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Boosting oxygen reduction activity and CO_(2) resistance on bismuth ferrite-based perovskite cathode for low-temperature solid oxide fuel cells below 600℃

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Journal of Energy Chemistry 2024年第3期90卷 600-609,I0013页

作者： Juntao Gao Zhiyun Wei Mengke Yuan zhe wang zhe Lü Qiang Li Lingling xu Bo Wei School of Physics Harbin Institute of TechnologyHarbin 150001HeilongjiangChina Key Laboratory of Functional Inorganic Material Chemistry Ministry of EducationSchool of Chemistry and Materials ScienceHeilongjiang UniversityHarbin 150080HeilongjiangChina School of Physics and Electronic Engineering Harbin Normal UniversityHarbin 150025HeilongjiangChina

Developing efficient and stable cathodes for low-temperature solid oxide fuel cells(LT-SOFCs) is of great importance for the practical ***,we propose a series of Sm-modified Bi_(0.7-x)Sm_xSr_(0.3)FeO_(3-δ) perovskites as highly-active catalysts for *** doping can significantly enhance the electrocata lytic activity and chemical stability of *** 600℃,Bi_(0.675)Sm_(0.025)Sr_(0.3)FeO_(3-δ)(BSSF25) cathode has been found to be the optimum composition with a polarization resistance of 0.098 Ω cm^2,which is only around 22.8% of Bi_(0.7)Sr_(0.3)FeO_(3-δ)(BSF).A full cell utilizing BSSF25 displays an exceptional output density of 790 mW cm^(-2),which can operate continuously over100 h without obvious *** remarkable electrochemical performance observed can be attributed to the improved O_(2) transport kinetics,superior surface oxygen adsorption capacity,as well as O_(2)p band centers in close proximity to the Fermi ***,larger average bonding energy(ABE) and the presence of highly acidic Bi,Sm,and Fe ions restrict the adsorption of CO_(2) on the cathode surface,resulting in excellent CO_(2) *** work provides valuable guidance for systematic design of efficient and durable catalysts for LT-SOFCs.

关键词： Low-temperature solid oxide fuel cell Perovskite cathode DFT calculations CO_(2) tolerance

Tunable quantum anomalous Hall effects in ferromagnetic van der Waals heterostructures

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National Science Review 2024年第3期11卷 100-107页

作者： Feng xue Yusheng Hou zhe wang Zhiming xu Ke He Ruqian Wu Yong xu Wenhui Duan Beijing Academy of Quantum Information Sciences State Key Laboratory of Low Dimensional Quantum Physics Department of Physics Tsinghua University Guangdong Provincial Key Laboratory of Magnetoelectric Physics and Devices Center for Neutron Science and Technology School of Physics Sun Yat-sen University State Key Laboratory of Surface Physics Key Laboratory of Computational Physical Sciences and Department of PhysicsFudan University Frontier Science Center for Quantum Information Department of Physics and Astronomy University of California-Irvine Tencent Quantum Laboratory Tencent Technology(Shenzhen)Co.Ltd RIKEN Center for Emergent Matter Science(CEMS) Institute for Advanced Study Tsinghua University

The quantum anomalous Hall effect（QAHE） has unique advantages in topotronic applications, but it is still challenging to realize the QAHE with tunable magnetic and topological properties for building functional devices. Through systematic first-principles calculations, we predict that the in-plane magnetization induced QAHE with Chern numbers C = ±1 and the out-of-plane magnetization induced QAHE with high Chern numbers C = ±3 can be realized in a single material candidate, which is composed of van der Waals（vdW）coupled Bi and MnBi2Te4monolayers. The switching between different phases of QAHE can be controlled in multiple ways, such as applying strain or（weak） magnetic field or twisting the vdW materials. The prediction of an experimentally available material system hosting robust, highly tunable QAHE will stimulate great research interest in the field. Our work opens a new avenue for the realization of tunable QAHE and provides a practical material platform for the development of topological electronics.

关键词： quantum anomalous Hall effect topological quantum phase transition van der Waals heterostructures tunable Chern number high Chern number

Retaining the self-released chalcogenate at reconstructed cobalt sites by self-transformed carbonate regulation for boosted oxygen evolution

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Journal of Energy Chemistry 2024年第10期97卷 46-54页

作者： Jingxuan Zhao zhe xue Qing wang Xiangyang Li Shoujie Liu xu Zhao School of Chemical Engineering and Technology Xi'an Jiaotong University Key Laboratory of Materials Physics Institute of Solid State Physics Hefei Institutes of Physical Science (HFIPS) Chinese Academy of Sciences School of Materials Science and Engineering Anhui University

The in-situ generated oxyanions at electrochemically reconstructed catalysts from metal-based nonoxide compounds have been proven to significantly accelerate oxygen evolution reaction（OER） ***,it remains a challenge to retain these self-released oxyanions at reconstructed catalysts,hindering its utilization as a tool to develop efficient OER ***,we demonstrate a versatile selftransformed carbonate regulation strategy to efficiently retain the self-released chalcogenate at Co oxyhydroxides reconstructed from carbon-incorporated Co selenides under OER *** selftransformed CO32-can induce electron accumulation and narrow d bond at Co sites to facilitate the Co3d-O 2p orbital hybridization between Co sites and SeOx2-for enhanced SeOx2-retention,which can accelerate the rate-limiting step for*OOH formation during *** to CoOOH-SeOx2-with limited SeOx2-residues,CoOOH-CO32-/SeOx2-with elevated SeOx2-retention by CO32-regulation exhibited a 5.6-fold increase in current density and a remarkable lower Tafel slope towards *** strategy paves a rational avenue to design efficient catalysts for electrooxidation reactions through finely regulating self-released oxyanions at reconstructed structures.

关键词： Carbonate regulation Chalcogenate retention Electrochemical reconstruction Orbital hybridization Oxygen evolution reaction

Task-Oriented Semantic Communication with Foundation Models

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China Communications 2024年第7期21卷 65-77页

作者： Chen Mingkai Liu Minghao Zhang zhe xu Zhiping wang Lei Key Laboratory of Broadband Wireless Communication and Sensor Network Technology Ministry of EducationNanjing University of Posts and TelecommunicationsNanjing 210003China School of Ocean Information Engineering Jimei UniversityXiamen 361021China Key Laboratory of Underwater Acoustic Communication and Marine Information Technology(Xiamen University) Ministry EducationXiamen 361005China

In the future development direction of the sixth generation(6G)mobile communication,several communication models are proposed to face the growing challenges of the *** rapid development of artificial intelligence(AI)foundation models provides significant support for efficient and intelligent communication *** this paper,we propose an innovative semantic communication paradigm called task-oriented semantic communication system with foundation ***,we segment the image by using task prompts based on the segment anything model(SAM)and contrastive language-image pretraining(CLIP).Meanwhile,we adopt Bezier curve to enhance the mask to improve the segmentation ***,we have differentiated semantic compression and transmission approaches for segmented ***,we fuse different semantic information based on the conditional diffusion model to generate high-quality images that satisfy the users'specific task ***,the experimental results show that the proposed system compresses the semantic information effectively and improves the robustness of semantic communication.

关键词： diffusion model foundation model joint source-channel coding task-oriented semantic communication

Development of multi-functional anchorage support dynamic-static coupling performance test system and its application

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International Journal of Mining Science and Technology 2024年第3期34卷 339-349页

作者： Qi wang Shuo xu Bei Jiang Chong Zhang zhe Sun Jingxuan Liu Cailin Jiao State Key Laboratory for Tunnel Engineering China University of Mining&Technology-BeijingBeijing 100083China Research Center of Geotechnical and Structural Engineering Shandong UniversityJinan 250061China

In underground engineering with complex conditions,the bolt(cable)anchorage support system is in an environment where static and dynamic stresses coexist,under the action of geological conditions such as high stresses and strong disturbances and construction conditions such as the application of high *** is essential to study the support components performance under dynamic-static coupling *** on this,a multi-functional anchorage support dynamic-static coupling performance test system(MAC system)is developed,which can achieve 7 types of testing functions,including single component performance,anchored net performance,anchored rock performance and so *** bolt and cable mechanical tests are conducted by MAC system under different prestress *** results showed that compared to the non-prestress condition,the impact resistance performance of prestressed bolts(cables)is significantly *** the prestress range of 50–160 k N,the maximum reduction rate of impact energy resisted by different types of bolts is 53.9%–61.5%compared to non-prestress *** the prestress range of 150–300 k N,the impact energy resisted by high-strength cable is reduced by76.8%–84.6%compared to non-prestress *** MAC system achieves dynamic-static coupling performance test,which provide an effective means for the design of anchorage support system.

关键词： Anchorage support system Development of test system Dynamic-static coupling test Combined stress

Beam based alignment using a neural network

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Nuclear Science and Techniques 2024年第4期35卷 108-118页

作者： Guan-Liang wang Ke-Min Chen Si-Wei wang zhe wang Tao He Masahito Hosaka Guang-Yao Feng Wei xu National Synchrotron Radiation Laboratory University of Science and Technology of ChinaHefei 230029China Diamond Light Source Oxfordshire OX110DEUK

Beams typically do not travel through the magnet centers because of errors in storage *** beam deviating from the quadrupole centers is affected by additional dipole fields due to magnetic field ***-based alignment(BBA)is often performed to determine a golden orbit where the beam circulates around the quadrupole center *** storage rings with many quadrupoles,the conventional BBA procedure is time-consuming,particularly in the commissioning phase,because of the necessary iterative *** addition,the conventional BBA method can be affected by strong coupling and the nonlinearity of the storage ring *** this study,a novel method based on a neural network was proposed to determine the golden orbit in a much shorter time with reasonable *** golden orbit can be used directly for operation or adopted as a starting point for conventional *** method was demonstrated in the HLS-II storage ring for the first time through simulations and online *** results of the experiments showed that the golden orbit obtained using this new method was consistent with that obtained using the conventional *** development of this new method and the corresponding experiments are reported in this paper.

关键词： Golden orbit Beam-based alignment Neural network Storage ring

Distributed dynamic task allocation for unmanned aerial vehicle swarm systems:A networked evolutionary game-theoretic approach

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Chinese Journal of Aeronautics 2024年第6期37卷 182-204页

作者： zhe ZHANG Ju JIANG Haiyan xu Wen-An ZHANG College of Automation Engineering Nanjing University of Aeronautics and AstronauticsNanjing 211106China College of Economics and Management Nanjing University of Aeronautics and AstronauticsNanjing 211106China College of Information Engineering Zhejiang University of TechnologyHangzhou 310023China

Task allocation is a key aspect of Unmanned Aerial Vehicle(UAV)swarm collaborative *** an continuous increase of UAVs’scale and the complexity and uncertainty of tasks,existing methods have poor performance in computing efficiency,robustness,and realtime allocation,and there is a lack of theoretical analysis on the convergence and optimality of the *** paper presents a novel intelligent framework for distributed decision-making based on the evolutionary game theory to address task allocation for a UAV swarm system in uncertain scenarios.A task allocation model is designed with the local utility of an individual and the global utility of the ***,the paper analytically derives a potential function in the networked evolutionary potential game and proves that the optimal solution of the task allocation problem is a pure strategy Nash equilibrium of a finite strategy ***,a PayOff-based Time-Variant Log-linear Learning Algorithm(POTVLLA)is proposed,which includes a novel learning strategy based on payoffs for an individual and a time-dependent Boltzmann *** former aims to reduce the system’s computational burden and enhance the individual’s effectiveness,while the latter can ensure that the POTVLLA converges to the optimal Nash equilibrium with a probability of *** simulation results show that the approach is optimal,robust,scalable,and fast adaptable to environmental changes,even in some realistic situations where some UAVs or tasks are likely to be lost and increased,further validating the effectiveness and superiority of the proposed framework and algorithm.

关键词： Task allocation Unmanned Aerial Vehicles(UAV) Game theory Log-linear learning Distributed optimization algorithm

Pig pangenome graph reveals functional features of non‑reference sequences

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Journal of Animal Science and Biotechnology 2024年第3期15卷 956-970页

作者： Jian Miao Xingyu Wei Caiyun Cao Jiabao Sun Yuejin xu zhe Zhang Qishan wang Yuchun Pan zhen wang College of Animal Sciences Zhejiang UniversityHangzhou 310058ZhejiangChina Yazhou Bay Science and Technology City Hainan Institute of Zhejiang UniversityYazhou DistrictBuilding 11Yongyou Industrial ParkSanya 572025HainanChina

Background The reliance on a solitary linear reference genome has imposed a significant constraint on our compre-hensive understanding of genetic variation in *** constraint is particularly pronounced for non-reference sequences(NRSs),which have not been extensively *** In this study,we constructed a pig pangenome graph using 21 pig assemblies and identified 23,831 NRSs with a total length of 105 *** findings revealed that NRSs were more prevalent in breeds exhibiting greater genetic divergence from the reference ***,we observed that NRSs were rarely found within coding sequences,while NRS insertions were enriched in immune-related Gene Ontology ***,our investigation also unveiled a close association between novel genes and the immune capacity of *** observed substantial differences in terms of frequencies of NRSs between Eastern and Western pigs,and the heat-resistant pigs exhibited a substantial number of NRS insertions in an 11.6 Mb interval on chromosome ***,we discovered a 665 bp insertion in the fourth intron of the TNFRSF19 gene that may be associated with the ability of heat tolerance in South-ern Chinese *** Our findings demonstrate the potential of a graph genome approach to reveal important functional features of NRSs in pig populations.

关键词： Heat tolerance Immune ability Non-reference sequences Pig pangenome

Optimal retrofitting scenarios of multi-objective energy-efficient historic building under different national goals integrating energy simulation,reduced order modelling and NSGA-II algorithm

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Building Simulation 2024年第6期17卷 933-954页

作者： Hailu Wei Yuanhao Jiao zhe wang Wei wang Tong Zhang School of Architecture Southeast UniversityNanjingJiangsu Province210096China Key Laboratory of Urban and Architectural Heritage Conservation(Southeast University) Ministry of EducationNanjingChina Department of Civil and Environmental Engineering The Hong Kong University of Science and TechnologyHong KongChina HKUST Shenzhen-Hong Kong Collaborative Innovation Research Institute FutianShenzhenChina

Retrofitting a historic building under different national goals involves multiple objectives,constraints,and numerous potential measures and packages,therefore it is time-consuming and challenging during the early design *** study introduces a systematic retrofitting approach that incorporates standard measures for the building envelope(walls,windows,roof),as well as the heating,cooling,and lighting *** retrofit objectives are delineated based on prevailing Chinese *** retrofit measures function as genes to optimize energy-savings,carbon emissions,and net present value(NPV)by employing a log-additive decomposition approach through energy simulation techniques and NSGA-II,yielding 185,163,and 8 ***,a weighted sum method is proposed to derive optimal solutions across multiple *** framework is applied to a courtyard building in Nanjing,China,and the outcomes of the implementation are scrutinized to ascertain the optimal retrofit package under various *** this retrofit,energy consumption can be diminished by up to 63.62%,resulting in an NPV growth of 151.84%,and maximum rate of 60.48%carbon *** three result values not only indicate that the optimal values are achieved in these three aspects of energy saving,carbon reduction and economy,but also show the possibility of possible equilibrium in this multi-objective optimization *** framework proposed in this study effectively addresses the multi-objective optimization challenge in building renovation by employing a reliable optimization algorithm with a computationally efficient reduced-order *** provides valuable insights and recommendations for optimizing energy retrofit strategies and meeting various performance objectives.

关键词： historic building energy-efficient retrofitting building energy simulation log-additive decomposition approach NSGA-II