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nanotechnology and Precision Engineering 2024年第3期7卷 71-78页

作者： wei Zhao Zongwei Xu Pengfei Wang Hanyi Chen State Key Laboratory of Precision Measuring Technology and Instruments Tianjin UniversityTianjin 300072China Department of Modern Physics University of Science and Technology of ChinaHefei 230026China

nitrogen vacancy(nV)color centers in diamond have useful applications in quantum sensing andﬂuorescent *** can be gen-erated experimentally by ion implantation,femtosecond lasers,and chemical vapor ***,there is a lack of studies of the yield of nV color centers at the atomic *** the molecular dynamics simulations described in this paper,nV color centers are pre-pared by ion implantation in diamond with pre-doped nitrogen and subsequent *** differences between the yields of nV color centers produced by implantation of carbon(C)and nitrogen(n)ions,respectively,are *** is found that C-ion implantation gives a greater yield of nV color centers and superior location *** effects of different pre-doping concentrations(400–1500 ppm)and implantation energies(1.0–3.0 keV)on the nV color center yield are analyzed,and it is shown that a pre-doping concentra-tion of 1000 ppm with 2 keV C-ion implantation can produce a 13%yield of nV color centers after 1600 K annealing for 7.4 ***,a brief comparison of the nV color center identiﬁcation methods is presented,and it is found that the error rate of an analysis utiliz-ing the identify diamond structure coordination analysis method is reduced by about 7%compared with conventional identiﬁcation+methods.

关键词： nV color center Ion implantation Molecular dynamics(MD)simulation Yield enhancement

Reduced-order modeling and vibration transfer analysis of a fluid-delivering branch pipeline that consider fluid–solid interactions

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Frontiers of Mechanical Engineering 2024年第2期19卷 75-97页

作者： Wenhao JI Hongwei MA wei SUn Yinhang CAO School of Mechanical Engineering and Automation Northeastern UniversityShenyang 110819China Key Laboratory of Vibration and Control of Aero-Propulsion Systems(Ministry of Education) Northeastern UniversityShenyang 110819China College of Power and Energy Engineering Harbin Engineering UniversityHarbin 150001China

The efficient dynamic modeling and vibration transfer analysis of a fluid-delivering branch pipeline(FDBP)are essential for analyzing vibration coupling effects and implementing vibration reduction ***,this study proposes a reduced-order dynamic modeling method suitable for FDBPs and then analyzes the vibration transfer *** the modeling method,the finite element method and absorbing transfer matrix method(ATMM)are integrated,considering the fluid–structure coupling effect and fluid *** dual-domain dynamic substructure method is developed to perform the reduced-order modeling of FDBP,and ATMM is adopted to reduce the matrix order when solving fluid ***,the modeling method is validated by experiments on an H-shaped branch ***,transient and steady-state vibration transfer analyses of FDBP are performed,and the effects of branch locations on natural characteristics and vibration transfer behavior are *** show that transient vibration transfer represents the transfer and conversion of the kinematic,strain,and damping energies,while steady-state vibration transfer characteristics are related to the vibration *** addition,multiple-order mode exchanges are triggered when branch locations vary in frequency-shift regions,and the mode-exchange regions are also the transformation ones for vibration transfer patterns.

关键词： fluid-delivering branch pipeline vibration transfer analysis reduced-order modeling fluid-solid interactions finite element method absorbing transfer matrix method

Active MoS_(2)-based electrode for green ammonia synthesis

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Chinese Journal of Chemical Engineering 2024年第1期65卷 268-275页

作者： Xin Liu Lei Yang Tao wei Shanping Liu Beibei Xiao School of Energy and Power Engineering Jiangsu University of Science and TechnologyZhenjiang 212003China Institute Charles Gerhardt Montpellier UMR-5253Universite de MontpellierCNRSENSCMPlace E.Bataillon34095 Montpellier Cedex 05France

nitrogen electro-reduction under mild conditions is one promising alternative approach of the energyconsuming Haber-Bosch process for the artificial ammonia *** critical aspect to unlocking this technology is to discover the catalysts with high selectivity and *** this work,the n_(2)-to-nH_(3)conversion on the functional MoS_(2)is fully investigated by density functional theory calculations since the layered MoS_(2)provides the ideal platform for the elaborating copies of the nitrogenase found in nature,wherein the functionalization is achieved via basal-adsorption,basal-substitution or edge-substitution of transition metal *** results reveal that the edge-functionalization is a feasible strategy for the activity promotion;however,the basal-adsorption and basal-substitution separately suffer from the electrochemical instability and the nRR ***,MoS_(2)functionalized via edge W-substitution exhibits an exceptional *** energetically favored reaction pathway is through the distal pathway and a limiting potential is less than 0.20 ***,this work escalates the rational design of the high-effective catalysts for nitrogen fixation and provides the explanation why the predicated catalyst have a good performance,paving the guidance for the experiments.

关键词： nitrogen reduction reaction Density functional theory calculations Molybdenum disulfide Electrochemistry Catalyst Thermodynamics

Processing of a low-costγ-γ'niPtAl coating with improved oxidation resistance

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Rare Metals 2024年第6期43卷 2832-2841页

作者： Yan Jiang Liang-Liang wei Jian He Hong-Bo Guo School of Materials Science and Engineering Beihang UniversityBeijing 100191China Key Laboratory of High-Temperature Structural Materials and Protective Coatings Ministry of Industry and Information TechnologyBeihang UniversityBeijing 100191China

A novelγ-γ'(ni solid solution—ni_(3)Al)niPtAl coating was produced on advanced single-crystal(SC)superalloy n5 by electroplating of a thin Pt coating with~3μm in thickness followed by heat treatment at 1000℃in *** comparison,a traditionalγ-γ'niPtAl coating was also produced by electroplating of a thick Pt coating with~6μm in thickness followed by heat treatment at 1100℃in *** novel coating has a mass gain of~0.5 mg·cm^(-2)after 100 h 1-h cyclic oxidation at 1150℃,showing better oxidation resistance than the traditional *** oxide scale mostly consisting ofα-Al_(2)O_(3)grew on the novel coating because the element Cr from the SC alloy substrate contributes to the formation ofα-Al_(2)O_(3).Pt content in the novel coating has significant effect on the oxidation *** optimized Pt content in the coating is about 16 at%,which is helpful to reduce the diffusion of harmful elements from the substrate into the coating but also to reduce the cost of the coating.

关键词： γ-γ'niPtAl coating Platinum Oxidation Al_(2)O_(3) Superalloy

Characterization of Fe-containing particles in Chengdu,southwest China,using single-particle aerosol mass spectrometry

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Journal of Environmental Sciences 2024年第2期136卷 110-120页

作者： Renjiang He Junke Zhang Luyao Chen wei Zhang Yingwei Xi School of Public Health Southwest Medical UniversityLuzhou 646000China Faculty of Geosciences and Environmental Engineering Southwest Jiaotong UniversityChengdu 611756China Sichuan Environmental Monitoring Center Chengdu 610074China

Single-particle aerosol mass spectrometry was used to study the characteristics of Fecontaining particles during winter in Chengdu,southwest *** mass concentrations of PM_(2.5)and PM_(10)during the study period were 64±38 and 89±49μg/m~3,respectively,and nO_(2)and particulate matter were high compared with most other regions of *** Fecontaining particles were divided into seven categories with different mass spectra,sources and aging *** highest contribution was from Fe mixed with carbonaceous components(Fe-C,23.1%)*** was more mixed with sulfate than nitrate and therefore the contribution of Fe mixed with sulfate(Fe-S,20.7%)particles was higher than that of Fe mixed with nitrate(Fe-n,12.5%)*** contributions from Fe-containing particles related to primary combustion were high in the small particle size range,whereas aged Fecontaining particles and dust-related particles were mostly found in the coarse particle size *** air masses mainly originated from the west and east of Chengdu,and the corresponding PM_(2.5)concentrations were 79±36 and 55±36μg/m~3,*** west and east air masses showed stronger contributions of Fe-containing particles related to biomass burning(Fe-B)and fossil fuel combustion(Fe-C and Fe-S)particles,*** southwest area contributed the most Fe-containing *** assessments of the effects of Fe-containing particles during heavy pollution period should pay more attention to Fe-C and Fe-S ***-reduction of Fe-containing particles should consider both local emissions and short-distance transmission from the surrounding areas.

关键词： Fe-containing particles Particle composition Potential source areas Evolution Chengdu

Tungsten oxide/nitrogen-doped carbon nanotubes composite catalysts for enhanced redox kinetics in lithium-sulfur batteries

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Chinese Journal of Chemical Engineering 2024年第3期67卷 58-67页

作者： Deqing He Zihao Xie Qian Yang wei Wang Chao Su School of Energy and Power Jiangsu University of Science and TechnologyZhenjiang 212100China State Key Laboratory of Materials-Oriented Chemical Engineering College of Chemical EngineeringNanjing Tech UniversityNanjing 211816China

The sluggish redox kinetics of polysulfides in lithium-sulfur(Li-S)batteries are a significant obstacle to their widespread adoption as energy storage ***,recent studies have shown that tungsten oxide(WO_(3))can facilitate the conversion kinetics of polysulfides in Li-S ***,we fabricated host materials for sulfur using nitrogen-doped carbon nanotubes(n-CnTs)and WO_(3).We used low-cost components and simple procedures to overcome the poor electrical conductivity that is a disadvantage of metal *** composites of WO_(3) and n-CnTs(WO_(3)/n-CnTs)create a stable framework structure,fast ion diffusion channels,and a 3D electron transport network during electrochemical reaction *** a result,the WO_(3)/n-CnT-Li2S6 cathode demonstrates high initial capacity(1162 mA·h·g^(-1) at 0.5℃),excellent rate performance(618 mA·h·g^(-1) at 5.5℃),and a low capacity decay rate(0.093%up to 600 cycles at 2℃).This work presents a novel approach for preparing tungsten oxide/carbon composite catalysts that facilitate the redox kinetics of polysulfide conversion.

关键词： Li-S batteries Composites Ion diffusion channels 3D electron transport network Redox kinetics

Self-assembled VS_(2) microflowers buffering volume change during charging and discharging towards high-performance zinc ion batteries

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Journal of Materials Science & Technology 2024年第6期173卷 107-113页

作者： Tingsheng Wang Wujie Gao Yuanxi Zhao Songcan Wang wei Huang Frontiers Science Center for Flexible Electronics Xi’an Institute of Flexible Electronics(IFE)Northwestern Polytechnical UniversityXi’an 710072China Key Laboratory of Flexible Electronics of Zhejiang Province Ningbo Institute of Northwestern Polytechnical UniversityNingbo 315103China School of Materials Science and Engineering Northwestern Polytechnical UniversityXi’an 710072China

VS_(2) has attracted increasing attention as a cathode material for aqueous zinc ion batteries because of its proper large layer spacing,weak interlayer interactions,multiple valence states of V,and excellent electrical conductivity,but its large volume change during charging and discharging leads to poor cycling ***,we report a one-step hydrothermal synthesis of VS_(2) microflowers with proper lamellar spacing,which provides a stable framework for the insertion/deinsertion of zinc ions and enhances the cycling stability,delivering an initial charge capacity of 128.3 mAh g^(-1) at 3 A g^(-1) and maintains a charge capacity of 100.1 mAh g^(-1) after 900 *** addition,the optimized VS_(2) cathode shows specific capacities of 215.7 and 150.5 mAh g^(-1) at the current densities of 0.1 and 2 A g^(-1),respectively,demonstrating that the microflower structure with a high specific surface area and a short diffusion distance also significantly enhances the rate performance.

关键词： Vanadium sulfide Microflower Zinc ion batteries Cathode materials Volume change

Promoted surface charge density from interlayer Zn–n_(4) configuration in carbon nitride for enhanced CO_(2) photoreduction

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nano Research 2024年第4期17卷 2400-2409页

作者： Xianjin Shi Yu Huang Gangqiang Zhu wei Peng Meijuan Chen State Key Laboratory of Loess and Quaternary Geology(SKLLQG) Key Laboratory of Aerosol Chemistry and PhysicsInstitute of Earth EnvironmentChinese Academy of SciencesXi’an 710061China Center of Excellence in Quaternary Science and Global Change Chinese Academy of SciencesXi’an 710061China University of Chinese Academy of Sciences Beijing 100049China School of Physics and Information Technology Shaanxi Normal UniversityXi’an 710062China School of Human Settlements and Civil Engineering Xi’an Jiaotong UniversityXi’an 710049China

The solar-driven reduction of CO_(2) into valuable products is a promising method to alleviate global environmental problems and energy ***,the low surface charge density limits the photocatalytic conversion performance of CO_(2).Herein,a polymeric carbon nitride(PCn)photocatalyst with Zn single atoms(Zn1/Cn)was designed and synthesized for CO_(2) *** results of the CO_(2) photoreduction studies show that the CO and CH_(4) yields of Zn1/Cn increased fivefold,reaching 76.9 and 22.9μmol/(g·h),respectively,in contrast to the unmodified ***+plasma-etched X-ray photoelectron spectroscopy and synchrotron radiation-based X-ray absorption fine structure results reveal that Zn single atom is mainly present in the interlayer space of PCn in the Zn–n_(4) *** characterizations indicate that the interlayer Zn–n_(4) configuration can amplify light absorption and establish an interlayer charge transfer ***-assisted Kelvin probe force microscopy confirms that more photogenerated electrons are delivered to the catalyst surface through interlayer Zn–n_(4) configuration,which increases its surface charge ***,in-situ infrared spectroscopy combined with density functional theory calculation reveals that promoted surface charge density accelerates key intermediates(*COOH)conversion,thus achieving efficient CO_(2) *** work elucidates the role of internal single atoms in catalytic surface reactions,which provides important implications for the design of single-atom catalysts.

关键词： single-atom catalysts photocatalytic CO_(2)reduction interlayer modification charge transfer dynamics surface charge density

Energy-efficient joint UAV secure communication and 3D trajectory optimization assisted by reconfigurable intelligent surfaces in the presence of eavesdroppers

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Defence Technology（防务技术） 2024年第1期31卷 537-543页

作者： Huang Hailong Mohsen Eskandari Andrey V.Savkin wei ni The Department of Aeronautical and Aviation Engineering The Hong Kong Polytechnic UniversityHong KongChina School of Electrical Engineering and Telecommunications University of New South WalesSydney2052Australia Data61 CSIROAustralia

We consider a scenario where an unmanned aerial vehicle(UAV),a typical unmanned aerial system(UAS),transmits confidential data to a moving ground target in the presence of multiple *** friendly reconfigurable intelligent surfaces(RISs) help to secure the UAV-target communication and improve the energy efficiency of the *** formulate an optimization problem to minimize the energy consumption of the UAV,subject to the mobility constraint of the UAV and that the achievable secrecy rate at the target is over a given *** present an online planning method following the framework of model predictive control(MPC) to jointly optimize the motion of the UAV and the configurations of the *** effectiveness of the proposed method is validated via computer simulations.

关键词： Unmanned aerial systems(UASs) Unmanned aerial vehicle(UAV) Communication security Eaves-dropping Reconfigurable intelligent surfaces(RIS) Autonomous navigation and placement Path planning Model predictive control

A comparative investigation on wear behaviors of physical and chemical vapor deposited bronze coatings for hydraulic piston pump

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Chinese Journal of Aeronautics 2024年第3期37卷 391-403页

作者： wei HAO Andrews LARBI Hongkang DOnG Dongyun WAnG Shenghu LI Zhejiang Provincial Key Laboratory of Urban Rail Transit Intelligent Operation and Maintenance Technology and Equipment Zhejiang Normal UniversityJinhua 321004China College of Engineering Zhejiang Normal UniversityJinhua 321004China Hangzhou Lilong Hydraulic Co. LtdHangzhou 311200China

The cylinder block/valve plate interface is one of the most critical frictional interfaces of the swashplate-type axial piston ***,the poor lubrication interface caused rapid wear and high friction loss in an elastohydrodynamic lubrication system,decreasing the pump *** resistant bronze coatings were fabricated on 38CrMoAl substrate by Physical Vapor Deposition(PVD)and Chemical Vapor Deposition(CVD),***-on-disc wear tests were performed to comparatively investigate the wear behaviors of the coatings and bulk ductile iron *** can be found that the PVD-bronze coating exhibited better wear resistance than the other two *** enhanced wear resistance was attributed to the unique composite microstructure and desired mechanical strength,which could resist to mechanical shear and spallation,decreasing friction *** appropriate hardness of(1.33±0.07)GPa could be beneficial for enhancing its wear *** PVD-bronze coating possessed a much lower and stable coefficient of friction(about 0.1)and wear rate(about 6000μm3.n-1.m-1)under the loading forces of about 100 n after 20 *** wear mechanism was the abrasive wear.

关键词： Aircraft hydraulic pump Bronze Coatings Wear resistance Mechanisms