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Triboelectric nanogenerator hybrid array driven by multiform natural energies and its applications in self-powered cathodic protection

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Science China(Technological Sciences) 2024年第3期67卷 878-890页

作者： SUN Weixiang YANG Di LUO Ning LI Hao wang daoai School of Materials Science and Engineering Shandong University of Science and TechnologyQingdao 266590China State Key Laboratoryof Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China Qingdao Center of Resource Chemistry and New Materials Qingdao 266100China

In view of the increasing energy shortage and environmental pollution, the collection of friction charges to achieve the conversion of various natural energies and provide in-situ cathodic protection for metals is a significant challenge. Here, we designed a dual device-structure TENG composite array with the triboelectric layer of linear siloxane-modified polyurethane(PU) coating. This array could achieve a comprehensive collection for multiple forms of nature energy and cathodic protection of metals in multi-weather conditions. For one thing, the wave-mode TENG based on tanker structure could collect wave energy and showed the output performance with a short-circuit current of 15.5 μA. For another thing, the droplet-mode TENG based on arc-shaped surface structure could collect raindrop kinetic energy and showed the output performance with a short-circuit current of 16.3 μA. Notably, the parallel array of wave-mode TENG(W-TENG) and droplet-mode TENG(D-TENG) could simultaneously collect wave energy and raindrop kinetic energy, which showed a short-circuit current of 30.7 μA. Besides, a selfpowered a cathodic protection system powered by the dual structure TENG array is assembled and the open-circuit potential drop of the carbon steel connected with the TENG array is about 450 mV. Compared with cathodic protection system powered by single structure TENG, the composite array could provide more effective corrosion resistance for marine equipment in rainy weather. Due to the characteristic for comprehensive collection of nature energy, the anti-corrosion system supplied by TENG parallel array possesses great application potential in the all-weather corrosion protection of metal machinery under complex marine conditions.

关键词： triboelectric nanogenerator hybrid structure array siloxane-modified polyurethane cathodic protection

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Hydrophobic MAO/FSG coating based TENG for self-healable energy harvesting and self-powered cathodic protection

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Science China(Technological Sciences) 2022年第3期65卷 726-734页

作者： LIU YuPeng SUN WeiXiang LI TingHua wang daoai State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China Qingdao Center of Resource Chemistry and New Materials Qingdao 266100China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China Technical Center of China Tobacco Yunnan Industrial Co. Ltd.Kunming 650231China

An organic/inorganic hybrid coating with self-healable hydrophobicity is prepared as triboelectrical layer by micro-arc oxidation(MAO)and fluorinated sol-gel(FSG)coating.The MAO/FSG hybrid coating-based TENG(MF-TENG)has a current output of31μA and voltage output of 870 V,which is eight times that of the MAO based TENG.Compared with organic coating,the organic/inorganic hybrid coating has good wear resistance.When the fluorine composition on the surface of the coating is damaged,the self-healing hydrophobicity and electrical output are achieved by transferring loaded perfluorosilane to the damaged surface.The fluorinated sol-gel coating is hydrophobic,which ensures that the coating has good corrosion resistance.Also,the electricity generated in triboelectrification could improve the anti-corrosion performance by cathodic protection.Based on the anti-corrosion,anti-wear and self-healing properties,the MF-TENG has potential applicability in the field of energy collection,energy supply,and corrosion protection.

关键词： triboelectric nanogenerator organic/inorganic hybrid coating energy collection corrosion resistance self-healing property

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A new strategy for tube leakage and blockage detection using bubble motion-based solid-liquid triboelectric sensor

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Science China(Technological Sciences) 2022年第2期65卷 282-292页

作者： ZHANG XiaoLong DONG Yang XU Xiang QIN HongLing wang daoai Hubei Key Laboratory of Hydroelectric Machinery Design&Maintenance China Three Gorges UniversityYichang 443002China State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China Qingdao Center of Resource Chemistry and New Materials Qingdao 266100China

Exploring a rapid, reliable, and practical means to detect blockages and leakages in liquid pipelines and accurately locate their positions is of great importance in practical engineering applications. Here, we report a bubble motion-based triboelectric sensor(BM-TES) for detecting and locating the blockages and leaks inside a plastic tube. This simple-designed, environment-friendly,non-damaging sensor is composed of several ring-shaped Cu electrodes distributed on a polytetrafluoroethylene tube. The selfpowered movement of the bubble under the action of buoyancy makes the inner wall of the tube change from the original solidliquid phase to the gas-solid-liquid phase, which results in a short-term contact and separation between the liquid and the wall.Based on the fractional triboelectric effect of the liquid-solid contact, an obvious real-time stable voltage peak will be generated where the detection bubble passes. The obvious peaks of the open-circuit voltage with respect to time correspond with the electrode distribution. Then, the peaks can be utilized as a robust and sensitive indicator for detecting blockage and leakage, as the number of obvious peaks of the open-circuit voltage is directly related to the blockage and leakage location. The blockage and leakage in a fluid tube were successfully detected using the BM-TES with an accuracy of 10 cm. In addition, the BE-TES was able to detect the water flow velocity in the pipe. The experimental results showed that BM-TES can provide a new strategy and method for liquid tube monitoring and has great potential application value in related fields.

关键词： solid-liquid triboelectric self-powered bubble blockage leakage

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A triboelectric/electromagnetic hybrid generator for efficient wind energy collection and power supply for electronic devices

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Science China(Technological Sciences) 2021年第9期64卷 2003-2011页

作者： XU GuanPing ZHENG YouBin FENG YanGe MA ShaoChen LUO Ning FENG Min CHEN ShouGang wang daoai State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China School of Materials Science and Engineering Ocean University of ChinaQingdao 266100China Qingdao Center of Resource Chemistry and New Materials Qingdao 266100China

Harvesting energy from ambient environment has been considered as a promising strategy for driving portable electronic devices in a sustainable way. A wind driven triboelectric-electromagnetic hybrid nanogenerator has been fabricated to convert wind energy into electricity. It is composed of an electromagnetic generator(EMG) and a triboelectric nanogenerator(TENG) with the output power of 35 and 0.32 mW, respectively when the wind speed is 5 m/s. Generally, TENG shows a low current output with a high voltage output characteristic, on the contrary the EMG shows a high current output and a low voltage output. This hybrid nanogenerator overcomes these problems and exhibits comprehensive and efficient performance on scavenging energy.Moreover, in view of the output performance and charging ability of the hybrid nanogenerator, it shows high stability, making it suitable for charging capacitors or batteries and driving portable electronics sustainably. A new structure of integrated TENG and EMG was designed to harvest wind energy, which shows potential applications in portable and small device power supply system, especially in the areas of remote mountains, deserts, islands, etc., as emergency power supply.

关键词： TENG electromagnetic generator wind energy self-powered selective power supply

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基于传统滑雪板的可穿戴式雪上摩擦力在线测量装置研究

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摩擦学学报（中英文） 2024年第1期44卷 97-106页

作者：于泽尧刘莹刘钰博万洋吴杨王道爱周峰南昌大学先进制造学院江西南昌330031 中国科学院兰州化学物理研究所固体润滑国家重点实验室甘肃兰州730000 烟台先进材料与绿色制造山东省实验室山东烟台264006 青岛市资源化学与新材料研究中心山东青岛266100

竞技滑雪运动中雪上摩擦阻力影响运动员比赛成绩,而雪上摩擦影响因素众多,雪上摩擦阻力评测一直是冰雪竞技运动中的一大挑战.本文中设计了1种基于传统滑雪板的可穿戴式雪上摩擦力在线测量装置,将多个三分量传感器合理布置在传统滑雪板上... 详细信息

竞技滑雪运动中雪上摩擦阻力影响运动员比赛成绩,而雪上摩擦影响因素众多,雪上摩擦阻力评测一直是冰雪竞技运动中的一大挑战.本文中设计了1种基于传统滑雪板的可穿戴式雪上摩擦力在线测量装置,将多个三分量传感器合理布置在传统滑雪板上,通过有线连接的方式,结合数据采集卡,对3个分量的力信号进行监测、采集和保存,并通过终端电脑实时反馈力信号变化.实验室静态测试中,该装置具有稳定的力学信号输出,并给出准确的摩擦系数测试结果.在模拟雪场测试时,其能够准确地评估不同雪上减阻蜡的润滑性能及其耐磨性能,还能够监测自由式滑雪运动中的犁式制动和犁式转弯等常规技术动作.该装置输出的力信号具有高精度和高灵敏度特性,为滑雪运动中雪上减阻蜡的性能评价、运动员施力动作监测等给出了1种可行方案.

关键词：滑雪板摩擦力在线测量装置三分量力传感器雪上摩擦力雪上减阻蜡性能评价动作监测

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Nanotribology of SiP nanosheets: Effect of thickness and sliding velocity

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Friction 2022年第12期10卷 2033-2044页

作者： Zishuai WU Tongtong YU Wei WU Jianxi LIU Zhinan ZHANG daoai wang Weimin LIU Center of Advanced Lubrication and Seal Materials School of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi’an 710072China State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China Qingdao Center of Resource Chemistry and New Materials Qingdao 266100China State Key Laboratory of Mechanical System and Vibration Shanghai Jiao Tong UniversityShanghai 200240China

Two-dimensional compounds combining group IV A element and group V A element were determined to integrate the advantages of the two groups.As a typical 2D group IV–V material,SiP has been widely used in photodetection and photocatalysis due to its high carrier mobility,appropriate bandgap,high thermal stability,and low interlayer cleavage energy.However,its adhesion and friction properties have not been extensively grasped.Here,large-size and high-quality SiP crystals were obtained by using the flux method.SiP nanosheets were prepared by using mechanical exfoliation.The layer-dependent and velocity-dependent nanotribological properties of SiP nanosheets were systematically investigated.The results indicate the friction force of SiP nanosheets decreases with the increase in layer number and reaches saturation after five layers.The coefficient of friction of multilayer SiP is 0.018.The mean friction force,frictional vibrations,and the friction strengthening effect can be affected by sliding velocity.Specially,the mean friction force increases with the logarithm of sliding velocity at nm/s scale,which is dominated by atomic stick-slip.The influence of frequency on frictional vibration is greater than speed due to the different influences on the change in contact quality.The friction strengthening saturation distance increases with the increase in speed for thick SiP nanosheets.These results provide an approach for manipulating the nanofriction properties of SiP and serve as a theoretical basis for the application of SiP in solid lubrication and microelectromechanical systems.

关键词： SiP nanosheet 2D material atomic force microscopy(AFM) nanotribology

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Electron transfer dominated triboelectrification at the hydrophobic/slippery substrate-water interfaces

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Friction 2023年第6期11卷 1040-1056页

作者： Yi CHEN Xiaojuan LI Chenggong XU daoai wang Jinxia HUANG Zhiguang GUO Weimin LIU State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou730000China Ministry of Education Key Laboratory for the Green Preparation and Application of Functional Materials Hubei UniversityWuhan430062China University of Chinese Academy of Sciences Beijing100049China

Triboelectric nanogenerator(TENG)based on triboelectrification has attracted wide attention due to its effective utilization of green energy sources such as marine energy.However,researches about liquid-liquid triboelectrification are still scanty as solid-liquid triboelectrification has been widely studied.Herein,this work focuses on the hydrophobic/slippery substrate-water interfacial triboelectrification based on the solid friction materials of polytetrafluoroethylene(PTFE)nanoparticles.The hydrophobic/slippery substrate-water interfacial triboelectrification are studied by assembling PTFE coated Al sheets and perfluoropolyether(PFPE)infused PTFE coated Al sheets(formed the slippery lubricant-infused surfaces(SLIPSs))as the friction electrode,and water as liquid friction materials,respectively.The results show that the hydrophobic TENG output performances improved as the PTFE nanoparticles cumulating,and the SLIPSs TENG output performances increased with the thinner PFPE thickness.Both the triboelectrification behavior of hydrophobic/SLIPSs TENG assembled in this work are dominated by the electron transfer.Thanks to the introduction of SLIPSs,the SLIPSs TENG exhibits superior stability and durability than the hydrophobic TENG.The investigation of hydrophobic/slippery substrate-water interfacial triboelectrification contributes to optimize the TENG performances,and expands the application in harsh environments including low temperature and high humidity on the ocean.

关键词： triboelectric nanogenerator(TENG) slippery lubricant-infused surfaces(SLIPSs) polytetrafluoroethylene(PTFE)nanoparticles perfluoropolyether(PFPE)

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Achieving macroscale superlubricity with ultra-short running-in period by using polyethylene glycol-tannic acid complex green lubricant

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Friction 2023年第5期11卷 748-762页

作者： Changhe DU Tongtong YU Zishuai WU Liqiang ZHANG Ruilin SHEN Xiaojuan LI Min FENG Yange FENG daoai wang State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China Qingdao Center of Resource Chemistry and New Materials Qingdao 266100China

Superlubricating materials can greatly reduce the energy consumed and economic losses by unnecessary friction.However,a long pre-running-in period is indispensable for achieving superlubricity;this leads to severe wear on the surface of friction pairs and has become one of the important factors in the wear of superlubricating materials.In this study,a polyethylene glycol-tannic acid complex green liquid lubricant(PEG10000-TA)was designed to achieve macroscale superlubricity with an ultrashort running-in period of 9 s under a contact pressure of up to 410 MPa,and the wear rate was only 1.19×10^(–8)mm^(3)·N^(−1)·m^(−1).This is the shortest running-in time required to achieve superlubricity in Si_(3)N_(4)/glass(SiO_(2)).The results show that the strong hydrogen bonds between PEG and TA molecules can significantly reduce the time required for the tribochemical reaction,allowing the lubricating material to reach the state of superlubrication rapidly.Furthermore,the strong hydrogen bond can share a large load while fixing free water molecules in the contact zone to reduce shear interaction.These findings will help advance the use of liquid superlubricity technology in industrial and biomedical.

关键词： superlubricity running-in period tannic acid green lubricant friction

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Triboelectrification based on double-layered polyaniline nanofibers for self-powered cathodic protection driven by wind

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Nano Research 2018年第4期11卷 1873-1882页

作者： Siwen Cui Youbin Zheng Jun Liang daoai wang State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical Physics Chinese Academy of Sciences Lanzhou 730000 China University of Chinese Academy of Sciences Beijing 100049 China

Polyaniline nanofibers （PANI NFs） are introduced to construct a wind-driven triboelectric nanogenerator （TENG） as a new power source for self-powered cathodic protection. PANI NFs serve as a friction layer to generate charges by harvesting wind energy as well as a conducting layer to transfer charges in TENG. A PANI NFs-based TENG exhibits a high output performance with a maximum output voltage of 375 V, short current circuit of 248 μA, and corresponding power of 14.5 mW under a wind speed of 15 m/s. Additionally, a self-powered anticorrosion system is constructed by using a PANI-based TENG as the power source. The immersion experiment and electrochemical measurements demonstrate that carbon steel coupled with the wind-driven TENG is effectively protected with an evident open circuit potential drop and negative shift in the corrosion potential. The smart self-powered device is promising in terms of applications to protect metals from corrosion by utilizing wind energy in ambient conditions.

关键词： polyaniline,triboelectric nanogenerator,wind-driven,self-powered,cathodic protection

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Hydrophobic organic coating based water–solid TENG for water-flow energy collection and self-powered cathodic protection

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Frontiers of Materials Science 2021年第4期15卷 601-610页

作者： Yupeng LIU Guoyun SUN Ying LIU Weixiang SUN daoai wang State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China Institute of Materials Science and Engineering Ocean University of ChinaQingdao 266100China Qingdao Center of Resource Chemistry and New Materials Qingdao 266100China School of Materials Science and Engineering Shandong University of Science and TechnologyQingdao 266100China

Water-solid triboelectric nanogenerators(TENGs),as new energy collection devices,have attracted increasing attention in ocean energy harvesting and selfpowered sensing.Polyacrylic acid(PAA)coating,usually used on the surface of marine equipment,has the property of anti-aging and anti-wear but limits triboelectrical output when used with TENGs.In this paper,polyacrylic acid coating was modified with fluorinated polyacrylate resin(F-PAA)to increase its triboelectrical output,by 6 times,and also to increase its anti-corrosion property.In addition,the corrosion resistance property can be further enhanced by cathodic protection using the electrical output generated by the water-flow triboelectrical energy transfer process.Given their easy fabrication,water-flow energy harvesting,and corrosion resistance,PAA/F-PAA coating-based TENGs have promising applications in river and ocean energy collection and corrosion protection.

关键词： TENG hydrophobic coating energy collection anticorrosion cathodic protection

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