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Novel enzymatically crosslinked chitosan hydrogels with free-radical-scavenging property and promoted cellular behaviors under hyperglycemia

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Progress in Natural Science:Materials International 2020年第5期30卷 661-668页

作者： dieu Linh tran Phuong Le thi Thai Thanh Hoang thi Ki Dong Park Department of Molecular Science and Technology Ajou University Biomaterials and Nanotechnology Research Group Faculty of Applied Sciences Ton Duc Thang University

The impairment of regenerative processes induced by high blood-glucose level(hyperglycemia) and excessive reactive oxygen species(ROS) contributes to the diabetic complication progression and development. In this study, an injectable, in situ crosslinkable chitosan hydrogel with ROS-scavenging capability was developed by conjugating gallic acid onto the chitosan backbone(CGA). We hypothesized that gallic acid serves as both antioxidant and crosslinking moieties to form hydrogel in situ by means of enzymatic crosslinking with horseradish peroxidase(HRP). The rapid gelation(from 30 s) was observed by vial tilting. The mechanical properties and microstructures of CGA hydrogels can be well controlled by varying the concentrations of H2O2. The ROSscavenging ability of these CGA hydrogels was demonstrated against DPPH radical, hydroxyl radical, and total reducing power. Notably, in an in vitro hyperglycemia environment, CGA hydrogels significantly improved the proliferation and migration of human dermal fibroblast cells, which are closely related to diabetic wound healing. These results suggest that CGA hydrogels have potential as advanced materials for the treatment of diabetes-related diseases via attenuating the excessive ROS production and improving cellular behaviors.

关键词： Chitosan Gallic acid Injectable hydrogel Hyperglycemia Free-radical-scavenging

Injectable reactive oxygen and nitrogen species-controlling hydrogels for tissue regeneration:current status and future perspectives

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Regenerative Biomaterials 2022年第1期9卷 1106-1130页

作者： Phuong Le thi dieu Linh tran Thai Thanh Hoang thi Yunki Lee Ki Dong Park Institute of Applied Materials Science Vietnam Academy of Science and TechnologyHo Chi Minh City 700000Vietnam Department of Orthopaedics Emory University School of MedicineAtlantaGA 30329USA Department of Molecular Science and Technology Ajou UniversitySuwon 443-749Republic of Korea

The dual role of reactive oxygen and nitrogen species(RONS)in physiological and pathological processes in biological systems has been widely *** has been recently suggested that the regulation of RONS levels under physiological and pathological conditions is a potential therapy to promote health and treat diseases,*** hydrogels have been emerging as promising biomaterials for RONS-related biomedical applications owing to their excellent biocompatibility,three-dimensional and extracellular matrix-mimicking structures,tunable properties and easy *** hydrogels have been developed as advanced injectable platforms for locally generating or scavenging RONS,depending on the specific conditions of the target *** this review article,the design principles and mechanism by which RONS are generated/scavenged from hydrogels are outlined alongside a discussion of their in vitro and in vivo ***,we highlight the advantages and recent developments of these injectable RONS-controlling hydrogels for regenerativemedicines and tissue engineering applications.

关键词： reactive oxygen/nitrogen species oxidative stress-related diseases injectable hydrogels reactive oxygen/nitrogen species-scavenging/releasing/responsive properties tissue regeneration

Biomass accumulation of Panax vietnamensis in cell suspension cultures varies with addition of plant growth regulators and organic additives

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Asian Pacific Journal of Tropical Medicine 2017年第9期10卷 907-915页

作者： Tuan tran Trong dieu-Hien Truong Hoang Chinh Nguyen dieu-Thai tran Huyen-trang Nguyen thi Giap Do Dang Ho Nguyen Huu Plant Cell Technology Department Institute of Tropical BiologyVietnam Academy of Science and Technology9/621 Ha Noi HighwayLinh TrungThu DucHo Chi Minh CityViet Nam Faculty of Applied Sciences Ton Duc Thang University19 Nguyen Huu ThoTan PhongDistrict 7Ho Chi Minh CityViet Nam Genetic Engineering Department Institute of Tropical BiologyVietnam Academy of Science and Technology9/621 Ha Noi HighwayLinh TrungThu DucHo Chi Minh CityViet Nam

Objective: To evaluate the impact of plant growth regulators including kinetin(KN),benzyl adenine and naphthalene acetic acid, yeast extract and casein hydrolyzate on biomass accumulation of Vietnamese ginseng Panax vietnamensis(P. vietnamensis) in cell suspension ***: Cell suspension cultures were established from friable calluses derived from leaves and petioles of 3-year-old in-vitro P. vietnamensis plants. The cell suspension cultures were grown in Murashige and Skoog basal media supplemented with various concentrations of KN, benzyl adenine, naphthalene acetic acid, and yeast extract and casein ***: All tested factors generated an increase in the cell biomass of P. vietnamensis in suspension culture, but the impact of each varies depended on the factor type, concentration, and incubation period. Addition of 2.0 mg/L KN resulted in the largest biomass increase after 24 d,(57.0 ± 0.9) and(3.1 ± 0.1) mg/m L fresh and dry weight, respectively,whereas addition of benzyl adenine or naphthalene acetic acid produced optimum levels of Panax cell biomass at 1.0 and 1.5 mg/L, respectively. Addition of the elicitor yeast extract led to a 1.4–2.4 fold increase in biomass of P. vietnamensis, while addition of casein hydrolyzate enhanced biomass accumulation 1.8–2.6 ***: The addition of each factor causes significant changes in biomass accumulation of P. vietnamensis. The largest biomass accumulation is from cultures grown in MS media containing 2.0 mg/L KN for 24 d. The outcome of the present study provides new insights into the optimal suspension culture conditions for studies on the in vitro cell biomass production of P. vietnamensis.

关键词： Panax vietnamensis Plant cell suspension culture Plant regulators Yeast extract Casein hydrolyzate Biomass

Static and dynamic analysis of functionally graded fluidinfiltrated porous skew and elliptical nanoplates using an isogeometric approach

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Frontiers of Structural and Civil Engineering 2023年第3期17卷 477-502页

作者： tran thi Thu THUY Faculty of Mechanical Engineering Hanoi University of IndustryHanoi 100000Vietnam

The analysis of static bending and free and forced vibration responses of functionally graded fluidinfiltrated porous(FGFP)skew and elliptical nanoplates placed on Pasternak’s two-parameter elastic foundation is performed for the first time using isogeometric analysis(IGA)based on the non-uniform rational B-splines(NURBSs)basis *** types of porosity distributions affect the mechanical characteristics of materials:symmetric distribution,upper asymmetric distribution,and lower asymmetric *** stress–strain relationship for Biot porous materials was determined using the elastic *** general equations of motion of the nanoplates were established using the four-unknown shear deformation plate theory in conjunction with the nonlocal elastic theory and Hamilton’s principle.A computer program that uses IGA to determine the static bending and free and forced vibration of a nanoplate was developed on MATLAB software *** accuracy of the computational program was validated via numerical comparison with confidence *** set of programs presents the influence of the following parameters on the static bending and free and forced vibrations of nanoplates:porosity distribution law,porosity coefficient and geometrical parameters,elastic foundation,deviation angle,nonlocal coefficient,different boundary conditions,and Skempton *** numerical findings demonstrated the uniqueness of the FGFP plate’s behavior when the porosities are saturated with liquid compared with the case without *** findings of this study have significant implications for engineers involved in the design and fabrication of the aforementioned type of ***,this can form the basis for future research on the mechanical responses of the structures.

关键词： static bending free and forced vibrations nonlocal theory isogeometric analysis fluid-infiltrated porous nanoplates

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Organic dye removal and recycling performances of graphene oxide-coated biopolymer sponge

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Progress in Natural Science:Materials International 2022年第5期32卷 634-642页

作者： thi Sinh Vo tran thi Bich Chau Vo School of Mechanical Engineering Sungkyunkwan University Department of Industrial Management Can Tho University

In this study, a biopolymer sponge(PS) with a crosslinked mixture of gelatin-chitosan-poly(vinyl alcohol) was dipped into graphene oxide(GO) solution to form a composite sponge(CS, GO-coated PS) by a combination of simple dip-coating and freeze-drying procedures, as a sponge-like adsorbent in organic dye removal *** morphological, chemical, crystalline, mechanical and thermal characterizations of the as-obtained sponges were further investigated for the possible changes in the structure of sponge-like adsorbent after coating the GO sheets on the 3D porous structure of PS. The results showed that the CS had possessed effectively organic dye removal performances comparing to the PS. In the adsorption, the Langmuir and pseudo-second-order models corresponding to a monolayer approach and a chemical adsorption were appropriated. The maximum adsorption capacity of Rhodamine B and Congo red reached 126.8 and 135.0 mg·g-1; and 145.6 and 148.6 mg·g-1corresponding onto the PS and CS. It indicates that the maximum adsorption capacity on the CS enhanced significantly comparing to those on the PS owing to the functional GO sheets coated in the 3D porous structure of PS, which leads to supplying further functional adsorption sides on the whole 3D porous structure of CS. Notably, the sponges-like adsorbents could be regenerated and used again without a remarkable decrease of dye removal ability occurred in 9 adsorbing–desorbing cycles. Therefore, the CS prepared in this study can become a potential adsorbent for actual applications because of non-toxic materials, proper structural features, low-cost material and operation, and reliable recyclability.

关键词： Graphene oxide Biopolymer sponge Organic dye Adsorption Dye removal Recyclability

Graphene oxide-covered melamine foam utilizing as a hybrid foam toward organic dye removal and recyclability

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Progress in Natural Science:Materials International 2022年第3期32卷 296-303页

作者： thi Sinh Vo tran thi Bich Chau Vo School of Mechanical Engineering Sungkyunkwan University Department of Industrial Management Can Tho University

Graphene-based adsorbents have been attracted extensive interest in recent years. Herein, graphene oxidecovered melamine foam(GO-covered MF) was designed and prepared by a mild submerge-covering method with the support of a super-hydrophilic melamine framework, showing its adsorption performances for various organic dyes. The structure morphology as well as chemical, thermal and mechanical properties of the as-obtained hybrid foam(HF) were further determined for the possible structure changes after covering the GO sheets on the MF framework. Moreover, the HF exhibited an excellent ability for organic dye adsorption application, and which was well fitted in the pseudo-second-order kinetic and Langmuir models corresponding to a chemical adsorption and a mono-layer approach during the adsorption process. The maximum adsorption capacity by using the asobtained HF corresponded to 258.56 mg g-1(methylene blue), 233.22 mg g-1(Rhodamine B), 206.92 mg g-1(methyl orange), and 184.93 mg g-1(Congo red), which are competitive with that of other graphene-based absorbents. In particular, the HF could be reused without a noticeable degradation of organic dye removal performance. As such, the HF prepared in this study can become an encouraging candidate for practical application owing to the reliable recyclability and low-cost.

关键词： Graphene oxide Melamine foam Organic dye Adsorption Hybrid foam Recyclability

Surface characterization of polyimide and polyethylene terephthalate membranes toward plasma and UV treatments

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Progress in Natural Science:Materials International 2022年第3期32卷 314-327页

作者： thi Sinh Vo tran thi Bich Chau Vo School of Mechanical Engineering Sungkyunkwan University Department of Industrial Management Can Tho University

this study is to bring an overview on various methods regarding the surface treatment performed on different polymeric membranes in relation to a deference between the treatment mechanism and their chemical ***, plasma and UV surface treatments(PST and UST) were utilized to treat the surfaces of two commercial membranes, i.e., aromatic polyimide and polyethylene terephthalate for various durations using a discharge electrode and an UV LED curing system, respectively. Based on the effects of PST and UST processes on the surface of these membranes, their surface properties have been characterized to surface morphology and hydrophilicity(or wettability), at same time the changes have probably occurred on their surface during the PST and UST processes. As a result, their hydrophilic behavior was significantly enhanced after conducting these treatment processes based on the investigation of water contact angle. Moreover, Fourier-transform infrared and Raman spectroscopy manifested the changes in the chemical bonds, interactions and orientations of molecules, which confirmed the apparition and insertion of polar functional groups after the surface treatments, and accordingly,their wettability was enhanced significantly. Also, optical microscopy images showed direct impactions on their surface and the evidence of slight surface aging/damage during the treatment processes based on the presentation of the strange streaks on the treated surfaces. In particular, the peel forces exhibited an increase comparing to the initial membranes, which is characteristically for enhancing their adhesion behavior. Hence, these results are needful for improving the surface properties of a material, and obtaining better adhesion behavior on the membrane-like materials and recycling polymer materials.

关键词： Plasma treatment UV treatment Polymeric membrane Aromatic polyimide Polyethylene terephthalate

transient response of doubly-curved bio-inspired composite shells resting on viscoelastic foundation subject to blast load using improved first-order shear theory and isogeometric approach

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Defence Technology（防务技术） 2024年第8期38卷 171-193页

作者： Thuy tran thi Thu Tu Nguyen Anh Hue Nguyen thi Hong Nguyen thi School of Mechanical and Automotive Engineering Hanoi University of IndustryHanoiViet Nam Faculty of Technical Fundamental University of Transport TechnologyHanoiViet Nam Faculty of Mechanical Engineering Thuyloi University175 Tay SonDong DaHanoiViet Nam

Investigating natural-inspired applications is a perennially appealing subject for scientists. The current increase in the speed of natural-origin structure growth may be linked to their superior mechanical properties and environmental resilience. Biological composite structures with helicoidal schemes and designs have remarkable capacities to absorb impact energy and withstand damage. However, there is a dearth of extensive study on the influence of fiber redirection and reorientation inside the matrix of a helicoid structure on its mechanical performance and reactivity. The present study aimed to explore the static and transient responses of a bio-inspired helicoid laminated composite(B-iHLC) shell under the influence of an explosive load using an isomorphic method. The structural integrity of the shell is maintained by a viscoelastic basis known as the Pasternak foundation, which encompasses two coefficients of stiffness and one coefficient of damping. The equilibrium equations governing shell dynamics are obtained by using Hamilton's principle and including the modified first-order shear theory,therefore obviating the need to employ a shear correction factor. The paper's model and approach are validated by doing numerical comparisons with respected publications. The findings of this study may be used in the construction of military and civilian infrastructure in situations when the structure is subjected to severe stresses that might potentially result in catastrophic collapse. The findings of this paper serve as the foundation for several other issues, including geometric optimization and the dynamic response of similar mechanical structures.

关键词： Blast load Modified first-order shear theory Biological composite structures

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Instability of colloidal lead halide perovskite nanocrystals:Causes,improvement,and evaluation

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Nano Research 2024年第12期17卷 10607-10619页

作者： thi Kim tran tran Hawi N.Nyiera Jing Zhao North Eagleville Road Department of ChemistryUniversity of ConnecticutStorrsConnecticut 06269USA

The instability of colloidal lead halide perovskite nanocrystals(NCs)presents a significant challenge for their application in optoelectronic *** review examines the primary causes of instability in these NCs and the proposed mechanisms of *** also introduces the recently developed synthesis and surface passivation methods to address the instability issue of colloidal perovskite ***,we focus on the various types of ligands and precursors introduced during NC synthesis or post-treatment and how they impact the structural and optical properties of the perovskite *** review also proposes a systematic approach to evaluating stability enhancement strategies by establishing key parameters and ranking them based on working and processing ***,we discuss the issues that need to be addressed in future research to achieve practical application of lead halide perovskite NCs in advanced optoelectronic systems.

关键词： lead halide perovskites colloidal nanocrystals stability optical properties