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Engineering 2024年第4期35卷 180-190页

作者： Qing-Lian Wu Ke-Xin Yuan Wei-Tong Ren Lin Deng Hua-Zhe wang Xiao-Chi Feng He-Shan Zheng Nan-Qi Ren wan-qian guo State Key Laboratory of Urban Water Resource and Environment Harbin Institute of TechnologyHarbin 150090China College of Architecture and Environment Sichuan UniversityChengdu 610065China State Key Laboratory of Urban Water Resource and Environment School of Civil and Environmental EngineeringHarbin Institute of Technology(Shenzhen)Shenzhen 518055China College of Chemistry and Chemical Engineering Qiqihar UniversityQiqihar 161006China

n-Caproate,which is produced via chain elongation(CE)using waste biomass,can supply various fossilderived products,thus advancing the realization of carbon *** released from the degradation of nitrogen-rich waste biomass can act as a nutrient or an inhibitor in anaerobic bioprocesses,including CE,with the distinction being primarily dependent on its ***,the optimal concentration of ammonia and the threshold of toxicity for open-culture n-caproate production using ethanol as an electron donor,along with the underlying mechanisms,remain *** study revealed that the optimal concentration of ammonia for n-caproate production was 2.0 g∙L^(-1),whereas concentrations exceeding this threshold markedly suppressed the CE *** of the mechanism revealed the involvement of two forms of ammonia(i.e.,ammonium ions and free ammonia)in this inhibitory *** ammonia levels(5.0 g∙L^(-1))induced excessive ethanol oxidation and suppressed the reverse β-oxidation(RBO)process,directly leading to the enhanced activities of enzymes(phosphotransacetylase and acetate kinase)responsible for acetate formation and diminished activities of butyryl-coenzyme A(CoA):acetyl-CoA transferase,caproyl-CoA:butyryl-CoA transferase,and caproyl-CoA:acetyl-CoA transferase that are involved in the syntheses of n-butyrate and ***,the composition of the microbial community shifted from Paraclostridium dominance(at 0.1 g∙L^(-1)ammonia)to a co-dominance of Fermentimonas,Clostridium sensu stricto 12,and Clostridium sensu stricto 15 at 2.0 g∙L^(-1)***,these CE-functional bacteria were mostly absent in the presence of excessive ammonia(5.0 g∙L^(-1)ammonia).Metagenomic analysis revealed the upregulation of functions such as RBO,fatty acid synthesis,K^(+)efflux,adenosine triphosphatase(ATPase)metabolism,and metal cation export in the presence of 2.0 g∙L^(-1)ammonia,collectively contributing to enhanced n-caproate produc

关键词： Ammonia inhibition Medium chain fatty acids n-Caproate Enzyme Metagenomics

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Chain Elongation Using Native Soil Inocula:Exceptional n-Caproate Biosynthesis Performance and Microbial Mechanisms

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Engineering 2024年第8期39卷 262-272页

作者： Lin Deng Yang Lv Tian Lan Qing-Lian Wu Wei-Tong Ren Hua-Zhe wang Bing-Jie Ni wan-qian guo State Key Laboratory of Urban Water Resource and the Environment Harbin Institute of TechnologyHarbin 150090China Centre for Technology in Water and Wastewater&School of Civil and Environmental Engineering University of Technology SydneySydneyNSW 2007Australia

This study demonstrates the feasibility and effectiveness of utilizing native soils as a resource for inocula to produce n-caproate through the chain elongation(CE)platform,offering new insights into anaerobic soil *** results reveal that all five of the tested soil types exhibit CE activity when supplied with high concentrations of ethanol and acetate,highlighting the suitability of soil as an ideal source for n-caproate *** with anaerobic sludge and pit mud,the native soil CE system exhibited higher selectivity(60.53%),specificity(82.32%),carbon distribution(60.00%),electron transfer efficiency(165.00%),and conductivity(0.59 ms∙cm^(-1)).Kinetic analysis further confirmed the superiority of soil in terms of a shorter lag time and higher yield.A microbial community analysis indicated a positive correlation between the relative abundances of Pseudomonas,Azotobacter,and Clostridium and n-caproate ***,metagenomics analysis revealed a higher abundance of functional genes in key microbial species,providing direct insights into the pathways involved in n-caproate formation,including in situ CO_(2)utilization,ethanol oxidation,fatty acid biosynthesis(FAB),and reverse beta-oxidation(RBO).The numerous functions in FAB and RBO are primarily associated with Pseudomonas,Clostridium,Rhodococcus,Stenotrophomonas,and Geobacter,suggesting that these genera may play roles that are involved or associated with the CE ***,this innovative inoculation strategy offers an efficient microbial source for n-caproate production,underscoring the importance of considering CE activity in anaerobic soil microbial ecology and holding potential for significant economic and environmental benefits through soil consortia exploration.

关键词： Soil Chain elongation n-caproate Reverse beta-oxidation Fatty acid biosynthesis Metagenomics

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Carbon quantum dots-based semiconductor preparation methods,applications and mechanisms in environmental contamination

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Chinese Chemical Letters 2020年第10期31卷 2556-2566页

作者： Qi-Shi Si wan-qian guo Hua-Zhe wang Bang-Hai Liu Nan-Qi Ren State Key Laboratory of Urban Water Resource and Environment Harbin Institute of TechnologyHarbin 150090China

Photocatalyst is the most widespread method in advanced oxidation technologies,but due to the photoinduced electron combine easily with hole and the wavele ngth of adsorption is limited which will affect some practical *** quantum dots(CQDs)is non-toxic and harmless green materials,it has the ability to improve the photocatalytic effect which is attributed to its good electrical and optical *** up-conversion effect,photosensitization and electrical conductivity are assistants which help promote the photocatalytic effect in environmental *** key mechanisms of CQDs to improve photocatalysis can be roughly divided into three categories:1)Up-conversion effect conve rts the incident light into the emitted light with high ene rgy to solve the problem which is the light absorption range;2)CQDs act as a photosensitizer instead of valence band to provide electrons to the conduction band of semiconductor;3)CQD s can be used as the internal or external electronic conductor in materials to alleviate the trend of electron and hole ***,CQDs and CQDs-based photocatalysts have different views to solve environmental problems,so it is necessary to integrate different ***,this review is mainly aimed at the recent researches about the preparation processes of CQD,CQD s-based photocatalysts,and their ability to remove environmental pollutants,with a special emphasis on the mechanism for depredating ***,this paper analyzes and discusses the prospects and challenges of CQDs in the environmental field.

关键词： CQDs CQDs modified semiconductor Photodegradation Environmental treatment Photoactive mechanism

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Compared effects of “solid-based” hydrogen peroxide pretreatment on disintegration and properties of waste activated sludge

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Chinese Chemical Letters 2022年第3期33卷 1293-1297页

作者： Hai-Chao Luo wan-qian guo Qi Zhao Hua-Zhe wang Nan-Qi Ren State Key Laboratory of Urban Water Resource and Environment Harbin Institute of TechnologyHarbin 150090China

The effects of two solid-based hydrogen peroxides sodium percarbonate(SPC) and calcium peroxide(CP)on waste activated sludge(WAS) disintegration were investigated. Both oxidants achieved efficient WAS disintegration for the synergistic effect of alkaline and oxidation. The strong alkaline condition led to the leakage of ammonia and the existence of abundant calcium ions accelerated the fixation of phosphorus via precipitation in CP WAS disintegration process. However, the spongy-like layer and low p H condition retarded the release of gaseous ammonia in SPC group. Hydroxyl radical was the main oxygen reactive species in SPC approaches which were more intense than CP by electron spin resonance(ESR) *** treated WAS contented more small particle size matter and total suspended solids(TSS) increased dramatically. In conclusion, CP pretreated sludge was more suitable for fertilization, while SPC was in favor of anaerobic digestion. This study clarified the differences between these two oxidants and their intermediates on nutrients release in sludge disintegration.

关键词： Waste activated sludge “Solid-based”hydrogen peroxide Oxygen reactive species Sludge disintegration Nutrients release

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Localizing vitamin-C through nanoconfinement enables high-rate CO_(2) electrolysis to ethylene

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Science China Materials 2024年第3期67卷 1006-1008页

作者： Zhengyi qian Shaojun guo School of Materials Science and Engineering Peking UniversityBeijing 100871China

The electrosynthesis of value-added fuels and chemicals from carbon dioxide reduction reaction(CO_(2)RR)is a promising approach for realizing the objectives of carbon neutrality[1].Nevertheless,the current production of desirable multicarbon(C_(2+))chemicals,such as ethylene(C_(2)H_(4)),still encounters challenges related to low selectivity,low current density,and the requirement for high-purity feeding gas[2].

关键词： enable purity dioxide

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Light People:*** May Lau,newly elected US NAE member in Hong Kong,talks about future of photonics and women in science

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Light(Science & Applications) 2024年第4期13卷 602-608页

作者： Yating wan Chenzi guo Electrical and Computer Engineering the ComputerElectrical and Mathematical Sciences and Engineering DivisionKing Abdullah University of Science and Technology23955-6900 ThuwalSaudi Arabia Changchun Institute of Optics Fine Mechanics and PhysicsChinese Academy of SciencesChangchunChina

Editorial Photonics technology remains a driving force in today’s scientific landscape,marked by continuous innovation and crossdisciplinary *** an enlighting conversation with Light:Science&Applications,*** May Lau,a pioneer in photonics research,shares her deep insights on the evolution of technologies of LEDs,lasers,challenges of hetero-epitaxy,and the future of micro-LEDs and quantum dot *** honored as a member of the US National Academy of Engineering(NAE)for her significant contributions to photonics and electronics using III-V semiconductors on silicon,*** stands out as the sole Hong Kong scholar inducted into the NAE this year,joining 114 new and 21 international *** this exclusive Light People interview,*** shares her journey as a pioneering woman in engineering,her commitment to mentorship and academia,and her perspective on advancing female representation in *** summary provided is distilled from ***’s thoughtful responses during the *** a deeper exploration of ***’s experiences and advice,the full interview is available in the Supplementary material.

关键词： interview lighting driving

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Harnessing data using symbolic regression methods for discovering novel paradigms in physics

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Science China(Physics,Mechanics & Astronomy) 2024年第6期67卷 1-11页

作者： Jianyang guo wan-Jian Yin College of Energy Soochow Institute for Energy and Materials Innovations(SIEMIS)Jiangsu Provincial Key Laboratory for Advanced Carbon Materials and Wearable Energy TechnologiesSoochow UniversitySuzhou 215006China Shanghai Qi Zhi Institute Shanghai 200232China Light Industry Institute of Electrochemical Power Sources Soochow UniversitySuzhou 215006China

In recent years,machine-learning methods have profoundly impacted research in the interdisciplinary fields of ***,most machine-learning models lack interpretability,and physicists doubt the credibility of their conclusions because they cannot be combined with prior physical ***,this review focuses on symbolic regression,which is an interpretable machine-learning ***,the relevant concepts of machine learning are introduced in conjunction with ***,we provide an overview of symbolic regression ***,the recent directions for the application of symbolic regression methods in different subfields of physics are outlined,and an overview of the ways in which the applications of symbolic regression have evolved in the realm of physics is *** major aim of this review is to introduce the basic principles of symbolic regression and explain its applications in the field of physics.

关键词： machine learning genetic programming symbolic regression

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Optimal regularity of positive solutions of the Hénon-Hardy equation and related equations

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Science China Mathematics 2024年第10期67卷 2283-2302页

作者： Zongming guo Fangshu wan College of Mathematics and Information Science Henan Normal UniversityXinxiang 453007China School of Mathematical Sciences University of Science and Technology of ChinaHefei 230026China School of Mathematical Sciences Anhui UniversityHefei 230601China

We present a new method to determine the optimal regularity of positive solutions u∈C^(4)(Ω\{0})∩C^(0)(Ω) of the Hénon-Hardy equation,i.e.,Δ^(2)u=|x|^(α)u^(p)inΩ,(0,1) where Ω■RN(N≥4) is a bounded smooth domain with 0∈Ω,α>-4,and p∈*** is clear that 0 is an isolated singular point of solutions of(0.1) and the optimal regularity of u in Ω relies on the parameter α.It is also important to see that the regularity of u at x=0 determines the regularity of u in Ω.We first establish asymptotic expansions up to arbitrary orders at x=0 of prescribed positive solutions u ∈C^(4)(Ω{0}) ∩ C^(0)(Ω)of(0.1).Then we show that the regularity at x=0 of each positive solution u of(0.1) can be determined by some terms in asymptotic expansions of the related positive radial solution of the equation(0.1) with Ω=B,where B is the unit ball of R^(N).The main idea works for more general equations with singular weights.

关键词： H´enon-Hardy equation positive solutions optimal regularity singular point asymptotic expansions

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Vibration Control of A Flexible Marine Riser System Subject to Input Dead Zone and Extraneous Disturbances

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China Ocean Engineering 2024年第2期38卷 271-284页

作者： ZHOU Li wanG guo-rong wan Min School of Mechatronic Engineering Southwest Petroleum UniversityChengdu 610500China Energy Equipment Institute Southwest Petroleum UniversityChengdu 610500China National Key Laboratory of Oil and Gas Reservoir Geology and Exploitation Southwest Petroleum UniversityChengdu 610500China

An observer-based adaptive backstepping boundary control is proposed for vibration control of flexible offshore riser systems with unknown nonlinear input dead zone and uncertain environmental *** control algorithm can update the control law online through real-time data to make the controller adapt to the environment and improve the control ***,based on the adaptive backstepping framework,virtual control laws and Lyapunov functions are designed for each *** direction interference observers are designed to track the timevarying boundary *** this basis,the inverse of the dead zone and linear state transformation are used to compensate for the original system and eliminate the adverse effects of the dead *** addition,the stability of the closed-loop system is proven by Lyapunov stability *** the system states are bounded,and the vibration offset of the riser converges to a small area of the initial ***,four examples of flexible marine risers are simulated in MATLAB to verify the effectiveness of the proposed controller.

关键词： adaptive backstepping control disturbance observer flexible marine riser input dead zone vibration control

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Recent Advances in Mechanistic Understanding of Metal-Free Carbon Thermocatalysis and Electrocatalysis with Model Molecules

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Nano-Micro Letters 2024年第7期16卷 74-97页

作者： Wei guo Linhui Yu Ling Tang Yan wan Yangming Lin CAS Key Laboratory of Design and Assembly of Functional Nanostructures Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002People’s Republic of China Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials Xiamen Institute of Rare Earth MaterialsHaixi InstituteChinese Academy of SciencesXiamen 361021People’s Republic of China State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002People’s Republic of China Institute of Urban Environment Chinese Academy of SciencesXiamen 361021People’s Republic of China

Metal-free carbon,as the most representative heterogeneous metal-free catalysts,have received considerable interests in electro-and thermo-catalytic reac-tions due to their impressive performance and *** the past decade,well-designed carbon catalysts with tunable structures and heteroatom groups coupled with various characterization techniques have proposed numerous reaction ***,active sites,key intermediate species,precise structure-activity relationships and dynamic evolution processes of carbon catalysts are still rife with controversies due to the monotony and limitation of used experimental *** this Review,we sum-marize the extensive efforts on model catalysts since the 2000s,particularly in the past decade,to overcome the influences of material and structure limitations in metal-free carbon *** both nanomolecule model and bulk model,the real contribution of each alien species,defect and edge configuration to a series of fundamentally important reactions,such as thermocatalytic reactions,electrocatalytic reactions,were systematically *** with in situ techniques,isotope labeling and size control,the detailed reaction mechanisms,the precise 2D structure-activity relationships and the rate-determining steps were revealed at a molecular ***,the outlook of model carbon catalysis has also been proposed in this work.

关键词： Metal-free carbon catalysts Model catalyst Electrocatalysis Active site Reaction mechanisms

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