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Domain-engineered BiFeO3 thin-film photoanodes for highly enhanced ferroelectric solar water splitting

Nano Research 2018年第2期11卷 642-655页

作者： Jaesun Song Taemin Ludvic kim Jongmin Lee Sam Yeon Cho Jaeseong Cha Sang Yun Jeong Hyunji An wan sik kim Yen-Sook Jung Jiyoon Park Gun Young Jung Dong-Yu kim Ji Young Jo Sang Don Bu Ho Won Jang Sanghan Lee School of Materials Science and Engineering Gwangju Institute of Science and Technology (GIST) Gwangju Republic of Korea Department of Materials Science and Engineering Research Institute of Advanced Materials Seoul National University Seoul Republic of Korea Department of Physics Chonbuk National University Jeonju Republic of Korea

In photoelectrochemical （PEC） water splitting, charge separation and collection by the electric field in the photoactive material are the most important factors for improved conversion efficiency. Hence, ferroelectric oxides, in which electrons are the majority carriers, are considered promising photoanode materials because their high built-in potential, provided by their spontaneous polarization, can signifi＇canfly enhance the separation and drift of photogenerated carriers. In this regard, the PEC properties of BiFeO3 thin-film photoanodes with different crystallographic orientations and consequent ferroelectric domain structures are investigated. As the crystallographic orientation changes from （001）pc via （ll0）pc to （lll）p~, the ferroelastic domains in epitaxial BiFeO3 thin films become mono-variant and the spontaneous polarization levels increase to 110 btC/cm2. Consequent136 the photocurrent density at 0 V vs. Ag/AgC1 increases approximately 5.3-fold and the onset potential decreases by 0.180 V in the downward polarization state. It is further demonstrated that ferroelectric switching in the （lll）pc BiFeO3 thin-film photoanode leads to an approximate change of 8,000% in the photocurrent density and a 0.330 V shift in the onset potential. This study strongly suggests that domain-engineered ferroelectric materials can be used as effective charge separation and collection layers for efficient solar water-splitting photoanodes.

关键词： BiFeO3 ferroelectric photoelectrochemical domain orientation pulsed laser deposition

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Aligned Ion Conduction Pathway of Polyrotaxane‑Based Electrolyte with Dispersed Hydrophobic Chains for Solid‑State Lithium–Oxygen Batteries

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Nano-Micro Letters 2025年第2期17卷 169-186页

作者： Bitgaram kim Myeong‑Chang Sung Gwang‑Hee Lee Byoungjoon Hwang Sojung Seo Ji‑Hun Seo Dong‑wan kim Department of Materials Science and Engineering Korea University145 Anam‑RoSeongbuk‑GuSeoul 02841Republic of Korea School of Civil Environmental and Architectural EngineeringKorea University145 Anam‑RoSeongbuk‑GuSeoul 02841Republic of Korea Materials Science and Chemical Engineering Center Institute for Advanced Engineering(IAE)Yongin 17180Republic of Korea

A critical challenge hindering the practical application of lithium–oxygen batteries(LOBs)is the inevitable problems associated with liquid electrolytes,such as evaporation and safety *** study addresses these problems by proposing a modified polyrotaxane(mPR)-based solid polymer electrolyte(SPE)design that simultaneously mitigates solvent-related problems and improves ***-SPE exhibits high ion conductivity(2.8×10^(−3)S cm^(−1)at 25℃)through aligned ion conduction pathways and provides electrode protection ability through hydrophobic chain *** this mPR-SPE into solid-state LOBs resulted in stable potentials over 300 *** situ Raman spectroscopy reveals the presence of an LiO_(2)intermediate alongside Li_(2)O_(2)during oxygen *** situ X-ray diffraction confirm the ability of the SPE to hinder the permeation of oxygen and moisture,as demonstrated by the air permeability *** present study suggests that maintaining a low residual solvent while achieving high ionic conductivity is crucial for restricting the sub-reactions of solid-state LOBs.

关键词： Solid polymer electrolyte Lithium-oxygen batteries Polyrotaxane ion conductivity Hydrophobic chain

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Improvement of erectile function by Korean red ginseng （Panax ginseng） in a male rat model of metabolic syndrome

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Asian Journal of Andrology 2013年第3期15卷 395-399页

作者： Sung-Dae kim Young-Joo kim Jung-sik Huh Sae-Woong kim Dong-wan Sohn Department of Urology School of Medicine Jeju National University Jeju 690767 Korea Department of Urology College of Medicine The Catholic University of Korea Seoul 150713 Korea

The seriousness of metabolic syndrome is not due to the disease itself but its promotion of other diseases, such as erectile dysfunction and cardiovascular and cerebrovascular diseases. We investigated the effects of Korean red ginseng （KRG, Panax ginseng） extract on erectile function in a rat model of metabolic syndrome. We divided the rats into three groups： control, metabolic syndrome＋normal saline （N/S） and metabolic syndrome ＋ KRG. To determine the occurrence of metabolic syndrome in all groups, body weight and various biochemical parameters （e.g., blood glucose, insulin, cholesterol） were measured, and the intra-abdominal glucose tolerance test was performed. To investigate penile erection, the peak intracavernosal pressure （ICP）, mean arterial pressure （MAP） and Masson＇s trichrome stain were evaluated. Erectile function was also investigated by measuring the cyclic guanosine monophosphate （cGMP） levels of the corpus cavernosum. We found that the various biochemical parameters and body weight were similar in the metabolic syndrome＋KRG group and the control group, although the values were slightly higher. The peak ICP/MAP ratio of the metabolic syndrome＋N/S group was markedly decreased compared to the other groups. The cGMP level of the corpus cavernosum in the metabolic syndrome＋N/S group was significantly lower than that of the other groups. As demonstrated in this model of metabolic syndrome with erectile dysfunction, KRG may improve erectile function.

关键词： erectile dysfunction ginseng metabolic syndrome penis

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Comparison of totally laparoscopic total gastrectomy using an endoscopic linear stapler with laparoscopic-assisted total gastrectomy using a circular stapler in patients with gastric cancer: a single-center experience

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World Journal of Gastroenterology 2017年第48期23卷 8553-8561页

作者： Chung sik Gong Byung sik kim Hee Sung kim department of gastric surgery asan medical centeruniversity of ulsan college of medicine

AIM To evaluate the safety and efficacy of totally laparoscopic total gastrectomy(TLTG) with esophagojejunostomy using a linear stapler compared with laparoscopic-assisted total gastrectomy(LATG) using a circular stapler in gastric cancer *** We retrospectively reviewed 687 patients who underwent laparoscopic total gastrectomy for gastric cancer at a single institution from August 2008 to August 2014. The patients were divided into two groups according to the type of operation: 421 patients underwent TLTG and 266 underwent LATG. Clinicopathologic characteristics and surgical outcomes in the two groups were compared and *** The TLTG group had higher mean ages at the time of operation(57.78 ± 11.20 years and 55.69 ± 11.96 years,P = 0.020) and more histories of abdominal surgery(20.2% and 12.4%,P = 0.008) compared with the LATG group. Surgical outcomes such as intraoperative and postoperative transfusions,combined operations,pain scores and administration of analgesics,and complications were similar between the two groups. However,compared with the LATG group,the TLTG group required a shorter operation time(149 min vs 170 min,P < 0.001),had lower postoperative hematocrit change(3.49% vs 4.04%,P = 0.002),less intraoperative events(3.1% vs 10.2%,P < 0.001),less intraoperative anastomosis events(2.4% vs 7.1%,P = 0.003),faster postoperative recovery such as median time to first flatus(3.30 d vs 3.60 d,P < 0.001),faster median commencement of soft diet(4.30 d vs 4.60 d,P < 0.001) and shorter length of postoperative hospital stay(6.75 d vs 7.02 d,P = 0.005). CONCLUSION The intracorporeal method for reconstruction of esophagojejunostomy using a linear stapler may be considered a feasible procedure comparing with extracorporeal anastomosis using circular stapler because TLTG is simpler and more straightforward than LATG. Therefore,TLTG can be recommended as an appropriate procedure for gastric cancer.

关键词： Totally laparoscopic total gastrectomy Laparoscopic-assisted total gastrectomy Gastric cancer

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Visible-light-activated N-doped CQDs/g-C3N4/Bi2WO6 nanocomposites with different component arrangements for the promoted degradation of hazardous vapors

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Journal of Materials Science & Technology 2020年第5期40卷 168-175页

作者： Mi Gyeong kim wan-Kuen Jo Department of Environmental Engineering Kyungpook National University 80 University RoadBukguDaegu702-701Republic of Korea

To investigate whether the arrangement of componentsin multi-composite photocatalysts may affect their photocatalytic properties,due to different charge-transfer routes,two ternary-nanocomposite photocatalysts with different component arrangements,comprising N-doped carbon quantum dots(NCQDs),g-C3N4(CN),and Bi2WO6(BWO)(hereafter referred to as NCQDs/CN/BWO),were developed,and the photocatalytic degradation of model hazardous vapors under visible-light illumination was *** I NCQDs/CN/BWO,which was developed by the combination of NCQDs/BWO and CN,exhibited photocatalytic ability superior to that of type II NCQDs/CN/BWO,which was developed by the combination of CN/BWO and NCQDs;the superior photocatalytic ability corresponded to the dual properties of NCQDs:charge mediation and upconversion ***,the photocatalytic ability of NCQDs/CN/BWO was greater than those of the reference catalysts;in addition,this photocatalyst exhibited outstanding photochemical ***,the effects of CN/(BWO+CN)weight ratio of the CN/BWO dual nanocomposites and the NCQDs/(BWO+CN+NCQDs)weight percentage of NCQDs/CN/BWO ternary nanocomposites on the pollutant removal efficiency were *** plausible mechanisms over the two NCQDs/CN/BWO photocatalysts for the degradation of hazardous vapors were *** component arrangement approach proposed herein afforded a technique toward the perceptive development of novel multi-component heterostructures for the photocatalytic degradation of hazardous vapors.

关键词： Component arrangement Charge-transfer route NCQDs dual role Charge mediator Upconversion photoluminescence

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Modified analogue forecasting in the hidden Markov frameworkfor meteorological droughts

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Science China(Technological Sciences) 2019年第1期62卷 151-162页

作者： CHEN Si CHUNG GunHui kim Byung sik kim Tae-Woong Department of Civil and Environmental Engineering Hanyang University Department of Civil Engineering Hoseo University Department of Urban Environmental Disaster Prevention Engineering Kangwon National University

An analogue method(AM) is a nonparametric approach that has been applied to predict the future states of a dynamic system by following the evolution of the analogues in the historical archive. In this study, we proposed a hidden Markov model(HMM)framework for a modified analogue forecasting(MAF) approach for meteorological droughts in Korea. The unobservable(hidden) state process in the framework aims to model the underlying drought state, while the observation process was formed from the time series of the standardized precipitation index(SPI) as a drought index. Within the framework, the likelihood estimator was used as the measure of similarity between past SPI analogues and current data. The MAF approach was conducted on the selected analogues to make forecasts at lead times of one and three months. The proposed model was applied to five selected stations in Korea using the SPI data from 1973 to 2016. The forecasting performance of the proposed model was tested during the validation period(2003–2016) using several statistical criteria and it was compared to a persistence-based benchmark model. The results showed significant improvement in the forecasting capacity, and satisfactory performance for numerical SPI forecasting and categorical drought forecasting. The results also suggested that the proposed model was able to provide useful information for determining future drought categories for early drought warning with a lead time of up to three months.

关键词： modified analogue forecasting hidden Markov model meteorological drought standardized precipitation index

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Chemical surface tuning of zinc metal anode toward stable,dendrite-less aqueous zinc-ion batteries

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Journal of Energy Chemistry 2023年第11期86卷 1-8,I0001页

作者： Pranav Kulkarni Sun-sik kim Hyun Young Jung Department of Energy Engineering Gyeongsang National UniversityJinju-siGyeongnam 52725South Korea Department of Energy System Engineering Gyeongsang National UniversityJinju-siGyeongnam 52725South Korea

The commercialization of Zn batteries is confronted with urgent challenges in the metal anode,such as dendrite formation,capacity loss,and cracking or ***,surface interfacial engineering of the Zn anode is introduced for achieving safety and dendritic-free cycling for high-performance aqueous Zn batteries through a simple but highly effective chemical etching-substitution *** chemical modification induces a rough peak-valley surface with a thin fluorine-rich interfacial layer on the Zn anode surface,which regulates the growth orientation via guiding uniform Zn plating/stripping,significantly enhances accessibility to aqueous electrolytes and improves wettability by reducing surface *** a result,such a synergetic surface effect enables uniform Zn plating/stripping with low polarization of 29 m V at a current density of 0.5 m A cm^(-2) with stable cyclic performance up to 1000 ***,a full cell composed of a fluorine-substituted Zn anode coupled with aβ-MnO_(2)or Ba-V_(6)O_(13)cathode demonstrates improved capacity retention to 1000 cycles compared to the pristine-Zn *** proposed valley deposition model provides the practical direction of surface-modified interfacial chemistries for improving the electrochemical properties of multivalent metal anodes via surface tuning.

关键词： Dendrite free Peak-Valley surface Zinc-ion batteries Surface modification Fluorinated interface

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Effect of post heat-treatment on the microstructure and high-temperature oxidation behavior of precipitation hardened IN738LC superalloy fabricated by selective laser melting

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Journal of Materials Science & Technology 2021年第17期76卷 95-103页

作者： Kyu-sik kim Sangsun Yang Myeong-Se kim Kee-Ahn Lee Department of Materials Science and Engineering Inha UniversityIncheon 22212Republic of Korea Korea Institute of Materials Science Changwon51508Republic of Korea Auratech Co. Ltd.Seongnam13449Republic of Korea

The present study investigated the effect of as-built and post heat-treated microstructures of IN738LC alloy fabricated via selective laser melting process on high temperature oxidation *** as-built microstructure showed fine cell and columnar structure due to high cooling *** element segregation was observed in inter-cell/inter-columnar *** post heat-treatment,the initially-observed cell structure disappeared,instead bimodal Ni_3(Al,Ti)particles *** temperature(1273 K and 1373 K)oxidation test results showed parabolic oxidation curves regardless of temperature and initial *** as-built IN738LC fabricated via the selective laser melting process displayed oxidation resistance similar to or slightly better than that of IN738LC fabricated via wrought or cast ***-treated SLM IN738LC,although had similar oxidation weight-gain values to those of the SLM asbuilt material at 1273K,showed relatively better oxidation resistance at 1373 *** Ni_3(Al,Ti)precipitate formed in the post heat treatment changed the local chemical composition,thereby led to changes in alumina former/chromia former location and fraction on the alloy *** was concluded that in heat-treated IN738LC increased alumina former fraction was found,and this resulted in excellent oxidation resistance and relatively low weight-gain.

关键词： IN738LC Selective laser melting High temperature oxidation Post heat-treatment Oxidation mechanism

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ON TRANSMISSION PROBLEM FOR VISCOELASTIC WAVE EQUATION WITH A LOCALIZED A NONLINEAR DISSIPATION

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Acta Mathematica Scientia 2013年第2期33卷 362-374页

作者： Jeong Ja BAE Seong sik kim Department of Mathematics Dongeui UniversityPusan 614-714Korea

In this article, we consider the global existence and decay rates of solutions for the transmission problem of Kirchhoff type wave equations consisting of two physically different types of materials, one component being a Kirchhoff type wave equation with time dependent localized dissipation which is effective only on a neighborhood of certain part of boundary, while the other being a Kirchhoff type viscoelastic wave equation with nonlinear memory

关键词： Existence of solution uniform decay transmission problem boundary valueproblem localized dissipation

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Degenerate s-Extended Complete and Incomplete Lah-Bell Polynomials

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Computer Modeling in Engineering & Sciences 2022年第6期130卷 1479-1495页

作者： Hye Kyung kim Dae sik Lee Department of Mathematics Education Daegu Catholic UniversityGyeongsan38430Korea School of Electronic and Electric Engineering Daegu UniversityGyeongsan38453Korea

Degenerate versions of special polynomials and numbers applied to social problems,physics,and applied mathematics have been studied variously in recent ***,the(s-)Lah numbers have many other interesting applications in analysis and *** this paper,we divide two *** first introduce new types of both degenerate incomplete and complete s-Bell polynomials respectively and investigate some properties of them ***,we introduce the degenerate versions of complete and incomplete Lah-Bell polynomials as multivariate forms for a new type of degenerate s-extended Lah-Bell polynomials and numbers *** investigate relations between these polynomials and degenerate incomplete and complete s-Bell polynomials,and derive explicit formulas for these polynomials.

关键词： Lah-Bell numbers and polynomials s-extended Lah-Bell numbers and polynomials complete s-Bell polynomials incomplete s-Bell polynomials s-Stirling numbers of second kind

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