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Vertically grown MoS_(2.nanosheets on graphene with defect-rich structure for efficient sodium storage

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Rare Metals 2024年第3期43卷 1062-1071页

作者： Ying wang jia-Peng He Han-Qing Pan Qing-Peng wang Lei Zhang yong-Chang Liu Qing-Hong wang School of Chemistry&Materials Science Jiangsu Key Laboratory of Green Synthetic Chemistry for Functional MaterialsJiangsu Normal UniversityXuzhou221116China institute of Biopharmaceutical Research Liaocheng UniversityLiaocheng252059China beijing Advanced Innovation Center for Materials Genome Engineering Institute for Advanced Materials and TechnologyState Key Laboratory for Advanced Metals and MaterialsUniversity of Science and Technology BeijingBeijing100083China Centre for Catalysis and Clean energy Gold Coast CampusGriffith UniversityGold CoastQLD4222Australia

The synthesis of a perpendicular growth structure of MoS_(2.nanosheets on graphene for efficient sodium storage is challenging yet ideal due to the benefits of open ion diffusion channels and high electronic *** this study,we have successfully fabricated a novel structure of vertical MoS_(2.nanosheets on graphene,with ZnS nanoparticles serving as bonding points(MoS_(2./ZnS/G),through a facile hydrothermal *** the synthesis process,Zn^(2.)not only acts as a landing site for the vertical growth of MoS_(2.nanosheets but also triggers the formation of a defect-rich structure in the final *** unique architecture of MoS_(2./ZnS/G effectively combines the advantages of a vertically aligned geometry and a defectrich structure for energy *** resulting structure displays shortened transport paths for electrons/ions,enhanced conductivity,improved structural integrity,and an increased number of active sites for promising electrochemical *** expected,when used as anode for sodium-ion batteries,the as-synthesize d MoS_(2./ZnS/G exhibits excellent rate capability(high capacity of 2.8 mAh·g^(-1)at 5 A·g^(-1))and good cycling stability(a capacity decay of 0.056%per cycle after 500 cycles at 1 A·g^(-1)).According to the kinetic investigations,the electrochemical process of the MoS_(2./ZnS/G sample is primarily governe d by a pseudocapacitive behavior,which enhances the charge/discharge kinetics and allows the MoS_(2./ZnS/G structure to remain intact during cycling.

关键词： MoS_(2. Perpendicular growth Graphene Sodium storage Electrochemical performance

Optimal Scheduling of Regional Integrated energy Systems Considering Hybrid Demand Response

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CSEE Journal of Power and energy Systems 2024年第3期10卷 1208-1219页

作者： Ganyun Lyu Bin Cao Dexiang jia Nan wang Jun Li Guangyu {2. Department of Electrical Engineering Nanjing Institute of TechnologyNanjing 211167China State Grid energy Research institute Co. LTDBeijing 102209China State Grid Integrated energy Service Group Co. LTDBeijing 100032China IEEE CSEE

Flexible load can optimize the load curve,which is an important means to promote renewable energy *** peculiarities of electricity,heat,cooling and gas loads are analyzed in this paper,considering the fuzzy degree of human perception for water temperature,and the characteristic model of hot water load is *** the fuzzy degree of human perception of ambient temperature,the characteristic model of cooling load is established by using PMV and PPD ***,considering four combinations of cut load,translatable load,transferable load and alternative load,and considering the coupling relationship of composite parts,different response models of load are established *** the minimum cost of the system,including operation and compensation costs as the objective function,the optimization scheduling model of the regional integrated energy system is established,and the Gurobi solver is used for simulation analysis to solve the optimal output and load response curve of each piece of *** results show that the load curve can be optimized,the flexible regulation ability of the regional integrated energy system can be enhanced,the energy loss of the system can be reduced,and the wind power consumption ability of the system can be increased by considering the integrated demand response.

关键词： Alternative load day ahead optimal scheduling integrated demand response PMV and PPD index regional integrated energy system

Ultra‑Efficient and Cost‑Effective Platinum Nanomembrane Electrocatalyst for Sustainable Hydrogen Production

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Nano-Micro Letters 2024年第6期16卷 95-110页

作者： Xiang Gao Shicheng Dai Yun Teng Qing wang Zhibo Zhang Ziyin Yang Minhyuk Park Hang wang Zhe jia Yunjiang wang yong Yang Department of Mechanical Engineering College of EngineeringCity University of Hong KongTat Chee AvenueKowloon TongKowloonHong KongPeople’s Republic of China State key laboratory of Nonlinear Mechanics Institute of MechanicsChinese Academy of SciencesBeijingPeople’s Republic of China School of Engineering Science University of Chinese Academy of SciencesBeijingPeople’s Republic of China laboratory for Microstructures Institute of MaterialsShanghai UniversityShanghaiPeople’s Republic of China School of Materials Science and Engineering Jiangsu Key Laboratory for Advanced Metallic MaterialsSoutheast UniversityNanjingPeople’s Republic of China Department of Materials Science and Engineering College of EngineeringCity University of Hong KongTat Chee AvenueKowloon TongKowloonHong KongPeople’s Republic of China

Hydrogen production through hydrogen evolution reaction(HER)offers a promising solution to combat climate change by replacing fossil fuels with clean energy ***,the widespread adoption of efficient electrocatalysts,such as platinum(Pt),has been hindered by their high *** this study,we developed an easy-to-implement method to create ultrathin Pt nanomembranes,which catalyze HER at a cost significantly lower than commercial Pt/C and comparable to non-noble metal *** Pt nanomembranes consist of highly distorted Pt nanocrystals and exhibit a heterogeneous elastic strain field,a characteristic rarely seen in conventional *** unique feature results in significantly higher electrocatalytic efficiency than various forms of Pt electrocatalysts,including Pt/C,Pt foils,and numerous Pt singleatom or single-cluster *** research offers a promising approach to develop highly efficient and cost-effective low-dimensional electrocatalysts for sustainable hydrogen production,potentially addressing the challenges posed by the climate crisis.

关键词： Platinum Hydrogen evolution reaction Lattice distortion Heterogeneous strain

Prediction of (n, 2.) reaction cross-sections of long-lived fission products based on tensor model

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NUCLEAR SCIENCE AND TECHNIQUES 2024年第10期35卷 1-14页

作者： Huang, jia-Li wang, Hui Huang, Ying-Ge Xiao, Er-Xi Feng, Yu-Jie Lei, Xin Gu, Fu-Chang Zhu, Long {2., yong-Jing Su, Jun Sun Yat Sen Univ Sino French Inst Nucl Engn & Technol Zhuhai 519082 Peoples R China China Inst Atom energy Key Lab Nucl Data Beijing 102413 Peoples R China China Inst Atom energy China Nucl Data Ctr Beijing 102413 Peoples R China

Interest has recently emerged in potential applications of (n, 2.) reactions of unstable nuclei. Challenges have arisen because of the scarcity of experimental cross-sectional data. This study aims to predict the (n, 2.) reaction cross-section of long-lived fission products based on a tensor model. This tensor model is an extension of the collaborative filtering algorithm used for nuclear data. It is based on tensor decomposition and completion to predict (n, 2.) reaction cross-sections; the corresponding EXFOR data are applied as training data. The reliability of the proposed tensor model was validated by comparing the calculations with data from EXFOR and different databases. Predictions were made for long-lived fission products such as 60Co, 79Se\documentclass[12.t]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$${{79}} {\mathrm{Se}}$$\end{document}, 93Zr\documentclass[12.t]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$${{93}}\mathrm{Zr}$$\end{document}, 107P\documentclass[12.t]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$${{107}}\mathrm{P}$$\end{document}, 12.Sn\documentclass[12.t]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$${{12.}}\mathrm{Sn}$$\end{document}, and 137Cs\documentclass[12.t]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepack

关键词： (n, 2.) Reaction cross-section Tensor model Machine learning Collaborative filtering algorithm Selective transmutation NUCLEAR-DATA TRANSMUTATION N,2.

Weatherability and heat resistance enhanced by interaction between AG2. and Mg/AI-LDH

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Rare Metals 2024年第6期43卷 2758-2768页

作者： Pei-Yao Yang Xiang-Cui Liu Yu-Chao wang Huan-Ran Zheng Jin-Xian wang {2.-Yi Zheng Meng-Jie Liu Dan-Ni Deng Yu Bai Ying-Bi chen Tong Zhang Zhi-Ming Liu yong-Peng Lei State key laboratory of Powder Metallurgy Powder Metallurgy Research InstituteCentral South UniversityChangsha 410083China Research institute of Chemical Defense Beijing 102205China

Although inorganic pigments in common spectral tuning materials show good weatherability and heat resistance,the limited color choices,weak coloring power,poor dispersibility,and a possibility of toxicity limit their *** the basis of organic pigments which possess a wide range of colors,high coloring power,good transparency,and high safety,herein,the modified pigment and biomimetic coating with improved weatherability,especially ultraviolet(UV)resistance(from 2.to 6 days),was achieved by intercalating acid green 2.(AG2.)pigment into Mg/Al-layered double hydroxides(Mg/Al-LDH).Furthermore,the heat resistance of AG2. was also significantly ***,the spectral stability of pigments after heat treatment is superior with almost unchanged spectral profile and green reflection *** formation of strong N-H bonds and the S-M(Mg,Al)bonds between Mg/Al-LDH laminates and AG2. molecules contributes to the *** work shows potential for biomimetic leaf materials in respect of reflective spectra stability.

关键词： Layered double hydroxide Biomimetic Acid green 2. Interaction Weatherability Heat resistance

Phosphine-Built-In Porous Organic Cage Supported Ultrafine Pd Nanoclusters Enable highly Efficient and Regioselective Hydrogenation of Epoxides

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CCS Chemistry 2024年第10期6卷 2476-2488页

作者： Xin Zhou Zhaozhan wang Zhe-Ning chen {2. Yang CAS key laboratory of Bio-Based Materials Qingdao Institute of Bioenergy and Bioprocess TechnologyChinese Academy of SciencesQingdao 266101 Shandong energy institute Qingdao 266101 College of Environment and Safety Engineering Qingdao University of Science and TechnologyQingdao 266101 State key laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002 University of chinese academy of sciences Beijing 100049 Fujian Provincial key {2. of Theoretical and Computational Chemistry Xiamen UniversityXiamen 361005

Selective hydrogenation of epoxides has been regarded as an atom-economical and straightforward method for the synthesis of ***,it remains a big challenge in the precise control of *** date,the reaction enabled by a reusable and high-performance heterogeneous catalyst with excellent regioselectivity is very ***,we develop highly loaded and ultrafine Pd nanoclusters(NCs)encapsulated on a phosphinebuilt-in porous organic cage(FPPOC)for the catalytic hydrogenation of epoxides by molecular *** from the unique characters of uniform dispersion and strong interaction between Pd NCs and FPPOC,the resultant Pd NCs exhibited superior catalytic activity and excellent regioselectivity for the hydrogenation of epoxides under milder conditions.A diverse set of terminal and internal epoxides was efficiently reduced to the corresponding linear or branched alcohols in an extremely regioselective manner,well tolerating diverse functional ***,the catalyst demonstrates high stability and could be reused up to 10 times with marginal decay in activity and ***,the catalyst is applicable for scale-up synthesis with a record turnover number as high as 16,111,to the best of our knowledge,outperforming those previous state-of-the-art *** experiments and characterizations in combination with density functional theory calculations provide insight into the superior activity and excellent regioselectivity.

关键词： porous organic cage phosphine-built-in palladium nanoclusters regioselective hydrogenation epoxides

Role of gallium wetting layer in high-quality ZnO growth on sapphire (0001) substrates

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Science China(physics,Mechanics & Astronomy) 2004年第5期47卷 612-620页

作者： ZENG Zhaoquan1,3, wang yong2. DU Xiaolong1, MEI Zengxia1, KONG Xianghe3, {2. Jinfeng1, XUE Qikun1 & ZHANG Ze2. 4 1. State key laboratory for Surface physics, institute of physics, chinese academy of sciences, beijing 100080, China 2. laboratory of Electron Microscopy, institute of physics, chinese academy of sciences, beijing 100080, China 3. College of physics and Engineering, Qufu Normal University, Qufu 2.3165, China 4. beijing University of Technology, beijing 10002., China 1. State key laboratory for Surface {2. Institute of Physics Chinese Academy of Sciences 100080 Beijing China 2. College of physics and Engineering Qufu Normal University 273165 Qufu China 3. laboratory of Electron Microscopy Institute of Physics Chinese Academy of Sciences 100080 Beijing China 4. beijing University of Technology 100022 Beijing China

A Ga wetting layer was used to modify the surface structure of sapphire (0001) substrate to prepare high-quality ZnO film by radio frequency plasma-assisted molecule beam epitaxy. We found that this Ga layer plays a crucial role in eliminating 30 rotation domains, controlling polarity and decreasing defect density in ZnO epilayers, as demonstrated by in situ reflection high {2. electron diffraction, ex situ high resolution X-ray diffraction and high resolution cross-sectional transmission electron microscopy. Zn-polar film of ZnO was determined by convergent beam electron diffraction. A Ga bilayer model is proposed to understand the effects of the Ga wetting layer on high-quality ZnO growth.

关键词： Ga wetting layer, sapphire, polarity, defect density, zinc oxide, rf-MBE, RHEED, HRXRD, TEM, CBED.

Sensitivity impacts owing to the variations in the type of zero-range pairing forces on the fission properties using the density functional theory

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Nuclear Science and Techniques 2024年第3期35卷 198-207页

作者： Yang Su Ze-Yu Li Li-Le Liu Guo-Xiang Dong Xiao-Bao wang yong-Jing {2. China Nuclear Data Center China Institute of Atomic EnergyBeijing 102413China School of Science Huzhou UniversityHuzhou 313000China

Using the Skyrme density functional theory,potential energy surfaces of^(2.0)Pu with constraints on the axial quadrupole and octupole deformations(q_(2.)and q_(30))were *** volume-like and surface-like pairing forces,as well as a combination of these two forces,were used for the Hartree–Fock–Bogoliubov *** in the least-energy fission path,fission barrier,pairing energy,total kinetic energy,scission line,and mass distribution of the fission fragments based on the different forms of the pairing forces were analyzed and *** fission dynamics were studied based on the timedependent generator coordinate method plus the Gaussian overlap *** results demonstrated a sensitivity of the mass and charge distributions of the fission fragments on the form of the pairing *** on the investigation of the neutron-induced fission of^(2.9)Pu,among the volume,mixed,and surface pairing forces,the mixed pairing force presented a good reproduction of the experimental data.

关键词： Nuclear fission Density functional theory Pairing force Potential energy surfaces Fission fragment distribution

Thermo-Flow Performances for the Main-Auxiliary Integrated Natural Draft Dry Cooling System

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Journal of Thermal Science 2024年第3期33卷 1010-1025页

作者： ZHANG Zongyang HOU Yichen ZHOU Hanyu jia He chen Lei KONG Yanqiang wang Weijia YANG Lijun DU Xiaoze key laboratory of Power Station {2. Transfer Conversion and System of Ministry of Education School of Energy Power and Mechanical EngineeringNorth China Electric Power UniversityBeijing102206China

Recently,natural draft dry cooling system with the main-auxiliary integrated air-cooled heat exchangers in the up and lower layers,has drawn attention to the electric power *** research firstly develops two physical models for the integrated cooling system,namely Case A and Case *** Case A,the main air-cooled heat exchanger is arranged in the upper layer and the auxiliary air-cooled heat exchanger arranged in the lower layer,while in Case B,the two heat exchanger systems are arranged in the opposite *** then,directing at the engineering TMCR and TRL 1 working conditions,the unit-local-overall thermo-flow characteristics of Case A and Case B are obtained and compared by numerical *** findings show that,for the auxiliary air-cooled exchanger,Case A has obviously higher cooling performances than Case B,with the difference varying from 5.46%to 7.55%.Whereas,for the main air-cooled exchanger,Case B shows the recovered cooling performances,with the difference changing from 1.15%to 2.99%.Case A is preferably recommended to the engineering application in consideration of more strict cooling demand of the auxiliary cooling ***,this research will provide some theoretical guidelines for the design and construction of the main-auxiliary integrated natural draft dry cooling system.

关键词： integrated dry cooling system main air-cooled heat exchanger auxiliary air-cooled heat exchanger upper layer and lower layer thermo-flow performances