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Enhanced helium ion irradiation tolerance in a Fe-Co-Ni-Cr-Al-ti high-entropy alloy with L12 nanoparticles

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Journal of Materials Science & technology 2023年第12期143卷 169-177页

作者： Y.L.Zhao F.L.Meng t.Yang J.H.Luan S.F.Liu G.M.Yeli w.t.lin w.H.Liu X.J.Liu C.t.Liu J.J.Kai School of Materials Science and Engineering Harbin Institute of Technology(Shenzhen)Shenzhen 518055China School of Materials Science and Engineering Southern University of Science and TechnologyShenzhen 518055China Department of Materials Science and Engineering Mechanical Behavior Division of Shenyang National Laboratory for Materials ScienceCity University of Hong KongHong KongChina Department of Mechanical Engineering City University of Hong KongHong KongChina Institute of Nuclear&New Energy technology Tsinghua UniversityBeijing 100084China

L12-strengthened high entropy alloys(HEAs)with excellent room and high-temperature mechanical prop-erties have been proposed as promising candidates as structural materials for advanced nuclear ***,knowledge about their radiation response is fairly *** the present work,a novel HEA with a high density of L12 nanoparticles was irradiated with He ion at 500°*** electron microscope(tEM)and atom probe tomography(APt)were employed to study the evolution of mi-crostructural stability and radiation-induced *** to the single-phase FeCoNiCr HEA,the main microstructural features were numerous large faulted dislocation loops and helium *** the irradiation resistance of the present L12-strengthened HEA is much improved in terms of reduced bubble size,which could be attributed to the considerable He trapping efficiency of the coherent pre-cipitate/matrix interface and the enhanced capability of the interface for damage elimination when the matrix channel width is *** analysis revealed that an inverse-Kirkendall-mechanism-dominated radiation-induced segregation(RIS)occurs around bubbles,where a significant Co enrichment and Ni de-pletion can be clearly *** addition,the competing dynamics of ballistic mixing and elemental clustering that raised from the irradiation-enhanced diffusion in a highly supersaturated matrix,along with the low precipitation nucleation barrier due to the small lattice misfit,lead to a dynamical pre-cipitation dissolution and re-precipitation appears under *** a promising phenomenon is expected to promote a potential self-healing effect and could in turn provide a sustainable irradiation tolerance over the operational lifetime of a reactor.

关键词： L12 nanoparticles High-entropy alloy Helium bubble Phase stability Radiation-induced segregation

He-enhanced heterogeneity of radiation-induced segregation in FeNiCoCr high-entropy alloy

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Journal of Materials Science & technology 2022年第6期101卷 226-233页

作者： w.t.lin G.M.Yeli G.wang J.H.lin S.J.Zhao D.Chen S.F.Liu F.L.Meng Y.R.Li F.He Y.Lu J.J.Kai Department of Mechanical Engineering City University of Hong KongHong KongChina Institute of Nuclear&New Energy technology Tsinghua UniversityBeijingChina Department of Physics Southern University of Science and TechnologyShenzhenChina Centre for Advanced Nuclear Safety and Sustainable Development City University of Hong KongHong KongChina School of Environmental Science and Engineering Southern University of Science and TechnologyShenzhenChina School of Materials Science and Engineering Shanghai UniversityShanghaiChina Nano-Manufacturing Laboratory(NML) City University of Hong Kong Shenzhen Research InstituteShenzhenChina

Radiation-induced segregation(RIS) is a typical non-equilibrium process that can dramatically alter the behavior of defect sinks and material properties under irradiation. However, RIS mechanisms have been rarely studied around small He bubbles owing to the technical challenges involved in direct measurements of local chemistry. Here, using state-of-the-art atom probe tomography, we report the RIS behavior near He bubbles in the Fe Ni Co Cr high-entropy alloy that indicates Co segregates most strongly, followed by weaker Ni segregation, whereas Fe and Cr are depleted almost to the same degree. Exceptionally, the magnitude of Co segregation around He bubbles is higher than previously measured values at voids and dislocation loops. Electron energy-loss spectroscopy was used to measure the He density and pressure inside individual bubbles. we demonstrate that He bubbles are over-pressurized at the irradiation temperature that could result in the vacancy bias and the subsequent vacancy-dominated RIS ***-principles calculations further reveal that there are repulsive interactions between He and Co atoms that may reduce the frequency of Co-vacancy exchange. As a result, He atoms likely retard Co diffusion via the vacancy mechanism and enhance the heterogeneity of RIS in Co-containing multicomponent alloys. these insights could provide the basis for understanding He effects in nuclear materials and open an avenue for tailoring the local chemical order of medium-and high-entropy alloys.

关键词： High-entropy alloy Radiation-induced segregation He bubbles Atom probe tomography Electron energy-loss spectroscopy

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超级贝氏体钢的热处理

热处理 2015年第6期30卷 44-50页

作者： H.t.Chang H.w.Yen w.t.lin C.Y.Huang J.R.Yang 顾剑锋 Department of Materials Science and Engineering National Taiwan University Iron and Steel R&D Department China Steel Corporation 本刊编委会上海交通大学

研究了分别含有0.0005%(质量分数)和0.0024%(质量分数)硼的两种试验用高硅高碳钢以获得超级贝氏体组织。奥氏体化后,试样分别在3种不同的等温温度(150℃、200℃和300℃)保温不同时间。采用带有显微硬度测定的光学显微镜和透射电镜观察... 详细信息

研究了分别含有0.0005%(质量分数)和0.0024%(质量分数)硼的两种试验用高硅高碳钢以获得超级贝氏体组织。奥氏体化后,试样分别在3种不同的等温温度(150℃、200℃和300℃)保温不同时间。采用带有显微硬度测定的光学显微镜和透射电镜观察试样的微观组织。结果表明,200℃等温转变10天后,两种钢均获得了高体积分数的含有纳米级贝氏体铁素体亚单元的束状组织,具有高达675 HV1的超高显微硬度。添加0.0024%(质量分数)硼能促进200℃等温处理初期的贝氏体相变,但对缩短相变的完成时间没有明显的影响。在150℃和300℃等温不能得到大量的贝氏体组织。

关键词：贝氏体硼热处理相变纳米级组织 tEM

Fine-tuning the spatial allocation of phytohormones for smart canopy, smart breeding, and smart agriculture

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Science China Life Sciences 2025年第1期 309-310页

作者： tao Zhou lin Li National Key Laboratory of Crop Genetic Improvement Huazhong Agricultural University HuBei HongShan Laboratory

the dual challenges of global climate change and population growth have increased demand for higher crop yields per unit area. the innovative technology of smart agriculture aims to synergize breeding, cultivation, and production through the application of biological and informatics technologies. Historically, the “Green Revolution” introduced semidwarf varieties of certain key crops by utilizing mutations affecting gibberellin pathways, which significantly increased planting densities and yields.

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Interannual variability of boreal summer intraseasonal oscillation over the northwestern Pacific influenced by the Pacific Meridional Mode

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Atmospheric and Oceanic Science Letters 2025年第1期18卷 6-11页

作者： Haoyu Zhou Pang-Chi Hsu lin Chen Yitian Qian Key Laboratory of Meteorological Disaster Ministry of Education/Joint International Research Laboratory of Climate and Environmental Change/Collaborative Innovation Center on Forecast and Evaluation of Meteorological DisastersNanjing University of Information Science and TechnologyNanjingChina

During the boreal summer,intraseasonal oscillations exhibit significant interannual variations in intensity over two key regions:the central-western equatorial Pacific(5°S-5°N,150°E-150°w)and the subtropical Northwestern Pacific(10°-20°N,130°E-175°w).the former is well-documented and considered to be influenced by the ENSO,while the latter has received comparatively less attention and is likely influenced by the Pacific Meridional Mode(PMM),as suggested by partial correlation analysis *** elucidate the physical processes responsible for the enhanced(weakened)intraseasonal convection over the subtropical northwestern Pacific during warm(cold)PMM years,the authors employed a moisture budget *** findings reveal that during warm PMM years,there is an increase in summer-mean moisture over the subtropical northwestern *** increase interacts with intensified vertical motion perturbations in the region,leading to greater vertical moisture advection in the lower troposphere and consequently resulting in convective *** a process is pivotal in amplifying intraseasonal convection *** observational findings were further verified by model experiments forced by PMM-like sea surface temperature patterns.

关键词： Boreal summer intraseasonal oscillation Interannual variability Pacific Meridional Mode Moisture budget analysis

Boosting bidirectional sulfur conversion enabled by introducing boron-doped atoms and phosphorus vacancies in Ni2P for lithium-sulfur batteries

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Journal of Energy Chemistry 2025年第1期100卷 760-769页

作者： lin Peng Yu Bai Hang Li Meixiu Qu Zhenhua wang Kening Sun Advanced Research Institute of Multidisciplinary Science Beijing Institute of Technology Beijing Key Laboratory of Chemical Power Source and Green Catalysis School of Chemistry and Chemical Engineering Beijing Institute of Technology

Lithium-sulfur （Li-S） batteries have gained great attention due to the high theoretical energy density and low cost,yet their further commercialization has been obstructed by the notorious shuttle effect and sluggish redox ***,we supply a strategy to optimize the electron structure of Ni2P by concurrently introducing B-doped atoms and P vacancies in Ni2P （Vp-B-Ni2P）,thereby enhancing the bidirectional sulfur *** study indicates that the simultaneous introduction of B-doped atoms and P vacancies in Ni2P causes the redistribution of electron around Ni atoms,bringing about the upward shift of d-band center of Ni atoms and effective d-p orbital hybridization between Ni atoms and sulfur species,thus strengthening the chemical anchoring for lithium polysulfides （LiPSs） as well as expediting the bidirectional conversion kinetics of sulfur ***,theoretical calculations reveal that the incorporation of B-doped atoms and P vacancies in Ni2P selectively promotes Li2S dissolution and nucleation ***,the Li-S batteries with Vp-B-Ni2P-separators present outstanding rate ability of 777 m A h g-1at 5 C and high areal capacity of 8.03 mA h cm-2under E/S of 5μL mg-1and sulfur loading of 7.20 mg *** work elucidates that introducing heteroatom and vacancy in metal phosphide collaboratively regulates the electron structure to accelerate bidirectional sulfur conversion.

关键词： Lithium sulfur batteries

Projective Hilbert modules and sequential approximations

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Science China Mathematics 2025年第1期 137-168页

作者： Lawrence G.Brown Huaxin lin Department of Mathematics Purdue University Department of Mathematics East China Normal University Department of Mathematics University of Oregon Shanghai Institute for Mathematics and Interdisciplinary Sciences

we show that when A is a separable C*-algebra,every countably generated Hilbert A-module is projective（with bounded module maps as morphisms）.we also study the approximate extensions of bounded module *** the case where A is a σ-unital simple C*-algebra with strict comparison,and every strictly positive lower semicontinuous affine function on quasitraces can be realized as the rank of an element in the Cuntz semigroup,we show that the Cuntz semigroup is equivalent to unitarily equivalent classes of countably generated Hilbert A-modules if and only if A has stable rank one.

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Electrocatalytic cleavage of a lignin β-O-4 model compound and coupling with nitrogen-containing aromatics using Prussian blue analogue-derived nickel–cobalt spinel

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Journal of Energy Chemistry 2025年第1期100卷 628-636页

作者： Yi Qi Xueying Chen Bowen Liu Xuliang lin Xueqing Qiu Yanlin Qin Guangdong Provincial Key Laboratory of Plant Resources Biorefinery School of Chemical Engineering and Light Industry Guangdong University of Technology Guangdong Provincial Laboratory of Chemistry and Fine Chemical Engineering Jieyang Center Guangdong Basic Research Center of Excellence for Ecological Security and Green Development Guangdong University of Technology

Electrochemical conversion of lignin for the production of high-value heterocyclic aromatic compounds has great *** demonstrate the targeted synthesis and cation modulation of NiCo2O4spinel nanoboxes,synthesized via cation exchange and calcination *** catalysts exhibit excellent efficacy in the electrocatalytic conversion of lignin model compounds,specifically 2-phenoxy-1-phenylethanol,into nitrogen-containing aromatics,achieving high conversion rates and *** catalysts were synthesized via a cation exchange and calcination oxidation process,using Prussian blue nanocubes as *** porous architecture and polymetallic composition of the NiCo2O4spinel demonstrated superior performance in electrocatalytic oxidative coupling,achieving a 99.2 wt%conversion rate of the 2-phenoxy-1-phenylethanol with selectivities of 37.5 wt%for quinoline derivatives and 31.5 wt%for *** innovations include the development of a sustainable one-pot synthesis method for quinoline derivatives,the elucidation of a multistage reaction pathway involving CAO bond cleavage,hydroxyaldol condensation,and CAN bond formation,and a deeper mechanistic understanding derived from DFt *** work establishes a new strategy for lignin valorization,offering a sustainable route to produce high-value nitrogen-containing aromatics from renewable biomass under mild conditions,without the need for additional reagents.

关键词： Spinel Biomass valorization Electrocatalysis Lignin oxidation Coupling

Pyroptosis,ferroptosis,and autophagy in spinal cord injury:regulatory mechanisms and therapeutic targets

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Neural Regeneration Research 2025年第10期20卷 2787-2806页

作者： Qingcong Zheng Du wang Rongjie lin weihong Xu Department of Spinal Surgery the First Affiliated Hospital of Fujian Medical UniversityFuzhouFujian ProvinceChina Arthritis Clinical and Research Center Peking University People’s HospitalBeijingChina Department of Orthopedic Surgery Fujian Medical University Union HospitalFuzhouFujian ProvinceChina

Regulated cell death is a form of cell death that is actively controlled by *** studies have shown that regulated cell death plays a key role after spinal cord *** and ferroptosis are newly discovered types of regulated cell deaths that have been shown to exacerbate inflammation and lead to cell death in damaged spinal ***,a complex form of cell death that is interconnected with various regulated cell death mechanisms,has garnered significant attention in the study of spinal cord *** injury triggers not only cell death but also cellular survival *** signaling pathways play pivotal roles in influencing the processes of both deterioration and repair in spinal cord injury by regulating pyroptosis,ferroptosis,and ***,this review aims to comprehensively examine the mechanisms underlying regulated cell deaths,the signaling pathways that modulate these mechanisms,and the potential therapeutic targets for spinal cord *** analysis suggests that targeting the common regulatory signaling pathways of different regulated cell deaths could be a promising strategy to promote cell survival and enhance the repair of spinal cord ***,a holistic approach that incorporates multiple regulated cell deaths and their regulatory pathways presents a promising multi-target therapeutic strategy for the management of spinal cord injury.

关键词： autophagy cell death ferroptosis inflammation pathological mechanisms pyroptosis regulated cell death regulatory pathways spinal cord injury therapeutic targets