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Viscosity and structure relationship with equimolar substitution of CaO with MgO in the CaO–MgO–Al_(2)O_(3)–SiO_(2)slag melts

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International Journal of Minerals,Metallurgy and Materials 2025年第1期32卷 70-79页

作者： yong Hou Shuo Zhang Jie Dang jia Guo Hanghang Zhou Xuewei Lü College of Materials Science and Engineering Chongqing UniversityChongqing 400044China Chongqing Key Laboratory of Vanadium-Titanium Metallurgy and New Materials Chongqing UniversityChongqing 400044China

Currently,the Al_(2)O_(3)content in the high-alumina slag systems within blast furnaces is generally limited to 16wt%–18.5wt%,making it challenging to overcome this *** most studies that concentrated on managing the MgO/Al_(2)O_(3)ratio or basicity,this paper explored the effect of equimolar substitution of MgO for CaO on the viscosity and structure of a high-alumina CaO-MgO-Al_(2)O_(3)-SiO_(2)slag system,providing theoretical guidance and data to facilitate the application of high-alumina *** results revealed that the viscosity first decreased and then increased with higher MgO substitution,reaching a minimum at 15mol%MgO *** transform infrared spectroscopy(FTIR)results found that the depths of the troughs representing[SiO_(4)]tetrahedra,[AlO_(4)]tetrahedra,and Si-O-Al bending became progressively deeper with increased MgO *** of the Raman spectra showed that the average number of bridging oxygens per Si atom and the X_(Q^(3))/X_(Q^(2))(X_(Q^(i))is the molar fraction of Q^(i) unit,and i is the number of bridging oxygens in a[SiO_(4)]tetrahedral unit)ratio increased from 2.30 and 1.02 to 2.52 and 2.14,respectively,indicating a progressive polymerization of the silicate structure.X-ray photoelectron spectroscopy(XPS)results highlighted that non-bridging oxygen content decreased from 77.97mol% to 63.41mol% with increasing MgO concentration,whereas bridging oxygen and free oxygen contents *** analysis demonstrated a gradual increase in the polymerization degree of the tetrahedral structure with the increase in MgO ***,bond strength is another important factor affecting the slag *** occurrence of a viscosity minimum can be attributed to the complex evolution of bond strengths of non-bridging oxygens generated during depolymerization of the[SiO_(4)]and[AlO_(4)]tetrahedral structures by CaO and MgO.

关键词： aluminosilicate viscosity structure spectroscopy

效率视角下中国2030年二氧化碳排放峰值目标的省区分解——基于零和收益DEA模型的研究

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环境科学学报 2017年第11期37卷 4399-4408页

作者：王勇贾雯毕莹东北财经大学统计学院大连116025 东北财经大学博士后科研流动站大连116025

实现2030年二氧化碳排放达到峰值不仅是中国在全球气候谈判中做出的国际承诺,也是中国实现经济结构转型的必然选择,而对二氧化碳排放峰值进行合理的区域分解是中国实现二氧化碳排放达峰的必要前提.本文首先对中国2030年二氧化碳排放峰... 详细信息

实现2030年二氧化碳排放达到峰值不仅是中国在全球气候谈判中做出的国际承诺,也是中国实现经济结构转型的必然选择,而对二氧化碳排放峰值进行合理的区域分解是中国实现二氧化碳排放达峰的必要前提.本文首先对中国2030年二氧化碳排放峰值进行初始的省区分解,利用DEA-BCC模型对初始省区分解方案进行效率评估,在此基础上利用零和收益DEA模型得到全部省区达到有效的中国二氧化碳排放峰值省区分解方案.本文研究表明:(1)大部分省区初始分解方案的效率值较低,只有2个省区的效率值达到DEA有效,且二氧化碳排放配额比重较大省区的分配效率值较小;(2)经过零和收益DEA模型的优化,省区分解方案的整体效率最终提升至有效边界,二氧化碳排放配额由效率较低的欠发达地区向效率较高的较发达地区转移,较发达和不发达的两类地区均分配到了较少的二氧化碳排放配额,最终二氧化碳排放权占比较多的地区主要为二氧化碳排放严重但减排潜力较大的省区.文章最后根据本文研究结论提出了具体的碳排放省区分解政策建议.

关键词：二氧化碳排放峰值省区分解效率零和收益DEA模型

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轮毂电机驱动电动汽车横摆稳定性控制

控制工程 2021年第6期28卷 1075-1085页

作者：汪永嘉合肥工业大学汽车与交通工程学院安徽合肥230009

针对轮毂电机驱动的电动汽车的横摆稳定性问题,提出了一种基于极限学习机(ELM)网络的直接横摆力矩控制方法。采用自适应积分终端滑模(AITSM)控制策略设计横摆角速度控制器,并通过ELM的快速在线学习能力实现在闭环系统中进行集总干扰估... 详细信息

针对轮毂电机驱动的电动汽车的横摆稳定性问题,提出了一种基于极限学习机(ELM)网络的直接横摆力矩控制方法。采用自适应积分终端滑模(AITSM)控制策略设计横摆角速度控制器,并通过ELM的快速在线学习能力实现在闭环系统中进行集总干扰估计和补偿。控制器的主要贡献在于,一是实现横摆角速度跟踪误差的有限时间收敛,二是引入了ELM扰动估计技术,减少了传统滑模控制对系统扰动先验知识的依赖。仿真结果表明,使用所提出的控制器策略,车辆横摆角速度跟踪精度和系统强鲁棒性得到了提升,实现了更好的车辆横摆稳定性和操控性能。

关键词：电动汽车积分终端滑模极限学习机

Industrial Control Anomaly Detection Based on Distributed Linear Deep Learning

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Computers, Materials & Continua 2025年第1期82卷 1129-1150页

作者： Shijie Tang yong Ding Huiyong wang School of Computer Science and Information Security Guilin University of Electronic TechnologyGuilin541004China School of Electronic Engineering and Automation Guilin University of Electronic TechnologyGuilin541004China Guangxi Engineering Research Center of Industrial Internet Security and Blockchain Guilin University of Electronic TechnologyGuilin541004China Institute of Cyberspace Technology HKCT Institute for Higher EducationHong Kong999077China School of Mathematics&Computing Science Guilin University of Electronic TechnologyGuilin541004China

As more and more devices in Cyber-Physical Systems(CPS)are connected to the Internet,physical components such as programmable logic controller(PLC),sensors,and actuators are facing greater risks of network attacks,and fast and accurate attack detection techniques are *** key problem in distinguishing between normal and abnormal sequences is to model sequential changes in a large and diverse field of time *** address this issue,we propose an anomaly detection method based on distributed deep *** method uses a bilateral filtering algorithm for sequential sequences to remove noise in the time series,which can maintain the edge of discrete *** use a distributed linear deep learning model to establish a sequential prediction model and adjust the threshold for anomaly detection based on the prediction error of the validation *** method can not only detect abnormal attacks but also locate the sensors that cause *** conducted experiments on the Secure Water Treatment(SWAT)and Water Distribution(WADI)public *** experimental results show that our method is superior to the baseline method in identifying the types of attacks and detecting efficiency.

关键词： Anomaly detection CPS deep learning MLP(multi-layer perceptron)

SYNTHESIS AND CRYSTAL STRUCTURE OF 5, 10, 15, 20, 22, 24-HEXAHYDRO-5, 5, 10, 10, 15, 15, 20, 20-OCTAMETHYL-PORPHINE

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Chinese Journal of Structural Chemistry 1992年第5期 376-379页

作者： Meng Ji-Ben Fu De-Chao wang yong-Mei jia Wen-LiDepartment of Chemistry , Nankai University , Tianjin Yiao Xin-Kan wang Hong-Gen Central Laboratory , Nankai University , Tianjin

The title com pound (HHOMP) has been synthesized with the pho-toinduced condensation of acetone and pyrrole in the presence of iodoaromatic hydrocarbons, and its molecular and crystal structures have been determined by X-ray analysis. C28H36N4, Mr = 428. 63, triclinic; space group P1; a =10. 165(3), b = 10. 185(2), c=13. 012(3)(?); α=85. 41(2), β=67. 84(2), γ= 89. 75(2)°; V = 1243 (?)3; Z = 2; D = 1. 145g. cm-3; μ= 0. 635cm-1; F (000) = 464. Although the HHOMP molecule twists, it is found that the four nitrogen atoms are still in a plane.

关键词： OCTAMETHYL-PORPHINE SYNTHESIS AND CRYSTAL STRUCTURE OF 5 HEXAHYDRO-5

Multivariate synergy for heightening ionic HOF robustness and proton conductivity

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Science China Chemistry 2025年

作者： Xiang-Tian Bai Li-Hui Cao Xu-yong Chen jia-Yu wang Zi-Ye Zhou Shaanxi Key Laboratory of Chemical Additives for Industry College of Chemistry and Chemical EngineeringShaanxi University of Science and Technology

Multicomponent crystalline materials construct more complex and diversified structures with different combinations and modes,which expands the material structure space and application *** this work,we have successfully synthesized two twocomponent ionic hydrogen-bonded organic frameworks （iHOF-32 and iHOF-33） and a three-component iHOF （iHOF-34）.Guanidine hydrochloride which is rich in N and H and has a short chain length strengthens the hydrogen bonding network of iHOF,thereby aiding in the efficient migration of *** rigid architecture of 1,1'-diamino-4,4'-bipyridine diiodide furnishes additional scaffolding for the iHOFs and enhances its robustness under harsh ***-34 accomplishes the combination of the ultra-high proton conductivity of iHOF-32 and the robustness of iHOF-33 by the synergistic interaction among the three components of *** addition,iHOF-34 was fabricated as a composite membrane with a peak proton conductivity of 1.55×10-1S cm-1,which is 3.8 times higher than that of recast Nafion,and has extensive potential in fuel *** self-assembly strategy of multicomponent HOFs opens up new avenues for constructing diverse structures while promising new opportunities for applications in the fields of proton conduction and energy storage.

关键词：

论“十七年”时期中国儿童小说的儿童形象嬗变

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齐鲁学刊 2016年第1期 156-160页

作者：王家勇沈阳师范大学文学院辽宁沈阳110034

实用主义教育观是"十七年"时期中国儿童小说儿童形象塑造的理论基础,但这个理论却在此时出现了异变,其对杜威的原点思想做了断章取义式的解读,只强调"实用"二字,只要求儿童小说能够起到"教训"作用。其原因有三:"十七年"时期儿童文学的... 详细信息

实用主义教育观是"十七年"时期中国儿童小说儿童形象塑造的理论基础,但这个理论却在此时出现了异变,其对杜威的原点思想做了断章取义式的解读,只强调"实用"二字,只要求儿童小说能够起到"教训"作用。其原因有三:"十七年"时期儿童文学的文艺指导方针即对毛泽东文艺思想的极端解读,百废待兴的社会主义建设事业对建设者和接班人的急需,前苏联儿童文学理论的引入。三者合力,最终致使"十七年"时期的儿童形象只集中表现于两大类:"少先队"和"革命儿童",并呈现出符合时代特征的嬗变轨迹。

关键词： “十七年” 中国儿童小说儿童形象嬗变

Enhanced post-combustion CO2 capture and direct air capture by plasma surface functionalization of graphene adsorbent

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Journal of Energy Chemistry 2025年第1期100卷 653-664页

作者： Rahul Navik Eryu wang Xiao Ding Huang Yunyi Yiyu Liu jia Li Guangdong-Hong Kong Joint Laboratory for Carbon Neutrality Jiangmen Laboratory of Carbon and Science and Technology Guangzhou HKUST Fok Ying Tung Research Institute The Hong Kong University of Science and Technology (Guangzhou) Carbon Neutrality and Climate Change Thrust Society Hub The Hong Kong University of Science and Technology (Guangzhou) Stoddart Institute of Molecular Science Department of Chemistry Zhejiang University

Graphene has enormous potential to capture CO2due to its unique properties and ***,graphene-based adsorbents have drawbacks of lower CO2adsorption capacity and poor *** work demonstrates a one-step rapid and sustainable N2/H2plasma treatment process to prepare graphene-based sorbent material with enhanced CO2adsorption *** treatment directly enriches amine species,increases surface area,and improves textural *** CO2adsorption capacity increases from 1.6 to 3.3 mmol/g for capturing flue gas,and from 0.14 to 1.3 mmol/g for direct air capture （DAC）.Importantly,the electrothermal property of the plasma-modified aerogels has been significantly improved,resulting in faster heating rates and significantly reducing energy consumption compared to conventional external heating for regeneration of *** aerogels display improved selectivity of 42 and 87 after plasma modification for 5 and 10 min,*** plasma-treated aerogels display minimal loss between 17%and 19% in capacity after 40 adsorption/desorption cycles,rendering excellent *** N2/H2plasma treatment of adsorbent materials would lower energy expenses and prevent negative effects on the global economy caused by climate change.

关键词： Carbon neutrality CO 2 capture Climate change Plasma treatment Graphene aerogel

Ideal Bi‑Based Hybrid Anode Material for Ultrafast Charging of Sodium‑Ion Batteries at Extremely Low Temperatures

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Nano-Micro Letters 2025年第3期17卷 152-167页

作者： Jie Bai jian Hui jia Yu wang Chun Cheng Yang Qing jiang Key Laboratory of Automobile Materials(Jilin University) Ministry of EducationSchool of Materials Science and EngineeringJilin UniversityChangchun 130022People’s Republic of China

Sodium-ion batteries have emerged as competitive substitutes for low-temperature applications due to severe capacity loss and safety concerns of lithium-ion batteries at−20°C or ***,the key capability of ultrafast charging at ultralow temperature for SIBs is rarely ***,a hybrid of Bi nanoparticles embedded in carbon nanorods is demonstrated as an ideal material to address this issue,which is synthesized via a high temperature shock *** a hybrid shows an unprecedented rate performance(237.9 mAh g^(−1)at 2 A g^(−1))at−60℃,outperforming all reported SIB anode *** with a Na_(3)V_(2)(PO_(4))_(3)cathode,the energy density of the full cell can reach to 181.9 Wh kg^(−1)at−40°*** on this work,a novel strategy of high-rate activation is proposed to enhance performances of Bi-based materials in cryogenic conditions by creating new active sites for interfacial reaction under large current.

关键词： Bi nanoparticles High temperature shock High-rate activation Ultrafast charging Low-temperature sodium-ion batteries