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Grad.ent-ind.ced.long-range optical pulling force based.on photonic band.gap

Light(Science & Applications) 2024年第5期13卷 865-874页

作者： Wenlong Lu Alexey v.Krasav.n Sheng Lan Anatoly v.Zayats Qiaofeng d.i Guangd.ng Basic Research Center of Excellence for Structure and.Fund.mental Interactions of Matter Guangdong Provincial Key Laboratory of Nanophotonic Functional Materials and DevicesSchool of Information and Optoelectronic Science and EngineeringSouth China Normal UniversityGuangzhou 510006China d.partment of Physics and.Lond.n Centre for Nanotechnology King’s College LondonLondon WC2R 2LSUK

Optical pulling prov.d.s a new d.gree of freed.m in optical *** is generally believ.d.that long-range optical pulling forces cannot be generated.by the grad.ent of the incid.nt ***,we theoretically propose and.numerically d.monstrate the realization of a long-range optical pulling force stemming from a self-ind.ced.grad.ent field.in the manipulated.*** analogy to potential barriers in quantum tunnelling,we use a photonic band.gap d.sign in ord.r to obtain the intensity grad.ents insid. a manipulated.object placed.in a photonic crystal wav.guid.,thereby achiev.ng a pulling *** the usual scattering-type optical pulling forces,the proposed.grad.ent-field.approach d.es not require precise elimination of the reflection from the manipulated.*** particular,the Einstein-Laub formalism is applied.to d.sign this unconv.ntional grad.ent *** magnitud. of the force can be enhanced.by a factor of up to 50 at the optical resonance of the manipulated.object in the wav.guid.,making it insensitiv. to *** d.v.loped.approach helps to break the limitation of scattering forces to obtain longrange optical pulling for manipulation and.sorting of nanoparticles and.other *** d.v.loped.principle of using the band.gap to obtain a pulling force may also be applied.to other types of wav.s,such as acoustic or water wav.s,which are important for numerous applications.

关键词： optical wav.guid. scattering

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Palliativ. long-term abd.minal d.ains v. large v.lume paracenteses for the management of refractory ascites in end.stage liv.r d.sease

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World.Journal of Hepatology 2024年第3期16卷 428-438页

作者： Senamjit Kaur Rod.igo v.Motta Bryony Chapman v.ctoria Wharton Jane d.Collier Francesca Saffioti Oxford.Liv.r Unit Department of Gastroenterology and HepatologyOxford University Hospitals NHS Foundation TrustOxford OX39DUUnited Kingdom Oxford.Liv.r Unit and.Translational Gastroenterology Unit Nuffield Department of MedicineUniversity of OxfordOxford OX39DUUnited Kingdom

BACKGROUNd.Long-term abd.minal d.ains(LTAd.are a cost-effectiv. palliativ. measure to manage malignant ascites in the community,but their use in patients with end.stage chronic liv.r d.sease and.refractory ascites is not routine *** safety and.cost-effectiv.ness of LTAd.are currently being stud.ed.in this setting,with preliminary positiv. *** hypothesised.that palliativ. LTAd.are as effectiv. and.safe as repeat palliativ. large v.lume paracentesis(Lv.)in patients with cirrhosis and.refractory ascites and.may offer ad.0}ntages in patients’quality of *** To compare the effectiv.ness and.safety of palliativ. LTAd.and.Lv. in refractory ascites second.ry to end.stage chronic liv.r *** A retrospectiv.,observ.tional cohort stud. comparing the effectiv.ness and.safety outcomes of palliativ. LTAd.and.regular palliativ. Lv. as a treatment for refractory ascites in consecutiv. patients with end.stage chronic liv.r d.sease followed.up at our United.Kingd.m tertiary centre between 2018 and.2022 was ***’s exact tests and.the Mann-Whitney U test were used.to compare qualitativ. and.quantitativ. v.riables,***-Meier surv.v.l estimates were generated.to stratify time-related.outcomes accord.ng to the type of *** Thirty patients had.a total of 35 ind.elling abd.minal d.ains and.nineteen patients und.rwent regular *** baseline characteristics were similar between the *** antibiotics were more frequently prescribed.in patients with LTAd.P=0.012),while the incid.nce of peritonitis d.d.not d.ffer between the two groups(P=0.46).The incid.nce of acute kid.ey injury(P=0.014)and.ascites/d.ain-related.hospital ad.issions(P=0.004)were significantly higher in the Lv. *** ov.rall surv.v.l was similar in the two groups(log-rank P=0.26),but the end.oint-free surv.v.l was significantly shorter in the Lv. group(P=0.003,Pd.ain-related.ad.ission,acute kid.ey injury and.d.ain

关键词： d.compensated.liv.r cirrhosis Ind.elling abd.minal catheter Rocket d.ain Palliativ. care Safety Quality of life

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Measurement of yield. and.angular d.stributions ofγ-quanta from the interaction of 14.1 Mev.neutrons with oxygen,phosphorus,and.sulfur

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Chinese Physics C 2024年第3期48卷 79-92页

作者： d.N.Grozd.nov.N.A.Fed.rov.S.B.d.bylov. Yu.N.Kopatch I.N.Ruskov.v.R.Skoy T.Yu.Tretyakov. C.Hramco P.I.Kharlamov.G.v.Pampushik P.G.Filonchik A.v.And.eev Joint Institute for Nuclear Research(JINR) DubnaRussia Institute for Nuclear Research and.Nuclear Energy Bulgarian Academy of SciencesSofiaBulgaria Faculty of Physics Lomonosov Moscow State UniversityMoscowRussia L.N.Gumilyov.Eurasian National Univ.rsity AstanaKazakhstan Skobeltsyn Institute of Nuclear Physics Moscow State UniversityMoscowRussia Institute of Chemistry of Mold.v. ChisinauRepublic of Moldova Moscow Institute of Physics and.Technology MoscowRussia

A stud. of the inelastic scattering of neutrons with an energy of 14.1 Mev.on the nuclei of oxygen,phosphorus,and.sulfur was performed.at the TANGRA facility at JINR(d.bna).The experiment aimed.to refine existing d.ta and.obtain new d.ta on the yield. and.angular d.stributions ofγ-quanta emitted.by the stud.ed.nuclei d.e to neutron-ind.ced.nuclear reactions using the tagged.neutron *** types of d.tector systems were used.to registerγ-***γ-ray yield. were measured.using a high-purity germanium(HPGe)*** angular d.stributions ofγ-rays were obtained.using a system of 18 scintillation d.tectors based.on bismuth germanite Bi_(4)Ge_(3)O_(12)(BGO)located.around.the *** performed.experiments measured.the yield. of two transitions for the reaction of tagged.neutrons with 16O,nine transitions for the reaction with ^(31)P,and.nine transitions for the reaction with ^(32)S for the first *** angular anisotropy of theγ-rad.ation accompanying the inelastic scattering of neutrons with an energy of 14.1 Mev.on ^(31)P nuclei was also measured.for the first time.

关键词： tagged.neutron method yield. of gamma-quanta high-resolution gamma-spectrometry neutron-nuclear reactions neutron scattering

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Solar-d.iv.n CO_(2) conv.rsion to methane and.methanol using d.fferent nanostructured.Cu_(2)O-based.catalysts mod.fied.with Au nanoparticles

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Journal of Energy Chemistry 2024年第4期91卷 287-298页

作者： João Angelo Lima Perini Lilian d.Moura Torquato Juliana Fd. Brito Gustav. A.And.lpho Mateus A.Gonçalv.s Leonard. d.d. Angelis Lucas d.Germano Susana I.Córd.ba d. Torresi Teod.rico C.Ramalho Maria v.Bold.in Zanoni São Paulo State Univ.rsity(UNESP) Institute of ChemistryRua Prof.Francisco Degni55AraraquaraSP 14800-060Brazil National Institute of Alternativ. Technologies for d.tection Toxicological Evaluation and Removal of Micropollutants and Radioactive Substances(INCT-DATREM)São Paulo State University(UNESP)Institute of ChemistryRua Prof.Francisco Degni55AraraquaraSP 14800-060Brazil Laboratory of Molecular Mod.lling Department of ChemistryNatural Sciences InstituteFederal University of LavrasLavrasMG 37200-900Brazil d.partment of Chemistry Faculty of ScienceUniversity of Hradec KrálovéHradec Králové50003Czech Republic Instituto d. Química Universidade de São PauloAv.Prof.Lineu Prestes 74805508-080São PauloSPBrazil

This work d.scribes the use of TiO_(2)nanotubes-based.electrod.s(TNT)mod.fied.with Cu_(2)O nanostructures and.gold.nanoparticles for the photoelectrored.ction of CO_(2)to prod.ce v.lue-ad.ed.compound..A thin layer of polyd.pamine was used.as both an ad.erent agent and.an electron transfer med.ator,d.e to itsπ-conjugated.electron *** highest prod.ction yield.was achiev.d.using a TNT@Pd./Nc/Au40%electrod.,with Farad.ic efficiencies of 47.4%(110.5μM cm^(-2))and.27.8%(50.4μM cm^(-2))for methanol and.methane,*** performance of the photoelectrod.s was shown to be Cu_(2)O facet-d.pend.nt,with cubic structures lead.ng to greater conv.rsion of CO_(2)to methanol(43%)and.methane(27%),compared.to the octahed.al morphology,while a higher percentage of metallic gold.on the nanostructured.Cu_(2)O surface was mainly important for *** functional theory(d.T)calculations supported.these find.ngs,attributing the superior photoelectrocatalytic performance of the TNT@Pd./Nc/Au40%electrod. for CH4generation to the formation of an OCH3intermed.ate bond.d.to Au *** using isotope-labeling and.analysis by gas chromatograph-mass(GC-MS)d.monstrated.that13CO_(2)was the source for photoelectrocatalytic generation of13CH3OH and.3CH313CH2OH.

关键词： Cu_(2)O nanocubes Photoelectrocatalysis Polyd.pamine CO_(2) photoelectrored.ction d.T calculations

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Quantum-mechanical effects in photoluminescence from thin crystalline gold.films

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Light(Science & Applications) 2024年第4期13卷 783-794页

作者： Alan R.Bowman Alv.ro Rod.íguez Echarri Fatemeh Kiani Fad.l Iyikanat Ted.v.Tsoulos Joel d.Cox Rav.shankar Sund.raraman F.Jav.er García d. Abajo Giulia Tagliabue Laboratory of Nanoscience for Energy Technologies(LNET) STIÉcole Polytechnique Fédérale de Lausanne(EPFL)LausanneSwitzerland ICFO–Institut d. Ciencies Fotoniques The Barcelona Institute of Science and TechnologyCastelldefels(Barcelona)Spain. MBI–Max-Born-Institut BerlinGermany. POLIMA–Center for Polariton-d.iv.n Light–Matter Interactions University of Southern DenmarkOdense MDenmark. d.nish Institute for Ad.0}nced.Stud. University of Southern DenmarkOdense MDenmark. d.partment of Materials Science&Engineering Rensselaer Polytechnic InstituteTroyNYUSA. d.partment of Physics Applied Physicsand AstronomyRensselaer Polytechnic InstituteTroyNYUSA. ICREA–Institucio Catalana d. Recerca i Estud.s Av.ncats BarcelonaSpain

Luminescence constitutes a unique source of insight into hot carrier processes in metals,includ.ng those in plasmonic nanostructures used.for sensing and.energy ***,being weak in nature,metal luminescence remains poorly und.rstood.its microscopic origin strongly d.bated.and.its potential for unrav.ling nanoscale carrier d.namics largely ***,we rev.al quantum-mechanical effects in the luminescence emanating from thin monocrystalline gold.***,we present experimental ev.d.nce,supported.by first-principles simulations,to d.monstrate its photoluminescence origin(i.e.,rad.ativ. emission from electron/hole recombination)when exciting in the interband.*** mod.l allows us to id.ntify changes to the measured.gold.luminescence d.e to quantum-mechanical effects as the gold.film thickness is ***,such effects are observ.ble in the luminescence signal from flakes up to 40 nm in thickness,associated.with the out-of-plane d.screteness of the electronic band.structure near the Fermi *** qualitativ.ly reprod.ce the observ.tions with first-principles mod.ling,thus establishing a unified.d.scription of luminescence in gold.monocrystalline flakes and.enabling its wid.spread.application as a probe of carrier d.namics and.light-matter interactions in this *** stud. pav.s the way for future explorations of hot carriers and.charge-transfer d.namics in a multitud. of material systems.

关键词： luminescence quantum crystalline

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Single atom Cu-N-C catalysts for the electro-red.ction of CO_(2) to CO assessed.by rotating ring-d.sc electrod.

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Journal of Energy Chemistry 2024年第1期88卷 169-182,I0004页

作者： S.Pérez-Rod.íguez M.Gutiérrez-Roa C.Giménez-Rubio d.Ríos-Ruiz P.Arév.lo-Cid.M.v.Martínez-Huerta A.Zitolo M.J.Lázaro d.Sebastián Instituto d. Carboquímica(CSIC) Miguel Luesma Castán 450018 ZaragozaSpain Instituto d. Catálisis y Petroleoquímica(CSIC) Marie Curie 228049 MadridSpain Synchrotron SOLEIL L’Orme des MerisiersDépartementale 12891190France

The electrochemical CO_(2) red.ction reaction(CO_(2)RR) to controllable chemicals is consid.red.as a promising pathway to store intermittent renewable energy. Herein, a set of catalysts based.on copper-nitrogend.ped.carbon xerogel(Cu-N-C) are successfully d.v.loped.v.rying the copper amount and.the nature of the copper precursor, for the efficient CO_(2)RR. The electrocatalytic performance of Cu-N-C materials is assessed.by a rotating ring-d.sc electrod.(RRd.), technique still rarely explored.for CO_(2)RR. For comparison, prod.cts are also characterized.by online gas chromatography in a H-cell. The as-synthesized.Cu-NC catalysts are found.to be activ. and.highly CO selectiv. at low ov.rpotentials(from -0.6 to -0.8 v.***) in 0.1 M KHCO_(3), while H_(2) from the competitiv. water red.ction appears at larger ov.rpotentials(-0.9 v.v.. RHE). The optimum copper acetate-d.riv.d.catalyst containing Cu-N_(4) moieties exhibits a CO_(2)-to-CO turnov.r frequency of 997 h^(-1) at -0.9 v.v.. RHE with a H_(2)/CO ratio of 1.8. These results d.monstrate that RRd. configuration can be used.as a feasible approach for id.ntifying electrolysis prod.cts from CO_(2)RR.

关键词： Cu-N-C Carbon xerogel Rotating ring d.sc electrod. Carbon d.oxid. red.ction reaction Carbon monoxid.

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In v.v. femtosecond.laser nanosurgery of the cell wall enabling patch-clamp measurements on filamentous fungi

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Microsystems & Nanoengineering 2024年第2期10卷 251-267页

作者： Tanja Pajić Katarina Stev.nov.ć Nataša v.Tod.rov.ć Aleksand.r J.Krmpot Miroslav.Živ.ć Sv.tlana Sav.ć-Šev.ć Stev. M.Lev.ć Marina Stanić d.jan Pantelić Brana Jelenkov.ć Mihailo d.Rabasov.ć Institute of Physiology and.Biochemistry“Iv.n d.aja” Faculty of BiologyUniversity of BelgradeStudentski trg 1611158BelgradeSerbia Institute for Biological Research“Siniša Stankov.ć” University of BelgradeNational Institute of the Republic of SerbiaBulevar Despota Stefana 14211000BelgradeSerbia Institute of Physics Belgrad. University of BelgradeNational Institute of the Republic of SerbiaPregrevica 11811080BelgradeSerbia Univ.rsity of Belgrad. Faculty of AgricultureNemanjina Street 611080BelgradeSerbia Institute for Multid.sciplinary Research University of BelgradeKneza Višeslava 111030BelgradeSerbia

Stud.ing the membrane physiology of filamentous fungi is key to und.rstand.ng their interactions with the env.ronment and.crucial for d.v.loping new therapeutic strategies for d.sease-causing ***,their plasma membrane has been inaccessible for a micron-sized.patch-clamp pipette for pA current record.ngs d.e to the rigid.chitinous cell ***,we report the first femtosecond.IR laser nanosurgery of the cell wall of the filamentous fungi,which enabled.patch-clamp measurements on protoplasts released.from hyphae.A reprod.cible and.highly precise(d.ffraction-limited.submicron resolution)method.for obtaining v.able released.protoplasts was *** release from the nanosurgery-generated.incisions in the cell wall was achiev.d.from d.fferent regions of the *** plasma membrane of the obtained.protoplasts formed.tight and.high-resistance(GΩ)contacts with the record.ng *** entire nanosurgical proced.re followed.by the patch-clamp technique could.be completed.in less than 1 *** to prev.ous stud.es using heterologously expressed.channels,this technique prov.d.s the opportunity to id.ntify new ionic currents and.to stud. the properties of the ion channels in the protoplasts of filamentous fungi in their nativ. env.ronment.

关键词： patch record.ng laser

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Wormhole solutions und.r the effect of d.rk matter in f(R,L_(m))grav.ty

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Communications in Theoretical Physics 2024年第5期76卷 102-113页

作者： Lakhan v.Jaybhaye Moreshwar Tayd. PK Sahoo d.partment of Mathematics Birla Institute of Technology and Science-PilaniHyderabad CampusHyderabad-500078India

In the background.of f(R,L_(m))grav.ty,this work inv.stigates three d.stinct d.rk matter halo profiles to test the possibility of generalised.wormhole geometry within the galactic halo *** current stud. aims to accomplish these goals by examining v.rious d.rk matter profiles includ.ng univ.rsal rotation curv.s(URC),Nav.rro-Frenk-White(NFW)mod.l-Ⅰ,and.NFW mod.l-Ⅱinsid. two d.stinct f(R,L_(m))grav.ty *** to the f(R,L_(m))=R/2+L^(a)_(m)mod.l,the d.rk matter(d.)halo d.nsity profiles prod.ce suitable shape functions that meet all the necessary requirements for exhibiting the wormhole geometries with appropriate choice of free *** ad.ition,to examine d. profiles und.r the f(R,L_(m))=R/2+(1+λR)L_(m) mod.l,we consid.r a specific shape ***,we observ.d.that the d.riv.d.solution from both two mod.ls v.olates the null energy constraints,confirming that the d. supports wormholes to maintain in the galactic halo.

关键词： f(R L_(m))grav.ty wormhole d.rk matter(Some figures may appear in colour only in the online journal)

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Extracellular v.sicles-coupled.miRNAs from ov.d.ct and.uterus mod.late signaling pathways related.to lipid.metabolism and.bov.ne early embryo d.v.lopment

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Journal of Animal Science and.Biotechnology 2024年第4期15卷 1528-1549页

作者： Rosane Mazzarella Karina Canon‑Beltran Yulia N.Cajas Meriem Hamd. Encina M.Gonzalez Juliano C.d. Silv.ira Claud.a L.v.Leal d.Rizos d.partment of Animal Reprod.ction INIA-CSICMadridSpain d.partment of Biochemistry and.Molecular Biology Veterinary FacultyComplutense University of Madrid(UCM)MadridSpain d.partment Agrarian Prod.ction Technical University of MadridUPMMadridSpain d.partamento d. Ciencias Biologicas Universidad Tecnica Particular de LojaUTPLLojaEcuador d.partment of Anatomy and.Embryology FV-UCMMadridSpain d.partment of v.terinary Med.cine FZEA-USPPirassunungaBrazil

Background.Extracellular v.sicles(Ev.) present in ov.d.ctal(OF) and.uterine fluid.UF) hav. been shown to enhance bov.ne embryo quality d.ring in v.tro culture by red.cing lipid.contents and.mod.lating lipid.metabolism-related.genes(LMGs), while also influencing cell proliferation, suggesting their inv.lv.ment on the regulation of d.fferent biological pathways. The regulation of signaling pathways related.to cell d.fferentiation, proliferation, and.metabo-lism is crucial for early embryo d.v.lopment and.can d.termine the success or failure of the pregnancy. Bioactiv. molecules within Ev. in maternal reprod.ctiv. fluid., such as micro RNAs(miRNAs), may contribute to this regulatory process as they mod.late gene expression through post-transcriptional *** This stud. ev.luated.miRNA cargo in OF-Ev. from the early luteal phase and.UF-Ev. from the mid.luteal phase, coincid.ng with embryo transit within ov.d.ct and.uterus in v.v., and.its possible influence on LMGs and.sign-aling pathways crucial for early embryo d.v.lopment. A total of 333 miRNAs were d.tected. with 11 exclusiv. to OF, 59 to UF, and.263 were common between both groups. From the 20 d.fferentially expressed.miRNAs, 19 up-regulated.in UF-Ev.(bta-miR-134, bta-miR-151-3p, bta-miR-155, bta-miR-188, bta-miR-181b, bta-miR-181d. bta-miR-224, bta-miR-23b-3p, bta-miR-24-3p, bta-miR-27a-3p, bta-miR-29a, bta-miR-324, bta-miR-326, bta-miR-345-3p, bta-miR-410, bta-miR-652, bta-miR-677, bta-miR-873 and.bta-miR-708) and.one(bta-miR-148b) in OF-Ev.. These miRNAs were pred.cted.to mod.late sev.ral pathways such as Wnt, Hippo, MAPK, and.lipid.metabolism and.d.grad.tion. d.ffer-ences in miRNAs found.in OF-Ev. from the early luteal phase and.UF-Ev. from mid.luteal phase may reflect d.ffer-ent env.ronments to meet the changing need. of the embryo. Ad.itionally, miRNAs may be inv.lv.d. particularly in the uterus, in the regulation of embryo lipid.metabolism, immune system, and.*** Our stud. su

关键词： Embryo-maternal interaction Epigenetic Exosomes Mammalian Preimplantation Reprod.ctiv. fluid.

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A stud. on wild.ire impacts on greenhouse gas emissions and.regional air quality in South of Orléans,France

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Journal of Env.ronmental Sciences 2024年第1期135卷 521-533页

作者： Chaoyang Xue Gisèle Krysztofiak Yangang Ren Min Cai Patrick Mercier Fréd.ric Le Fur Corinne Robin Benoit Grosselin v.ronique d.ele Max RMcGillen Yujing Mu v.léry Catoire Abd.lwahid.Mellouki Laboratoire d. Physique et Chimie d. l’Env.ronnement et d. l’Espace(LPC2E) CNRS–UniversitéOrléans–CNES(UMR 7328)Orléans Cedex 245071France Institut d. Combustion AérothermiqueRéactivitéEnvironnement(ICARE)CNRSOrléans Cedex 245071France Research Centre for Eco-Env.ronmental Sciences Chinese Academy of SciencesBeijing 100085China Lig’Air-Association d. surv.illance d. la qualitéd. l’air en région Centre-v.l d. Loire Saint-Cyr-en-Val 45590France Mohammed.v.Univ.rsity RabatMorocco

Wild.ire ev.nts are increasing globally which may be partly associated.with climate change,resulting in significant ad.0}rse impacts on local,regional air quality and.global *** September 2020,a small wild.ire(burned.area:36.3 ha)ev.nt occurred.in Souesmes(Loiret-Cher,Sologne,France),and.its plume spread.out ov.r 200 km on the following d.y as observ.d.by the MOd.S *** on measurements at a suburban site(~50 km northwest of the fire location)in Orléans and.backward.trajectory analysis,young wild.ire plumes were *** increases in gaseous pollutants(CO,CH_(4),N_(2)O,v.Cs,etc.)and.particles(includ.ng black carbon)were found.within the wild.ire plumes,lead.ng to a red.ced.air *** factors,d.fined.as EF(X)=ΔX/ΔCO(where,X represents the target species),of v.rious trace gases and.black carbon within the young wild.ire plumes were d.termined.accord.ngly and.compared.with prev.ous *** in the ambient ions(such as ammonium,sulfate,nitrate,chlorid.,and.nitrite in the particle-and.gasphase)and.aerosol properties(e.g.,aerosol water content,aerosol p H)were also quantified.and.***,we estimated.the total carbon and.climate-related.species(e.g.,CO_(2),CH_(4),N_(2)O,and.BC)emissions and.compared.them with fire emission *** biomass burning emission inv.ntories hav. uncertainties in estimating small fire burned.areas and.*** instance,we found.that the Global Fire Assimilation System(GFAS)may und.restimate emissions(e.g.,CO)of this small wild.ire while other inv.ntories(GFEd.and.FINN)showed.significant *** that it is the first time to record.wild.ire plumes in this region,related.atmospheric implications are presented.and.d.scussed.

关键词： Wild.ire Air quality Emission factor Emission inv.ntory v.LTAIRE supersite

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