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Ganoderma lucidum:a comprehensive review of phytochemistry,efficacy,safety and clinical study

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Food Science and Human Wellness 2024年第2期13卷 568-596页

作者： Sijia wu Siyuan Zhang Bo Peng Dechao Tan Mingyue wu Jinchao Wei yitao Wang Hua Luo Macao Centre for Research and Development in Chinese Medicine State Key Laboratory of Quality Research in Chinese MedicineInstitute of Chinese Medical SciencesUniversity of MacaoMacao SAR 999078China College of Pharmacy Guangxi Medical UniversityNanning 530021China Guangxi University of Chinese Medicine Nanning 530001China

Ganoderma lucidum,one of the most well-known edible fungi,is believed to be very beneficial for longevity and vitality.A long usage history suggests that G.lucidum has various clinical therapeutic effects.And experimental studies have confirmed that G.lucidum has multiple pharmacological effects,including antitumor,anti-microbial,anti-HIV protease,and antidiabetic activity and so on.With the deepening of research,more than 300 compounds have been isolated from G.lucidum.There is an increasing population of G.lucidum-based products,and its international development is expanding.Currently,G.lucidum has drawn much attention to its chemical composition,therapeutic effect,clinical value,and safety.This paper provides a comprehensive review of these aspects to enhance the global promotion of G.lucidum.

关键词： Ganoderma lucidum Phytochemistry Efficacy Safety Clinical study

Ca and Sr co-doping induced oxygen vacancies in 3DOM La_(2-x)Sr_(x)Ce_(2-y)CayO_(7-δ)catalysts for boosting low-temperature oxidative coupling of methane

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Journal of Energy Chemistry 2024年第4期91卷 331-344页

作者： Tongtong wu Yuechang Wei Jing Xiong yitao Yang Zhenpeng Wang Dawei Han Zhen Zhao Jian Liu State Key Laboratory of Heavy Oil Processing China University of PetroleumBeijing 102249China Key Laboratory of Optical Detection Technology for Oil and Gas China University of PetroleumBeijing 102249China

It is urgent to develop catalysts with application potential for oxidative coupling of methane(OCM)at relatively lower temperature.Herein,three-dimensional ordered macro porous(3 DOM)La_(2-x)Sr_(x)Ce_(2-y)CayO_(7-δ)(A_(2)B_(2)O_(7)-type)catalysts with disordered defective cubic fluorite phased structure were successfully prepared by a colloidal crystal template method.3DOM structure promotes the accessibility of the gaseous reactants(O2and CH4)to the active sites.The co-doping of Ca and Sr ions in La_(2-x)Sr_(x)Ce_(2-y)CayO_(7-δ)catalysts improved the formation of oxygen vacancies,thereby leading to increased density of surface-active oxygen species(O_(2)^(-))for the activation of CH4and the formation of C2products(C2H6and C2H4).3DOM La_(2-x)Sr_(x)Ce_(2-y)CayO_(7-δ)catalysts exhibit high catalytic activity for OCM at low temperature.3DOM La1.7Sr0.3Ce1.7Ca0.3O7-δcatalyst with the highest density of O_(2)^(-)species exhibited the highest catalytic activity for low-temperature OCM,i.e.,its CH4conversion,selectivity and yield of C2products at 650℃are 32.2%,66.1%and 21.3%,respectively.The mechanism was proposed that the increase in surface oxygen vacancies induced by the co-doping of Ca and Sr ions boosts the key step of C-H bond breaking and C-C bond coupling in catalyzing low-temperature OCM.It is meaningful for the development of the low-temperature and high-efficient catalysts for OCM reaction in practical application.

关键词： 3DOM catalysts Ca ions Sr ions Low-temperature oxidative couplingof methane Oxygen vacancies O_(2)^(-) species

Irrigation and nitrogen fertiliser optimisation in protected vegetable fields of northern China:Achieving environmental and agronomic sustainability

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Journal of Integrative Agriculture 2024年第3期23卷 1022-1033页

作者： Bingqian Fan yitao Zhang Owen Fenton Karen Daly Jungai Li Hongyuan Wang Limei Zhai Xiaosheng Luo Qiuliang Lei Shuxia wu Hongbin Liu State Key Laboratory of Efficient Utilization of Arid and Semi-arid Arable Land in Northern China/Key Laboratory of Nonpoint Source Pollution Control Ministry of Agriculture and Rural Affairs/lnstitute of Agricultural Resources and Regional PlanningChinese Academy of Agricultural SciencesBeijing 100081China Institute of Geographic Sciences and Natural Resources Research Chinese Academy of SciencesBeijing 100101China Teagasc Environmental Research CentreWexford Y35Ireland Institute of Plant Nutrition Resources and Environmental SciencesHenan Academy of Agricultural SciencesZhengzhou 450002China

Globally,sub-optimal use of nitrogen (N) fertiliser and elevated N irrigation groundwater have led to high leached nitrate (NO_(3)^(–)) losses from protected vegetable field systems.Optimising fertiliser and irrigation management in different soil types is crucial to reduce future N loads from such systems.The present 4-year study examined leached N loads from lysimeter monitoring arrays set up across 18 protected vegetable system sites encompassing the dominant soil types of northern China.The treatments applied at each field site were:1) a high N and high irrigation input treatment (HNHI);2) a low N but high irrigation input treatment (LNHI) and 3) a low N with low irrigation input treatment (LNLI).Results showed that the mean annual leached total nitrogen loads from the HNHI,LNHI and LNLI treatments were 325,294 and 257 kg N ha^(–1) in the fluvo-aquic soil,114,100 and 78 kg N ha^(–1) in the cinnamon soil and 79,68 and 57 kg N ha^(–1) in the black soil,respectively.The N dissolved in irrigation water in the fluvo-aquic soil areas was 8.26-fold higher than in the cinnamon areas.A structural equation model showed that N fertiliser inputs and leaching water amounts explained 14.7 and 81.8%of the variation of leached N loads,respectively.Correspondingly,reducing irrigation water by 21.5%decreased leached N loads by 20.9%,while reducing manure N and chemical N inputs by 22 and 25%decreased leached N loads by only 9.5%. This study highlights that protected vegetable fields dominated by fluvo-aquic soil need management to curtail leached N losses in northern China.

关键词： agriculture water quality nitrate groundwater irrigation management

A Modified Cohesive Zone Model for Simulation of Delamination Behavior in Laminated Composites

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Transactions of Nanjing University of Aeronautics and Astronautics 2019年第5期36卷 724-732页

作者： wu yitao LIAN Wei Shanghai YS Information Technology Co. Ltd.Shanghai 200240P.R.China Shanghai Aircraft Design and Research Institute Shanghai 201210P.R.China

Considering the promotion effect of interlaminar normal tensile stress and the inhibition effect of interlaminar normal compressive stress,two kinds of elimination initial criteria were proposed in this paper.Based on these two delamination initial criteria,a modified cohesive zone model(CZM)was established to simulate the delamination behavior in laminated composites.Numerical simulations of double cantilever beam(DCB),mixed-mode bending(MMB)and end notched flexure(ENF)tests were conducted.The results show that the proposed model can do a better job than common ones when it is used to predict laminates’delamination under interlaminar compression stress.Moreover,a factor r,named cohesive strength coefficient,was defined in this paper on account of the difference between cohesive strength and interlaminar fracture strength.With changing factor r,it shows that a moderate variation of cohesive strength will not cause significant influences on global load-displacement responses.Besides,in order to obtain a good balance between prediction accuracy and computational efficiency,there shall be two or three numerical elements within the cohesive zone.

关键词： composite laminate delamination numerical analysis cohesive zone model

Anti-oxidant anti-inflammatory and antibacterial tannin-crosslinked citrate-based mussel-inspired bioadhesives facilitate scarless wound healing

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Bioactive Materials 2023年第2期20卷 93-110页

作者： Keke wu Meimei Fu yitao Zhao Ethan Gerhard Yue Li Jian Yang Jinshan Guo Department of Histology and Embryology NMPA Key Laboratory for Safety Evaluation of CosmeticsSchool of Basic Medical SciencesGuangdong Provincial Key Laboratory of Bone and Joint Degeneration DiseasesThe Third Affiliated Hospital of Southern Medical UniversitySouthern Medical UniversityGuangzhouChina Department of Biomedical Engineering Pennsylvania State UniversityUniversity ParkPA16802USA

The revolutionary role of tissue adhesives in wound closure,tissue sealing,and bleeding control necessitates the development of multifunctional materials capable of effective and scarless healing.In contrast to the use of traditionally utilized toxic oxidative crosslinking initiators(exemplified by sodium periodate and silver nitrate),herein,the natural polyphenolic compound tannic acid(TA)was used to achieve near instantaneous(90%bacterial death upon near-infrared(NIR)irradiation).In vivo evaluation in both an infected full-thickness skin wound model and a rat skin incision model demonstrated that 3A-TCMBAs+NIR treatment could promote wound closure and collagen deposition and improve the collagen Ⅰ/Ⅲ ratio on wound sites while simultaneously inhibiting the expression of pro-inflammatory cytokines.Further,phased angiogenesis was observed via promotion in the early wound closure phases followed by inhibition and triggering of degradation&remodeling of the extracellular matrix(ECM)in the late stage(supported by phased CD31(platelet endothelial cell adhesion molecule-1)PDGF(platelet-derived growth factor)and VEGF(vascular endothelial growth factor)expression as well as elevated matrix metalloprotein-9(MMP-9)expression on day 21),resulting in scarless wound healing.The significant convergence of material and bioactive properties elucidated above warrant further exploration of 3A-TCMBAs as a significant,new class of bioadhesive.

关键词： Anti-oxidant Hydrogen bond crosslinking Phased angiogenesis Scarless wound healing Tannic acid

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电催化两电子水氧化制备过氧化氢的研究进展

物理化学学报 2024年第4期40卷 11-25页

作者：林柳孙泽民陈华添赵莲孙明月杨逸涛廖振升吴鑫宇李欣欣唐城北京师范大学文理学院先进材料研究中心广东珠海519087 清华大学化学工程系绿色反应工程与工艺北京市重点实验室北京100084

过氧化氢(H_(2)O_(2))是一种环境友好的化学氧化剂,广泛应用于水处理、医疗消毒、化学合成等工业领域。电催化两电子水氧化反应(2e^(-)WOR)是一种可以在温和条件下直接从水中生产H_(2)O_(2)的方法。然而,受限于反应机理认识和催化材料... 详细信息

过氧化氢(H_(2)O_(2))是一种环境友好的化学氧化剂,广泛应用于水处理、医疗消毒、化学合成等工业领域。电催化两电子水氧化反应(2e^(-)WOR)是一种可以在温和条件下直接从水中生产H_(2)O_(2)的方法。然而,受限于反应机理认识和催化材料设计的不足,2e^(-)WOR的催化选择性和活性仍然较低。本文综述了近年来通过2e^(-)WOR反应路径电合成H_(2)O_(2)的研究进展,首先介绍了2e^(-)WOR的催化机理和研究方法,强调了理论计算加速高选择性、高活性和高稳定性催化剂研究的作用,并讨论了电合成H_(2)O_(2)的不同定量方法和原位表征手段;然后详细总结了高性能2e^(-)WOR电催化剂的调控策略,包括缺陷、掺杂、晶面和界面工程,同时指出了反应器创新设计的重要性;最后展望了电合成H_(2)O_(2)的研究挑战和机遇。

关键词：水氧化反应过氧化氢催化剂设计电化学机理理论研究

基于主动光场调控的超快光纤激光器研究进展(特邀)

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激光与光电子学进展 2024年第1期61卷 270-286页

作者：刘嘉豪罗智超张泽贤杨奕涛伍代轩刘萌罗爱平徐文成华南师范大学信息光电子科技学院广东广州510006

综述了近期基于腔内空间光调制器的超快光纤激光器的研究进展,总结了目前基于腔内空间光调制器的超快光纤激光器所能实现的基本功能和输出特性,同时介绍了本课题组基于腔内空间光调制器的研究成果,最后对腔内空间光调制器驱动的超快光... 详细信息

综述了近期基于腔内空间光调制器的超快光纤激光器的研究进展,总结了目前基于腔内空间光调制器的超快光纤激光器所能实现的基本功能和输出特性,同时介绍了本课题组基于腔内空间光调制器的研究成果,最后对腔内空间光调制器驱动的超快光纤激光器的发展趋势和应用前景进行了展望。

关键词：激光器超快光纤激光器空间光调制器光场调控脉冲整形色散管理

河北省塞罕坝地区气温和降水变化的环流特征及关键因子

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沙漠与绿洲气象 2024年第3期18卷 63-68页

作者：吴萍萍贾硕郭义涛叶正谦承德市气象站河北承德067000 承德市气象局河北承德067000 雄安新区气象局河北雄安071700 围场县气象局河北围场068450

对塞罕坝地区多年气温和降水的大尺度环流异常进行合成分析,研究其环流特征及关键因子。结果表明:1962-2020年塞罕坝地区气温总体呈偏高趋势,春、秋、冬季降水呈偏多趋势,夏季降水呈偏少趋势。大尺度环流背景下,各季节影响塞罕坝地区气... 详细信息

对塞罕坝地区多年气温和降水的大尺度环流异常进行合成分析,研究其环流特征及关键因子。结果表明:1962-2020年塞罕坝地区气温总体呈偏高趋势,春、秋、冬季降水呈偏多趋势,夏季降水呈偏少趋势。大尺度环流背景下,各季节影响塞罕坝地区气温和降水的主要因子不同,通过挑选最优因子分析得出:塞罕坝地区受大气环流指数影响明显,春季太平洋-北美遥相关型指数(PNA)、夏季北大西洋涛动指数(NAO)、秋季西太平洋遥相关型指数(WP)、冬季高原季风指数(PMI)与该地气温和降水有较好的关系。

关键词：塞罕坝环流特征关键因子气温降水

Vacancy-enhanced Mo-N_(2) interaction in MoSe_(2) nanosheets enables efficient electrocatalytic NH_(3) synthesis

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Chinese Chemical Letters 2023年第1期34卷 474-477页

作者： Shuhong wu Meng Zhang Shengmei Huang Lihai Cai Dannong He yitao Liu School of Materials Science and Engineering Shanghai Jiao Tong UniversityShanghai 200240China National Engineering Research Center for Nanotechnology Shanghai 200240China Innovation Center for Textile Science and Technology Donghua UniversityShanghai 200051China Institute of Systems Engineering Academy of Military SciencesBeijing 102300China

NH_(3) plays an essential role in human life since it is an important raw material for fertilizers,plastics and rubbers production.As an NH_(3) synthesis technology under ambient conditions,electrocatalytic N_(2) reduction reaction(NRR)has great potential to replace the energy-intensive Haber-Bosch process.The key of electrocatalytic NRR is the exploration of efficient catalysts.Transition metal Mo is promising since it exists naturally in nitrogenase due to the unique Mo-N_(2) interaction;particularly in the form of 2D material such as MoSe_(2),the surface area is maximized for more active sites.However,the NRR performance of MoSe_(2) is still unsatisfactory because Mo is only exposed at the semi-open edge,and the electronegative Se-mantled surface area remains inaccessible to N_(2).Herein,we propose a simple and effective strategy to create high-concentration Se vacancies in MoSe_(2) through heteroatom doping induced lattice strain,which effectively enhances the Mo-N_(2) interaction on the surface area.In result,high NH_(3) yield(3.04×10^(–10)mol s^(–1)cm^(–2))and Faraday efficiency(21.61%)are attained at–0.45 V vs.RHE in 0.1 mol/L Na_(2)SO_(4).

关键词： MoSe_(2)nanosheets Doping Se vacancies Mo-N_(2)interaction Electrocatalysis NH_(3)synthesis