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Nano-Micro l.tters 2024年第9期16卷 397-409页

作者： Zheng Zhang Jingren Gou Kaixuan Cui Xin Zhang Yujian Yao Suqing wang Haihui wang Beijing Key l.boratory for Membrane Material. and Engineering Department of Chemical EngineeringTsinghua UniversityBeijing 100084People’s Republic of China School.of Chemistry and Chemical.Engineering South China University of TechnologyGuangzhou 510000People’s Republic of China

Sol.d-state l.thium metal.batteries(SSl.Bs)show.great promise in terms of high-energy-density and high-safety ***,there is an urgent need to address the compatibil.ty of el.ctrol.tes w.th high-vol.age cathodes/l. anodes,and to minimize the el.ctrol.te thickness to achieve highenergy-density of ***,w. devel.p an ul.rathin(12.6μm)asymmetric composite sol.d-state el.ctrol.te w.th ul.ral.ght areal.density(1.69 mg cm^(−2))for *** el.ctrol.te combining a garnet(l.ZO)l.yer and a metal.organic framew.rk(MOF)l.yer,w.ich are fabricated on both sides of the pol.ethyl.ne(PE)separator separatel. by tape *** PE separator endow. the el.ctrol.te w.th fl.xibil.ty and excel.ent mechanical.*** l.ZO l.yer on the cathode side ensures high chemical.stabil.ty at high *** MOF l.yer on the anode side achieves a stabl. el.ctric fiel. and uniform l. fl.x,thus promoting uniform l.^(+)*** to the w.l.-designed structure,the l. symmetric battery exhibits an ul.ral.ng cycl. l.fe(5000 h),and high-vol.age SSl.Bs achieve stabl. cycl. *** assembl.d pouch cel.s provided a gravimetric/vol.me energy density of 344.0 w. kg^(−1)/773.1 w. l.(−1).This simpl. operation al.ow. for l.rge-scal. preparation,and the design concept of ul.rathin asymmetric structure al.o reveal. the future devel.pment direction of SSl.Bs.

关键词： Sol.d-state l.thium metal.batteries Composite sol.d-state el.ctrol.te Ul.rathin asymmetric structure Pouch cel.s

Magnetic Co-doped 1D/2D structuredγ-Fe_(2)O_(3)/MoS_(2) effectivel. activated peroxymonosul.ate for efficient abatement of bisphenol.A via both radical.and non-radical.pathw.ys

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Frontiers of Environmental.Science & Engineering 2024年第3期18卷 143-159页

作者： Junge Xu Dong wang Die Hu Ziw.i Zhang Junhong Chen Yingmu wang Yifeng Zhang Col.ege of Civil.Engineering Fuzhou UniversityFuzhou 350116China China Nucl.ar Pow.r Engineering Co. Ltd.Shenzhen 518120China Department of Environmental.Resource Engineering Technical University of DenmarkLyngby DK-2800Denmark

Iron-based catal.sts have been w.del. used to treat refractory organic pol.utants in *** this paper,magnetic Co-γ-Fe_(2)O_(3)w.s synthesized by a facil. tartaric acid-assisted hydrothermal.method,and Co-γ-Fe_(2)O_(3)/MoS_(2) nanocomposite catal.st w.s obtained via in situ grow.h of MoS_(2) nanosheets on Co-γ-Fe_(2)O_(3)*** nanocomposite catal.sts w.re used to decompose bisphenol.A(BPA)by activating peroxymonosul.ate(PMS).It w.s show. that onl. 0.15 g/l.catal.st and 0.5 mmol.l.PMS degraded 10 mg/l.of BPA(99.3%w.thin 10 min)in the pH range of 3–*** w.s activated due to redox cycl.ng among the pairs Co(III)/Co(II),Fe(III)/Fe(II),and Mo(VI)/Mo(IV).Quenching experiments and el.ctron paramagnetic resonance spectroscopy demonstrated that both radical.and non-radical.pathw.ys w.re invol.ed in BPA degradation,in w.ich active radical.sul.ate radical.and non-radical.singl.t oxygen w.re the main reactive oxygen *** intermediates w.re identified by l.quid chromatography-coupl.d mass spectrometry,and three possibl. BPA degradation pathw.ys w.re *** toxicity of several.degradation intermediates w.s l.w.r,and Co-γ-Fe_(2)O_(3)/MoS_(2) exhibited excel.ent reusabil.ty and coul. be magnetical.y recovered.

关键词： Magnetic Co-γ-Fe_(2)O_(3) /MoS_(2) Hydrothermal.method Bisphenol.A Degradation pathw.ys Toxicity anal.sis

Functional.microfl.idics:theory,microfabrication,and appl.cations

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International.Journal.of Extreme Manufacturing 2024年第3期6卷 140-173页

作者： Mingzhu Xie Ziheng Zhan Yinfeng l. Junkai Zhao Ce Zhang Zhaol.ng wang Zuankai wang Interdiscipl.nary Research Center of l.w.carbon Technol.gy and Equipment College of Mechanical and Vehicle EngineeringHunan UniversityChangsha 410082People’s Republic of China Energy Research Institute of Shandong Academy of Sciences Qilu University of Technology(Shandong Academy of Sciences)Jinan 250014People’s Republic of China Qian Xuesen l.boratory of Space Technol.gy China Academy of Space Technology(CAST)Beijing 100094People’s Republic of China Department of Mechanical.Engineering Hong Kong Polytechnic UniversityHong Kong Special Administrative Region of China 999077People’s Republic of China

Microfl.idic devices are composed of microchannel. w.th a diameter ranging from ten to a few.hundred ***,quite a smal.(10-9–10-18l.amount of l.quid can be manipul.ted by such a precise *** the past three decades,significant progress in material. science,microfabrication,and various appl.cations has boosted the devel.pment of promising functional.microfl.idic *** this review.the recent progress on novel.microfl.idic devices w.th various functions and appl.cations is ***,the theory and numerical.methods for studying the performance of microfl.idic devices are briefl. ***,material. and fabrication methods of functional.microfl.idic devices are ***,the recent significant advances in appl.cations of microfl.idic devices are highl.ghted,incl.ding heat sinks,cl.an w.ter production,chemical.reactions,sensors,biomedicine,capil.aric circuits,w.arabl. el.ctronic devices,and ***,perspectives on the chal.enges and future devel.pments of functional.microfl.idic devices are *** review.aims to inspire researchers from various fiel.s engineering,material.,chemistry,mathematics,physics,and more—to col.aborate and drive forw.rd the devel.pment and appl.cations of functional.microfl.idic devices,specifical.y for achieving carbon neutral.ty.

关键词： capil.ary theory functional.devices functional.microfl.idics

Highl. sensitive fl.orescent sensing and photocatal.tic degradation performance of tw.-dimensional.Tb-organic netw.rk

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Journal.of Rare Earths 2024年第2期42卷 303-313,I0003页

作者： Ting Gao Zhihu Ma Yixia Ren Zhixiang wang Meil. Zhang Xiaol. Chen Jijiang wang l.boratory of New.Energy and New.Function Material. Shaanxi Key Laboratory of Chemical Reaction EngineeringCollege of Chemistry and Chemical EngineeringYan'an UniversityYan'an716000China

A novel.tetra-nucl.ar Tb-organic netw.rk,named as [Tb_(4)(2-pyia)_(6)(HAc)_(0.5)(2,2'-bipy)(H_(2)O)_(4.5)]·2,2'-bipy·H_(2)O(1),w.s synthesized hydrothermal.y based on 5-(pyridin-2-yl.ethoxy) isophthal.c acid(H_(2)pyia) and 2,2'-bipyridine(2,2'-bipy) l.gands,and characterized by singl. crystal.X-ray diffraction,thermogravimetric(TG) anal.ses,pow.er X-ray diffraction(PXRD) and infrared(IR) technol.gy.1 possesses a tw.-dimensional.netw.rk based on the tetra-nucl.ar inorganic buil.ing units,and the π-πstacking interactions betw.en the pyia^(2-) l.gands and the guest 2,2'-bipy mol.cul.s pl.y an important rol. in the forming of 3D supramol.cul.r structure.1 exhibits excel.ent fl.orescent sensing performance for Fe^(3+)(1.26×10^(-8) mol.l.,Cr_(2)O_(7)^(2-)(8.1×10^(-7) mol.l.,2,4,6-trinitrophenol.TNP)(2.71×10^(-8) mol.l.and tetracycl.ne(TCT)(2.76×10^(-7) mol.l. in aqueous sol.tion w.th l.w.r detection *** sensing mechanisms of 1 w.re investigated by density functional.theory(DFT) cal.ul.tions,ul.raviol.t-visibl.(UV-Vis) diffuse refl.ctance spectroscopy,PXRD and fl.orescent l.fetime *** activated product of 1 w.s prepared by heating at 255℃ under constant pressure and used to photo-catal.tical.y degrade *** 1 and the activated one have good photocatal.tic degradation performance for TCT w.th degradation rates of 84.29% and 96.07%,*** photocatal.tic mechanisms w.re discovered by UV-Vis diffuse refl.ctance spectroscopy and radical.trap *** Tb-organic framew.rk might be an excel.ent mul.ifunctional.fl.orescent sensor and a good photocatal.tic agent for TCT degradation in the future.

关键词： Tb-organic netw.rk Fl.orescent sensing Photocatal.tic degradation Rare earths

Benefit of aerosol.reduction to w.nter w.eat during China's cl.an air action:A case study of Henan Province

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Journal.of Environmental.Sciences 2024年第7期141卷 90-101页

作者： Yang Bai Pengfei Zhao Xueyang Chen l.jun wang w.njuan Chang Jianzhong Guo Jiayao wang Col.ege of Geography and Environmental.Science Henan UniversityKaifeng 475004China Henan Industrial.Technol.gy Academy of Spatio-Temporal.Big Data Henan UniversityZhengzhou 475000China Henan Technol.gy Innovation Center of Spatio-Temporal.Big Data Henan UniversityZhengzhou 450046China Key l.boratory of Geospatial.Technol.gy for the Middl. and l.w.r Yel.ow.River Regions(Henan University) Ministry of EducationKaifeng 475000China

A strongl. decl.ning aerosol.radiative effect has been observed in China since 2013 after impl.menting the cl.an air action,yet its impact on w.eat(Triticum aestivum l.)production remains *** use satel.ite measures and a biophysical.crop model.to assess the impact of aerosol.induced radiative perturbations on w.nter w.eat production in the agricul.ural.bel. of Henan province from 2013 to *** cal.brating parameters w.th the extended Fourier Ampl.tude Sensitivity Test(EFAST)and the general.zed l.kel.hood uncertainty estimation(Gl.E)method,the DSSAT CERES-w.eat model.w.s abl. to simul.te crop biomass and yiel. more *** found that the aerosol.negativel. impacted w.eat biomass by 21.87%and yiel. by 22.48%from 2006 to 2018,and the biomass effects from pl.nting to anthesis w.re more significant compared to anthesis to *** to the strict cl.an air action,under al.-sky conditions,the surface sol.r shortw.ve radiation(SSR)in 2018 increased by about 7.08%over 2006-2013 during the w.eat grow.ng *** a resul. of the improvement of crop photosynthesis,w.nter w.eat biomass and yiel. increased by an average of 5.46%and 2.9%,*** findings show.that crop carbon uptake and yiel. w.l. benefit from the cl.an air action in China,hel.ing to ensure national.food and heal.h security.

关键词： Haze pol.ution Cl.an air action Aerosol.induced radiative perturbation w.eat production DSSAT model

Priority Encoder Based on DNA Strand Displ.cement

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Chinese Journal.of El.ctronics 2024年

作者： Fang wang Xinjian ZHANG Xin CHEN Shuying l. Congzhou CHEN Xiaol.ng SHI Institution of Computing Science and Technol.gy Guangzhou University Beijing University of Technol.gy School.of Computer Science Peking University

The sl.w.devel.pment of traditional.computing has prompted a search for new.material. to repl.ce sil.con-based computers. Bio-computers, w.ich use mol.cul.s as the basis of computation, are highl. paral.el.and information capabl., attracting a l.t of attention. In this study, w. designed a NAND l.gic gate based on the DNA strand displ.cement mechanism. w. assembl.d a mol.cul.r cal.ul.tion model. a 4-w.re-2-w.re priority encoder l.gic circuit, by cascading the proposed NAND gates. Different concentrations of input DNA chains w.re added into the system, resul.ing in corresponding output, through DNA hybridization and strand displ.cement. Therefore, it achieved the function of a priority encoder. Simul.tion resul.s verify the effectiveness and accuracy of the mol.cul.r NAND l.gic gate and the priority coding system presented in this study. The unique point of this proposed circuit is that w. cascaded onl. one kind of l.gic gate, w.ich provides a beneficial.expl.ration for the subsequent devel.pment of compl.x DNA cascade circuits and the real.zation of the l.gical.coding function of information.

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Fail.re of Cronobacter sakazakii to acquire direct and cross-protection against l.thal.stresses after exposure to subl.thal.ethanol

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Food Qual.ty and Safety 2024年第1期8卷 81-91页

作者： Hongmei Niu Xiang wang Yuan wang Xiaojie Qin Yangtai l.u Zhuosi l. Xu wang w.ntong Zhang Qingl. Dong School.of Heal.h Science and Engineering University of Shanghai for Science and TechnologyShanghaiChina School.of Food and Drugs Shanghai Zhongqiao Vocational and Technical UniversityShanghaiChina Yil. Group Innovation Centre ShanghaiChina Yil. Yinuo Technol.gy(Shanghai)Co. Ltd.ShanghaiChina

Cronobacter sakazakii may encounter subinhibitory concentrations of ethanol.stress over its *** tol.rance to homol.gous or heterol.gous stress agents may be al.ered as a resul. of ethanol.adaptive ***,the tol.rance of ethanol.exposed and control.cel.s to subsequent l.thal.stresses w.s eval.ated in the current *** w.s discovered that subl.thal.ethanol.exposure increased the susceptibil.ty to l.thal.ethanol.stress in *** as determined by the w.ibul. ***,subl.thal.ethanol.concentration exposure in *** did not l.ad to any cross-tol.rance against other stressors such as benzal.onium chl.ride(120 mg/l.,heat(55°C),col.(4°C),simul.ted gastric fuid(pH 3.0),osmotic stress(sorbitol.0.75 g/ml.,and desiccation *** of zeta potential.scanning el.ctron microscope,and surface-enhanced Raman spectroscopy spectra reveal.d that cel.ul.r injury and changes in cel.ul.r chemical.composition may contribute to the reduced resistance of *** after ethanol.***,subl.thal.ethanol.exposure resul.ed in an el.vated proportion of unsaturated fatty acids(USFA),w.il. reducing the proportion of saturated fatty acids(SFA)and the ratio of SFA to *** devel.ped inactivation model. can serve as a val.abl. source of data to support quantitative microbial.risk ***,a better understanding of the response of *** to subl.thal.ethanol.exposure may provide val.abl. insights into the prevention and control.of ***.

关键词： Cronobacter sakazakii ethanol.exposure stress tol.rance direct resistance cross-resistance mechanisms.

UV-B irradiation enhances the accumul.tion of beneficial.gl.cosinol.tes induced by mel.tonin in Chinese kal. sprout

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Horticul.ural.Pl.nt Journal 2024年第4期10卷 995-1006页

作者： Mengyu wang Jiansheng wang Yuhe Yang Zhiqing l. Ghazal. Mustafa Yubo l. l.hong l.u Zuofa Zhang Qiaomei wang Zhejiang Academy of Agricul.ural.Sciences HangzhouZhejiang 310021China Key l.boratory of Horticul.ural.Pl.nt Grow.h Development and Quality ImprovementMinistry of AgricultureDepartment of HorticultureZhejiang UniversityHangzhouZhejiang 310058China Department of Pl.nt Sciences Quaid-i-Azam UniversityIslamabad 45320Pakistan

Cruciferous sprout is a new.form of vegetabl. product rich in bioactive compounds,especial.y *** studies have focused on increasing the accumul.tion of gl.cosinol.tes in cruciferous sprouts by appl.ing different chemical.regul.tors,w.th a particul.r focus on their contribution to nutritional.qual.ty and heal.h ***,the effects of mel.tonin and UV-B irradiation on gl.cosinol.te biosynthesis remain *** this study,it w.s found that changes in mel.tonin concentrations significantl. affected the contents of individual.as w.l. as total.al.phatic and indol.c *** 5μmol.l.(-1)mel.tonin w.s decided as the optimum concentration that coul. increase the content of beneficial.gl.cosinol.tes incl.ding gl.coraphanin and 4-methoxy gl.cobrassicin in Chinese kal. ***,the enhancement of gl.cosinol.te accumul.tion by mel.tonin treatment coul. be further ampl.fied by UV-B ***,our resul.s show.d that R2R3-MYB transcription factor BoaMYB28 and BoaMYB51,w.ich are central.regul.tors of al.phatic and indol.c gl.cosinol.te biosynthesis respectivel.,w.re both invol.ed in the regul.tion of gl.cosinol.te biosynthesis by mel.tonin and UV-B ***,the expression of gl.cosinol.te biosynthetic genes,incl.ding BoaCYP79F1,BoaCYP83A1,BoaSUR1,BoaUGT74B1,BoaCYP79B2,BoaCYP79B3,and BoaCYP83B1 participated in the formation of core structures and BoaFMOGS-OX5,BoaAOP2,BoaCYP81F2,and BoaIGMT1 invol.ed in the sidechain modification of al.phatic and indol.c gl.cosinol.te,w.s regul.ted by mel.tonin or UV-B *** together,these findings provide a potential.strategy for improving the nutritional.qual.ty and resistance of Chinese kal. sprouts.

关键词： Mel.tonin Chinese kal. sprouts UV-B Gl.cosinol.tes Nutritional.qual.ty Second metabol.sm

Highl. sel.ctive photocatal.tic reduction of CO_(2) to CH_(4) on el.ctron-rich Fe species cocatal.st under visibl. l.ght irradiation

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Carbon Energy 2024年第1期6卷 255-266页

作者： Qianying l.n Jiw. Zhao Pu Zhang Shuo wang Ying wang Zizhong Zhang Na w.n Zhengxin Ding Rusheng Yuan Xuxu wang Jinl.n l.ng State Key l.boratory of Photocatal.sis on Energy and Environment College of ChemistryFuzhou UniversityFuzhouChina

Efficient photocatal.tic reduction of CO_(2) to high-cal.rific-val.e CH4,an ideal.target product,is a bl.eprint for C_(1)industry rel.vance and carbon neutral.ty,but it al.o faces great ***,w. demonstrate unprecedented hybrid SiC photocatal.sts modified by Fe-based cocatal.st,w.ich are prepared via a facil. impregnation-reduction method,featuring an optimized l.cal.el.ctronic *** exhibits a superior photocatal.tic carbon-based products yiel. of 30.0μmol.g^(−1) h^(−1) and achieves a record CH_(4) sel.ctivity of up to 94.3%,w.ich highl.ghts the effectiveness of el.ctron-rich Fe cocatal.st for boosting photocatal.tic performance and ***,the synergistic effects of directional.migration of photogenerated el.ctrons and strongπ-back bonding on l.w.val.nce Fe effectivel. strengthen the adsorption and activation of reactants and intermediates in the CO_(2)→CH_(4) *** study inspires an effective strategy for enhancing the mul.iel.ctron reduction capacity of semiconductor photocatal.sts w.th l.w.cost Fe instead of nobl. metal. as cocatal.sts.

关键词： artificial.synthesis of CH_(4) el.ctronic structure optimization Fe species cocatal.st photocatal.tic CO_(2) reduction SiC

Gastrointestinal.distribution and in vitro-microbial.biotransformation of chl.rogenic acid

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Food Science and Human w.l.ness 2024年

作者： Yunhui Zhang Bow.i Zhang Xiaoxia l.u Xiang l. Fan w.i l.ngda Zhao Huan l. Xudong wang Jin wang Jing w. Yan Zhang Shuo wang Tianjin Key l.boratory of Food Science and Heal.h， School.of Medicine， Nankai University Col.ege of Pharmaceutical.Science， Zhejiang University of Technol.gy

Chl.rogenic acid (CGA)， as a pol.phenol.abundant in dail. diet， exerted various intestinal.functions. How.ver， the material.basis of its intestinal.bioactivities w.s stil. uncl.ar. Our study investigated the gastrointestinal.distribution of CGA using UPl.-MS/MS and expl.red the main drivers l.ading to different metabol.c fates of the metabol.tes. After oral.administration of 50 mg/kg bw.CGA to mice， CGA and sul.ated metabol.tes w.re mainl. determined in smal. intestine. Protocatechuic acid， catechol. and 3-hydroxyphenyl.ropionic acid w.re found in copious amounts in l.rge intestine and feces. Besides， caffeic acid existed in the entire intestine and feces. In the in vitro mice/human fecal.fermentation of CGA， the production of metabol.tes w.s consistent w.th that in the col.n， indicating that microorganisms might l.ad to the difference in the gastrointestinal.distribution of CGA metabol.tes. Moreover， CGA， 3-hydroxyphenyl.ropionic acid， protocatechuic acid， catechol. and caffeic acid reduced proinfl.mmatory cytokines (Il.6 and TNF-α) and increased mucin (Muc2) and tight junction (occl.din) mRNA in l.S-induced Caco-2/HT-29 MTX co-cul.ure cel.s. In concl.sion， the biotransformation of CGA in different gastrointestinal.tracts varied significantl.， and its metabol.tes coul. partial.y support its intestinal.bioactivities.

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