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Coupling of Adhesion and Anti‑Freezing Properties in Hydrogel Electrolytes for Low‑Temperature Aqueous‑Based Hybrid Capacitors

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Nano-Micro Letters 2024年第2期16卷 15-31页

作者： Jingya Nan Yue sun Fusheng Yang Yijing Zhang Yuxi Li Zihao wang Chuchu wang Dingkun wang Fuxiang Chu Chunpeng wang Tianyu Zhu Jianchun Jiang Institute of Chemical Industry of Forest Products Chinese Academy of ForestryKey Laboratory of Biomass Energy and MaterialJiangsu ProvinceNanjing 210042JiangsuPeople’s Republic of China Co‑Innovation Center of Efficient Processing and Utilization of Forest Resources Nanjing Forestry UniversityNanjing 210037JiangsuPeople’s Republic of China Energy Technologies Area Lawrence Berkeley National LaboratoryBerkeleyCA 94720USA Department of Materials science and Engineering Clemson UniversityClemsonSC 29634USA

solid-state zinc-ion capacitors are emerging as promising candidates for large-scale energy storage owing to improved safety,mechanical and thermal stability and easy-to-direct *** electrolytes are appealing solid-state electrolytes because of eco-friendliness,high conductivity and intrinsic ***,the electrolyte/electrode interfacial contact and anti-freezing properties of current hydrogel electrolytes are still challenging for practical applications of zinc-ion ***,we report a class of hydrogel electrolytes that couple high interfacial adhesion and anti-freezing *** synergy of tough hydrogel matrix and chemical anchorage enables a well-adhered interface between hydrogel electrolyte and ***,the cooperative solvation of ZnCl2 and LiCl hybrid salts renders the hydrogel electrolyte high ionic conductivity and mechanical elasticity simultaneously at low *** significantly,the Zn||carbon nanotubes hybrid capacitor based on this hydrogel electrolyte exhibits low-temperature capacitive performance,delivering high-energy density of 39 Wh kg^(-1)at-60°C with capacity retention of 98.7%over 10,000 *** the benefits of the well-adhered electrolyte/electrode interface and the anti-freezing hydrogel electrolyte,the Zn/Li hybrid capacitor is able to accommodate dynamic deformations and function well under 1000 tension cycles even at-60°*** work provides a powerful strategy for enabling stable operation of low-temperature zinc-ion capacitors.

关键词： Interfacial adhesion Anti-freezing Hydrogel electrolytes Low-temperature hybrid capacitors Dynamic deformati

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Microstructural evolution and deformation behavior of friction stir welded twin-induced plasticity steel

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Journal of Materials science & Technology 2024年第2期169卷 68-81页

作者： Ke Qiao Kuaishe wang Jia wang Zhengyang Hao Yating Xiang Peng Han Jun Cai Qi Yang Wen wang school of Metallurgical Engineering National and Local Joint Engineering Research Center for Functional Materials ProcessingXi’an University of Architecture and TechnologyXi’an 710055China shanghai Research Institute of Materials Shanghai 200437China

The weldability of twin-induced plasticity(TWIP)steel with ultra-high strength via friction stir welding(FsW)technique was investigated,and microstructural evolution and deformation behavior of whole and micro-zones of FsW TWIP joint were studied for the first *** results showed that the content of recrystallized grains in the stir zone(sZ)increased from 10.5%of basal material(BM)to 14.2%,and that of heat affected zone(HAZ)increased to 78.6%.The percentage of annealing twins decreased from 26.8%in BM to 11%in sZ,while increased to 35%in *** with the BM,the ultimate tensile strength and yield strength of the FsW joint increased to 1036 and 550 MPa,respectively,reaching 106.7%and 110.9%of BM,*** elongation of the entire joint was 50.5%,which was lower than that of BM due to the nonuniform deformation during the tensile *** engineering strain was mainly concentrated in BM and sZ and transferred to each other during the tensile test,while the engineering strain in HAZ was always the ***,the tensile fracture occurred in the *** order of ultimate tensile strength of micro-zones in the FsW joint was as follows:HAZ>BM≈*** order of yield strength was as follows:HAZ>BM>sZ.

关键词： Twin-induced plasticity steel Friction stir welding Microstructure Mechanical property Deformation behavior

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A cascade of in situ conversion of bicarbonate to CO_(2) and CO_(2) electroreduction in a flow cell with a Ni-N-s catalyst

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Journal of Energy Chemistry 2024年第1期88卷 183-193,I0005页

作者： Linghui Kong Min wang Yongxiao Tuo shanshan Zhou Jinxiu wang Guangbo Liu Xuejing Cui Jiali wang Luhua Jiang Nanomaterials and Electrocatalysis Laboratory College of Materials Science and EngineeringQingdao University of Science and TechnologyQingdao 266042ShandongChina state Key Laboratory of Heavy Oil Processing College of New EnergyChina University of Petroleum(East China)Qingdao 266580ShandongChina

Combination of CO_(2) capture using inorganic alkali with subsequently electrochemical conversion of the resultant HCO_(3)^(-)to high-value chemicals is a promising route of low cost and high *** electrochemical reduction of HCO_(3)^(-)is challenging due to the inaccessible of negatively charged molecular groups to the electrode ***,we adopt a comprehensive strategy to tackle this challenge,i.e.,cascade of in situ chemical conversion of HCO_(3)^(-)to CO_(2) and CO_(2) electrochemical reduction in a flow *** a tailored Ni-N-s single atom catalyst(sACs),where sulfur(s)atoms located in the second shell of Ni center,the CO_(2)electroreduction(CO_(2)ER)to CO is *** experimental results and density functional theory(DFT)calculations reveal that the introduction of s increases the p electron density of N atoms near Ni atom,thereby stabilizing^(*)H over N and boosting the first proton coupled electron transfer process of CO_(2)ER,i.e.,^(*)+e^(-)+^(*)H+^(*)CO_(2)→^(*)*** a result,the obtained catalyst exhibits a high faradaic efficiency(FE_(CO)~98%)and a low overpotential of 425 mV for CO production as well as a superior turnover frequency(TOF)of 47397 h^(-1),outcompeting most of the reported Ni *** importantly,an extremely high FECOof 90%is achieved at 50 mA cm^(-2)in the designed membrane electrode assembly(MEA)cascade electrolyzer fed with liquid *** work not only highlights the significant role of the second coordination on the first coordination shell of the central metal for CO_(2)ER,but also provides an alternative and feasible strategy to realize the electrochemical conversion of HCO_(3)^(-)to high-value chemicals.

关键词： s doped Ni-N-C single atom catalysts CO_(2)electrochemical reduction DFT calculations Membrane electrode assembly Reduction of bicarbonate

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Rapid lithium-ion insertion/extraction and migration behavior of Na_(2)WO_(4)-encapsulated lithium-rich layered oxide cathode

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Rare Metals 2024年第8期43卷 3647-3660页

作者： Yu-shen Zhao Fan-Fan wang Jian-Cang wang Peng-Fei wang Ting-Feng Yi Jun-Hong Zhang school of Materials science and Engineering Northeastern UniversityShenyangShenyang 110819China Key Laboratory of Dielectric and Electrolyte Functional Material Hebei Province School of Resources and MaterialsNortheastern University at QinhuangdaoQinhuangdao 066004China shandong Provincial Key Laboratory of Chemical Energy storage and Novel Cell Technology College of Chemistry and Chemical EngineeringLiaocheng UniversityLiaocheng 252059China

Due to the low cost,high working voltage and high storage capacity,Li-rich Mn-based layered compounds show promise as the cathode materials for lithiumion batteries(LIBs).However,the side reactions at the solid-liquid interface of the cathode will lead to rapid capacity decay and inferior rate ***,this article proposes a liquid-phase dispersion strategy to introduce a Na_(2)WO_(4)layer on the Li_(1.2)Ni_(0.13)-Co_(0.13)Mn_(0.54)O_(2) cathode,which can reduce the side effects between raw materials and electrolyte and promote the insertion/extraction rate of Li^(+),thus enhancing the material stability and rate *** a result,the capacity retention rate is 96.9%after 200 cycles under ***,the capacities are 177.5,149.5,111.1 and58.3 mAh·g^(-1)at 1C,2C,5C and 10C,implying a superior fast charging *** exceptional performance can be ascribed to both the increased conductivity and enhanced structural stability of the cathode ***'s more,based on the investigation of ion insertion/extraction behavior in electrode materials and the ion migration kinetics in the electrolyte,this study suggests that coating Li-rich Mn-based materials with Na_(2)WO_(4)can be a promising strategy to improve their performance in LIBs.

关键词： Li-ion battery Coating Rate performance Li_(1.2)Ni_(0.13)Co_(0.13)Mn_(0.54)O_(2) Reaction kinetics

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Differences and similarities in radial growth of Betula species to climate change

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Journal of Forestry Research 2024年第2期35卷 176-187页

作者： Di Liu Yang An Zhao Li Zhihui wang Yinghui Zhao Xiaochun wang Center for Ecological Research Key Laboratory of Sustainable Forest Ecosystem ManagementMinistry of EducationCollege of ForestryNortheast Forestry UniversityHarbin 150040People’s Republic of China Changan Park in shijiazhuang Shijiazhuang 050000People’s Republic of China shijiazhuang Landscape Greening Engineering Project Construction Center Shijiazhuang 050000People’s Republic of China Heilongjiang Institute of Meteorological science Harbin 150030People’s Republic of China school of Life Qufu Normal UniversityQufu 273100People’s Republic of China

Betula platyphylla and Betula costata are important species in mixed broadleaved-Korean pine(Pinus koraiensis)***,the specific ways in which their growth is affected by warm temperatures and drought remain *** address this issue,60 and 62 tree-ring cores of *** and *** were collected in Yichun,*** dendrochronological methods,the response and adaptation of these species to climate change were examined.A“hysteresis effect”was found in the rings of both species,linked to May–september moisture conditions of the previous *** growth of *** was positively correlated with the standardized precipitation-evapotranspiration index(sPEI),the precipitation from september to October of the previous year,and the relative humidity in October of the previous *** of *** is primarily restricted by moisture conditions from september to *** contrast,*** growth is mainly limited by minimum temperatures in May–June of both the previous and current *** droughts,*** had a faster recovery rate compared to *** the context of rising temperatures since 1980,the correlation between *** growth and monthly sPEI became positive and strengthened over time,while the growth of *** showed no conspicuous *** findings suggest that the growth of *** is already affected by warming temperatures,whereas *** may become limited if warming continues or *** change could disrupt the succession of these species,possibly accelerating the succession of pioneer *** results of this research are of great significance for understanding how the growth changes of birch species under warming and drying conditions,and contribute to understanding the structural adaptation of mixed broadleaved-Korean pine(Pinus koraiensis)forests under climate change.

关键词： Tree rings Betula platyphylla Betula costata Climate response Moving correlation Extreme drought

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Multi-spherical interactions and mechanisms of hydrocarbon enrichment in the southeast Asian archipelagic tectonic system

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science China Earth sciences 2024年第2期67卷 566-583页

作者： Rixiang ZHU Hongjun wang Huajian wang Xiaomei wang Bo WAN wang ZHANG Houqin ZHU Yuke LIU Junlai LIU Qingren MENG Fang HAO Zhijun JIN state Key Laboratory of Lithospheric Evolution Institute of Geology and GeophysicsChinese Academy of SciencesBeijing100029China state Key Laboratory of Enhanced Oil and Gas Recovery PetroChina Research Institute of Petroleum Exploration and DevelopmentBeijing100083China school of Earth sciences and Resources China University of GeosciencesBeijing100083China state Key Laboratory of Deep Oil and Gas China University of Petroleum(East China)Qingdao266580China Institute of Energy Peking UniversityBeijing100871China

Global cooling began since 50 Ma,but a warm climate was maintained in the archipelagic tectonic system in southeast Asia where a wealth of Cenozoic oil and gas resources was formed and *** the perspective of Earth system,this study analyzes Cenozoic tectonic activities,climatic and environmental evolution,and petroleum enrichment in southeast Asia,and provides the following insights:(1)subduction of oceanic plates and the extension of overlying continental lithosphere resulted in widespread volcanic eruptions as well as the formation of rift basins and shallow marine shelves,leading to complex interactions between deep tectonic processes and Earth’s surface including mountains,basins,and seas.(2)Microcontinental accretion and prolonged stay in equatorial low-latitude regions have changed trade winds into monsoons,altered ocean current pathways and flow rates,and profoundly affected rainfall and climate.(3)The archipelagic tectonic system,coupled with a hot and rainy climate,fostered tropical rainforests,mangroves,and phytoplankton,providing abundant organic matter and promoting the development of petroleum resources.(4)Combinations of rift basin development and marine transgression and regression led to an effective superposition of source-reservoir-seal combinations from multiplepetroleum *** deep burial of organic matter and high geothermal gradients facilitated the generation and large-scale accumulation of oil and gas.(5)Multi-spherical(such as atmosphere,biosphere,hydrosphere and lithosphere)interactions on the Earth,which resulted from the convergence of multiple tectonic plates,are believed as the primary driver for exceptional enrichments of Cenozoic oil and gas resources in southeast *** understandings are significant for developing theories of oil and gas enrichment under the guidance of Earth system *** order to continue making significant oil and gas exploration discoveries in the deep-layers,deep-waters,and unconventio

关键词： southeast Asia Archipelagic tectonic system Interactions of Earth’s spheres Oil and gas resources Cenozoic

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A New Industrial Intrusion Detection Method Based on CNN-BiLsTM

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Computers, Materials & Continua 2024年第6期79卷 4297-4318页

作者： Jun wang Changfu si Zhen wang Qiang Fu College of Computer science and Technology Shenyang University of Chemical TechnologyShenyang110142China

Nowadays,with the rapid development of industrial Internet technology,on the one hand,advanced industrial control systems(ICs)have improved industrial production ***,there are more and more cyber-attacks targeting industrial control *** ensure the security of industrial networks,intrusion detection systems have been widely used in industrial control systems,and deep neural networks have always been an effective method for identifying cyber *** intrusion detection methods still suffer from low accuracy and a high false alarm ***,it is important to build a more efficient intrusion detection *** paper proposes a hybrid deep learning intrusion detection method based on convolutional neural networks and bidirectional long short-term memory neural networks(CNN-BiLsTM).To address the issue of imbalanced data within the dataset and improve the model’s detection capabilities,the synthetic Minority Over-sampling Technique-Edited Nearest Neighbors(sMOTE-ENN)algorithm is applied in the preprocessing *** algorithm is employed to generate synthetic instances for the minority class,simultaneously mitigating the impact of noise in the majority *** approach aims to create a more equitable distribution of classes,thereby enhancing the model’s ability to effectively identify patterns in both minority and majority *** the experimental phase,the detection performance of the method is verified using two data *** results show that the accuracy rate on the CICIDs-2017 data set reaches 97.7%.On the natural gas pipeline dataset collected by Lan Turnipseed from Mississippi state University in the United states,the accuracy rate also reaches 85.5%.

关键词： Intrusion detection convolutional neural network bidirectional long short-term memory neural network multi-head self-attention mechanism

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Progress in systematics and biogeography of Orchidaceae

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Plant Diversity 2024年第4期46卷 425-434页

作者： Yajun wang Hanchen wang Chao Ye Zhiping wang Chongbo Ma Dongliang Lin Xiaohua Jin state Key Laboratory of Plant Diversity and specialty Crops Institute of Botanythe Chinese Academy of SciencesBeijing 100093China University of Chinese Academy of sciences Beijing 100093China China National Botanical Garden Beijing 100093China

Orchidaceae are one of the largest families of angiosperms in terms of species *** the last decade,numerous studies have delved into reconstructing the phylogenetic framework of Orchidaceae,leveraging data from plastid,mitochondrial and nuclear *** studies have provided new insights into the systematics,diversification and biogeography of Orchidaceae,establishing a robust foundation for future ***,pronounced controversies persist regarding the precise placement of certain lineages within these phylogenetic *** address these discrepancies and deepen our understanding of the phylogenetic structure of Orchidaceae,we provide a comprehensive overview and analysis of phylogenetic studies focusing on contentious groups within Orchidaceae since 2015,delving into discussions on the underlying reasons for observed topological *** also provide a novel phylogenetic framework at the subtribal ***,we examine the tempo and mode underlying orchid species diversity from the perspective of historical biogeography,highlighting factors contributing to extensive ***,we delineate avenues for future research aimed at enhancing our understanding of Orchidaceae phylogeny and diversity.

关键词： Diversification Orchid phylogenetics Phylogenetic conflicts Biogeography Taxonomy

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Oral administration of Bacillus coagulans TQ-35 alleviates allergic responses in OVA-sensitive BALB/c mice

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Food science and Human Wellness 2024年第3期13卷 1246-1257页

作者： Yifan wang shanjun Chen Chong wang Yi Zhang Hongliang Zeng Linglin Fu Yanbo wang Food safety Key Laboratory of Zhejiang Province School of Food Science and BiotechnologyZhejiang Gongshang UniversityHangzhou 310018China College of Food science Fujian Agriculture and Forestry UniversityFuzhou 350002China school of Food and Health Beijing Technology and Business UniversityBeijing 100048China

Bacillus coagulans has been extensively studied so far,but there has been a lack of research on its usage in *** this study,we designed to assess the effect of different concentrations of *** on food allergy in a BALB/c mouse model of ovalbumin(OVA)-induced food allergy and its effect on gut *** assessment of symptoms,specific immunoglobulin E(IgE),T-cell differentiation,and related gene expression levels in sensitized mice by assay indicated that high doses of oral *** could alleviate allergic *** with ***,in the high-dose group,significantly reduced IgE and IgG1 levels and modulated the balance of T helper type 1 cell(Th1)and Th2 and the expression of relevant genes in the spleen.16s rRNA analysis showed that probiotics improved the structure of the microbiota,in particular by boosting the percentage of Clostridia,Bacteroides vulgatus and Enterococcus faecium,and by increasing the abundance of microbial species,thereby modulating the immune ***,this study can provide insights into the practical application of *** doses to alleviate OVA allergy.

关键词： Bacillus coagulans TQ-35 Food allergy Ovalbumin(OVA) Gut microbiota

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Enhanced degradation of tetracycline by gas-liquid discharge plasma coupled with g-C_(3)N_(4)/TiO_(2)

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Plasma science and Technology 2024年第9期26卷 69-78页

作者： Zhenhai wang Zikai ZHOU sen wang Zhi FANG College of Electrical Engineering and Control science Nanjing Tech UniversityNanjing 211816People’s Republic of China

Plasma-catalysis is considered as one of the most promising technologies for antibiotic degradation in *** the plasma-catalytic system,one of the factors affecting the degradation effect is the performance of the photocatalyst,which is usually restricted by the rapid recombination of electrons and holes as well as narrow light absorption *** this research,a photocatalyst g-C_(3)N_(4)/TiO_(2) was prepared and coupled with gas-liquid discharge(GLD)to degrade tetracycline(TC).The performance was examined,and the degradation pathways and mechanisms were *** show that a 90%degradation rate is achieved in the GLD with g-C_(3)N_(4)/TiO_(2) over a 10 min *** the pulse voltage is conducive to increasing the degradation rate,whereas the addition of excessive g-C_(3)N_(4)/TiO_(2) tends to precipitate agglomerates,resulting in a poor degradation *** redox properties of the g-C_(3)N_(4)/TiO_(2) surface promote the generation of oxidizing active species(H2O2,O3)in *** quenching experiments showed that·OH,hole(h^(+)),play important roles in the TC degradation by the discharge with g-C_(3)N_(4)/TiO_(2).Two potential degradation pathways were proposed based on the *** toxicity of tetracycline was reduced by treatment in the ***,the g-C_(3)N_(4)/TiO_(2) composites exhibited excellent recoverability and stability.

关键词： gas-liquid discharge plasma-catalysis g-C_(3)N_(4)/TiO_(2) TC degradation

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