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Constructing electron-blocking grain boundaries in garnet to suppress lithium dendrite growth

Journal of Advanced Ceramics 2024年第2期13卷 166-175页

作者： Xing Xiang zecheng Fang Congkun Du Zhenzhen Zhao Jiajia Chen Yanhua Zhang Huihu wang Chenhuinan Wei Fei Chen Qiang Shen Hubei Provincial Key Laboratory of Green Materials for Light Industry Hubei University of TechnologyWuhan 430068China Hubei Longzhong Laboratory Wuhan University of Technology Xiangyang Demonstration ZoneXiangyang 441000China Collaborative Innovation Center of Green Light-weight Materials and Processing Hubei University of TechnologyWuhan 430068China New Materials and Green Manufacturing Talent Introduction and Innovation Demonstration Base Hubei University of TechnologyWuhan 430068China State Key Lab of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China

Li_(7)La_(3)Zr_(2)O_(12)(LLZO)is considered as a promising solid-state electrolyte due to its high ionic conductivity,wide electrochemical window,and excellent electrochemical stability.However,its application in solid-state lithium metal batteries(SSLMBs)is impeded by the growth of lithium dendrites in LLZO due to some reasons such as its high electronic conductivity.In this study,lithium fluoride(LiF)was introduced into Ta-doped LLZO(LLZTO)to modify its grain boundaries to enhance the performance of SSLMBs.A nanoscale LiF layer was uniformly coated on the LLZTO grains,creating a threedimensional continuous electron-blocking network at the grain boundaries.Benefiting from the electronic insulator LiF and the special structure of the modified LLZTO,the symmetric cells based on LLZO achieved a high critical current density(CCD)of 1.1 mA·cm^(-2)(in capacity-constant mode)and maintained stability over 2000 h at 0.3 mA·cm^(-2).Moreover,the full cells combined with a LiFePO_(4)(LFP)cathode,demonstrated excellent cycling performance,retaining 97.1% of capacity retention after 500 cycles at 0.5 C.Therefore,this work provides a facile and effective approach for preparing a modified electrolyte suitable for high-performance SSLMBs.

关键词： solid electrolyte garnet lithium dendrite microstructure solid-state batteries

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Sinian hydrocarbon accumulation conditions and exploration potential at the northwest margin of the Yangtze region, China

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Petroleum Exploration and Development 2022年第2期49卷 272-284页

作者： YANG Yu wang zecheng WEN Long XIE Wuren FU Xiaodong LI Wenzheng PetroChina Southwest Oil&Gas Field Company Chengdu 610051China PetroChina Research Institute of Petroleum Exploration&Development Beijing 100083China

Based on outcrop, drilling, logging and seismic data, the reservoir forming conditions, reservoir forming model and exploration potential of the ultra-deep Sinian Dengying Formation at the northwest margin of Yangtze craton region were examined.(1) This area is in craton rifting stage from Sinian to Early Cambrian, characterized by syn-sedimentary faults and rapid subsidence, significant sedimentary differences, and development of Dengying Formation platform margins on both sides of the rift.(2) The Sinian–Cambrian in this area has two sets of high-quality source rocks, Doushantuo Formation and Maidiping-Qiongzhusi Formation;of which, the latter has a thickness of 150–600 m and hydrocarbon generation intensity of(100-200)×10;m;/km;.(3) The mounds and shoals in the platform margin of Sinian Dengying Formation controlled by faults are thick and distributed in rows and zones;they are reformed by contemporaneous–quasi-contemporaneous and supergene karstification jointly, forming pore-type reservoirs with a thickness of 200-400 m.(4) The two sets of source rocks enter oil generation windows from Permian to Early Triassic, and the oil migrates a short distance to the lithologic traps of mounds and shoals to form a huge scale paleo-oil reservoir group;from Late Triassic to Jurassic, the oil in the paleo-oil reservoirs is cracked into gas, laying the foundation of present natural gas reservoirs.(5) The mound-shoal body at the platform margin of Dengying Formation and the two sets of high-quality source rocks combine into several types of favorable source-reservoir combinations, which, with the advantage of near-source and high-efficiency reservoir formation, and can form large lithologic gas reservoirs. The Mianyang-Jiange area is a potential large gas field with trillion cubic meters of reserves. According to seismic prediction, the Laoguanmiao structure in this area has the Deng-2 Member mound-shoal reservoir of about 1300 km^(2), making it a ultra-deep target worthy of exploration in the near future.

关键词： craton rift Dengying Formation source rock fault-controlled platform margin belt lithologic petroleum reservoir northwest margin of Yangtze craton region

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Geological characteristics of the southern segment of the Late Sinian–Early Cambrian Deyang-Anyue rift trough in Sichuan Basin, SW China

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Petroleum Exploration and Development 2023年第2期50卷 321-333页

作者： LI Rong wang Yongxiao wang zecheng XIE Wuren LI Wenzheng GU Mingfeng LIANG Zirui PetroChina Research Institute of Petroleum Exploration&Development Beijing 100083China PetroChina Hangzhou Geological Research Institute Hangzhou 310023China Sinopec Exploration Company Chengdu 610000China

Based on the latest drilling, seismic and field outcrop data, the geological characteristics(e.g. strata, development and sedimentary evolution) of the southern segment of the Late Sinian–Early Cambrian Deyang–Anyue rift trough in the Sichuan Basin are analyzed. First, the strata in the southern segment are complete. The first to second members of Dengying Formation(Deng 1 + Deng 2) are found with relatively stable thickness(400–550 m), and the third to fourth members(Deng 3+ Deng 4) show great thickness difference between the marginal trough and the inner trough, which is up to 250 m. The Cambrian Maidiping Formation and Qiongzhusi Formation in southern Sichuan Basin are relatively thin, with the thickness changing greatly and frequently. Second, the Deyang–Anyue rift trough extended southward during the Deng 4 period, affecting southern Sichuan Basin. Compared to the middle and northern segments of the rift trough, the southern segment is generally wide, gentle and shallow, with multiple steps, and alternating uplifts and sags, which are distributed in finger shape. Third, the Deng 1 + Deng 2 in southern Sichuan Basin records the dominance of carbonate platform and unobvious sedimentary differentiation, and the Deng 4 exhibits obvious sedimentary differentiation, namely, basin–slope–secondary slope–slope–secondary slope–platform margin–restricted platform, from the inner trough to the marginal trough. Fourth, the rift trough in southern Sichuan Basin has evolved in four stages: stabilization of Deng 1–Deng 2, initialization of Deng 3–Deng 4, filling of Maidiping–Qiongzhusi, and extinction of Canglangpu Formation.

关键词： Deyang-Anyue rift trough geological characteristics secondary slope development and evolution Cambrian Maidiping Formation Cambrian Qiongzhusi Formation Sinian Dengying Formation Sichuan Basin

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Exploring the potential of oil and gas resources in Sichuan Basin with Super Basin Thinking

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Petroleum Exploration and Development 2022年第5期49卷 977-990页

作者： wang zecheng SHI Yizuo WEN Long JIANG Hua JIANG Qingchun HUANG Shipeng XIE Wuren LI Rong JIN Hui ZHANG Zhijie YAN Zengmin PetroChina Research Institute of Petroleum Exploration&Development Beijing 100083China PetroChina Southwest Oil&Gas Field Company Chengdu 610051China

Based on the contemporary strategy of Petro China and the“Super Basin Thinking”initiative,we analyze the petroleum system,the remaining oil and gas resource distribution,and the Super Basin development scheme in the Sichuan Basin with the aim of unlocking its full resource potential.We conclude that,(1)The three-stage evolution of the Sichuan Basin has resulted in the stereoscopic distribution of hydrocarbon systems dominated by natural gas.The prospecting Nanhua-rift stage gas system is potentially to be found in the ultra-deep part of the basin.The marine-cratonic stage gas system is distributed in the Sinian to Mid-Triassic formations,mainly conventional gas and shale gas resources.The foreland-basin stage tight sand gas and shale oil resources are found in the Upper Triassic-Jurassic formations.Such resource base provides the foundation for the implementation of Super Basin paradigm in the Sichuan Basin.(2)To ensure larger scale hydrocarbon exploration and production,technologies regarding deep to ultra-deep carbonate reservoirs,tight-sand gas,and shale oil are necessarily to be advanced.(3)In order to achieve the full hydrocarbon potential of the Sichuan Basin,pertinent exploration strategies are expected to be proposed with regard to each hydrocarbon system respectively,government and policy supports ought to be strengthened,and new cooperative pattern should be established.Introducing the“Super Basin Thinking”provides references and guidelines for further deployment of hydrocarbon exploration and production in the Sichuan Basin and other developed basins.

关键词： Super Basin Thinking marine carbonate reservoir tight sand gas shale oil total petroleum system stacked hydrocarbon accumulation Sichuan Basin

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Petroleum geology of marl in Triassic Leikoupo Formation and discovery significance of Well Chongtan1 in central Sichuan Basin,SW China

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Petroleum Exploration and Development 2023年第5期50卷 1092-1104页

作者： wang zecheng XIN Yongguang XIE Wuren WEN Long ZHANG Hao XIE Zengye ZHANG Jianyong TIAN Han LI Wenzheng FU Xiaodong SUN Haofei wang Xiaofang HU Guoyi ZHANG Yu PetroChina Research Institute of Petroleum Exploration&Development Beijing 100083China Research Institute of Petroleum Exploration&Development PetroChina Southwest Oil&Gas Field CompanyChengdu 610041China Exploration Department PetroChina Southwest Oil&Gas Field CompanyChengdu 610041China

In 2022,the risk exploration well Chongtan1(CT1)in the Sichuan Basin revealed commercial oil and gas flow during test in a new zone–the marl of the second submember of the third member of Leikoupo Formation(Lei-32)of Middle Triassic,recording a significant discovery.However,the hydrocarbon accumulation in marl remains unclear,which restricts the selection and deployment of exploration area.Focusing on Well CT1,the hydrocarbon accumulation characteristics of Lei-32 marl are analyzed to clarify the potential zones for exploration.The following findings are obtained.First,according to the geochemical analysis of petroleum and source rocks,oil and gas in the Lei-32 marl of Well CT1 are originated from the same marl.The marl acts as both source rock and reservoir rock.Second,the Lei-32 marl in central Sichuan Basin is of lagoonal facies,with a thickness of 40–130 m,an area of about 40000 km^(2),a hydrocarbon generation intensity of(4–12)×10^(8) m^(3)/km^(2),and an estimated quantity of generated hydrocarbons of 25×10^(12) m^(3).Third,the lagoonal marl reservoirs are widely distributed in central Sichuan Basin.Typically,in Xichong–Yilong,Ziyang–Jianyang and Moxi South,the reservoirs are 20–60 m thick and cover an area of 7500 km^(2).Fourth,hydrocarbons in the lagoonal marl are generated and stored in the Lei-32 marl,which means that marl serves as both source rock and reservoir rock.They represent a new type of unconventional resource,which is worthy of exploring.Fifth,based on the interpretation of 2D and 3D seismic data from central Sichuan Basin,Xichong and Suining are defined as favorable prospects with estimated resources of(2000–3000)×10^(8) m^(3).

关键词： Sichuan Basin central Sichuan Basin Triassic Leikoupo Formation lagoonal marl source-reservoir integration marine unconventional oil and gas

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Assessment of tree-ring mercury radial translocation and age effect in Masson pine:Implications for historical atmospheric mercury reconstruction

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Journal of Environmental Sciences 2024年第4期138卷 266-276页

作者： Xu Liu Xun wang Dingyong wang College of Resources and Environment Southwest UniversityChongqing 400715China State Key Laboratory of Environmental Geochemistry Institute of GeochemistryChinese Academy of SciencesGuiyang 550081China

The tree ring has been regarded as an emerging archive to reconstruct historical atmospheric mercury(Hg)trends,but with the large knowledge gaps in the reliability.In this study,we comprehensively evaluated the Hg source,radial translocation and age effect of Masson pine(Pinus massoniana)tree ring at Mt.Jinyun in Chongqing,to assess the suitability of such tree ring as the archive of atmospheric Hg.Results showed that distinct variabilities among Masson pine tree-ring Hg concentration profiles.The Hg concentration significantly increased along with stem height(P<0.05),indicating the Hg in tree rings mainly derived from foliage uptake atmospheric Hg.We found a distinct age effect that the tree ring of young trees had the higher Hg concentration.Besides,we used the advection-diffusion model to demonstrate how Hg concentration shifted by the advection or/and diffusion in tree rings.The modeling results showed that the advection induced radial translocation during the young growth period of tree was a plausible mechanism to result in the tree-ring Hg record largely different from the trend of anthropogenic Hg emissions in Chongqing.We finally suggest that in further Hg dendrochemistry,better discarding the tree-ring Hg profile of the young growth period to reduce impacts of the radial translocation and age effect.

关键词： Masson pine Tree-ring mercury Radial translocation Tree age effect

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Pushing the boundaries: an interview with Dae-Hyun Kim on terahertz devices

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National Science Review 2024年第3期11卷 42-45页

作者： Defu wang the Center for Carbon-based Electronics School of Electronics Peking University

Ⅲ–Ⅴ compound semiconductors, such as InGaAs/InAlAs, exhibit exceptional carrier transport properties, establishing them as fundamental elements in terahertz(THz) applications crucial for the development of 6G netwo...

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CO_(2)激光退火不同外径锗芯光纤的扫描速度研究

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光子学报 2024年第4期53卷 84-94页

作者：杜亦凡赵子文钟双栖马泽成王少业上海大学通信与信息工程学院上海200444 上海大学特种光纤与光接入网重点实验室上海200444 上海大学特种光纤与先进通信国际合作联合实验室上海200444

对内径为41~43μm,外径约为188μm、251μm和270μm的锗芯光纤进行激光退火实验,研究CO_(2)激光沿光纤轴向扫描速度对锗芯拉曼峰频率和光传输损耗特性的影响。研究发现,激光扫描速度是决定退火后光纤特性的重要参数。对不同外径的光纤,... 详细信息

对内径为41~43μm,外径约为188μm、251μm和270μm的锗芯光纤进行激光退火实验,研究CO_(2)激光沿光纤轴向扫描速度对锗芯拉曼峰频率和光传输损耗特性的影响。研究发现,激光扫描速度是决定退火后光纤特性的重要参数。对不同外径的光纤,达到最优退火效果的激光扫描速度不同,188μm、251μm和270μm外径的锗芯光纤分别为10 mm·s^(-1)、14 mm·s^(-1)和16 mm·s^(-1),光传输损耗分别为3.435 dB·cm^(-1)、2.147 dB·cm^(-1)和3.578 dB·cm^(-1)。使用COMSOL软件对退火过程中纤芯表面固定点的温度变化进行了模拟仿真研究,仿真结果显示激光退火过程中温度呈脉冲形变化。相同外径条件下,激光扫描速度提高,温度脉冲的峰值升高、谷值降低、单脉冲持续时间缩短;相同扫描速度条件下,光纤外径减小,温度脉冲峰值提高,谷值降低。

关键词：锗芯光纤 CO_(2)激光退火激光扫描速度 COMSOL仿真温度变化模拟

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Enrichment of anammox biomass during mainstream wastewater treatment driven by achievement of partial denitrification through the addition of bio-carriers

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Journal of Environmental Sciences 2024年第3期137卷 181-194页

作者： Yuqing Ma Bo wang Xiaodi Li Shuo wang Wen wang Yongzhen Peng National Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology Engineering Research Center of BeijingBeijing University of TechnologyBeijing 100124China

Anammox is widely considered as the most cost-effective and sustainable process for nitrogen removal.However,how to achieve the enrichment of anammox biomass remains a challenge for its large-scale application,especially in mainstream wastewater treatment.In this study,the feasibility of enrichment of anammox biomass was explored through the realization of partial denitrification and the addition of bio-carriers.By using ordinary activated sludge,a sequencing batch reactor(SBR)followed by an up-fow anaerobic sludge bed(UASB)was operated at 25±2℃ for 214 days.The long-term operation was divided into five phases,in which SBR and UASB were started-up in Phases I and II,respectively.By eliminating oxygen and adjusting the infow ratios in Phases III-V,advanced nitrogen removal was achieved with the effuent total nitrogen being 4.7 mg/L and the nitrogen removal efficiency being 90.5%in Phase V.Both in-situ and ex-situ activity tests demonstrated the occurrence of partial denitrification and anammox.Moreover,16S rRNA high-throughput sequencing analysis revealed that Candidatus Brocadia was enriched from below the detection limit to in biofilms(0.4%in SBR,2.2%in UASB)and the foc sludge(0.2%in SBR,1.3%in UASB),while Thauera was mainly detected in the foc sludge(8.1%in SBR,8.8%in UASB),which might play a key role in partial denitrification.Overall,this study provides a novel strategy to enrich anammox biomass driven by rapid achievement of partial denitrification through the addition of bio-carriers,which will improve large-scale application of anammox processes in mainstream wastewater treatment.

关键词： Enrichment Anammox biomass Bio-carriers Partial denitrification Mainstream wastewater

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Performance and mechanism of La-Fe metal-organic framework as a highly efficient adsorbent for fluoride removal from mine water

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Journal of Environmental Sciences 2024年第5期139卷 245-257页

作者： Chaomin Jia Jianbing wang Huijiao wang Sichao Zhu Xiaohui Zhang Yuxiang wang School of Chemical&Environmental Engineering China University of Mining&Technology-BeijingBeijing 100083China Beijing Polytechnic Beijing 100176China Chinese Society for Urban Studies Beijing 100835China

Water fluoride pollution has caused non-negligible harm to the environment and humans,and thus it is crucial to find a suitable treatment technology.In this study,La-Fe@PTA adsorbent was synthesized for the defluoridation of mine water.The results showed that the optimum conditions for defluoridation by La-Fe@PTA were p H close to 7.0,the initial F-concentration of 10 mg/L,the dosage of 0.5 g/L and the adsorption time of 240 min.Compared with SO_4^(2-),Cl^(-),NO_(3)^(-),Ca^(2+)and Mg^(2+),CO_(3)^(2-)and HCO_(3)^(-)presented severer inhibition on fluoride uptake by La-Fe@PTA.The adsorption process fits well with the pseudo-second-order kinetic model and Freundlich model,and the maximum adsorption capacity of Langmuir model was 95 mg/g.Fixed-bed adsorption results indicated that fluoride in practical fluorinated mine water could be effectively removed from 3.6 mg/L to less than 1.5 mg/L within130 bed volume(BV)by using 1.5 g La-Fe@PTA.Furthermore,the adsorbent still had good adsorption capacity after regeneration,which confirms the great application potential of La-Fe@PTA as a fluoride ion adsorbent.The mechanism analysis showed that La-Fe@PTA adsorption of fluorine ions is a physicochemical reaction driven by electrostatic attraction and ion exchange.

关键词： Adsorption La-Fe@PTA Fluoride ion Mine water Mechanism

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