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Journal of Rare Earths 2024年第1期42卷 1-15,I0001页

作者： Julio Corredoira-Vázquez Cristina gonzález-barreira Paula Oreiro-martínez Ana m.garcía-Deibe Jesús Sanmartín-matalobos matilde Fondo Departamento de Química Inorganica Facultade de QuímicaUniversidade de Santiago de CompostelaCampus Vida15782Santiago de CompostelaSpain Phantom-g CICECO-Aveiro Institute of MaterialsDepartment of PhysicsUniversity of Aveiro3810-193AveiroPortugal Institute of materials(imATUS) Universidade de Santiago de Compostela15782Santiago de CompostelaSpain

In this paper,the lanthanoid complexes of N_(5) and N_(6) macrocycle ligands,without pendant arms or additional heteroatoms,are *** review covers the period from 2015 to the current date,since in 2014 Schiff base macrocyclic ligands incorporating the pyridine moiety,and their complexes,were revised,and in 2015 the chemistry of pentaaza macrocycle ligands with rare earth metals was also *** and phthalocyanine ligands are not included in this review,which primarily focuses on complexes with Schiff bases and amines without pendant arms or any additional donor other than *** synthetic methods,structural characterization,based on single X-ray crystal data,and properties of the lanthanoid complexes,with special attention to magneto-structural correlations,are presented herein.

关键词： Lanthanoid N_(5),N_(6)macrocycle Coordination chemistry Chirality biological activity molecule magnet

An app to assist farmers in the identification of diseases and pests of coffee leaves using deep learning

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Information Processing in Agriculture 2022年第1期9卷 38-47页

作者： Jose g.m.Esgario Pedro b.C.de Castro Lucas m.Tassis Renato A.Krohling LAbCIN-Nature Inspired Computing Federal University of Espirito SantoAv.Fernando Ferrari514CEP 29075-910 VitoriaEspırito SantoESBrazil LAbCIN-Nature Inspired Computing and PPGI-Graduate Program in Computer Scienceand Production Engineering DepartmentFederal University of Espirito SantoAv.Fernando Ferrari514CEP 29075-910 VitoriaEspırito SantoESBrazil

In recent years,deep learning methods have been introduced for segmentation and classi-fication of leaf lesions caused by pests and *** the commonly used approaches,convolutional neural networks have provided results with high *** purpose of this work is to present an effective and practical system capable of seg-menting and classifying different types of leaf lesions and estimating the severity of stress caused by biotic agents in coffee leaves using convolutional neural *** proposed approach consists of two stages:a semantic segmentation stage with severity calculation and a symptom lesion classification *** stage was tested separately,highlighting the positive and negative points of each *** obtained very good results for the severity estimation,suggesting that the model can estimate severity values very close to the real *** the biotic stress classification,the accuracy rates were greater than 97%.Due to the promising results obtained,an App for Android platform was developed and imple-mented,consisting of semantic segmentation and severity calculation,as well as symptom classification to assist both specialists and farmers to identify and quantify biotic stresses using images of coffee leaves acquired by smartphone.

关键词： Convolutional neural networks Semantic segmentation Coffee leaf Pests and diseases App.development

Synthesis and characterization of a 1,3-dibutylimidazolium azide([bbIm][N_(3)]) : A promising green energetic ionic liquid

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Defence Technology（防务技术） 2024年第8期38卷 1-15页

作者： Nawel matmat Amir Abdelaziz Djalal Trache Achour Sabrina Ahmed Fouzi Tarchoun Hani boukeciat Sourbh Thakur Weiqiang Pang Thomas m.Klapotke Energetic materials Laboratory(EmLab) Teaching and Research Unit of Energetic ProcessesEcole Militaire PolytechniqueBP 17 Bordj El-BahriAlgiers 16046Algeria Department of Organic Chemistry Bioorganic Chemistry and BiotechnologySilesian University of TechnologyB.Krzywoustego 444-100 GliwicePoland Xi'an modern Chemistry Research Institute Xi'an 710065China Energetic materials Research Department of ChemistryLudwig-Maximilian UniversityMunich Butenandtstrasse 5-13(D)D-81377 MunichGermany

In the pursuit of advancing imidazolium-based energetic ionic liquids (EILs),the current study is devoted to the synthesis and characterization of 1,3-dibutyl-imidazolium azide ([bbIm][N_(3)]),as a novel member in this ionic liquids *** chemical structure of this EIL was rigorously characterized and confirmed using FTIR spectroscopy,1D,and 2D-NmR *** thermal behavior assessment was conducted through DSC and TgA *** analysis revealed an endothermic glass transition at T_(g)=-61℃,followed by an exothermic degradation event at T_(onset)=311℃.Similarly,TgA thermograms exhibited a one-stage decomposition process resulting in 100% mass loss of the ***,the short-term thermal stability of the azide EIL was investigated by combining the non-isothermal TgA data with the TAS,it-KAS,and VYA/CE isoconversional kinetic ***,the Arrhenius parameters(E_(a)=154 kJ·mol^(-1),Log(A/s^(-1))=11.8) and the most probable reaction model g(a) were *** observed high decomposition temperatures and the significantly elevated activation energy affirm the enhanced thermal stability of the modified *** findings revealed that[bbIm][N_(3)]EIL can be a promising candidate for advanced energetic material application.

关键词： 1,3-dibutyl-imidazolium azide[bbIm][N_(3)] Energetic imidazolium-base ionic liquids 1D-/2D-NmR analyses Short-term thermal stability Isoconversional approaches

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三轴形变核ba中的奇异集体激发模式

物理学报 2024年

作者：韦锐周厚兵王思成丁兵强赟华贾晨旭陈红星郭松 C.m.Petrache D.mengoni A.Astier E.Dupont 吕冰锋 D.bazzacco A.boso A.goasduff F.Recchia D.Testov F.galtarossa g.Jaworski D.R.Napoli S.Riccetto m.Siciliano J.J.Valiente-Dobon C.Andreoiu F.H.garcia K.Ortner K.Whitmore A.Ata?-Nyberg T.b?ck b.Cederwall E.A.Lawrie I.Kuti D.Sohler T.marchlewski J.Srebrny A.Tucholski 意大利国家核物理研究所帕多瓦分部中国科学院大学西蒙菲莎大学化学系广西核物理与核技术重点实验室意大利国家核物理研究所莱尼亚罗国家实验室国家研究基金会iThemba加速器科学实验室西开普大学物理与天文系费拉拉大学理学与自然科学院帕多瓦大学物理和天文学系皇家理工学院物理系广西师范大学物理科学与技术学院中国科学院近代物理研究所 HUN-REN原子核研究所 15. 华沙巴斯德拉大学重离子实验室巴黎萨克雷大学

利用意大利Legnaro实验室串列静电加速器提供的65 meV13C束流与122Sn靶的熔合蒸发反应布居了131ba的高自旋态，并搭建了新的能级纲图。新的能级纲图由15条转动带组成，包括三对手征双重带，其中两对正宇称手征带为赝自旋-手征四重带。... 详细信息

利用意大利Legnaro实验室串列静电加速器提供的65 meV13C束流与122Sn靶的熔合蒸发反应布居了131ba的高自旋态，并搭建了新的能级纲图。新的能级纲图由15条转动带组成，包括三对手征双重带，其中两对正宇称手征带为赝自旋-手征四重带。正负宇称手征带通过一系列增强的E1跃迁连接，表明它们之间存在八极关联。在低自旋区域搭建了一条新的转动带，通过一系列γ跃迁向νh11/2晕带退激。这种能级结构与摇摆带相似，但基于现有的实验证据还难以将它确认为摇摆带，不能排除其它集体激发机制，如γ振动的影响。

关键词：高自旋态手征带赝自旋八极关联摇摆运动

The role of physical properties in explosive welding of copper to stainless steel

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Defence Technology（防务技术） 2023年第4期22卷 88-98页

作者： g.H.S.F.L.Carvalho I.galvao R.mendes R.m.Leal A.b.moreira A.Loureiro Univ Coimbra CEMMPREDepartamento de Engenharia Mec^anicaRua Luís Reis Santos3030-788CoimbraPortugal Department of Industrial Engineering University of FirenzeVia di Santa Marta 350139FirenzeItaly ISEL Departamento de Engenharia Mec^anicaInstituto Politecnico de LisboaRua Conselheiro Emídio Navarro 11959-007LisboaPortugal Univ Coimbra ADAILEDAPDepartamento de Engenharia Mec^anicaRua Luís Reis Santos3030-788CoimbraPortugal LIDA-ESAD.CR Instituto Politecnico de LeiriaRua Isidoro Inacio Alves de Carvalho2500-321Caldas da RainhaPortugal Univ.Porto LAETA/INEGIDept.Eng.Metalúrgica e de MateriaisR.Dr.Roberto Frias4200-465PortoPortugal

This paper investigates the effects of the physical properties on the microstructure and weldability of explosive welding by joining two metals with a significant contrast in thermophysical properties:stainless steel and *** welds between stainless steel and copper were obtained,and the interfacial morphology was wavy,regardless of the position of the *** weldability of dissimilar pairs was found to be more dependent on the relationship between the physical properties of the base materials than on the absolute value of the material *** there is a significant difference in thermal conductivity between the flyer and the base plate,together with a material with a low melting temperature,the weldability of the pair is often *** relative position of the plates affects the interfacial microstructure even when similar morphologies are *** the metallic pairs studied,the wave size was bigger for the configuration in which the ratio between the density of the flyer and the density of the base plate is *** same phenomenon was observed for the impedance:bigger waves were found for a smaller ratio between the impedance of the flyer and the impedance of the base plate.

关键词： Explosive welding Solid-state Copper-stainless steel Dissimilar Interface morphology Weldability

Unveiling bulk and surface radiation forces in a dielectric liquid

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Light(Science & Applications) 2022年第5期11卷 925-934页

作者： N.g.C.Astrath g.A.S.Flizikowski b.Anghinoni L.C.malacarne m.L.baesso T.Požar m.Partanen I.brevik D.Razansky S.E.bialkowski Department of Physics Universidade Estadual de MaringáMaringáPRBrazil Faculty of mechanical Engineering University of LjubljanaLjubljanaSlovenia Department of Electronics and Nanoengineering Aalto UniversityAaltoFinland Department of Energy and Process Engineering Norwegian University of Science and TechnologyTrondheimNorway Institute for biomedical Engineering and Institute of Pharmacology and Toxicology Faculty of MedicineUniversity of ZurichZurichSwitzerland Institute for biomedical Engineering Department of Information Technology and Electrical EngineeringETH ZurichZurichSwitzerland Department of Chemistry and biochemistry Utah State UniversityLoganUTUSA

Precise control over light-matter interactions is critical for many optical manipulation and material characterization methodologies,further playing a paramount role in a host of nanotechnology ***,the fundamental aspects of interactions between electromagnetic fields and matter have yet to be established unequivocally in terms of an electromagnetic momentum ***,we use tightly focused pulsed laser beams to detect bulk and boundary optical forces in a dielectric *** the optical convoluted signal,we decouple thermal and nonlinear optical effects from the radiation forces using a theoretical interpretation based on the microscopic Ampère force *** is shown,for the first time,that the time-dependent pressure distribution within the fluid chiefly originates from the electrostriction *** results shed light on the contribution of optical forces to the surface displacements observed at the dielectric air-water interfaces,thus shedding light on the long-standing controversy surrounding the basic definition of electromagnetic momentum density in matter.

关键词： dielectric momentum surface

Reviewing perovskite oxide sites influence on electrocatalytic reactions for high energy density devices

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Journal of Energy Chemistry 2023年第6期81卷 1-19,I0002页

作者： Lorrane C.C.b.Oliveira Raissa Venâncio Paulo V.F.de Azevedo Chayene g.Anchieta Thayane C.m.Nepel Cristiane b.Rodella Hudson Zanin gustavo Doubek Advanced Energy Storage Division Laboratory of Advanced Batteries(LAB)Center for Innovation on New Energies(CINE)School of Chemical EngineeringUniversity of Campinas(Unicamp)CampinasSao Paulo 13083-852Brazil Advanced Energy Storage Division Center for Innovation on New Energies(CINE)Brazilian Renewable Energies(BREnergies)groupManufacturing GroupSchool of Electrical and Computer EngineeringUniversity of Campinas(UNICAMP)CampinasSão Paulo 13083-852Brazil Paul Scherrer Institut(PSI) Swiss Light Source(SLS)Forschungsstrasse 1115232 Villigen PSIAargauSwitzerland brazilian Center for Research in Energy and materials(CNPEm)/brazilian Synchrotron Light Laboratory(LNLS) CampinasSão Paulo 13083-100Brazil

batteries,fuel cells,and supercapacitors are electrochemical devices already on the market and still need a boost in kinetics to match the high energy density demand of *** have attracted the scientific community's attention in the last decade due to their electrocatalytic activity,chemical and structural properties,tunability,low cost,and *** have been made to understand the active sites and the operational mechanisms in perovskite oxides to shape them as an electrocatalyst in advanced energy *** the role of perovskites is the key to engineering more controlled and efficient electrocatalysts via chemical synthesis,and there is still much to *** review highlights the use of perovskites in different energy storage and conversion *** A,b,and A&b doping-site effects are analyzed to understand the opportunities and challenges related to this class of *** addition,the synthesis methods and the properties related to the doping site are described and summarized.

关键词： Perovskites Energy storage systems Electrocatalysts battery Oxide fuel cells Capacitors

The development of semiconductor detectors for radiometers of alpha‑radiation and the examination of the volumetric activity of radon in various areas

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Radiation Detection Technology and methods 2023年第3期7卷 457-463页

作者： b.S.Radzhapov S.A.Radzhapov F.g.mullagalieva m.A.Zufarov Physical-Technical Institute of Scientific Association of“Physics-Sun” Chingiz Aytmatov Str.2 B100084 TashkentUzbekistan Institute of materials Science Scientific Association of“Physics-Sun”Uzbekistan Academy of Sciences Parkent102226 TashkentUzbekistan

Purpose Development of highly sensitive semiconductor detectors of large diameter and manufacturing of a measuring complex—a radiometer based on the developed detectors for studying the activity of alpha particles and the volumetric activity of radon in various *** The detectors were manufactured using surface-barrier and heterojunction *** etchant formulations for silicon have been *** obtain plane-parallelism of the plates during chemical etching,a special dynamic setup was *** structure of the radiometer,electrical circuits,and device software have been *** The results of the development of technology for the manufacture of detectors of large dimensions(30-100 mm in diameter)are *** of the electrical and radiometric characteristics of surface-barrier n detectors and detectors based on Al-αge-pSi-Au heterojunctions were carried *** principle of operation of the electronic components of a radiometer made using these detectors is also *** The data of monitoring of radon content in soil air are *** results showed that the concentration varies depending on temperature,humidity,and time of *** gSm/SmS module allows the device to operate in real time.

关键词： Silicon Semiconductor detectors Radiometer Alpha-radiation Heterojunction

Comparative analysis of extreme ultraviolet solar radiation proxies during minimum activity levels

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Earth and Planetary Physics 2023年第5期7卷 540-547页

作者： A.g.Elias C.R.martinis b.F.de Haro barbas F.D.medina b.S.Zossi m.Fagre T.Duran Laboratorio de Ionosfera Atmosfera Neutra y MagnetosferaFacultad de Ciencias Exactas y Tecnologia(FACET)Universidad Nacional de Tucuman(UNT)Tucuman 4000Argentina Instituto de Física del Noroeste Argentino Consejo Nacional de Investigaciones Cientificas y Tecnicas(CONICET)-UNTTucuman 4000Argentina Center for Space Physics Astronomy DepartmentBoston UniversityMA 02215USA CONICET Tucuman 4000Argentina Laboratorio de Telecomunicaciones Departamento de ElectricidadElectrónica y ComputaciónFACETUNTTucuman4000Argentina Departamento de Física Universidad Nacional del Sur(UNS)Bahia Blanca 8000Argentina Instituto de Física del Sur CONICET-UNSBahia Blanca 8000Argentina

Four extreme ultraviolet(EUV)solar radiation proxies(magnesium II core-to-wing ratio(mgII),Lymanαflux(Fα),10.7-cm solar radio flux(F10.7),and sunspot number(Rz))were analyzed during the last four consecutive solar activity minima to investigate how they differ during minimum periods and how well they represent solar EUV *** variability within each minimum and between minima was compared by considering monthly means.A comparison was also made of their role in filtering the effect of solar activity from the critical frequency of the ionospheric F2 layer,foF2,which at mid to low latitudes depends mainly on EUV solar *** last two solar cycles showed unusually low EUV radiation levels according to the four *** the connection between the EUV“true”variation and that of solar proxies,according to the foF2 filtering analysis,mgII and Fαbehaved in a more stable and suitable way,whereas Rz and F10.7 could be overestimating EUV levels during the last two minima,implying they would both underestimate the inter-minima difference of EUV when compared with the first two minima.

关键词： solar EUV radiation solar minimum foF2 solar activity solar EUV proxy

Stochastic Programming for Hub Energy management Considering Uncertainty Using Two-Point Estimate method and Optimization Algorithm

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Computer modeling in Engineering & Sciences 2023年第12期137卷 2163-2192页

作者： Ali S.Alghamdi mohana Alanazi Abdulaziz Alanazi Yazeed Qasaymeh muhammad Zubair Ahmed bilal Awan m.g.b.Ashiq Department of Electrical Engineering College of EngineeringMajmaah UniversityAl-Majmaah11952Saudi Arabia Department of Electrical Engineering College of EngineeringJouf UniversitySakaka72341Saudi Arabia Department of Electrical Engineering College of EngineeringNorthern Border UniversityAr’Ar73222Saudi Arabia Automation and Control Department College of Engineering TechnologyUniversity of Doha for Science and TechnologyDoha24449Qatar Department of Electrical and Computer Engineering College of Engineering and Information TechnologyAjman UniversityAjman20550United Arab Emirates Department of Physics College of ScienceImam Abdulrahman Bin Faisal UniversityDammam31441Saudi Arabia

To maximize energy profit with the participation of electricity,natural gas,and district heating networks in the day-ahead market,stochastic scheduling of energy hubs taking into account the uncertainty of photovoltaic and wind resources,has been carried *** has been done using a new meta-heuristic algorithm,improved artificial rabbits optimization(IARO).In this study,the uncertainty of solar and wind energy sources is modeled using Hang’s two-point estimating method(TPEm).The IARO algorithm is applied to calculate the best capacity of hub energy equipment,such as solar and wind renewable energy sources,combined heat and power(CHP)systems,steamboilers,energy storage,and electric cars in the *** standard ARO algorithmis developed to mimic the foraging behavior of rabbits,and in this work,the algorithm’s effectiveness in avoiding premature convergence is improved by using the dystudynamic inertia weight *** proposed IARO-based scheduling framework’s performance is evaluated against that of traditional ARO,particle swarm optimization(PSO),and salp swarm algorithm(SSA).The findings show that,in comparison to previous approaches,the suggested meta-heuristic scheduling framework based on the IARO has increased energy profit in day-ahead electricity,gas,and heating markets by satisfying the operational and energy hub ***,the results show that TPEm approach dependability consideration decreased hub energy’s profit by 8.995%as compared to deterministic planning.

关键词： Stochastic energy hub scheduling energy profit uncertainty Hong’s two-point estimate method improved artificial rabbits optimization