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Multi-endpoint assays reveal more severe toxicity induced by chloraminated effluent organic matter than chloraminated natural organic matter

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Journal of Environmental Sciences 2024年第1期135卷 310-317页

作者： Hai-Yan wang De-xiu Wu Ye Du Xiao-Tong Lv Qian-yuan Wu State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental SciencesBeijing 100012China Environmental Protection Key Laboratory of Microorganism Application and Risk Control Guangdong Provincial Engineering Research Center for Urban Water Recycling and Environmental SafetyTsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China College of Architecture and Environment Sichuan UniversityChengdu 610000China

Disinfection by chloramination produces toxic byproducts and the difference in toxicity of reclaimed and drinking water treated by chloramination remains *** study investigated cytotoxic effects at the same concentrations of dissolved organic matter and showed that chloraminated effluent organic matter(EfOM)induced 1.7 times higher cytotoxicity than chloraminated natural organic matter(NOM)applied to simulate drinking *** EfOM induced more reactive nitrogen species than chloraminated NOM,and chloraminated EfOM and NOM induced similar and higher levels of reactive oxygen species than the negative control,***,intracellular macromolecule damage indicated by DNA/RNA damage marker 8–hydroxy-(deoxy)guanosine and the intracellular protein carbonyl concentration induced by chloraminated EfOM was higher and slightly more than that induced by chloraminated NOM,*** data were consistent with the effects on cell physiological *** cycle arrest mainly occurred in G2 phase by chloraminated EfOM and *** apoptotic cells,which could return to normal,increased upon exposure to high concentrations of chloraminated EfOM and ***,necrotic cells were significantly increased from 0.5%to 2.5%when the concentration increased from 20-to 60-fold chloraminated EfOM,but were not obviously changed by chloraminated *** results indicated that the comprehensive intracellular changes induced by toxic substances in chloraminated EfOM were more irreversible and induced more cell death than chloraminated NOM.

关键词： Cytotoxicity Intracellular active nitrogen/oxygen Intracellular oxidative damage Cell necrosis Reclaimed water

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A Tri-Salt Composite Electrolyte with Temperature Switch Function for Intelligently Temperature-Controlled Lithium Batteries

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Energy & Environmental Materials 2024年第6期7卷 84-93页

作者： Ende Fu Huimin wang Yating Zhang Zhenxue Xiao xiu Zheng Shuai Hao Xueping Gao Institute of New Energy Material Chemistry School of Materials Science and EngineeringNankai UniversityTianjin300350 China

The intense research of lithium-ion batteries has been motivated by their successful applications in mobile devices and electronic *** emerging of intelligent control in kinds of devices brings new requirements for battery *** high-energy lithium batteries are expected to respond or react under different environmental *** this work,a tri-salt composite electrolyte is designed with a temperature switch function for intelligently temperature-controlled lithium ***,the halide Li_(3)YBr_(6)together with LiTFSI and LiNO_(3)works as active fillers in a low-melting-point polymer matrix(polyethyleneglycol dimethyl ether(PEGDME)and polyethylene oxide(PEO)),which is further filled into the pre-lithiated alumina fiber *** 60°C,the composite electrolyte exists in the liquid state and fully contacts with the working electrodes on the liquid–solid interface,effectively minimizing the interfacial resistance and leading to high discharge capacity in the *** electrolyte is changed into a solid state below 30°C so that the ionic conductivity is significantly reduced and the interface resistance is increased dramatically on the solid–solid ***,by simply adjusting the temperature,the cell can be turned“ON”or“OFF”*** novel function of the composite electrolyte has enlightening significance in developing intelligently temperature-controlled lithium batteries.

关键词： composite electrolyte halide electrolyte low melting point solid-state battery temperature switch function

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Statistical analysis and interpretation on lightning impulse breakdown voltages of ester liquids under varying field uniformity

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High Voltage 2024年第1期9卷 22-34页

作者： Haichuan yu Qiang Liu Zhongdong wang Department of Electrical and Electronic Engineering The University of ManchesterManchesterUK Department of Engineering University of ExeterExeterUK

Ester liquids(ELs),as the alternative transformer liquids to the conventional mineral oils(MOs),have been increasingly used in power transformers with high voltage *** various properties,the lightning impulse breakdown voltages(LIBDVs)have been studied elaborately in the past two decades under different electric field *** electric field uniformities do have an effect on the breakdown characteristics,for example,breakdown mechanisms,polarity effects,and differences of LIBDV between ELs and MOs,which is quantitatively investigated based on the LIBDVs collected from the *** breakdown mechanism transition phenomenon between streamer initiation dominated breakdown and streamer propagation dominated breakdown has been reviewed ***,the transition field factor boundaries to observe the polarity effect on LIBDVs are taken at around 20 for ELs and 10 for ***,the transition field factor boundaries to observe the LIBDV distinctions between ELs and MOs are about 109 and 14 under positive and negative lightning impulse,*** systematic analysis and interpretation on the transition field factor boundaries among different phenomena can provide insights on insulation design of ELs filled power transformers.

关键词： field lightning breakdown

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Multiple Normalized Solutions for Nonlinear Biharmonic Schr?dinger Equations in ■with L-Subcritical Growth

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Acta Mathematicae Applicatae Sinica 2024年

作者： Jun wang Li wang Ji-xiu wang Department of Mathematics Sun Yat-sen University College of Science East China Jiaotong University School of Mathematics and Statistics Hubei University of Arts and Science

In this article, we consider the existence of normalized solutions for the following nonlinear biharmonic Schr?dinger equations:■where c, ε > 0, N ≥ 5, λ ∈ R is a Lagrange multiplier and is unknown, h ∈ C（■N, [0, ∞）), f : R → R is continuous function satisfying L2-subcritical growth. When ε is small enough, we get multiple normalized solutions. Moreover, we also obtain orbital stability of the solutions.

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Femtosecond laser-induced periodic surface structures on hard and brittle materials

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Science China(Technological Sciences) 2024年第1期67卷 19-36页

作者： ZHAO GuoXu wang Gong LI yunFei wang Lei LIAN yuDong yu yu ZHAO Hui wang yuLei LU ZhiWei Center for Advanced Laser Technology Hebei University of TechnologyTianjin 300401China Hebei Key Laboratory of Advanced Laser Technology and Equipment Tianjin 300401China State Key Laboratory of Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityChangchun 130012China School of Information and Electrical Engineering Hebei University of EngineeringHandan 056038China

Hard and brittle materials have high hardness,excellent optical stability,chemical stability,and high thermal ***,they have huge application potential in various fields,such as optical components,substrate materials,and quantum information,especially under harsh conditions,such as high temperatures and high *** laser direct writing technology has greatly promoted the development of femtosecond laser-induced periodic surface structure(Fs-LIPSS or LIPSS by a femtosecond laser)applications of hard and brittle materials due to its high precision,controllability,and three-dimensional processing *** far,LIPSSs have been widely used in material surface treatment,optoelectronic devices,and ***,a consensus has not been reached regarding the formation mechanism of LIPSSs on hard and brittle *** this paper,three widely accepted LIPSS formation mechanisms are introduced,and the characteristics and applications of LIPSSs on diamonds,silicon,silicon carbide,and fused silica surfaces in recent years are *** addition,the application prospects and challenges of LIPSSs on hard and brittle materials by a femtosecond laser are discussed.

关键词： laser-induced periodic surface structures hard and brittle materials femtosecond laser

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Semi-supervised remote sensing image scene classification with prototype-based consistency

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Chinese Journal of Aeronautics 2024年第2期37卷 459-470页

作者： Yang LI Zhang LI Zi wang Kun wang Qifeng yu College of Aerospace Science and Engineering National University of Defense TechnologyChangsha 410073China

Deep learning significantly improves the accuracy of remote sensing image scene classification,benefiting from the large-scale ***,annotating the remote sensing images is time-consuming and even tough for *** neural networks trained using a few labeled samples usually generalize less to new unseen *** this paper,we propose a semi-supervised approach for remote sensing image scene classification based on the prototype-based consistency,by exploring massive unlabeled *** this end,we,first,propose a feature enhancement module to extract discriminative *** is achieved by focusing the model on the foreground ***,the prototype-based classifier is introduced to the framework,which is used to acquire consistent feature *** conduct a series of experiments on NWPU-RESISC45 and Aerial Image Dataset(AID).Our method improves the State-Of-The-Art(SOTA)method on NWPU-RESISC45 from 92.03%to 93.08%and on AID from 94.25%to 95.24%in terms of accuracy.

关键词： Semi-supervised learning Remote sensing Scene classification Prototype network Deep learning

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High corrosion and wear resistant electroless Ni–P gradient coatings on aviation aluminum alloy parts

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International Journal of Minerals,Metallurgy and Materials 2024年第1期31卷 155-164页

作者： Bo wang Jiawei Li Zhihui Xie Gengjie wang Gang yu College of Chemistry and Chemical Engineering Hunan UniversityChangsha 410012China Chemical Synthesis and Pollution Control Key Laboratory of Sichuan Province/College of Chemistry and Chemical Engineering China West Normal UniversityNanchong 637002China Zhongchuan Machinery Ltd.Co. Aero Engine Corporation of ChinaChangsha 410200China

A Ni–P alloy gradient coating consisting of multiple electroless Ni–P layers with various phosphorus contents was prepared on the aviation aluminum alloy. Several characterization and electrochemical techniques were used to characterize the different Ni–P coatings’ morphologies, phase structures, elemental compositions, and corrosion protection. The gradient coating showed good adhesion and high corrosion and wear resistance, enabling the application of aluminum alloy in harsh environments. The results showed that the double zinc immersion was vital in obtaining excellent adhesion (81.2 N). The optimal coating was not peeled and shredded even after bending tests with angles higher than 90°and was not corroded visually after 500 h of neutral salt spray test at 35℃. The high corrosion resistance was attributed to the misaligning of these micro defects in the three different nickel alloy layers and the amorphous structure of the high P content in the outer layer. These findings guide the exploration of functional gradient coatings that meet the high application requirement of aluminum alloy parts in complicated and harsh aviation environments.

关键词： aluminum alloy electroless nickel coating corrosion adhesion

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Tuning Surface Molecular Design of Porous Carbon for Blue Energy Harvesting

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Research 2024年第1期2023卷 651-662页

作者： Jian yu Zhong-Lin wang Tianwei Ma Department of Civil and Environmental Engineering University of Hawaii at MānoaHonoluluHI 96822USA Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of SciencesBeijing 101400China College of Engineering Texas A&M University-Corpus ChristiCorpus ChristiTX 78412USA

Capacitive mixing is a promising blue energy technology due to its membrane-free electricity generation and long electrode life ***,because of limited performance,existing systems do not lend themselves to practical *** it is a crucial factor directly influencing electrode behavior,surface chemistry has largely been overlooked in capacitive ***,we show that manipulating surface functionalization alone can tune the responses of electrodes to produce a high voltage rise without altering the pore structure of the *** findings reveal that the spontaneous electrode potential of a surface-modified carbon electrode shifts negatively proportional to the surface charge due to the surface groups,which explains why and how manipulating the surface chemistry can improve the power generation capacity.

关键词： electrode Porous mixing

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Insight into the adsorption behavior and mechanism of trace impurities from H_(2)O_(2) solution on functionalized zirconia by tuning the structure of amino groups

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Frontiers of Chemical Science and Engineering 2024年第5期18卷 83-94页

作者： yu Meng Yitong wang Guozhu Li Guozhu Liu Li wang Key Laboratory for Green Chemical Technology of Ministry Education School of Chemical Engineering and TechnologyTianjin UniversityTianjin 300072China Haihe Laboratory of Sustainable Chemical Transformations Tianjin 300192China

Primary,secondary and tertiary amino-functionalized zirconia(ZrO_(2)-NH_(2),ZrO_(2)-NH and ZrO_(2)-N)was synthesized by the postgrafting method for the adsorption removal of typical metallic ions,phosphate and total oxidizable carbon from a real H_(2)O_(2) ***_(2)-NH_(2),ZrO_(2)-NH and ZrO_(2)-N exhibited similar pore sizes and sequentially increased zeta *** adsorption results of single and binary simulated solutions showed that the removal efficiency increased in the order of Fe^(3+)>Al^(3+)>Ca^(2+)>Na^(+).There is competitive adsorption between metallic ions,and Fe^(3+) has an advantage over the other metals,with a removal efficiency of 90.7%.The coexisting phosphate could promote the adsorption of metallic ions,while total oxidizable carbon had no effect on *** adsorption results of the real H_(2)O_(2)solution showed that ZrO_(2)-NH_(2) exhibited the best adsorption affinity for metallic ions,as did phosphate and total oxidizable carbon,with a total adsorption capacity of 120.9 mg·g_(-1).Density functional theory calculations revealed that the adsorption process of metallic ions involves electron transfer from N atoms to metals and the formation of N-metal bonds.

关键词： adsorption metallic ion phosphate total oxidizable carbon zirconia H_(2)O_(2)

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Research on the cuttings discharge in air cushion chamber of slurry shield based on CFD-DEM coupling method Author links open overlay panel

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Particuology 2024年第8期91卷 88-105页

作者： Han wang Wantao Ding Weimin Yang Chengzhen wang Wenduan yu Zhicheng wang School of Qilu Transportation Shandong UniversityJinan250002China China Railway 14th Bureau Group Co. LtdJinan250101China

The rapid discharge of cuttings from the air cushion chamber is crucial for the construction safety and excavation efficiency of the slurry *** studies have mainly focused on the transport characteristics of cuttings in the slurry discharge pipe,while the complete process of cuttings entering the slurry discharge pipe from the air cushion chamber until they are discharged was often *** on the CFD-DEM coupling method and combined with actual engineering,this paper established a numerical model that can more completely reflect the cuttings discharge process during slurry shield tunneling,and the effects of the slurry velocity at slurry gate and scouring pipes,inclination angle of slurry discharge pipe,cuttings diameter and shape coefficient were investigated by analyzing the variation in the mass flow rate,mass of discharged cuttings,and discharged *** results revealed that increasing the slurry velocity can promote the discharge of *** keep the discharged rate at a high level,it is recommended that the slurry velocity at the slurry gate should be greater than 0.15 m/*** the inclination angle of the discharge pipe is conducive to the rapid discharge of *** with large diameter or small shape coefficient are more prone to accumulate in the air cushion chamber and cause clogging *** research results not only help to improve engineers'understanding of cuttings discharge in slurry shield,but also provide practical guidance for formulating relevant construction measures.

关键词： Slurry shield CFD-DEM coupling method Cuttings discharge Aircushion chamber Slurry discharge pipe

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