graph topology that conforms to the ground truth,and efficiently extract node features pertinent to downstream *** extensive experiment with actual Ethereum transaction data demonstrates that AMBGAT obtains competitive performance in the classification of Ethereum accounts while accurately estimating the graph topology.

关键词： Internet of things Graph representation learning Node classification Security mechanism

Water–solid contact electrification and catalysis adjusted by surface functional groups

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Nano Research 2024年第4期17卷 3344-3351页

作者： Yusen su Andy Berbille Zhong Lin Wang wei Tang CAS Center for Excellence in Nanoscience Beijing Institute of Nanoenergy and NanosystemsChinese Academy of SciencesBeijing100083China School of Nanoscience and Technology University of Chinese Academy of SciencesBeijing100049China Georgia Institute of Technology AtlantaGA 30332-0245USA

Chemical functional groups on solid surfaces greatly influence contact electrification(CE)at water–solid *** studies of their effects mainly swapped materials or bonded related molecules to a substrate,introducing other factors of *** work aims at unambiguously demonstrating the role of functional groups in water-polymer *** study the contribution of functional groups,by using ion coupled plasma etching to modify a high-density polyethylene(HDPE)film,a polymer with a naturally quasi-null charge transfer ***(HDPE–F)and hydroxyl(HDPE–OH)functional groups are generated and endowed HDPE with charge withdrawing ***–F withdraws 2.5–2.7 times more charges than HDPE–***,the surface charges accumulated generate electrostatic forces,altering the droplets *** phenomenon provides another approach to study CE,helping to evaluate the contribution of electrons to solid–liquid ***,employing HDPE–F to perform contact-electro-catalysis shows its activity is 2.4 times higher than that of commercial fluorinated films.

关键词： contact-electro-catalysis charge transfer solid–liquid interfaces contact electrification

Enhancement of comprehensive properties of Nb-Si based in-situ composites by Ho rare earth doping

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Rare Metals 2024年第9期43卷 4508-4520页

作者： wei wei Qi Wang Rui-Run Chen Chao-Wen Zheng Yan-Qing su National Key Laboratory for Precision Hot Processing of Metals School of Materials Science and EngineeringHarbin Institute of TechnologyHarbin 150001China

This study examines the microstructure,mechanical properties(with a focus on room-temperature toughness),and oxidation resistance of Ho-doped NbDSi based in-situ *** base alloy consists of the coarse primary Nb_(5)Si_(3)phase and the Nb_(5)Si_(3)+Nbss(Nb solid solution)eutectic *** doping influences the solidification *** the Ho doping is higher than0.2 at%,the alloys transform into eutectic *** can be solid-solved in trace amounts in the Nbss ***,most of Ho forms a stable Ho oxide phase,which alleviates oxygen contamination problem to some ***,the interface separation between Ho oxide and other phases reduces the plastic deformation ***,with 0.4 at%Ho doping,the K_(Q)value is18.03 MPa·m^(1/2),which is 31.1%higher than that of the base *** strength of the Ho-doped alloys does not deteriorate with an increase in ***,the large network-like Ho_(2)O_(3)in the 0.8Ho alloy causes a decrease in toughness and *** addition,the Ho oxide phase effectively blocks the inward oxygen *** 0.8 at%Ho doping,the oxidation mass gain per unit area is 10.16 mg·cm^(2),which is 39.7%lower than that of the base alloy.

关键词： Nb-Si based composites Rare earth elements Ho Microstructure Properties

Anion-induced differential assembly and structural transformation of supramolecular coordination cages

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Chinese Chemical Letters 2024年第3期35卷 268-272页

作者： Shao-Ping Zheng Yao-wei Xu Pei-yang su Chen-Hui Liu Yin-Hui Huang Yu-Lin Lu Zhang-Wen wei Zhiwei Jiao Hai-Sen Xu Cheng-Yong su MOE Laboratory of Bioinorganic and Synthetic Chemistry Lehn Institute of Functional MaterialsSchool of ChemistrySun Yat-sen UniversityGuangzhou 510006China Institute of Environmental Research at Greater Bay Area Guangzhou UniversityGuangzhou 510006China State Key Laboratory of Organometallic Chemistry Shanghai Institute of Organic ChemistryChinese Academy of SciencesShanghai 200032China

The intimate host-anion interactions will regulate thermodynamics and kinetics in the self-assembly of cationic cages mimicking biological ***,we report construction and transformation of three Pd(Ⅱ)-based metal-organic cages(MOCs)depending on different *** conversions of the lantern-shaped MOC-34 into either octahedral MOC-35 or tricapped trigonal prism MOC-36 are induced by BF_(4)^(–)or NO_(3)^(–),***-36 is kinetically favored and can undergo quantitative conversion to the thermodynamically preferred MOC-35 upon heating,accelerated by excess BF_(4)^(–)to motivate dissociative dynamics of Pd-vertices and lower activation barrier of cage *** guest encapsulation behaviors of MOC-35 and MOC-36 have also been *** results manifest a significance of host-anion dynamics beyond complementary anion template,shedding light on the understanding of intricate anion recognition in nature.

关键词： supramolecular coordination cage Dynamic host-anion interactions Structural transformation Anion receptor Guest inclusion

A multi-agent collaboration scheme for energy-efficient task scheduling in a 3D UAV-MEC space

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Frontiers of Information Technology & Electronic Engineering 2024年第6期25卷 824-838页

作者： yang LI Ziling wei Jinshu su Baokang ZHAO College of Computer National University of Defense TechnologyChangsha 410073China Academy of Military Sciences Beijing 100091China

Multi-access edge computing(MEC)presents computing services at the edge of networks to address the enormous processing requirements of intelligent *** to the maneuverability of unmanned aerial vehicles(UAVs),they can be used as temporal aerial edge nodes for providing edge services to ground users in ***,MEC environment is usually dynamic and *** is a challenge for multiple UAVs to select appropriate service ***,most of existing works study UAV-MEC with the assumption that the flight heights of UAVs are fixed;i.e.,the flying is considered to occur with reference to a two-dimensional plane,which neglects the importance of the *** this paper,with consideration of the co-channel interference,an optimization problem of energy efficiency is investigated to maximize the number of fulfilled tasks,where multiple UAVs in a threedimensional space collaboratively fulfill the task computation of ground *** the formulated problem,we try to obtain the optimal flight and sub-channel selection strategies for UAVs and schedule strategies for *** on the multi-agent deep deterministic policy gradient(MADDPG)algorithm,we propose a curiosity-driven and twin-networks-structured MADDPG(CTMADDPG)algorithm to solve the formulated *** uses the inner reward to facilitate the state exploration of agents,avoiding convergence at the sub-optimal ***,we adopt the twin critic networks for update stabilization to reduce the probability of Q value *** simulation results show that CTMADDPG is outstanding in maximizing the energy efficiency of the whole system and outperforms the other benchmarks.

关键词： Multi-access edge computing Multi-agent reinforcement learning Unmanned aerial vehicles Task scheduling

Transient Response and Ionic Dynamics in Organic Electrochemical Transistors

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Nano-Micro Letters 2024年第11期16卷 191-223页

作者： Chao Zhao Jintao yang wei Ma State Key Laboratory for Mechanical Behavior of Materials Xi’an Jiaotong UniversityXi′an 710049People’s Republic of China

The rapid development of organic electrochemical transistors(OECTs)has ushered in a new era in organic electronics,distinguishing itself through its application in a variety of domains,from high-speed logic circuits to sensitive biosensors,and neuromorphic devices like artificial synapses and organic electrochemical random-access *** recent strides in enhancing OECT performance,driven by the demand for superior transient response capabilities,a comprehensive understanding of the complex interplay between charge and ion transport,alongside electron–ion interactions,as well as the optimization strategies,remains *** review aims to bridge this gap by providing a systematic overview on the fundamental working principles of OECT transient responses,emphasizing advancements in device physics and optimization *** review the critical aspect of transient ion dynamics in both volatile and non-volatile applications,as well as the impact of materials,morphology,device structure strategies on optimizing transient *** paper not only offers a detailed overview of the current state of the art,but also identifies promising avenues for future research,aiming to drive future performance advancements in diversified applications.

关键词： Organic electrochemical transistors Transient response Ion dynamics Electronic dynamics Volatility and non-volatility

Composite Converter Combined APFC with Switched-capacitor Converter

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CSEE Journal of Power and Energy Systems 2024年第1期10卷 281-291页

作者： Qing Fu Yishan Chen Yixing su yang Hang School of Physics Sun Yat-Sen UniversityGuangzhou 510275China

To reduce switch numbers and voltage stress in semiconductor devices,this paper proposes a novel single-phase converter combined Active Power Factor Correction(APFC)with switched-capacitor *** addition,dynamic voltage regulation and voltage gain are improved by integrating the boost converter and switching capacitor *** interstage bulk capacitor is no longer *** average current control with redistribution of voltage in cells is proposed to obtain voltage lift ability of the switching capacitor cells and maintain a high-power *** study and verify the proposed converter preliminarily,theoretical analysis and simulation are presented in the ***,a 50o W prototype with two different configurations is built for experimental *** proposed converter can reach 95.62%of maximum efficiency,0.99 of power factor,and 3.55%of THD with 600 V output voltage,simultaneously.

关键词： AC-DC converter composite conveter power factor correction switched capacitor

Exploring the potential of constructing a hybrid supercapacitor with FeCoNi-LDH porous material containing oxygen vacancies for high-performance energy storage applications

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Nano Research 2024年第9期17卷 8134-8144页

作者： Jihao su Ling yang Dengbin Yu Shaojun Dong State Key Laboratory of Electroanalytical Chemistry Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China College of Chemistry Jilin UniversityChangchun 130022China University of Science and Technology of China Hefei 230026China

A significant challenge in developing high-performance hybrid supercapacitors(HSCs)is the need to reasonably construct advanced architectures that consist of various components and exhibit superior electrochemical capacitance *** FeCoNi-layered double hydroxide(FeCoNi-LDH)porous material has a specific capacitance of 1960 F·g^(-1)when used as the anode material at 1 A·g^(-1).The FeCoNi-LDH material exhibits nanoplates with a distinct spindle morphology on their *** to the combined action of the three metals and abundant oxygen vacancies,they exhibit unique rate performance and cycle *** electronic structure of LDH and the regulation of oxygen vacancy were confirmed by density functional theory(DFT)*** suggests that the strength of hydroxide can reduce the energy required for oxygen vacancy formation in FeCoNi-LDH nanosheets and enhance ion and charge transfer,as well as electrolyte adsorption on the electrode *** FeCoNi-LDH//activated carbon(AC)HSC has an energy density of 53.2 Wh·kg^(-1)at a power density of 800 W·kg^(-1),surpassing other devices composed of comparable materials during the same *** study made significant advances in the design and synthesis of a ternary LDH porous structure with distinct oxygen vacancies,as well as its potential application in electrochemical energy storage.

关键词： oxygen vacancy FeCoNi-layered double hydroxide(FeCoNi-LDH) theory calculation electrode material hybrid supercapacitor

Overexpression of wild-type HRAS drives non-alcoholic steatohepatitis to hepatocellular carcinoma in mice

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Zoological Research 2024年第3期45卷 551-566页

作者： Chen Ling su-su Liu Yu-Ya Wang Gui-Tao Huo Yan-wei yang Nan Xu Hong Wang Yong Wu Yu-Fa Miao Rui Fu Yu-wei Zhao Chang-Fa Fan College of Life Sciences Northwest UniversityProvincial Key Laboratory of Biotechnology of Shaanxi ProvinceXi’anShaanxi 710069China Division of Animal Model Research Institute for Laboratory Animal ResourcesNational Institutes for Food and Drug Control(NIFDC)Beijing 102629China National Center for Safety Evaluation of Drugs National Institutes for Food and Drug Control(NIFDC)Beijing 100176China Division of HIV/AIDS and Sexually Transmitted Virus Vaccines Institute for Biological Products ControlNational Institutes for Food and Drug Control(NIFDC)Beijing 102629China Division of Laboratory Animal Monitoring Institute for Laboratory Animal ResourcesNational Institutes for Food and Drug Control(NIFDC)Beijing 102629China

Hepatocellular carcinoma(HCC),a prevalent solid carcinoma of significant concern,is an aggressive and often fatal disease with increasing global incidence rates and poor therapeutic *** etiology and pathological progression of non-alcoholic steatohepatitis(NASH)-related HCC is multifactorial and ***,no single animal model can accurately mimic the full NASH-related HCC pathological progression,posing considerable challenges to transition and mechanistic ***,a novel conditional inducible wild-type human HRAS overexpressed mouse model(HRAS-HCC)was established,demonstrating 100%morbidity and mortality within approximately one month under normal dietary and lifestyle *** symptoms of HCC such as ascites,thrombus,internal hemorrhage,jaundice,and lung metastasis were successfully replicated in ***-depth pathological features of NASH-related HCC were demonstrated by pathological staining,biochemical analyses,and typical marker gene *** murine anti-PD-1 and sorafenib treatment effectively prolonged mouse survival,further confirming the accuracy and reliability of the *** on protein-protein interaction(PPI)network and RNA sequencing analyses,we speculated that overexpression of HRAS may initiate the THBS1-COL4A3 axis to induce NASH with severe fibrosis,with subsequent progression to ***,our study successfully duplicated natural sequential progression in a single murine model over a very short period,providing an accurate and reliable preclinical tool for therapeutic evaluations targeting the NASH to HCC continuum.

关键词： HRAS THBS1 HCC driver factor NASH Fibrosis Cirrhosis HCC Treatment evaluation