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Li-Rich Organosulfur Cathode with Boosted Kinetics for High-Energy Lithium-Sulfur Batteries

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Energy & Environmental Materials 2024年第4期7卷 118-125页

作者： Ting Ma Jiaojiao Deng Yuxiao Lin Qinghua liang liang Hu Xiaohu wang Jun Liu Xinsheng Zhao Yinwei Li Ding nan Xiaoliang Yu College of Chemistry and Chemical Engineering Inner Mongolia University Inner Mongolia Key Laboratory of Graphite and Graphene for Energy Storage and Coating School of Materials Science and Engineering Inner Mongolia University of Technology Shenzhen Key Laboratory on Power Battery Safety and Shenzhen Geim Graphene center Tsinghua Shenzhen International Graduate School (SIGS) School of physics and Electronic Engineering Jiangsu Normal University Key Laboratory of Rare Earth Ganjiang Innovation Academy Chinese Academy of Sciences department of Mechanical Engineering Research Institute for Smart EnergyThe Hong Kong Polytechnic University

Organosulfur materials containing sulfur-sulfur bonds are an emerging class of high-capacity cathodes for lithium ***,it remains a great challenge to achieve rapid conversion reaction kinetics at practical testing conditions of high cathode mass loading and low electrolyte *** this study,a Li-rich pyrolyzed polyacrylonitrile/selenium disulfide（pPAN/Se2S3） composite cathode is synthesized by deep lithiation to address the above challenges.

关键词： Electrolytes

Latest cosmological constraints on Cardassian expansion models including the updated gamma-ray bursts

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Research in Astronomy and astrophysics 2011年第9期11卷 1019-1030页

作者： nan liang Pu-Xun Wu Zong-Hong Zhu department of Astronomy Beijing Normal University Beijing 100875 China center for High Energy physics Peking University Beijing 100871 China center of Nonlinear Science and department of physics Ningbo University Ningbo 315211 China

We constrain the Cardassian expansion models from the latest observa- tions, including the updated Gamma-ray bursts （GRBs）, which are calibrated using a cosmology independent method from the Union2 compilation of type Ia supernovae （SNe Ia）. By combining the GRB data with the joint observations from the Union2 SNe Ia set, along with the results from the Cosmic Microwave Background radia- tion observation from the seven-year Wilkinson Microwave Anisotropy Probe and the baryonic acoustic oscillation observation galaxy sample from the spectroscopic Sloan Digital Sky Survey Data Release. we find significant constraints on the model oarameters of the original Cardassian model ΩM0=0.282-0.014^0.015,n=0.03-0.05^＋0.05 and n=-0.16-3.26^＋0.25,β=0.76-0.58^＋0.34 of the modified polytropic Cardassian model, which are consistent with the ACDM model in a l-or confidence region. From the reconstruction of the deceleration parameter q（z） in Cardassian models, we obtain the transition redshift ZT = 0.73 ± 0.04 for the original Cardassian model and ZT = 0.68 ± 0.04 for the modified polytropic Cardassian model.

关键词： gamma-rays bursts -- cosmology cosmological parameters

Alloy strategy to synthesize Pt-early transition metal oxide interfacial catalysts

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nano Research 2024年第4期17卷 3390-3397页

作者： Shi-Long Xu Hang nan Wanqun Zhang Yue Lin Sheng-Qi Chu Hai-Wei liang Hefei National Research center for Physical Sciences at the Microscale Department of ChemistryUniversity of Science and Technology of ChinaHefei 230026China School of Materials and Chemical Engineering Anhui Jianzhu UniversityHefei 230601China Institute of High Energy physics Chinese Academy of SciencesBeijing 100049China

Metal oxide supported metal catalysts show promising catalytic performance in many industry-relevant ***,the enhancement of performance is often limited by the insufficient metal/metal oxide *** this work,we demonstrate a general synthesis of Pt-early transition metal oxide(Pt-MO_(x),M=Ti,Zr,V,and Y)catalysts with rich interfacial sites,which is based on the air-induced surface segregation and oxidation of M in the supported Pt-M alloy *** characterizations verify the dynamic structural response of Pt-M alloy catalysts to air and the formation of Pt-MO_(x) catalysts with abundant interfacial *** prepared Pt-TiO_(x) interfacial catalysts exhibit improved performance in hydrogenation reactions of benzaldehyde,nitrobenzene,styrene,and furfural,as a result of the heterolytic dissociation of H_(2) at Pt-metal oxide interfacial sites.

关键词： Pt-early transition metal oxide interfacial catalyst alloy oxidation strategy interfacial sites hydrogenation reactions heterolytic dissociation

Spin Evolution of the Magnetar SGR J1935+2154

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Research in Astronomy and astrophysics 2024年第1期24卷 201-211页

作者： Ming-Yu Ge Yuan-Pei Yang Fang-Jun Lu Shi-Qi Zhou Long Ji Shuang-nan Zhang Bing Zhang liang Zhang Pei wang Kejia Lee Weiwei Zhu Jian Li Xian Hou Qiao-Chu Li Key Laboratory of Particle astrophysics Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China South-Western Institute For Astronomy Research Yunnan UniversityKunming 650504China Purple Mountain Observatory Chinese Academy of SciencesNanjing 210023China Key Laboratory of Stellar and Interstellar physics and School of physics and Optoelectronics Xiangtan UniversityXiangtan 411105China School of physics and Astronomy Sun Yat-Sen UniversityZhuhai 519082China university of Chinese Academy of Sciences Chinese Academy of SciencesBeijing 100049China Nevada center for astrophysics University of NevadaLas VegasNV 89154USA department of physics and Astronomy University of NevadaLas VegasNV 89154USA National Astronomical Observatories Chinese Academy of SciencesBeijing 100101China department of Astronomy Peking UniversityBeijing 100871China CAS Key Laboratory for Research in Galaxies and Cosmology Department of AstronomyUniversity of Science and Technology of ChinaHefei 230026China School of Astronomy and Space Science University of Science and Technology of ChinaHefei 230026China Yunnan Observatories Chinese Academy of SciencesKunming 650216China School of Astronomy and Space Science Nanjing UniversityNanjing 210023China Key laboratory of Modern Astronomy and astrophysics Nanjing UniversityNanjing 210023China

Fast radio bursts(FRBs)are short pulses observed in radio frequencies usually originating from cosmological *** discovery of FRB 200428 and its X-ray counterpart from the Galactic magnetar SGR J1935+2154suggests that at least some FRBs can be generated by ***,the majority of X-ray bursts from magnetars are not associated with radio *** fact that only in rare cases can an FRB be generated raises the question regarding the special triggering mechanism of *** we report long time spin evolution of SGR J1935+2154 until the end of *** to v and v,the spin evolution of SGR J1935+2154 could be divided into two *** first stage evolves relatively steady evolution until 2020 April *** the burst activity in2020,the spin of SGR J1935+2154 shows strong variations,especially for *** the burst activity in 2022October,a new spin-down glitch with△v/v=(-7.2±0.6)×10^(-6)is detected around MJD 59876,which is the second event in SGR J1935+*** the end,spin frequency and pulse profile do not show variations around the time of FRB 200428 and radio bursts 221014 and 221021,which supply strong clues to constrain the trigger mechanism of FRBs or radio bursts.

关键词： (stars:)pulsars:general (stars:)pulsars:individual(SGR J1935+2154) X-rays:bursts

Frontiers in high entropy alloys and high entropy functional materials

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Rare Metals 2024年第10期43卷 4639-4776页

作者： Wen-Tao Zhang Wen Huang Fu-Jie Yu Qi Zhao Xin-Dong Zhu Tao Feng Yao Jiang Xiao-Ming Li Xue-Fei Miao He Zhu Si Lan Xue-Qian wang Bao-Long Shen Zhe Jia Feng-Qi Zhang Wei wang Qi Liu Yang Ren Xun-Li wang Xiao-Ya Cui Xiao-Yang wang Ya-nan Chen Bing-Bing Fan Meng-Ru Li Qi-Long Gao Jia-Ming Guo Zeng-Bao Jiao Zhi-Min Guo Yu-Ping Zhao Qian Yu Rui Huang Ling-Kun Zhang Yi-Ping Lu Xu-Bo Li Huai-Jun Lin Yan Ma Wei-Ming Yang Zhi-Hua Shen Hai-Yan He Yong-Gang Sun Yong-Jiang Huang De-Zhuang wang Qing-Feng Liu Fei-Yang wang Hui Liu Hong-Hui Wu Li-Qiang wang Yang Lu nan wang Tian-Li wang Wei-Bing Liao Yi-Han wang Yuan Wu Yu-Zhen Yin Jie Pan Yi Zhang Qing wang Jian-Yang Zhang Tao Yang Yasir Sohail Jin-Yu Zhang Hua Ji Qiang Li Wei-Di Liu Zhi-Gang Chen Xiong-Jun Liu Wen Ma liang Mao Zhen-Duo Wu School of Materials Science and Engineering Nanjing University of Science and Technology Jiangsu Key Laboratory for Advanced Metallic Materials School of Materials Science and Engineering Southeast University department of physics City University of Hong Kong School of Materials Science and Engineering Tianjin University School of physics and Microelectronics Zhengzhou University department of Mechanical Engineering Research Institute for Advanced Manufacturing The Hong Kong Polytechnic University center of Electron Microscopy and State Key Laboratory of Silicon Materials School of Materials Science and Engineering Zhejiang University Key Laboratory of Solidification Control and Digital Preparation Technology (Liaoning Province) School of Materials Science and Engineering Dalian University of Technology Institute of Advanced Wear & Corrosion Resistance and Functional Materials Jinan University School of Mechanics and Civil Engineering China University of Mining and Technology School of Physical Sciences Great Bay University School of Materials Science andEngineering Harbin Institute of Technology State Key Laboratory of Materials-Oriented Chemical Engineering College of Chemical Engineering Nanjing Tech University beij.ng Advanced Innovation center for Materials Genome Engineering Research Institute for Carbon Neutrality University of Science and Technology Beijing department of Mechanical Engineering The University of Hong Kong School of Computing Macquarie University Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province College of Physics and Optoelectronic Engineering Shenzhen University State Key Laboratory for Advanced Metals and Materials University of Science and Technology Beijing State Key Laboratory of Materials Processing and Die & Mould Technology School of Materials Science and Engineering Huazhong University of Science and Technology Institute of materials Shanghai University department of Materials Science and Engineering C

Owing to their exceptional properties, high-entropy alloys(HEAs) and high-entropy materials have emerged as promising research areas and shown diverse applications. Here,the recent advances in the field are comprehensively reviewed,organized into five sections. The first section introduces the background of HEAs, covering their definition, significance,application prospects, basic properties, design principles, and microstructure. The subsequent section focuses on cutting-edge high-entropy structural materials, highlighting developments such as nanostructured alloys, grain boundary engineering,eutectic systems, cryogenic alloys, thin films, micro-nano-lattice structures, additive manufacturing, high entropy metallic glasses, nano-precipitate strengthened alloys, composition modulation, alloy fibers, and refractory systems. In the following section, the emphasis shifts to functional materials, exploring HEAs as catalysts, magneto-caloric materials, corrosion-resistant alloys, radiation-resistant alloys, hydrogen storage systems, and materials for biomedicine. Additionally, the review encompasses functional high-entropy materials outside the realm of alloys, including thermoelectric, quantum dots, nanooxide catalysts, energy storage materials, negative thermal expansion ceramics,and high-entropy wave absorption materials. The paper concludes with an outlook, discussing future directions and potential growth areas in the field. Through this comprehensive review,researchers, engineers, and scientists may gain valuable insights into the recent progress and opportunities for further exploration in the exciting domains of high-entropy alloys and functional materials.

关键词： Cutting-edge structural materials Cutting-edgefunctional materials High entropy alloys

Testing the distance-duality relation with a combination of cosmological distance observations

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Research in Astronomy and astrophysics 2011年第10期11卷 1199-1208页

作者： Shuo Cao nan liang department of Astronomy Beijing Normal University Beijing 100875 China center for High Energy physics Peking University Beijing 100871 China

We propose an accurate test of the distance-duality （DD） relation, η = DL（z）（1 ＋ z）^-2/DA（z） = 1 （where DL and DA are the luminosity distances and angular diameter distances, respectively）, with a combination of cosmological observational data of Type Ia Supernovae （SNe Ia） from the Union2 set and the galaxy cluster sample under an assumption of the spherical model. In order to avoid bias brought on by redshift non-coincidence between observational data and to consider redshift error bars of both clusters and SNe Ia in the analysis, we carefully choose the SNe Ia points which have the minimum acceptable redshift difference of the galaxy cluster sample （│△Z│min = σz,SN ＋σz,cluster）. By assuming η to be a constant and defined as functions of the redshift parameterized by six different expressions, we find that there exists no observable evidence for variations in the DD relation based on the collected data, since related statistical tests are well satisfied within the 1σ confidence level for most cases. Further, considering different values of △z as constraints, we also find that the choice of △z may play an important role in this model-independent test of the DD relation for the spherical sample of galaxy clusters.

关键词： distance scale -- galaxies clusters general -- supernovae general

The role of strain and polar discontinuity in magnetism in LaMnO_3/SrTiO_3/LaAlO_3(001) heterostructures

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Science Bulletin 2018年第15期63卷 949-951页

作者： liang Wu Changjian Li Jing Ma Cewen nan X.Renshaw wang School of Materials Science and Engineering State Key Laboratory of New Ceramics and Fine Processing Tsinghua University department of Materials Science and Engineering National University of Singapore School of Physical and Mathematical Sciences & School of Electrical and Electronic Engineering Nanyang Technological University

Creating novel interfacial effects in quantum-matter-based heterostructures is at the heart of condensed matter physics and materials science[1].Utilizing the subtle interplay among charge,spin,orbit and lattice degrees of freedom,these interfacial effects can spawn tailored functionalities and act as additional building blocks for the future oxide *** the various interfacial effects,the inevitable strain effect induced by unequal lattice constants and the ubiquitous charge redistribution effect at inter-

关键词：磁力材料科学电子学氧化物物理格子

The In-Flight Realtime Trigger and Localization Software of GECAM

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Research in Astronomy and astrophysics 2024年第10期24卷 11-24页

作者： Xiao-Yun Zhao Shao-Lin Xiong Xiang-Yang Wen Xin-Qiao Li Ce Cai Shuo Xiao Qi Luo Wen-Xi Peng Dong-Ya Guo Zheng-Hua An Ke Gong Jin-Yuan Liao Yan-Qiu Zhang Yue Huang Lu Li Xing Wen Fei Zhang Jing Duan Chen-Wei wang Dong-Li Shi Peng Zhang Qi-Bin Yi Chao-Yang Li Yan-Bing Xu Xiao-Hua liang Ya-Qing Liu Da-Li Zhang Xi-Lei Sun Fan Zhang Gang Chen Huan-Yu wang Sheng Yang Xiao-Jing Liu Min Gao Mao-Shun Li Jin-Zhou wang Xing Zhou Yi Zhao wang-Chen Xue Chao Zheng Jia-Cong Liu Xing-Bo Han Jin-Ling Qi Jia Huang Ke-Ke Zhang Can Chen Xiong-Tao Yang Dong-Jie Hou Yu-Sa wang Rui Qiao Xiang Ma Xiao-Bo Li Ping wang Xin-Ying Song Li-Ming Song Shi-Jie Zheng Bing Li Hong-Mei Zhang Yue Zhu Wei Chen Jian-Jian He Zhen Zhang Jin Hou Hong-Jun wang Yan-Chao Hao Xiang-Yu wang Zong-Yuan Yang Zhi-Long Wen Zhi Chang Yuan-Yuan Du Rui Gao Xiao-Fei Lan Yan-Guo Li Gang Li Xu-Fang Li Fang-Jun Lu Hong Lu Bin Meng Feng Shi Hui wang Hui-Zhen wang Yu-Peng Xu Jia-Wei Yang Xue-Juan Yang Shuang-nan Zhang Chao-Yue Zhang Cheng-Mo Zhang Zhi-Cheng Tang Cheng Cheng Key Laboratory of Particle astrophysics Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China university of Chinese Academy of Sciences Chinese Academy of SciencesBeijing 100049China School of Information Science and Technology Southwest Jiaotong UniversityChengdu 611756China Key Laboratory of Stellar and Interstellar physics and department of physics Xiangtan UniversityXiangtan 411105China physics and Space Science College China West Normal UniversityNanchong 637002China department of Astronomy Beijing Normal UniversityBeijing 100875China Innovation Academy for Microsatellites of CAS Shanghai 201203China Changchun university of Science and Technology Changchun 130022China Chinese Academy of Sciences South America center for Astronomy National Astronomical ObservatoriesCASBeijing 100101China

Realtime trigger and localization of bursts are the key functions of GECAM,an all-sky gamma-ray monitor launched on 2020 December *** developed a multifunctional trigger and localization software operating in the CPU of the GECAM Electronic *** onboard software has the following features:high trigger efficiency for real celestial bursts with a suppression of false triggers caused by charged particle bursts and background fluctuation,dedicated localization algorithm optimized for both short and long bursts,and low time latency of the trigger information which is downlinked through the Global Short Message Communication service of the global BeiDou navigation *** paper provides a detailed description of the design and development of the trigger and localization software system for *** covers the general design,workflow,the main functions,and the algorithms used in the *** paper also includes on-ground trigger tests using simulated gamma-ray bursts generated by a dedicated X-ray tube,as well as an overview of the performance for real celestial bursts during its in-orbit operation.

关键词： telescopes instrumentation:detectors methods:observational

Acceleration of bidirectional sulfur conversion kinetics and inhibition of lithium dendrites growth via a“ligand-induced”transformation strategy

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nano Research 2023年第7期16卷 9496-9506页

作者： Wei Zhou Minzhe Chen Dengke Zhao Jiacheng Dan Chuheng Zhu Wen Lei Li-Jun Ma nan wang Xinghua liang Ligui Li New Energy Research Institute School of Environment and EnergySouth China University of TechnologyHigher Education Mega CenterGuangzhou 510006China The State Key Laboratory of Refractories and Metallurgy Wuhan University of Science and TechnologyWuhan 430081China Key Laboratory of Theoretical Chemistry of Environment Ministry of Education School of Chemistry and EnvironmentSouth China Normal UniversityGuangzhou 510631China Siyuan laboratory Guangzhou Key Laboratory of Vacuum Coating Technologies and New Energy MaterialsDepartment of PhysicsJinan UniversityGuangzhou 510632China Guangxi Key Laboratory of Automobile Components and Vehicle Technology Guangxi University of Science and TechnologyLiuzhou 545006China

The introduction of materials with dual-functionalities,i.e.,the catalytic(adsorption)features to inhibit shuttle effects at the cathode side,and the capability to facilitate homogenous Li-ion fluxes at the anode side,is a promising strategy to realize high performance lithium-sulfur batteries(LSBs).Herein,a facile and rational organic“ligand-induced”(trimesic acid(TMA))transformation tactic is proposed,which achieves the regulation of electronic performance and d-band center of bimetallic oxides(NiFe_(2)O_(4))to promote bidirectional sulfur conversion kinetics and stabilize the Li plating/striping during the charge/discharge *** battery assembled with NiFe_(2)O_(4)-TMA modified separator exhibits a remarkable initial specific capacity of 1476.6 mAh·g^(-1)at 0.1 C,outstanding rate properties(661.1 mAh·g^(-1)at 8.0 C),and excellent cycling ***“ligand-induced”transformation tactic proposed in this work will open a whole new possibility for tuning the electronic structure and d-band center to enhance the performance of LSBs.

关键词： organic“ligand-induced”transformation NiFe_(2)O_(4)-trimesic acid(TMA) bidirectional sulfur conversion high sulfur loading