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A green cross-linking method for the preparation of renewable threedimensional graphene sponges for efficient adsorption of Congo red dye

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Chinese Journal of Chemical Engineering 2024年第2期66卷 84-93页

作者： Zhuang Liu Bo gao Haoyuan Han Yuling Li Haiyang Fu Donghui wei Key Laboratory for Ecological Metallurgy of Multimetallic Mineral(Ministry of Education) Northeastern UniversityShenyang 110819China

Graphene-based materials possess significant potential for the treatment of dye wastewater due to their exceptional adsorption properties toward stubborn ***,their utilization is hindered by high preparation costs,low yields,environmental pollution during synthesis,and challenges in regenerating the *** study proposes a novel approach to address these limitations by developing nitrogen-doped three-dimensional(3D)polyvinyl alcohol(PVA)crosslinked graphene sponges(N-PGA)using a cross-linking method with ammonium *** method offers a relatively mild,environmentally friendly *** carbonate serves as both a reducing and modifying agent,facilitating the formation of the intrinsic structure of N-PGA and acting as a nitrogen ***,PVA is utilized as the cross-linking *** results demonstrate that N-PGA exhibits a favorable internal 3D hierarchical porous structure and possesses robust mechanical *** measured specific surface area(BET)of N-PGA was as high as406.538 m^(2)·g^(-1),which was favorable for its efficient adsorption of Congo red(CR)dye *** an initial concentration of 50 mg·L^(-1),N-PGA achieved an impressive removal rate of 89.6%and an adsorption capacity of 112 mg·g^(-1)for CR ***,it retained 79%of its initial adsorption capacity after 10 cycles,demonstrating excellent regeneration *** summary,the synthesized N-PGA displays remarkable efficacy in the adsorption of CR dye in wastewater,opening up new possibilities for utilizing 3D porous graphene nanomaterials as efficient adsorbents in wastewater treatment.

关键词： Green chemistry Graphene sponge Adsorbents Adsorption Congo red Regeneration

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Enhancing efficiency and stability of organic solar cells through a simplified four-step synthesis of fully non-fused ring electron acceptor

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Journal of Energy Chemistry 2024年第6期93卷 601-608,I0015页

作者： Chenyang Han Huanhuan gao Yanna Sun Yuanyuan Kan Zhaozhao Bi wei Ma Yani Zhang Juan Antonio Zapien Yingguo Yang Ke gao College of New Energy Xi’an Shiyou UniversityXi’an 710065ShaanxiChina Shandong Provincial Key Laboratory for Science of Material Creation and Energy Conversion Institute of Frontier ChemistrySchool of Chemistry and Chemical EngineeringShandong UniversityQingdao 266237ShandongChina State Key Laboratory for Mechanical Behavior of Materials Xi’an Jiaotong UniversityXi’an 710049ShaanxiChina Department of Materials Science and Engineering City University of Hong KongKowloonHong Kong 99907China School of Microelectronics Fudan UniversityShanghai 200433China

Design and synthesis of superior cost-effective non-fullerene acceptors(NFAs)are still big challenges for facilitating the commercialization of organic solar cells(OSCs),yet to be ***,two medium bandgap fully non-fused ring electron acceptors(NFREAs,medium bandgap,i,e.,1,3-1,8 eV),namely PTR-2Cl and PTR-4Cl are synthesized with only four steps by using intramolecular noncovalent interaction central core,structured alkyl side chain orientation linking units and flanking with different electron-withdrawing end *** them,PTR-4C1 exhibits increased average electrostatic potential(ESP)difference with polymer donor,enhanced crystallinity and compactπ-πstacking compared with the control molecule *** a result,the PTR-4Cl-based OSC achieved an impressive power conversion efficiency(PCE)of 14.72%,with a much higher open-circuit voltage(V_(OC))of 0.953 V and significantly improved fill factor(FF)of 0.758,demonstrating one of the best acceptor material in the top-performing fully NFREA-based OSCs with both high PCE and V_(OC).Notably,PTR-4Cl-based cells maintain a good T_80lifetime of its initial PCE after over 936 h under a continuous thermal annealing treatment and over1300 h T_(80)lifetime without *** work provides a cost-effective design strategy for NFREAs on obtaining high V_(OC),efficient exciton dissociation,and ordered molecular packing and thus high-efficiency and stable OSCs.

关键词： Organic solar cells Fully non-fused ring acceptors End group engineering Morphology regulation High efficiency

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Influence of sintering time on microstructure and properties of hot oscillatory pressing sintered W–Cu refractory alloys

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Tungsten 2024年第2期6卷 323-332页

作者： Zi-Qian Wu wei Zhao Ka gao Shi-Hao Du Qing-Quan Kong De-Jian Sun Yang gao School of Materials Science and Engineering Zhengzhou University of AeronauticsZhengzhou 450015China School of Mechanical Engineering University of Shanghai for Science and TechnologyShanghai 200093China Department of General Medicine Changhai HospitalShanghai 200000China Hubei Key Laboratory of Mechanical Transmission and Manufacturing Engineering Wuhan University of Science and TechnologyWuhan 430081China Sichuan Province Engineering Technology Research Center of Powder Metallurgy Chengdu UniversityChengdu 610106China

W–Cu refractory alloys are widely used in aerospace,aviation,electronics,power,and other fi ***,because of its large melting point diff erence between alloy elements,the conventional powder metallurgy method required a long time of high temperature sintering is very likely to cause low density and abnormal grain size ***,90W-10Cu refractory alloys were successfully prepared by hot oscillatory pressing(HOP)under diff erent sintering time in this *** the infl uence of sintering time on the microstructure,grain size,density,Vickers hardness,room-tensile property,and electrical conductivity of the W–Cu refractory alloy was systematically *** results showed that during the short sintering time(30–90 min),the density,Vickers hardness,tensile strength,and electrical conductivity of the W–Cu refractory alloy increased signifi cantly to 98.7%,163.29 HV 30,507.3 MPa,and 14.2%International Annealed Copper Standard with the sintering time increasing,respectively,while its grain size showed no obvious *** the sintering time further increased to 120 min,the density was basically consistent with the sintering time of 90 ***,the prolonged high temperature sintering resulted in the grain growth of the samples,which caused the deterioration of the Vickers hardness,room-tensile strength,and conductivity properties of the W–Cu refractory *** the same sintering time,the density,Vickers hardness,and electrical conductivity of the HOP sintered W–Cu refractory alloy were signifi cantly higher than those of the HP sintered *** was indicated that high density,fi ne-grain,and excellent properties W–Cu refractory alloys could be prepared by hot oscillatory pressing under appropriate sintering time.

关键词： W–Cu refractory alloy Hot oscillatory pressing Sintering time Microstructure Property

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Stable α-CsPbI3 with extremely red emission for expanding the color gamut

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Science China(Information Sciences) 2024年第5期67卷 311-317页

作者： Yong ZHANG Xin wei Lei gao weijie ZHAO Changjiu SUN Junli wei Mingjian YUAN Zhenhua NI Junpeng LU Hongwei LIU School of Physics and Key Laboratory of MEMS of the Ministry of Education Southeast University Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education) Renewable Energy Conversion and Storage Center (RECAST) College of Chemistry Nankai University Jiangsu Key Lab on Opto-Electronic Technology School of Physics and TechnologyNanjing Normal University

The wider color gamut represents the better reproducibility of the real natural colors. Perovskite materials exhibit promising potential in full-color wide-gamut displays because of the wide tunability and high saturability of their photon emission. However, the full-color wide gamut(>100% Rec.2020) has not been constructed due to the lack of the extreme red primary color(～700 nm). Herein, the widest color gamut is realized, whereinα-CsPbI3 is used to generate the extreme red primary color. An in-situ encapsulation approach is advised to stabilizeα-CsPbI3 at room temperature by means of polyvinylpyrrolidone(PVP).Theα-CsPbI3 encapsulated by PVP(denoted as P-CPI) shows highly saturated(FWHM(full width at half maximum) ～28 nm) and extremely(～697 nm) red emission. The green emission is provided by P-CPBr(CsPbBr3 with PVP) which is also synthesized using the universal in-situ encapsulation approach. With the assistance of a commercial Ga N chip, the RGB gamut is extended to the widest(151% NTSC, 113%Rec.2020).

关键词： all-inorganic perovskite wide color gamut LED display carrier recombination

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Influence of sea-land breeze on the formation and dissipation of severe dense fog and its burst reinforcement in the Yellow Sea coastal area,China

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Science China Earth Sciences 2024年第2期67卷 432-449页

作者： Ya gao Duanyang LIU Shuqi YAN Wenjun ZHOU Hongbin WANG Fan ZU Qin MEI Chuanxiang YI Ye sheng Key Laboratory of Transportation Meteorology of China Meteorological Administration Nanjing210041China Yancheng Meteorological Bureau Yancheng224000China Nanjing Joint Institute for Atmospheric Sciences Nanjing210041China Key Laboratory of Disaster Weather Chinese Academy of Meteorological SciencesBeijing100086China

Based on the global reanalysis data of the National Centers for Environmental Prediction(NCEP)/National Center for Atmospheric Research,the surface meteorological observation data,sounding data and satellite observation data,this paper comprehensively analyzes the evolution process and formation mechanism of a persistent severe dense fog process occurred on February 15–17,2015 in Yancheng,eastern *** the numerical simulation experiment of Weather Research and Forecast(WRF)model,we further analyze the impact of sea-land breeze on the formation and burst reinforcement of *** show that the precipitation caused by the southwesterly airflow in front of the upper-level trough and the low-pressure inverted trough are conducive to the formation of early rain fog,while the nighttime clear radiance under the control of surface cold high and the infiltration of weak cold advection are conducive to the formation and development of later radiation-advection *** WRF model simulates the fog evolution process,which is basically consistent with the actual fog area,and the simulation results are credible to a certain *** simulation results show that the establishment of sea breeze has an advection cooling effect on the near surface layer,which is conducive to the formation and development of the inversion layer on the near surface,providing stable stratification conditions for the formation and burst reinforcement of *** one hand,the strengthening of sea breeze circulation can continuously transport water vapor to the study *** the other,the occurrence of ultra-low level jet is favorable for the accumulation of low-level water *** the same time,the inversion intensity further strengthens,which is in favor of the burst reinforcement and long-term maintenance of fog.

关键词： Radiation-advection fog Sea-land breeze Atmospheric boundary layer Fog burst reinforcement WRF model

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Yinhuang granule alleviates carbon tetrachloride-induced liver fibrosis in mice and its mechanism

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World Journal of Hepatology 2024年第2期16卷 264-278页

作者： Hao Ouyang Hui Miao Zhen Li Duan Wu Si-Cheng gao Yao-Yao Dai Xiao-Di gao Hai-sheng Chai wei-Ye Hu Jun-Feng Zhu Department of Liver Yueyang Hospital of Integrated Traditional Chinese and Western MedicineShanghai University of Traditional Chinese MedicineShanghai 201203China State Key Laboratory of Bioreactor Engineering East China University of Science and TechnologyShanghai 201203China

BACKGROUND Liver fibrosis is a formidable global medical challenge,with no effective clinical treatment currently *** granule(YHG)is a proprietary Chinese medicine comprising Scutellariae Radix and Lonicerae Japonicae *** is frequently used for upper respiratory tract infections,pharyngitis,as well as acute and chronic *** To investigate the potential of YHG in alleviating carbon tetrachloride(CCl4)-induced liver fibrosis in *** To induce a hepatic fibrosis model in mice,this study involved intraperitoneal injections of 2 mL/kg of CCl4 twice a week for 4 ***,liver fibrosis mice in the low dose of YHG(0.4 g/kg)and high dose of YHG(0.8 g/kg)groups were orally administered YHG once a day for 4 *** alanine/aspartate aminotransferase(ALT/AST)activity and liver hydroxyproline content were *** red and Masson's trichrome staining assay were *** polymerase chain reaction,western-blot and enzyme-linked immunosorbent assay were *** glutathione content,superoxide dismutase activity level,reactive oxygen species and protein carbonylation amount were *** The administration of YHG ameliorated hepatocellular injury in CCl4-treated mice,as reflected by decreased serum ALT/AST activity and improved liver histological *** also attenuated liver fibrosis,evident through reduced liver hydroxyproline content,improvements in Sirius red and Masson's trichrome staining,and lowered serum hyaluronic acid ***,YHG hindered the activation of hepatic stellate cells(HSCs)and ameliorated oxidative stress injury and inflammation in liver from CCl4-treated *** prompted the nuclear accumulation of nuclear factor erythroid 2-related factor 2(Nrf2)and upregulated the expression of Nrf2-dependent downstream antioxidant *** addition,YHG promoted mitochondrial biogenesis in liver from CCl4-treated mice,as demonstrated by increased liver adenosine triphosphate content,

关键词： Yinhuang granule Liver fibrosis Hepatic stellate cells Oxidative injury Nuclear factor erythroid 2-related factor 2 Inflammation

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Clinicopathological characteristics and typing of multilocular cystic renal neoplasm of low malignant potential

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World Journal of Clinical Cases 2024年第14期12卷 2332-2341页

作者： Wen-Long gao Gang Li Dong-sheng Zhu Yuan-Jie Niu Department of Urology The Second Hospital of Tianjin Medical UniversityTianjin 300211China Department of Pediatric Surgery The First People’s Hospital of LianyungangLianyungang 222000Jiangsu ProvinceChina

BACKGROUND Up until now,no research has been reported on the association between the cli-nical growth rate of multilocular cystic renal neoplasm of low malignant potential(MCRNLMP)and computed tomography(CT)imaging *** study sought to examine the correlation between them,with the objective of distin-guishing unique features of MCRNLMP from renal cysts and exploring effective management *** To investigate optimal management strategies of *** We retrospectively collected and analyzed data from 1520 patients,comprising 1444 with renal cysts and 76 with MCRNLMP,who underwent renal cyst decom-pression,radical nephrectomy,or nephron-sparing surgery for renal cystic disease between January 2013 and December 2021 at our *** of MC-RNLMP utilized the Bosniak classification for imaging and the 2016 World Health Organization criteria for clinical *** Our meticulous exploration has revealed compelling findings on the occurrence of ***,it comprises 1.48%of all cases involving simple renal cysts,5.26%of those with complex renal cysts,and a noteworthy 12.11%of renal tumors coexisting with renal cysts,indicating a statistically significant difference(P=0.001).Moreover,MCRNLMP constituted a significant 22.37%of the patient po-pulation whose cysts demonstrated a rapid growth rate of≥2.0 cm/year,whereas it only represented 0.66%among those with a growth rate below 2.0 cm/*** the 76 MCRNLMP cases studied,none of the nine patients who underwent subsequent nephron-sparing surgery or radical nephrectomy following renal cyst decompression experienced recurrence or *** the remaining 67 patients,who were actively monitored over a 3-year postoperative period,only one showed suspicious recurrence on CT *** MCRNLMP can be tentatively identified and categorized into three types based on CT scanning and growth rate *** treating MCRNLMP,partial nephrectomy is preferred,while rad

关键词： Renal cysts Multilocular cystic renal neoplasm of low malignant potential Computed tomography Diagnosis Treatment

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Sparse representation scheme with enhanced medium pixel intensity for face recognition

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CAAI Transactions on Intelligence Technology 2024年第1期9卷 116-127页

作者： Xuexue Zhang Yongjun Zhang Zewei Wang wei Long weihao gao Bob Zhang State Key Laboratory of Public Big Data Institute for Artificial IntelligenceCollege of Computer Science and TechnologyGuizhou UniversityGuiyangGuizhouChina Department of Computer and Information Science University of MacaoAvenida da UniversidadeTaipaMacaoChina

Sparse representation is an effective data classification algorithm that depends on the known training samples to categorise the test *** has been widely used in various image classification *** in sparse representation means that only a few of instances selected from all training samples can effectively convey the essential class-specific information of the test sample,which is very important for *** deformable images such as human faces,pixels at the same location of different images of the same subject usually have different ***,extracting features and correctly classifying such deformable objects is very ***,the lighting,attitude and occlusion cause more *** the problems and challenges listed above,a novel image representation and classification algorithm is ***,the authors’algorithm generates virtual samples by a non-linear variation *** method can effectively extract the low-frequency information of space-domain features of the original image,which is very useful for representing deformable *** combination of the original and virtual samples is more beneficial to improve the clas-sification performance and robustness of the ***,the authors’algorithm calculates the expression coefficients of the original and virtual samples separately using the sparse representation principle and obtains the final score by a designed efficient score fusion *** weighting coefficients in the score fusion scheme are set entirely ***,the algorithm classifies the samples based on the final *** experimental results show that our method performs better classification than conventional sparse representation algorithms.

关键词： computer vision face recognition image classification image representation

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Frequency and Reliability Analysis of Load-Bearing Composite Beams

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Automotive Innovation 2024年第1期7卷 194-207页

作者： Junlei wei Lingyu Sun Xinli gao Wenfeng Pan Jiaxin Wang Jinxi Wang School of Transportation Science and Engineering Beihang University37 Xueyuan RoadHaidian DistrictBeijing 100191China Beijing Key Laboratory for High-Efficient Power Transmission and System Control of New Energy Resource Vehicle Beihang University37 Xueyuan RoadHaidian DistrictBeijing 100191China Beijing Hangshu Vehicle Data Research Institute Co. Ltd.Beijing 100062China

The increasing utilization of fiber-reinforced thermoplastics(FRTPs)as a substitute for metal in load-bearing structures poses challenges related to NVH issues arising from frequency variations and reliability concerns stemming from fiber dispersion within the resin *** this study,the steel automobile seat beam serves as a benchmark for *** beams are designed and fabricated using two distinct processes:compression molding and injection ***,their modal frequency and reliability are meticulously *** investigations are conducted to explore the influence of various factors,including the combination of laminates and ribs,as well as the stacking sequence of laminates,on the modal *** findings reveal that the modal frequency and vibration mode are subject to alterations based on the fiber type,beam material,and laminate stacking ***,in comparison to the steel benchmark,the first-order frequency of the FRTP beam in this study experiences a 6.59%increase while simultaneously achieving a weight reduction of 32.42%.To assess reliability,a comprehensive analysis is performed,considering a six-fold standard *** analysis yields the permissible range of fluctuation for material elastic constants,bending performance,and frequency ***,the FRTP beams meet the required reliability *** results provide valuable insights for comprehending the stiffness-dependent response and effectively controlling structural performance when implementing FRTP for weight reduction purposes.

关键词： Automobile Fiber-reinforced thermoplastics Lightweight design Frequency change Reliability analysis

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Full-Scale Isogeometric Topology Optimization of Cellular Structures Based on Kirchhoff-Love Shells

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Computer Modeling in Engineering & Sciences 2024年第6期139卷 2479-2505页

作者： Mingzhe Huang Mi Xiao Liang gao Mian Zhou wei Sha Jinhao Zhang State Key Lab of Intelligent Manufacturing Equipment and Technology Huazhong University of Science and TechnologyWuhan430074China

Cellular thin-shell structures are widely applied in ultralightweight designs due to their high bearing capacity and strength-to-weight *** this paper,a full-scale isogeometric topology optimization(ITO)method based on Kirchhoff-Love shells for designing cellular tshin-shell structures with excellent damage tolerance ability is *** method utilizes high-order continuous nonuniform rational B-splines(NURBS)as basis functions for Kirchhoff-Love shell *** geometric and analysis models of thin shells are unified by isogeometric analysis(IGA)to avoid geometric approximation error and improve computational *** topological configurations of thin-shell structures are described by constructing the effective density field on the *** volume constraints are imposed in the proximity of each control point to obtain bone-like cellular *** facilitate numerical implementation,the p-norm function is used to aggregate local volume constraints into an equivalent global *** numerical examples are provided to demonstrate the effectiveness of the proposed *** simulation and comparative analysis,the results indicate that the cellular thin-shell structures optimized by the proposed method exhibit great load-carrying behavior and high damage robustness.

关键词： Cellular thin-shell structures isogeometric analysis full-scale topology optimization Kirchhoff–Love shells

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