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Two-Dimensional Metallophthalocyanine Nanomaterials for Electrocatalytic Energy Conversion

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Energy & Environmental Materials 2024年第4期7卷 364-385页

作者： Xinqi wang shaohui Sun Jiahao Yao Hao Wan Renzhi Ma Wei Ma School of Chemical Engineering and Zhongyuan Critical Metals Laboratory Zhengzhou University Research Center for Materials Nanoarchitectonics (MANA) National Institute for Materials Science (NIMS)

Crowing energy demand drives the rapid development of clean and reliable energy *** the past years,the exploration of novel materials with considerable efficiency and durability has drawn attention in the area of elec... 详细信息

关键词： conjugated nanostructure electrocatalysis 2D metallophthalocyanines

Chemical Scissors Tailored Nano‑Tellurium with High‑Entropy Morphology for Efficient Foam‑Hydrogel‑Based Solar Photothermal Evaporators

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Nano-Micro Letters 2024年第3期16卷 149-168页

作者： Chenyang Xing Zihao Li Ziao wang shaohui Zhang Zhongjian Xie Xi Zhu Zhengchun Peng State Key Laboratory of Radio FrequencyHeterogeneous Integration Shenzhen UniversityShenzhen 518060People’s Republic of China Center for Stretchable Electronics and NanoSensors College of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhen 518060People’s Republic of China School of Science and Engineering The Chinese University of Hong KongShenzhenShenzhen 518172People’s Republic of China Institute of Pediatrics Shenzhen Children’s HospitalShenzhen 518038GuangdongPeople’s Republic of China International Collaborative Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of Education Institute of Microscale OptoelectronicsShenzhen UniversityShenzhen 518060People’s Republic of China

The development of tellurium(Te)-based semiconductor nanomaterials for efficient light-to-heat conversion may offer an effective means of harvesting sunlight to address global energy ***,the nanosized Te(nano-Te)materials reported to date suffer from a series of drawbacks,including limited light absorption and a lack of surface ***,we report the preparation of nano-Te by electrochemical exfoliation using an electrolyzable room-temperature ionic ***,cations,and their corresponding electrolytic products acting as chemical scissors can precisely intercalate and functionalize bulk *** resulting nano-Te has high morphological entropy,rich surface functional groups,and broad light *** also constructed foam hydrogels based on poly(vinyl alcohol)/nano-Te,which achieved an evaporation rate and energy efficiency of 4.11 kg m^(−2)h^(−1)and 128%,respectively,under 1 sun ***,the evaporation rate was maintained in the range 2.5-3.0 kg m^(−2)h^(−1)outdoors under 0.5-1.0 sun,providing highly efficient evaporation under low light conditions.

关键词： Tellurium High entropy Electrochemical modification Solar absorption Evaporation rate

Experimental study on the influences of cutter geometry and material on scraper wear during shield TBM tunnelling in abrasive sandy ground

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第2期16卷 410-425页

作者： shaohui Tang Xiaoping Zhang Quansheng Liu Qi Zhang Xinfang Li Haojie wang Key Laboratory of Safety for Geotechnical and Structural Engineering of Hubei Province School of Civil EngineeringWuhan UniversityWuhan430072China State Key Laboratory of Water Resources and Hydropower Engineering Science Wuhan UniversityWuhan430072China

When shield TBM tunnelling in abrasive sandy ground,the rational design of cutter parameters is critical to reduce tool wear and improve tunnelling ***,the influence mechanism of cutter parameters on scraper wear remains unclear due to the lack of a reliable test *** and material optimisation are often based on subjective experience,which is unfavourable for improving scraper geological *** the present study,the newly developed WHU-SAT soil abrasion test was used to evaluate the variation in scraper wear with cutter geometry,material and *** influence mechanism of cutter parameters on scraper wear has been revealed according to the scratch characteristics of the scraper *** geometry and material parameters have been optimised to reduce scraper *** results indicate that the variation in scraper wear with cutter geometry is related to the cutting resistance,frictional resistance and stress *** appropriate increase in the front angle(or back angle)reduces the cutting resistance(or frictional resistance),while an excessive increase in the front angle(or back angle)reduces the edge angle and causes stress *** optimal front angle,back angle and edge angle for quartz sand samples areα=25°,β=10°andγ=55°,*** wear resistance of the modelled scrapers made of different metal materials is related to the chemical elements and *** wear resistances of the modelled scrapers made of 45#,06Cr19Ni10,42CrMo4 and 40CrNiMoA are 0.569,0.661,0.691 and 0.728 times those made of WC-Co,*** the alloy hardness is less than 47 HRC(or greater than 58 HRC),scraper wear decreases slowly with increasing alloy hardness as the scratch depth of the particle asperity on the metal surface stabilizes at a high(or low)***,when the alloy hardness is between 47 HRC and 58 HRC,scraper wear decreases rapidly with increasing alloy hardness as the scratch depth transitions

关键词： Shield TBM Scraper wear Cutter shape Metal material Alloy hardness

Candidate genes conferring ethylene-response in cultivated peanuts determined by BSA-seq and fine-mapping

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The Crop Journal 2024年第3期12卷 856-865页

作者： Yanyan Tang Zhong Huang shaohui Xu Wenjie Zhou Jianjun Ren Fuxin Yu Jingshan wang Wujun Ma Lixian Qiao College of Agronomy Qingdao Agricultural UniversityQingdao 266109ShandongChina Murdoch University Food Futures InstitutePerthWA 6150Australia The Characteristic Laboratory of Crop Germplasm Innovation and Application Provincial Department of EducationCollege of AgronomyQingdao Agricultural UniversityQingdao 266109ShandongChina Academy of Dongying Efficient Agricultural Technology and Industry on Saline and Alkaline Land in Collaboration with Qingdao Agricultural University Dongying 257347ShandongChina

Ethylene plays essential roles in plant growth,development and stress *** ethylene signaling pathway and molecular mechanism have been studied extensively in Arabidopsis and rice but limited in ***,we established a sand-culture method to screen pingyangmycin mutagenized peanut lines based on their specific response to ethylene(“triple response”).An ethylene-insensitive mutant,inhibition of peanut hypocotyl elongation 1(iph1),was identified that showed reduced sensitivity to ethylene in both hypocotyl elongation and root *** bulked segregant analysis sequencing,a major gene related to iph1,named AhIPH1,was preliminarily mapped at the chromosome Arahy.01,and further narrowed to a 450-kb genomic region through substitution mapping strategy.A total of 7014 genes were differentially expressed among the ACC treatment through RNA-seq analysis,of which only the Arahy.5BLU0Q gene in the candidate mapping interval was differentially expressed between WT and mutant *** sequence variations,functional annotation and transcriptome analysis revealed that a predicated gene,Arahy.5BLU0Q,encoding SNF1 protein kinase,may be the candidate gene for *** gene contained two single-nucleotide polymorphisms at promoter region and was more highly expressed in iph1 than *** findings reveal a novel ethylene-responsive gene,which provides a theoretical foundation and new genetic resources for the mechanism of ethylene signaling in peanuts.

关键词： Ethylene-insensitive Hypocotyl elongation AhIPH1 Candidate gene Genetic resources

A projected Newton algorithm based on chemically allowed interval for chemical equilibrium computations

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Frontiers of Chemical Science and Engineering 2024年第3期18卷 25-37页

作者： Hongbin Lu shaohui Tao Xiaoyan Sun Li Xia Shuguang Xiang Institute of Process Systems Engineering College of Chemical EngineeringQingdao University of Science and TechnologyQingdao266042China

The chemical equilibrium equations utilized in reactive transport modeling are complex and nonlinear,and are typically solved using the Newton-Raphson *** this algorithm is known for its quadratic convergence near the solution,it is less effective far from the solution,especially for ill-conditioned *** such cases,the algorithm may fail to converge or require excessive *** address these limitations,a projected Newton method is introduced to incorporate the concept of *** method constrains the Newton step by utilizing a chemically allowed interval that generates feasible descending ***,we utilize the positive continuous fraction method as a preconditioning technique,providing reliable initial values for solving the *** numerical results are compared with those derived using the regular Newton-Raphson method,the Newton-Raphson method based on chemically allowed interval updating rules,and the bounded variable least squares method in six different test *** numerical results highlight the robustness and efficacy of the proposed algorithm.

关键词： chemical equilibrium reactive transport modeling numerical methods projected Newton method

Delicate chemical structure regulation of nonfullerene acceptor for efficient and large thickness organic solar cells

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Science China Chemistry 2024年第5期67卷 1596-1604页

作者： Zhe Zhang Wanying Feng Yunxin Zhang shaohui Yuan Yuyang Bai Peiran wang Zhaoyang Yao Chenxi Li Tainan Duan Xiangjian Wan Bin Kan Yongsheng Chen State Key Laboratory and Institute of Elemento-Organic Chemistry Frontiers Science Center for New Organic MatterThe Centre of Nanoscale Science and Technology and Key Laboratory of Functional Polymer MaterialsRenewable Energy Conversion and Storage Center(RECAST)College of ChemistryNankai UniversityTianjin 300071China School of Materials Science and Engineering National Institute for Advanced MaterialsNankai UniversityTianjin 300350China Chongqing Institute of Green and Intelligent Technology Chongqing SchoolUniversity of Chinese Academy of Sciences(UCAS Chongqing)Chinese Academy of SciencesChongqing 400722China

Inspired by the success of CH-series acceptors, a small-molecular acceptor, CH-Tz was reported by adopting a new conjugationextended electron-deficient unit([1,2,5]thiadiazolo[3,4-b]pyrazine) on the central core. Owing to the enhanced inter-/intramolecular interactions, CH-Tz exhibited near-infrared absorption and an effective three-dimensional molecular packing network in its single crystal. When blended with polymer donor PM6, the binary device achieved a high power conversion efficiency(PCE) of 18.54%, with a notable short-circuit current density(J_(sc)) of 27.54 m A cm-2and an excellent fill factor(FF) over 80%,which can be partly ascribed to the balanced charge transport properties in the blend film. After employing D18-Cl as the third component, an enhanced PCE of 18.85% was achieved due to a more obvious fiber network. Impressively, the CH-Tz-based OSC devices show excellent thermal stability and thickness insensitivity. Record-breaking Jscof 28.92 m A cm-2was reached for PM6:D18-Cl:CH-Tz ternary device with a thickness of 560 nm. Besides, CH-Tz shows potential in fabricating multicomponent high-performance organic solar cells, where over 19% efficiency could be realized in the quaternary device. Our work advances the strong influence of electron-deficient central units on molecular photovoltaic properties and guides the design of acceptors for stable and large-thickness organic solar cells.

关键词： organic solar cells non-fullerene acceptor central unit large thickness molecular packing

Cation-Anion Redox Active Organic Complex for High Performance Aqueous Zinc Ion Battery

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Energy & Environmental Materials 2024年第1期7卷 60-67页

作者： Lilin Zhang Yining Chen Zongyuan Jiang Jingwei Chen Cong Wei Wenzhuo Wu shaohui Li Qun Xu School of Materials Science and Engineering Zhengzhou UniversityZhengzhou 450001China Henan Institute of Advanced Technology Zhengzhou UniversityZhengzhou 450001China School of Materials Science and Engineering Ocean University of China Qingdao 266100China

Organic redox compounds are attractive cathode materials in aqueous zinc-ion batteries owing to their low cost,environmental friendliness,multiple-electron-transfer reactions,and resource ***,the realized energy density is constrained by the limited capacity and low ***,copper-tetracyanoquinodimethane(CuTCNQ),an organic charge-transfer complex is evaluated as a zinc-ion battery cathode owing to the good electron acceptation ability in the cyano groups that improves the voltage *** electrochemical activation,electrolyte optimization,and adoption of graphene-based separator,CuTCNQ-based aqueous zinc-ion batteries deliver much improved rate performance and cycling stability with anti-self-discharge *** structural evolution of CuTCNQ during discharge/charge are investigated by ex situ Fourier transform infra-red(FT-IR)spectra,ex situ X-ray photoelectron spectroscopy(XPS),and in situ ultraviolet visible spectroscopy(UV-vis),revealing reversible redox reactions in both cuprous cations(Cu^(+))and organic anions(TCNQ^(x-1)),thus delivering a high voltage output of 1.0 V and excellent discharge capacity of 158 mAh g^(-1).The remarkable electrochemical performance in Zn//CuTCNQ is ascribed to the strong inductive effect of cyano groups in CuTCNQ that elevated the voltage output and the graphene-modified separator that inhibited CuTCNQ dissolution and shuttle effect in aqueous electrolytes.

关键词： cathode materials cyano groups electrochemical activation organic charge-transfer complex zinc-ion battery

A Stable Fuzzy-Based Computational Model and Control for Inductions Motors

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工程与科学中的计算机建模(英文) 2024年第1期138卷 793-812页

作者： Yongqiu Liu shaohui Zhong Nasreen Kausar Chunwei Zhang Ardashir Mohammadzadeh Dragan Pamucar School of Mechanical and Electrical Engineering Guangdong University of Science&TechnologyDongguan523083China School of Information Hunan Open UniversityChangsha410081China Department of Mathematics Faculty of Arts and SciencesYildiz Technical UniversityEsenlerIstanbul34220Turkey Multidisciplinary Center for Infrastructure Engineering Shenyang University of TechnologyShenyang110870China Faculty of Organizational Sciences University of BelgradeBelgrade11000Serbia College of Engineering Yuan Ze UniversityTaoyuan320315TaiwanChina

In this paper,a stable and adaptive sliding mode control(SMC)method for induction motors is *** the parameters of this system has been one of the existing *** solve this challenge,a new self-tuning type-2 fuzzy neural network calculates and updates the control system parameters with a fast *** to the dynamic changes of the system,in addition to the parameters of the SMC,the parameters of the type-2 fuzzy neural network are also updated *** conditions for guaranteeing the convergence and stability of the control system are *** the simulation part,in order to test the proposed method,several uncertain models and load torque have been ***,the results have been compared to the SMC based on the type-1 fuzzy system,the traditional SMC,and the PI *** average RMSE in different scenarios,for type-2 fuzzy SMC,is 0.0311,for type-1 fuzzy SMC is 0.0497,for traditional SMC is 0.0778,and finally for PI controller is 0.0997.

关键词： Sliding mode control self-tuning type-2 fuzzy systems inductions motor parameters uncertainty

Lignite-Based Hierarchical Porous C/SiOx Composites as High-Performance Anode for Potassium-Ion Batteries

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Energy & Environmental Materials 2024年第4期7卷 107-117页

作者： Zexu Yang Shouwang Zhao Rongji Jiao Gengyu Hao Yunying Liu Wenxiu He Jingwei Chen Guixiao Jia Jinlong Cui shaohui Li School of Chemistry and Chemical Engineering Aerogel Functional Nanomaterials Laboratory Inner Mongolia University of Science & Technology School of Materials Science and Engineering Ocean University of China School of Materials Science and Engineering Zhengzhou University

Silicon oxide （SiOx,0 详细信息

Silicon oxide （SiOx,0

关键词： anode hierarchical porous C/SiOx K4SiO4 lignite potassium-ion batteries