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Design Strategies for Aqueous Zinc Metal Batteries with High Zinc Utilization: From Metal Anodes to Anode-Free Structures

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Nano-Micro Letters 2024年第4期16卷 305-349页

作者： Xianfu Zhang Long Zhang Xinyuan Jia wen Song Yongchang liu School of Materials Science and Engineering University of Science and Technology Beijing30 College RoadBeijing 100083People’s Republic of China Beijing Advanced Innovation Center for Materials Genome Engineering Institute for Advanced Materials and TechnologyState Key Laboratory for Advanced Metals and MaterialsUniversity of Science and Technology BeijingBeijing 100083People’s Republic of China

Aqueous zinc metal batteries(AZMBs)are promising candidates for next-generation energy storage due to the excellent safety, environmental friendliness, natural abundance, high theoretical specific capacity, and low redox potential of zinc(Zn) metal. However,several issues such as dendrite formation, hydrogen evolution, corrosion, and passivation of Zn metal anodes cause irreversible loss of the active materials. To solve these issues, researchers often use large amounts of excess Zn to ensure a continuous supply of active materials for Zn anodes. This leads to the ultralow utilization of Zn anodes and squanders the high energy density of AZMBs. Herein, the design strategies for AZMBs with high Zn utilization are discussed in depth, from utilizing thinner Zn foils to constructing anode-free structures with theoretical Zn utilization of 100%, which provides comprehensive guidelines for further research. Representative methods for calculating the depth of discharge of Zn anodes with different structures are first summarized. The reasonable modification strategies of Zn foil anodes, current collectors with pre-deposited Zn, and anode-free aqueous Zn metal batteries(AF-AZMBs) to improve Zn utilization are then detailed. In particular, the working mechanism of AF-AZMBs is systematically introduced. Finally, the challenges and perspectives for constructing high-utilization Zn anodes are presented.

关键词： Aqueous zinc metal batteries Zinc anodes High zinc utilization Depth of discharge Anode-free structures

Exploring the Effect of Plasticity on the Phase Imaging of TM-AFM Through Molecular Dynamics Simulations

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Acta Mechanica Solida Sinica 2024年第2期37卷 297-304页

作者： Guolin liu Yu Zeng Yaxin Chen Zheng wei School of Mechanical and Electrical Engineering Beijing University of Chemical TechnologyBeijing100029China

In the tapping-mode atomic force microscope(TM-AFM),the probe tip continuously taps the sample surface,which may cause plastic deformation of the sample and result in energy *** energy dissipation of the probe is closely related to the scanned phase *** quantify the energy dissipation due to plastic indentations of the sample,this study utilized a combination of molecular dynamics(MD)simulations and experiments on single-crystal copper samples,including multiple nano-indentation *** energy dissipation of the probe due to the plastic deformation of the sample was calculated by integrating the hysteresis curve of the indentation depth versus the force applied to the *** simulation results are in good agreement with the experimental *** sets of results have demonstrated that the plastic energy dissipation decreases as the number of indentations increases,and eventually the energy of the probe tends to *** equilibrium energy dissipation is associated with other dissipation ***,it was observed that,after hundreds of taps,the dissipated energy of plastic deformation could be ignored,implying that the scanned image may not reflect the plasticity information of the sample after multiple taps of the probe on the sample surface for scanning.

关键词： Atomic force microscopy Force-distance curves Nano-indentations Plasticity Molecular dynamics

Auto-parametric resonance of a continuous-beam-bridge model under two-point periodic excitation:an experimental investigation and stability analysis

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Earthquake Engineering and Engineering Vibration 2024年第2期23卷 445-454页

作者： Li Yuchun Shen Chao liu wei Li Dong Department of Hydraulic Engineering College of Civil EngineeringTongji UniversityShanghai 200092China

The auto-parametric resonance of a continuous-beam bridge model subjected to a two-point periodic excitation is experimentally and numerically investigated in this *** auto-parametric resonance experiment of the test model is conducted to observe and measure the auto-parametric resonance of a continuous beam under a two-point excitation on *** parametric vibration equation is established for the test model using the finite-element *** auto-parametric resonance stability of the structure is analyzed by using Newmark's method and the energy-growth exponent *** effects of the phase difference of the two-point excitation on the stability boundaries of auto-parametric resonance are studied for the test *** with the experiment,the numerical instability predictions of auto-parametric resonance are consistent with the test phenomena,and the numerical stability boundaries of auto-parametric resonance agree with the experimental *** a continuous beam bridge,when the ratio of multipoint excitation frequency(applied to the columns)to natural frequency of the continuous girder is approximately equal to 2,the continuous beam may undergo a strong auto-parametric *** with the present experiment and analysis,a hypothesis of Volgograd Bridge's serpentine vibration is discussed.

关键词： auto-parametric resonance continuous beam bridge model two-point excitation experimental investigation stability analysis vibration of Volgograd Bridge

Polymer-encapsulated metal complex catalysts:An emerging and efficient platform for electrochemical CO_(2) reduction

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Journal of Materials Science & Technology 2024年第5期172卷 33-50页

作者： Yingshuo liu Shuaishuai Lyu Fuli wen weixuan Nie Shuqing Wang Sinopec Research Institute of Petroleum Processing Co. Ltd.Beijing 100083China School of Engineering Westlake UniversityHangzhou 310024China

Over the past decade,electrocatalytic reduction of CO_(2)has gained substantial ***,hardly any of the previous reviews have focused on the systematic discussion of polymer-molecular catalyst composites as an emerging system for the electrochemical transformation of CO_(2)to value-added *** this review,we first give a brief overview of the general features of solid-state and molecular catalysts,and then advance the discussion to polymer-catalyst composite systems,with particular emphasis on polymer-encapsulated molecular catalysts,where the coordination environment surrounding molecular catalysts can be modified via polymer encapsulation to promote the overall performance of CO_(2)*** elucidation of the possible reaction mechanisms of this emerging electrocat-alytic system along with proposed optimization strategies is also summarized and discussed based on recently published reports,followed by the challenges and prospects of their industrial applications at the end of this *** this review,we hope the audience can gain a comprehensive understanding of the electrocatalytic mechanism of the coordinating polymers and valuable insights into engineering the microenvironment surrounding the metal complexes for potential future research directions.

关键词： Polymer-molecular catalyst composite Polymer encapsulation Coordination environment CO_(2)electrocatalysis Electrocatalytic mechanism

Non-Convex Optimization of Resource Allocation in Fog Computing Using Successive Approximation

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Journal of Systems Science & Complexity 2024年第2期37卷 805-840页

作者： LI Shiyong liu Huan LI wenzhe SUN wei School of Economics and Management Yanshan UniversityQinhuangdao 066000China

Fog computing can deliver low delay and advanced IT services to end users with substantially reduced energy ***,with soaring demands for resource service and the limited capability of fog nodes,how to allocate and manage fog computing resources properly and stably has become the ***,the paper investigates the utility optimization-based resource allocation problem between fog nodes and end users in fog *** authors first introduce four types of utility functions due to the diverse tasks executed by end users and build the resource allocation model aiming at utility ***,for only the elastic tasks,the convex optimization method is applied to obtain the optimal results;for the elastic and inelastic tasks,with the assistance of Jensen’s inequality,the primal non-convex model is approximated to a sequence of equivalent convex optimization problems using successive approximation ***,a two-layer algorithm is proposed that globally converges to an optimal solution of the original ***,numerical simulation results demonstrate its superior performance and *** with other works,the authors emphasize the analysis for non-convex optimization problems and the diversity of tasks in fog computing resource allocation.

关键词： Fog computing non-convex optimization optimal resource allocation successive approximation method utility function

Modulated-ISRJ rejection using online dictionary learning for synthetic aperture radar imagery

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Journal of Systems Engineering and Electronics 2024年第2期35卷 316-329页

作者： wei Shaopeng ZHANG Lei LU Jingyue liu Hongwei College of Oceanography and Space Informatics China University of Petroleum(East China)Qingdao 266580China School of Electronics Engineering Xidian UniversityXi’an 710071China School of Electronics and Communication Engineering Shenzhen Campus of Sun Yat-sen UniversityGuangzhou 518107China School of Computer Science and Technology Xidian UniversityXi’an 710071China

In electromagnetic countermeasures circumstances,synthetic aperture radar(SAR)imagery usually suffers from severe quality degradation from modulated interrupt sampling repeater jamming(MISRJ),which usually owes considerable coherence with the SAR transmission waveform together with periodical modulation *** paper develops an MISRJ suppression algorithm for SAR imagery with online dictionary *** the algorithm,the jamming modulation temporal properties are exploited with extracting and sorting MISRJ slices using fast-time *** dictionary learning is followed to separate real signals from jamming *** the learned representation,time-varying MISRJs are suppressed *** simulated and real-measured SAR data are also used to confirm advantages in suppressing time-varying MISRJs over traditional methods.

关键词： synthetic aperture radar(SAR) modulated interrupt sampling jamming(MISRJ) online dictionary learning

Regulatory Mechanisms for Transcriptional Bursting Revealed by an Event-Based Model

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Research 2024年第3期2023卷 217-231页

作者： Renje Wu Bangyan Zhou wei Wang Feng liu National Laboratory of Solid State Microstructures Department of Physicsand Collaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210093P.R.China Institute for Brain Sciences Nanjing UniversityNanjing 210093P.R.China.

Gene transcription often occurs in discrete bursts, and it can be difficult to deduce the underlying regulatory mechanisms for transcriptional bursting with limited experimental data. Here, we categorize numerous states of single eukaryotic genes and identify 6 essential transcriptional events, each comprising a series of state transitions;transcriptional bursting is characterized as a sequence of 4 events, capable of being organized in various configurations, in addition to the beginning and ending events. By associating transcriptional kinetics with mean durations and recurrence probabilities of the events, we unravel how transcriptional bursting is modulated by various regulators including transcription factors. Through analytical derivation and numerical simulation, this study reveals key state transitions contributing to transcriptional sensitivity and specificity, typical characteristics of burst profiles, global constraints on intrinsic transcriptional noise, major regulatory modes in individual genes and across the genome, and requirements for fast gene induction upon stimulation. It is illustrated how biochemical reactions on different time scales are modulated to separately shape the durations and ordering of the events. Our results suggest that transcriptional patterns are essentially controlled by a shared set of transcriptional events occurring under specific promoter architectures and regulatory modes, the number of which is actually limited.

关键词： kinetics essentially constraints

Recent advances in fabrication and functions of neuromorphic system based on organic field effect transistor

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International Journal of Extreme Manufacturing 2024年第2期6卷 273-295页

作者： Yaqian liu Minrui Lian wei Chen Huipeng Chen School of Physics and Electronic Engineering Zhengzhou University of Light IndustryHenan 450002People’s Republic of China Institute of Optoelectronic Display National&Local United Engineering Lab of Flat Panel Display TechnologyFuzhou UniversityFuzhou 350002People’s Republic of China Joint School of National University of Singapore and Tianjin University International Campus of Tianjin UniversityFuzhou 350207People’s Republic of China Department of Chemistry National University of Singapore3 Science Drive 3Singapore 117543Singapore Department of Physics National University of Singapore3 Science Drive 3Singapore 117543Singapore

The development of various artificial electronics and machines would explosively increase the amount of information and data,which need to be processed via in-situ *** synapse devices can store and process signals in a parallel way,thus improving fault tolerance and decreasing the power consumption of artificial *** organic field effect transistor(OFET)is a promising component for bioinspired neuromorphic systems because it is suitable for large-scale integrated circuits and flexible *** this review,the organic semiconductor materials,structures and fabrication,and different artificial sensory perception systems functions based on neuromorphic OFET devices are ***,a summary and challenges of neuromorphic OFET devices are *** review presents a detailed introduction to the recent progress of neuromorphic OFET devices from semiconductor materials to perception systems,which would serve as a reference for the development of neuromorphic systems in future bioinspired electronics.

关键词： organic field effect transistor neuromorphic systems synaptic transistor sensory perception systems device fabrication

Transient Stability Analysis and Design of VSGs with Different DC-Link Voltage Controllers

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CSEE Journal of Power and Energy Systems 2024年第2期10卷 593-604页

作者： Chao Shen wei Gu Wanxing Sheng Keyan liu School of Electrical Engineering Southeast UniversityNanjingChina Power Distribution Research Department China Electric Power Research InstituteBeijing 100192China

Virtual synchronous control has been widely studied for the advantages of emulating inertia for voltage source converters (VSCs). A constant dc-link voltage is usually assumed in existing literature to estimate transient stability of virtual synchronous generators (VSGs). However, actual power supply in the dc-side of VSGs is limited and different dc-link voltage controllers are needed to achieve power balance between DC side and AC side. Addition of dc-link voltage controller has great influence on transient behavior of VSGs, which has not been investigated by previous research. To fill this gap, this paper gives insights into the effect of dc-link voltage dynamics on transient stability of VSGs. First, two typical kinds of VSGs with dc-link voltage controllers are introduced. Then, mathematical models considering dc-link dynamics are established and the effect of dc-link voltage controllers on transient synchronization stability of VSGs is revealed through equal area criterion (EAC). It is found that dc-link voltage controller would reduce stability margin of VSGs and design-oriented transient stability analysis is carried out quantitively using critical clearing time (CCT). Finally, simulation results are given to validate correctness of theoretical analysis.

关键词： DC-link voltage dynamics equal area criterion(eac) transient synchronization stability virtual synchronous generator(VSG)