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Bio-Based Rigid Polyurethane Foams for Cryogenic Insulation

Journal of Renewable Materials 2024年第3期12卷 585-602页

作者： Laima Vevere Beatrise Sture vladimir yakushin Mikelis Kirpluks Ugis Cabulis Latvian State Institute of Wood Chemistry RigaLV-1006Latvia

Cryogenic insulation material rigid polyurethane(PU)foams were developed using bio-based and recycled *** obtained from tall oil fatty acids produced as a side stream of wood biomass pulping and recycled polyethylene terephthalate were used to develop rigid PU foam *** 4th generation physical blowing agents with low global warming potential and low ozone depletion potential were used to develop rigid PU foam cryogenic insulation with excellent mechanical and thermal *** rigid PU foams had a thermal conductivity coefficient as low as 0.0171 W/m·K and an apparent density of 37-40 kg/m^(3).The developed rigid PU foams had anisotropic compression strength properties,which were higher parallel to the foaming ***,the compression strength was also influenced by the type of applied bio-based *** bio-based polyols with higher OH group functionality delivered higher crosslinking density of polymer matrix;thus,the mechanical properties were also *** mechanical strength of the foams increased when materials were tested at liquid nitrogen temperature due to the stiffening of the polymer *** thermal properties of the developed materials were determined using differential scanning calorimetry,dynamic mechanical analysis,and thermogravimetric analysis ***,the developed rigid PU foams had good adhesion to the aluminium substrate before and after applying cyroshock and an excellent safety coefficient of *** PU foams developed using Solstice LBA delivered adhesion strength of~0.5 MPa and may be considered for application as cryogenic insulation in the aerospace industry.

关键词： Cryogenic insulation polyurethanes tall oil 4th generation physical blowing agents

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