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Photovoltaic-powered supercapacitors for driving overall water splitting:A dual-modulated 3D architecture

Carbon Energy 2022年第6期4卷 1262-1273页

作者： Zixu Sun Lijuan Sun See Wee Koh Junyu Ge Jipeng Fei Mengqi Yao Wei Hong Shude Liu Yusuke yamauchi Hong Li Key Lab for Special Functional Materials of Ministry of Education National and Local Joint Engineering Research Center for High-Efficiency Display and Lighting TechnologyCollaborative Innovation Center of Nano Functional Materials and ApplicationsSchool of Materials Science and EngineeringHenan UniversityKaifengPeople's Republic of China School of Mechanical and Aerospace Engineering Nanyang Technological UniversitySingaporeSingapore School of Electronic and Information Zhongyuan University of TechnologyZhengzhouPeople's Republic of China JST-ERATO yamauchi Material Space-Tectonics Project National Institute for Materials Science(NIMS)TsukubaIbarakiJapan Australian Institute for Bioengineering and Nanotechnology(AIBN) The University of QueenslandBrisbaneQueenslandAustralia

Due to the growing demand for clean and renewable hydrogen fuel,there has been a surge of interest in electrocatalytic water-splitting devices driven by renewable energy ***,the feasibility of self-driven water splitting is limited by inefficient connections between functional modules,lack of highly active and stable electrocatalysts,and intermittent and unpredictable renewable energy ***,we construct a dualmodulated three-dimensional(3D)NiCo_(2)O_(4)@NiCo_(2)S_(4)(denoted as NCONCS)heterostructure deposited on nickel foam as a multifunctional electrode for electrocatalytic water splitting driven by photovoltaic-powered *** to a stable 3D architecture configuration,abundant active sites,efficient charge transfer,and tuned interface properties,the NCONCS delivers a high specific capacity and rate performance for supercapacitors.A twoelectrode electrolyzer assembled with the NCONCS as both the anode and the cathode only requires a low cell voltage of 1.47 V to achieve a current density of 10 mA cm^(−2) in alkaline electrolyte,which outperforms the state-of-the-art bifunctional *** calculations suggest that the generated heterointerfaces in NCONCS improve the surface binding capability of reaction intermediates while regulating the local electronic structures,which thus accelerates the reaction kinetics of water *** a proof of concept,an integrated configuration comprising a two-electrode electrolyzer driven by two series-connected supercapacitors charged by a solar cell delivers a high product yield with superior durability.

关键词： hybrid energy systems interface engineering morphology control solar-to-hydrogen trifunctional electrode

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Species-dependent effects of the phenolic herbicide ioxynil with potential thyroid hormone disrupting activity: modulation of its cellular uptake and activity by interaction with serum thyroid hormone-binding proteins

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Journal of Environmental Sciences 2012年第5期24卷 949-955页

作者： Sakura Akiyoshi Gobun Sai Kiyoshi yamauchi Department of Biological Science Faculty of Science Shizuoka University

Ioxynil, a phenolic herbicide, is known to exert thyroid hormone （TH） disrupting activity by interfering with TH-binding to plasma proteins and a step of the cellular TH-signaling pathway in restricted animal species. However, comparative studies are still lacking on the TH disruption. We investigated the interaction of [125I] ioxynil with serum proteins from rainbow trout, bullfrog, chicken, pig, rat, and mouse, using native polyacrylamide gel electrophoresis. Candidate ioxynil-binding proteins, which included lipoproteins, albumin and transthyretin （TTR）, differed among the vertebrates tested. Rainbow trout and bullfrog tadpole serum had the lowest binding activity for ioxynil, whereas the eutherian serum had the highest binding activity. The cellular uptake of, and response to, ioxynil were suppressed by rat serum greater than by tadpole serum. The cellular uptake of [125I]ioxynil competed strongly with phenols with a single ring, but not with THs. Our results suggested that ioxynil interferes with TH homeostasis in plasma and with a step of cellular TH-signaling pathway other than TH-uptake system, in a species-specific manner.

关键词： endocrine disruption ioxynil thyroid hormone serum transthyretin uptake

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Cobalt phthalocyanine-based conjugated polymer as efficient and exclusive electrocatalyst for CO_(2) reduction to ethanol

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Materials Reports(Energy) 2023年第1期3卷 100-106,I0004页

作者： Dong Jiang Ran Bu Wei Xia Yichen Hu Mengchen Zhou Enqing Gao Toru Asahi Yusuke yamauchi Jing Tang School of Chemistry and Molecular Engineering Shanghai Key Laboratory of Green Chemistry and Chemical ProcessesEast China Normal UniversityShanghai200062China Department of Life Science&Medical Bioscience School of Advanced Science and EngineeringWaseda University2-2 Wakamatsu-choShinjukuTokyo 162-8480 Japan International Center for Materials Nanoarchitectonics(WPI-MANA) National Institute for Materials Science(NIMS)1-1 NamikiTsukuba305-0044IbarakiJapan Australian Institute for Bioengineering and Nanotechnology(AIBN) The University of QueenslandBrisbane4072QueenslandAustralia Institute of Eco-Chongming Shanghai202162China

Electrocatalytic conversion of carbon dioxide to high value-added chemicals is a promising method for solving the energy crisis and global *** active metal-containing conjugated polymers have been widely studied for heterogeneous carbon dioxide *** the present contribution,we designed and synthesized a stable cobalt phthalocyanine-based conjugated polymer,named CoPPc-TFPPy-CP,and also explored its electro-catalytic application in carbon dioxide reduction to liquid products in an aqueous *** the catalyst,cobalt phthalocyanine acts as building blocks connected with 1,3,6,8-tetrakis(4-formyl phenyl)pyrenes via imine-linkages,leading to mesoporous formation polymers with the pore size centered at *** the central co-balt atoms shifted to a higher oxidation state after *** these chemical and structural natures,the catalyst displayed a remarkable electrocatalytic CO_(2) reduction performance with an ethanol Faradaic efficiency of 43.25%at-1.0V vs *** at the same time,the electrochemical reduction process catalyzed by cobalt phthalocyanine produced only carbon monoxide and *** the best of our knowledge,CoPPc-TFPPy-CP is the first example among organic polymers and metal-organic frameworks that produces ethanol from CO_(2) with a remarkable selectivity.

关键词： Cobalt phthalocyanine based conjugated polymer Carbon dioxide electroreduction Liquid products Ethanol

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Size control and electronic manipulation of Ru catalyst over B,N codoped carbon network for high-performance hydrogen evolution reaction

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Nano Research 2023年第5期16卷 6212-6219页

作者： Shuai Xu Mang Niu Guowei Zhao Shujun Ming Xingyun Li Qilong Zhu Liang-Xin Ding Minjun Kim Asma A.Alothman Mohammed Sheikh Saleh Mushab Yusuke yamauchi Institute of Materials for Energy and Environment Institute of Biochemical EngineeringCollege of Materials Science and EngineeringQingdao UniversityQingdao 266071China Hubei Key Laboratory of Processing and Application of Catalytic materials Huanggang Normal UniversityHuanggang 438000China State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of Sciences(CAS)Fuzhou 350002China Guangdong Provincial Key Lab of Green Chemical Product Technology School of Chemistry and Chemical EngineeringSouth China University of TechnologyGuangzhou 510640China Australian Institute for Bioengineering and Nanotechnology(AIBN)and School of Chemical Engineering The University of QueenslandBrisbaneQueensland 4072Australia Department of Chemistry College of ScienceKing Saud UniversityRiyadh 11451Saudi Arabia

Exploring highly efficient Pt-free catalysts for hydrogen evolution reaction(HER)is of great importance for hydrogen(H2)***,a novel HER electrocatalyst having abundant ultra-small(2–3 nm)Ru electronically confined by a B,N codoped polar carbon surface(Ru/(B-N)-PC)was *** Ru/(B-N)-PC catalyst exhibits a low overpotential of 15 mV at the current density of 10 mA·cm^(−2),a low Tafel slope of 22.6 mV·dec^(−1),superior durability,which outperforms the benchmark Pt/C *** experimental characterizations and theory calculations suggest that an electron communication established between B,N co-doped carbon surface and ultra-small Ru nanoparticles with electrons transferred from N atoms to Ru and backtransferred from Ru to B atoms,which exerts a moderate electronic modification of ***,in turn,affords a modest H adsorption energy and a lower H2O dissociation barrier,leading to the high-performance hydrogen evolution *** work provides meaningful insight into the size control and electronic modulation of Ru catalyst for intrinsic HER activity improvement.

关键词： hydrogen evolution reaction Ru catalyst carbon support doping

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Gas6-Tyro3 signaling is required for Schwann cell myelination and possible remyelination

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Neural Regeneration Research 2016年第2期11卷 215-216页

作者： Tomohiro Torii Junji yamauchi apan Graduate School of Medical and Dental Sciences Tokyo Medical and Dental University Bunkyo Tokyo lapan

Myelin plays important roles in vertebrates,ensuring the rapid propagation of action potentials and the long-term integrity of axons,but the molecular mechanisms of myelin formation remain poorly *** studies have demo... 详细信息

关键词： cell Gas6-Tyro3 signaling is required for Schwann cell myelination and possible remyelination LINGO

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Changes in serum thyroid hormone levels and thyroid gland activity of artificially maturing female Japanese eel (Anguilla japonica)

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Acta Oceanologica Sinica 2003年第1期22卷 111-122页

作者：曲宪成 Massaki Nagae Sinji Adachi Kohei yamauchi Fisheries College Shanghai Fisheries University334 Jungong RoadShanghai 200090China Faculty of Environmental Studies Course of Environmental Conservation and PlanningNagasaki University1-14 Bunkyo-machiNagasaki 852-8521Japan Department of Biology Faculty of FisheriesHokkaido University3-1-1 Minato-choHakodate 041-0821Japan

In order to evaluate the involvement of the thyroid gland in reproduction, thyroid functioning was described in female cultivated Japanese eel (Anguilla japonica) in progressive stages of sexual maturation induced by chum salmon pituitary homogenate (SPH) treatment. Serum thyroid hormones, thyroxine (T4) and triiodothyronine (T3) were also measured in each stage. Thyroid gland activity (epithelial cell height) was high before SPH injection (previtellogenic stage), further increasing at the early vitellogenic stage, thereafter decreasing to late vitellogenic and migratory nucleus stages. The profiles of both T3 and T4 changed during vitellogenesis, being high during previtellogenic and early vitellogenic stages, and subsequently declining, thus mimicking thyroid gland activity. These results suggest that the thyroid has relation with eel ovarian development during artificial maturation.

关键词： Thyroid activity thyroxine (T4) triiodothyronine (T3) Japanese eel artificial maturation

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Non-genetic contributions of the sperm nucleus to embryonic development

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Asian Journal of Andrology 2011年第1期13卷 31-35页

作者： Yasuhiro yamauchi Jeffrey A Shaman W Steven Ward Department Anatomy and Reproductive Biology Institute for Biogenesis Research John A. Burns School of Medicine University of Hawaii at Manoa Honolulu HI USA GLP Services GENEWlZ Inc. 115 Corporate Blvd. South Plainfield NJ 07080 USA

Recent data from several laboratories have provided evidence that the newly fertilized oocyte inherits epigenetic signals from the sperm chromatin that are required for proper embryonic development. For the purposes of this review, the term epigenetic is used to describe all types of molecular information that are transmitted from the sperm cell to the embryo. There are at least six different forms of epigenetic information that have already been established as being required for proper embryogenesis in mammals or for which there is evidence that it may do so. These are （i） DNA methylation; （ii） sperm-specific histones, （iii） other chromatin-associated proteins; （iv） the perinuclear theca proteins; （v） sperm-born RNAs and, the focus of this review; and （vi） the DNA loop domain organization by the sperm nuclear matrix. These epigenetic signals should he considered when designing protocols for the manipulation and cryopreservation of spermatozoa for assisted reproductive technology as necessary components for effective fertilization and subsequent embryo development.

关键词： embryogenesis epigenetics sperm DNA sperm nuclear matrix DNA loop domain organization

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Study of Optical Fibers Strain-Temperature Sensitivities Using Hybrid Brillouin-Rayleigh System

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Photonic Sensors 2014年第1期4卷 1-11页

作者： Kinzo Kishida Yoshiaki yamauchi Artur Guzik Neubrex Co.Ltd. Sakaemachi-dori 1-1-24Chuo-kuKobeHyogo650-0023Japan

在这份报纸，象在工业应用的分布式的光纤维察觉到的挑战(DOFS ) 一样的最近的进步被讨论。比作过去常测量紧张或温度的传感器的广阔市场，在工业水平的分布式的光纤维察觉到的成功(DOFS ) 很最多被限制。为更宽的接受的这缺乏的原因之... 详细信息

在这份报纸，象在工业应用的分布式的光纤维察觉到的挑战(DOFS ) 一样的最近的进步被讨论。比作过去常测量紧张或温度的传感器的广阔市场，在工业水平的分布式的光纤维察觉到的成功(DOFS ) 很最多被限制。为更宽的接受的这缺乏的原因之一是在商业地可得到的系统和实际工业要求之间的失配，特别为空间分辨率和精确。这些要求在纸被组织并且澄清。它也描述混合 Brillouin-Rayleigh 系统，它展出紧张计量器超过那些的能力。系统的原则就纤维刻度方法论而言被说明。为决定紧张，温度，和水疗院压力要求的公式被导出并且讨论。最后，应用的例子被举。

关键词：温度变化光纤应变系统混合瑞利分布式光纤传感敏感温度传感器

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Machine learning adaptation of intraocular lens power calculation for a patient group

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Eye and Vision 2021年第5期8卷 422-430页

作者： Yosai Mori Tomofusa yamauchi Shota Tokuda Keiichiro Minami Hitoshi Tabuchi Kazunori Miyata Miyata Eye Hospital 6‑3 Kurahara‑choMiyakonojoMiyazaki 885‑0051Japan Department of Ophthalmology Tsukazaki Hospital68‑1 WakuAboshi‑kuHimejiHyogo 671‑1227Japan Department of Technology and Design Thinking for Medicine Hiroshima University1‑2‑3 KasumiMinami‑kuHiroshima 734‑8553Japan

Background:To examine the effectiveness of the use of machine learning for adapting an intraocular lens(IOL)power calculation for a patient ***:In this retrospective study,the clinical records of 1,611 eyes of 1,169 Japanese patients who received a single model of monofocal IOL(SN60WF,Alcon)at Miyata Eye Hospital were reviewed and *** biometric metrics and postoperative refractions of 1211 eyes of 769 patients,constants of the SRK/T and Haigis formulas were *** SRK/T formula was adapted using a support vector *** errors in the use of adapted formulas as well as the SRK/T,Haigis,Hill-RBF and Barrett Universal II formulas were evaluated with data from 395 eyes of 395 distinct *** prediction errors,median absolute errors,and percentages of eyes within±0.25 D,±0.50 D,and±1.00 D,and over+0.50 D of errors were compared among ***:The mean prediction errors in the use of the SRT/K and adapted formulas were smaller than the use of other formulas(P<0.001).In the absolute errors,the Hill-RBF and adapted methods were better than *** performance of the Barrett Universal II was not better than the others for the patient *** were the least eyes with hyperopic refractive errors(16.5%)in the use of the adapted ***:Adapting IOL power calculations using machine learning technology with data from a particular patient group was effective and promising.

关键词： Machine learning Adaptation Intraocular lens power calculation Patient ethnicity Patient race Region of patient SRK/T formula

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Distribution and relative activity of matrix metalloproteinase-2 in human coronal dentin

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International Journal of Oral Science 2011年第4期3卷 192-199页

作者： Lee W. Boushell Masaru Kaku Yoshiyuki Mochida Mitsuo yamauchi Department of Operative Dentistry School of Dentistry University of North Carolina Department of Bio-Prosthodontics Medical and Dental Science Niigata University Graduate School Chuo-ku Department of Periodontology and Oral Biology Division of Oral Biology Boston University Henry M. Goldman School of Dental Medicine Center for Advanced Biomedical Research Dental Research Center School of Dentistry University of North Carolina

The presence of matrix metalloproteinase-2 （MMP-2） in dentin has been reported, but its distribution and activity level in mature human coronal dentin are not well understood. The purpose of this study was to determine the MMP-2 distribution and relative activity in demineralized dentin. Crowns of twenty eight human molars were sectioned into inner （ID）, middle （MD）, and outer dentin （OD） regions and demineralized. MMP-2 was extracted with 0.33 mol·L-1 EDTA/2 mol·L-1 guanidine-HCl, pH 7.4, and MMP-2 concentration was estimated with enzyme-linked immunoabsorbant assay （ELISA）. Further characterization was accomplished by Western blotting analysis and gelatin zymography. The mean concentrations of MMP-2 per mg dentin protein in the dentin regions were significantly different （P=0.043）： 0.9 ng （ID）, 0.4 ng （MD）, and 2.2 ng （OD）, respectively. The pattern of MMP-2 concentration was OD〉ID〉MD. Western blotting analysis detected -66 and -72 kDa immunopositive proteins corresponding to pro- and mature MMP-2, respectively, in the ID and MD, and a -66 kDa protein in the OD. Gelatinolytic activity consistent with MMP-2 was detected in all regions. Interestingly, the pattern of levels of Western blot immunodetection and gelatinolytic activity was MD〉ID〉OD. The eoneentration of MMP-2 in human coronal dentin was highest in the region of dentin that contains the dentinoenamel junction and least in the middle region of dentin. However, levels of Western blot immunodetection and gelatinolytic activity did not correlate with the estimated regional concentrations of MMP-2, potentially indicating region specific protein interactions.

关键词： matrix metalloproteinase-2 human coronal dentin distribution gelatinolytic activity

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