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Universal insertion of molecules in ionic compounds under pressure

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National Science Review 2024年第1期11卷 120-128页

作者： Feng Peng Yanming ma Chris j.Pickard Hanyu Liu maosheng Miao College of Physics and Electronic Information Luoyang Normal University Department of Chemistry and Biochemistry California State University Northridge State Key Laboratory of Superhard materials & Key Laboratory of material Simulation Methods and Software of Ministry of Education College of Physics Jilin University International Center of Future Science Jilin University Department of materials Science & Metallurgy University of Cambridge Advanced Institute for materials Research Tohoku University Department of Earth Science University of California Santa Barbara

Using first-principles calculations and crystal structure search methods, we found that many covalently bonded molecules such as H2, N2, CO2, NH3, H2O and CH4may react with NaC l, a prototype ionic solid,and form stable compounds under pressure while retaining their molecular structure. These molecules,despite whether they are homonuclear or heteronuclear, polar or non-polar, small or large, do not show strong chemical interactions with surrounding Na and Cl ions. In contrast, the most stable molecule among all examples, N2, is found to transform into cyclo-N5-anions while reacting with NaC l under high pressures. It provides a new route to synthesize pentazolates, which are promising green energy materials with high energy density. Our work demonstrates a unique and universal hybridization propensity of covalently bonded molecules and solid compounds under pressure. This surprising miscibility suggests possible mixing regions between the molecular and rock layers in the interiors of large planets.

关键词： molecule-solid hybrid materials high-pressure crystal structure prediction density functional theory planet interior

Microarray analysis of signalling interactions between inflammation and angiogenesis in subchondral bone in temporomandibular joint osteoarthritis

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Biomaterials Translational 2024年第2期5卷 175-184页

作者： Qin w. Gao j. Yan j. Han X. Lu w. ma Z. Niu L. jiao K. Department of Stomatology Tangdu Hospital and State Key Laboratory of Oral and Maxillofacial Reconstruction and Regeneration School of Stomatology The Fourth Military Medical University Shaanxi Province Xi’an China State Key Laboratory of Oral and maxillofacial Reconstruction and Regeneration and National Clinical Research Centre for Oral Diseases Shaanxi Key Laboratory of Stomatology School of Stomatology The Fourth Military Medical University Shaanxi Province Xi’an China

Inflammation and angiogenesis, the major pathological changes of osteoarthritis (OA), are closely associated with joint pain; however, pertinent signalling interactions within subchondral bone of osteoarthritic joints and potential contribution to the peripheral origin of OA pain remain to be elucidated. Herein we developed a unilateral anterior crossbite mouse model with osteoarthritic changes in the temporomandibular joint. Microarray-based transcriptome analysis, besides quantitative real-time polymerase chain reaction, was performed to identify differentially expressed genes (DEGs). Overall, 182 DEGs (fold change ≥ 2, P were identified between the control and unilateral anterior crossbite groups: 168 were upregulated and 14 were downregulated. On subjecting significant DEGs to enrichment analyses, inflammation and angiogenesis were identified as the most affected. Inflammation-related DEGs were mainly enriched in T cell activation and differentiation and in the mammalian target of rapamycin/nuclear factor-κB/tumour necrosis factor signalling. Furthermore, angiogenesis-related DEGs were mainly enriched in the Gene Ontology terms angiogenesis regulation and vasculature development and in the KEGG pathways of phosphoinositide 3-kinase-protein kinase B/vascular endothelial growth factor/hypoxia-inducible factor 1 signalling. Protein– protein interaction analysis revealed a close interaction between inflammation-and angiogenesis-related DEGs, suggesting that phosphatidylinositol-4,5-bisphosphate 3-kinase catalytic subunit delta (Pi3kcd), cathelicidin antimicrobial peptide (Camp), C-X-C motif chemokine receptor 4 (Cxcr4), and MYB proto-oncogene transcription factor (Myb) play a central role in their interaction. To summarize, our findings reveal that in subchondral bone of osteoarthritic joints, signal interaction is interrelated between inflammation and angiogenesis and associated with the peripheral origin of OA pain; moreover, our data highlight potential t

关键词： angiogenesis inflammation osteoarthritic pain osteoarthritis subchondral bone temporomandibular joint (TMj)

Potential Secretory Transporters and Biosynthetic Precursors of Biological Nitrification Inhibitor 1,9-Decanediol in Rice as Revealed by Transcriptome and Metabolome Analyses

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Rice science 2024年第1期31卷 87-102页

作者： DI Dongwei ma Mingkun ZHANG Xiaoyang LU Yufang Herbert j.KRONZUCKER SHI weiming State Key Laboratory of Soil and Sustainable Agriculture Institute of Soil ScienceChinese Academy of SciencesNanjing 210008China School of Food Science and Engineering Foshan UniversityFoshan 528000China School of BioSciences The University of MelbourneParkvilleVIC 3010Australia University of Chinese Academy of Sciences Beijing 100049China

Biological nitrification inhibitors(BNIs)are released from plant roots and inhibit the nitrification activity of microorganisms in soils,reducing NO_(3)^(‒)leaching and N2O emissions,and increasing nitrogenuse efficiency(NUE).Several recent studies have focused on the identification of new BNIs,yet little is known about the genetic loci that govern their biosynthesis and *** applied a combined transcriptomic and metabolomic analysis to investigate possible biosynthetic pathways and transporters involved in the biosynthesis and release of BNI 1,9-decanediol(1,9-D),which was previously identified in rice root *** results linked four fatty acids,icosapentaenoic acid,linoleate,norlinolenic acid,and polyhydroxy-α,ω-divarboxylic acid,with 1,9-D biosynthesis and three transporter families,namely the ATP-binding cassette protein family,the multidrug and toxic compound extrusion family,and the major facilitator superfamily,with 1,9-D release from roots into the soil *** finding provided candidates for further work on the genes implicated in the biosynthesis and secretion of 1,9-D and pinpoint genetic loci for crop breeding to improve NUE by enhancing 1,9-D secretion,with the potential to reduce NO_(3)^(‒)leaching and N2O emissions from agricultural soils.

关键词： 1,9-decanediol biological nitrification inhibitor metabolomic analysis nitrogen-use efficiency transcriptomic analysis

Nuance of inward rectifying potassium(Kir)channel dysfunctions in neurodegenerative diseases

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Neural Regeneration Research 2024年第6期19卷 1195-1196页

作者： Benjamin Garland Linlin ma Griffith Institute for Drug Discovery&School of Environment and Science Griffith UniversityNathanBrisbaneQLDAustralia

Neurodegenerative disorders are highly prevalent and diverse in *** manifestation largely depends on the cell types involved,with aberrant inflammatory episodes progressively inducing a constellation of phenotypes that are classified into specific diseases based on their neuropathological *** two most prevalent neurodegenerative diseases worldwide,Alzheimer’s disease(AD)and Parkinson’s disease(PD),for example,share notable similarities,yet they differ in terms of the specific cell types lost within the central nervous system(CNS).The significant and progressive loss of cortical and certain subcortical neurons in various regions is a major defining trait of *** contrast,the specific loss of dopaminergic neurons(DA)within the substantial nigra pars compacta(SNpc)is sufficient to cause motor symptoms associated with *** devastating condition arising from neurodegeneration within the CNS,amyotrophic lateral sclerosis(ALS),results in the progressive death of upper and lower motor *** degeneration originates in oligodendrocytes,whose defective myelination abilities lead to the denervation of the anterior horn,aggravating motor neuron death.

关键词： diseases degenerative degeneration

Elastic wave insulation and propagation control based on the programmable curved-beam periodic structure

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Applied mathematics and Mechanics(English Edition) 2024年第10期45卷 1791-1806页

作者： jiajia maO Hong CHENG Tianxue ma Beijing Key Laboratory of Nonlinear Vibrations and Strength of Mechanical Structures Department of Mechanics School of Mathematics Statistics and MechanicsBeijing University of Technology Department of Mechanics School of Physical Science and EngineeringBeijing Jiaotong University

Curved-beams can be used to design modular multistable metamaterials(MMMs) with reprogrammable material properties, i.e., programmable curved-beam periodic structure(PCBPS), which is promising for controlling the elastic wave *** PCBPS is theoretically equivalent to a spring-oscillator system to investigate the mechanism of bandgap, analyze the wave propagation mechanisms, and further form its geometrical and physical criteria for tuning the elastic wave propagation. with the equivalent model, we calculate the analytical solutions of the dispersion relations to demonstrate its adjustability, and investigate the wave propagation characteristics through the PCBPS. To validate the equivalent system, the finite element method(FEM) is *** is revealed that the bandgaps of the PCBPS can be turned on-and-off and shifted by varying its physical and geometrical characteristics. The findings are highly promising for advancing the practical application of periodic structures in wave insulation and propagation control.

关键词： 74j05 74Q10 curved-beam based periodic structure dispersion relation equivalent stiffness O326 spring-oscillator system wave propagation

Enhanced properties of stone coal-based composite phase change materials for thermal energy storage

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International journal of Minerals,Metallurgy and materials 2024年第1期31卷 206-215页

作者： Baoshan Xie Huan ma Chuanchang Li jian Chen Key Laboratory of Renewable Energy Electric-Technology of Hunan Province School of Energy and Power EngineeringChangsha University of Science and TechnologyChangsha 410114China State Key Laboratory of Disaster Prevention and Reduction for Power Grid Changsha University of Science and TechnologyChangsha 410114China

Phase change materials (PCMs) can be incorporated with low-cost minerals to synthesize composites for thermal energy storage in building *** coal (SC) after vanadium extraction treatment shows potential for secondary utilization in composite *** prepared SC-based composite PCMs with SC as a matrix,stearic acid (SA) as a PCM,and expanded graphite (EG) as an *** combined roasting and acid leaching treatment of raw SC was conducted to understand the effect of vanadium extraction on promoting loading *** showed that the combined treatment of roasting at 900℃ and leaching increased the SC loading of the composite by 6.2%by improving the specific surface *** loading capacity and thermal conductivity of the composite obviously increased by 127%and 48.19%,respectively,due to the contribution of 3wt% *** data were supported by the high load of 66.69%and thermal conductivity of 0.59 w·m^(-1)·K-1of the designed *** obtained composite exhibited a phase change temperature of 52.17℃,melting latent heat of 121.5 j·g^(-1),and good chemical *** SC-based composite has prospects in building applications exploiting the secondary utilization of minerals.

关键词： thermal energy storage phase change material stone coal vanadium extraction secondary utilization

Simulation of nuclear isomer production in laser-induced plasma

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matter and Radiation at Extremes 2024年第5期9卷 1-9页

作者： Zhiguo ma Yumiao wang Yi Yang Youjing wang Kai Zhao Yixin Li Changbo Fu wanbing He Yugang ma Key Laboratory of Nuclear Physics and Ion-Beam Application(MoE) Institute of Modern PhysicsFudan UniversityShanghai 200433China

Nuclear isomers play essential roles in various fields,including stellar nucleosynthesis,nuclear clocks,nuclear batteries,clean nuclear energy,and-ray *** technological advances in high-intensity lasers have made it possible to excite or de-excite nuclear isomers using table-top laser *** a particle-in-cell code,we investigate the interaction of a laser with a nanowire array and calculate the production rates of the^(73m)Ge(E_(1)=13.3 keV)and^(107m)Ag(E_(1)=93.1 keV)***^(73m1)Ge,production by Coulomb excitation is found to contribute a peak efficiency of 1.0×10^(19) particles s^(−1)j^(−1),while nuclear excitation by electron capture(NEEC)contributes a peak of 1.65×10^(11)particles s^(−1)j^(−1).These results indicate a high isomeric production ratio,as well as demonstrating the potential for confirming the existence of NEEC,a long-expected but so far experimentally unobserved fundamental process.

关键词： process. isomers excitation

Night warming increases wheat yield by improving pre-anthesis plant growth and post-anthesis grain starch biosynthesis

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journal of Integrative Agriculture 2024年第2期23卷 536-550页

作者： Yonghui Fan Boya Qin jinhao Yang Liangliang ma Guoji Cui wei He Yu Tang wenjing Zhang Shangyu ma Chuanxi ma Zhenglai Huang College of Agronomy Anhui Agricultural University/Key Laboratory of Wheat Biology and Genetic Improvement in South Yellow&Huai River ValleyMinistry of Agriculture and Rural AffairsHefei 230036China Xianyang Central Station for Agricultural Technology Extension Xianyang 712000China

Global climate change is characterized by asymmetric warming,i.e.,greater temperature increases in winter,spring,and nighttime than in summer,autumn,and *** experiments were conducted using four wheat cultivars,namely‘Yangmai 18’(YM18),‘Sumai 188’(SM188),‘Yannong 19’(YN19),and‘Annong 0711’(AN0711),in the two growing seasons of 2019-2020 and 2020-2021,with passive night warming during different periods in the early growth *** treatments were night warming during the tillering-jointing(Nw_(T-j)),jointing-booting(Nwj-B),and booting-anthesis(NwB-A)stages,with ambient temperature(NN)as the *** effects of night warming during different stages on wheat yield formation were investigated by determining the characteristics of dry matter accumulation and translocation,as well as sucrose and starch accumulation in wheat *** wheat yields of all four cultivars were significantly higher in Nw_(T-j)than in NN in the 2-year *** yield increases of semi-winter cultivars YN19 and AN0711 were greater than those of spring cultivars YM18 and *** Nw_(T-j)increased wheat yield mainly by increasing the 1,000-grain weight and the number of fertile spikelets,and it increased dry matter accumulation in various organs of wheat at the anthesis and maturity stages by increasing the growth rate at the vegetative growth *** flag leaf and spike showed the largest increases in dry matter ***_(T-j)also increased the grain sucrose and starch contents in the early and middle grain-filling stages,promoting yield ***,night warming between the tillering and jointing stages increased the pre-anthesis growth rate,and thus,wheat dry matter production,which contributed to an increase in wheat yield.

关键词： wheat asymmetric warming dry matter accumulation and translocation starch yield

Reduced-order modeling and vibration transfer analysis of a fluid-delivering branch pipeline that consider fluid–solid interactions

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Frontiers of Mechanical Engineering 2024年第2期19卷 75-97页

作者： wenhao jI Hongwei ma wei SUN Yinhang CAO School of Mechanical Engineering and Automation Northeastern UniversityShenyang 110819China Key Laboratory of Vibration and Control of Aero-Propulsion Systems(Ministry of Education) Northeastern UniversityShenyang 110819China College of Power and Energy Engineering Harbin Engineering UniversityHarbin 150001China

The efficient dynamic modeling and vibration transfer analysis of a fluid-delivering branch pipeline(FDBP)are essential for analyzing vibration coupling effects and implementing vibration reduction ***,this study proposes a reduced-order dynamic modeling method suitable for FDBPs and then analyzes the vibration transfer *** the modeling method,the finite element method and absorbing transfer matrix method(ATMM)are integrated,considering the fluid–structure coupling effect and fluid *** dual-domain dynamic substructure method is developed to perform the reduced-order modeling of FDBP,and ATMM is adopted to reduce the matrix order when solving fluid ***,the modeling method is validated by experiments on an H-shaped branch ***,transient and steady-state vibration transfer analyses of FDBP are performed,and the effects of branch locations on natural characteristics and vibration transfer behavior are *** show that transient vibration transfer represents the transfer and conversion of the kinematic,strain,and damping energies,while steady-state vibration transfer characteristics are related to the vibration *** addition,multiple-order mode exchanges are triggered when branch locations vary in frequency-shift regions,and the mode-exchange regions are also the transformation ones for vibration transfer patterns.

关键词： fluid-delivering branch pipeline vibration transfer analysis reduced-order modeling fluid-solid interactions finite element method absorbing transfer matrix method